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JAEA Reports

Evaluation of the minimum critical amount for heterogeneous lattice systems composed of fuel rods utilized in low-power water-moderated research and test reactors by using continuous-energy Monte Carlo code MVP with JENDL-4.0

Yanagisawa, Hiroshi

JAEA-Technology 2021-023, 190 Pages, 2021/11

JAEA-Technology-2021-023.pdf:5.25MB

Computational analyses on nuclear criticality characteristics were carried out for heterogeneous lattice systems composed of water moderator and fuel rods utilized in lowpower research and test reactors, in which the depletion of fuel due to burnup is relatively small, by using the continuous-energy Monte Carlo code MVP Version 2 with the evaluated nuclear data library JENDL-4.0. In the analyses, the minimum critical number of fuel rods was evaluated using calculated neutron multiplication factors for the heterogeneous systems of the uranium dioxide fuel rod in the Static Experiments Critical Facility (STACY) and the Tank-type Critical Assembly (TCA), and the uranium-zirconium hydride fuel rod in the Nuclear Safety Research Reactor (NSRR). In addition, six sorts of the ratio of reaction rates, which are components of neutron multiplication factors, were calculated in the analyses to explain the variation of neutron multiplication factors with the ratio of water moderator to fuel volume in a unit fuel rod cell. Those results of analyses are considered to be useful for the confirmation of reasonableness and validity of criticality safety measures as data showing criticality characteristics for water-moderated heterogeneous lattice systems composed of the existing fuel rods in research and test reactors, of which criticality data are not sufficiently provided by the Criticality Safety Handbook.

JAEA Reports

Direction of future safety research to be conducted by Sector of Nuclear Safety Research and Emergency Preparedness (FY 2021 Edition)

Planning and Co-ordination Office, Sector of Nuclear Safety Research and Emergency Preparedness

JAEA-Review 2021-019, 58 Pages, 2021/11

JAEA-Review-2021-019.pdf:2.26MB

In response to the directives of the 4th medium-to-long-term objectives, Japan Atomic Energy Agency will formulate the 4th medium-to-long-term plan and run its operation according to the plan from the fiscal year 2022. Consequently, the Sector of Nuclear Safety Research and Emergency Preparedness has reviewed the strategies of the safety research for contributing to the demand, "the continuous improvement of nuclear safety and the effectiveness of nuclear disaster prevention". It was also discussed how to proceed the safety research over the medium-to-long-term plan period based on the proposed new strategies. From the viewpoint of developing human resources and maintaining research capabilities in the sector, discussion was made on measures to pass on the knowledge and skills of senior and mid-career researchers to young researchers. The main elements of the proposed strategies are: (1) to efficiently and effectively develop both problem-solving research and advanced or leading research, considering the importance and needs on the nuclear safety and corresponding to regulatory trends and introduction of new technologies, (2) to produce research results of high quality for social implementation, including proactive proposal of measures for enhancing rationality of nuclear safety and regulation by utilizing risk information, and (3) to promote development of human resources and maintenance of technological base through challenging new research subjects. This report summarizes results of the discussion on the medium-to-long-term safety research strategies and the research plans based on the proposed strategies.

Journal Articles

Development of effectiveness evaluations technology of the measures for improving resilience of nuclear structures at ultra high temperature

Onoda, Yuichi; Nishino, Hiroyuki; Kurisaka, Kenichi; Yamano, Hidemasa

Proceedings of Asian Symposium on Risk Assessment and Management 2021 (ASRAM 2021) (Internet), 11 Pages, 2021/10

The effectiveness evaluations technology of the measures for improving resilience by applying a fracture control concept under ultra-high temperature conditions has developed for prototype sodium-cooled fast reactor Monju as a model plant, and the trial evaluation has conducted using this technology in this paper. The important accident sequences to which the fracture control concept is expected to be applied under ultra-high temperature condition are identified by investigating the results of the existing researches of level-2 probabilistic risk assessment for Monju. Accident sequences categorized in protected loss of heat sink and loss of reactor level are both identified as such important accident sequences which has the potential to prevent core damage. This study has developed the technology to evaluate the effectiveness of improving resilience, where the headings which stand for success or failure of the measures to improve resilience are introduced into the event tree, the branch probability of them is set, and the effectiveness of improving resilience is expressed as the reduction of core damage frequency. As a result of the trial evaluation of the effectiveness for the measures to improve resilience, it is confirmed that core damage frequency can be reduced by applying fracture control concept. The branch probability of the measures to improve resilience proposed in this study is tentatively assigned based on the assumption. This value is expected to be quantified by the forthcoming analyses of the integrity for the reactor vessel structure at ultra-high temperature. The technology developed in this study will be applied for the evaluation of improving resilience of the next generation sodium-cooled fast reactor.

Journal Articles

Evolution of the reaction and alteration of mudstone with ordinary Portland cement leachates; Sequential flow experiments and reactive-transport modelling

Bateman, K.; Murayama, Shota*; Hanamachi, Yuji*; Wilson, J.*; Seta, Takamasa*; Amano, Yuki; Kubota, Mitsuru*; Ouchi, Yuji*; Tachi, Yukio

Minerals (Internet), 11(9), p.1026_1 - 1026_23, 2021/09

 Times Cited Count:0

Journal Articles

Concepts and basic designs of various nuclear fuels, 5; Fuels for high temperature gas-cooled reactor and molten salt reactor

Ueta, Shohei; Sasaki, Koei; Arita, Yuji*

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 63(8), p.615 - 620, 2021/08

no abstracts in English

Journal Articles

Growing need for humanities and social science studies in uranium waste disposal

Yasuda, Hiroshi*; Fumoto, Hiromichi*; Saito, Tatsuo

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 63(8), p.610 - 614, 2021/08

Regarding the handling of uranium bearing waste, which is contaminated with uranium, which is a naturally occurring radionuclide, and its descendant nuclides, in recent years, the Japan Nuclear Regulatory Commission, etc. have been carefully and actively deliberated based on the knowledge of natural science and safety engineering. It was carried out, and as of March 2021, a certain policy has been shown. On the other hand, when disposing of uranium waste, which may cause dose exposure to future generations, the authors consider not only the science and engineering perspectives that have been conducted so far, but also the humanities and social science perspectives. We have been discussing with experts in related fields, thinking that it is necessary. In this report, we will introduce the background that brought about such an idea and the direction of future discussions.

Journal Articles

ISCN/JAEA-IAEA online SSAC training development

Kawakubo, Yoko; Stevens, R.*; Pickett, S.*; Sekine, Megumi; Noro, Naoko; Inoue, Naoko

Proceedings of INMM & ESARDA Joint Annual Meeting (Internet), 10 Pages, 2021/08

JAEA Reports

Study on the radioactivity evaluation method of biological shielding concrete of JPDR for near surface disposal

Kochiyama, Mami; Okada, Shota; Sakai, Akihiro

JAEA-Technology 2021-010, 61 Pages, 2021/07

JAEA-Technology-2021-010.pdf:3.56MB
JAEA-Technology-2021-010(errata).pdf:0.75MB

It is necessary to evaluate the radioactivity inventory in wastes in order to dispose of radioactive wastes generated from dismantling nuclear reactor in the shallow ground. In this report, we examined radioactivity evaluation method for near surface disposal about biological shield concrete near the core generated from the dismantling of JPDR. We calculated radioactive concentration of the target biological concrete using the DORT code and the ORIGEN-S code, and we estimated radioactivity concentration Di (Bq/t). For DORT calculation, the cross-section library created from the MATXSLIB-J40 file from JENDL-4.0 was used, and for ORIGEN-S, the attached library of SCALE6.0 was used. As a result of comparing the calculation results of the radioactivity concentration with the past measured values in the radial direction and the vertical direction, we found that the trends were generally the same. We calculated radioactive concentration of the target biological concrete Di (Bq/t), and we compared with the estimated Ci (Bq/t) equivalent to the dose criteria of trench disposal calculated for 140 nuclides. As a result we inferred that the except for about 2% of target waste could be disposed of in the trench disposal facility. We also preselected important nuclides for trench disposal based on the ratios (Di/Ci) for each nuclide, H-3, C-14, Cl-36, Ca-41, Co-60, Sr-90, Eu-152 and Cs-137 were selected as important nuclides.

JAEA Reports

Horonobe Underground Research Laboratory Project; Investigation program for the 2021 fiscal year

Nakayama, Masashi

JAEA-Review 2021-009, 54 Pages, 2021/07

JAEA-Review-2021-009.pdf:5.02MB

The Horonobe URL Project is being pursued by the JAEA to enhance the reliability of relevant disposal technologies for geological disposal of High-level Radioactive Waste through investigations of the deep geological environment within the host sedimentary rock at Horonobe Town in Hokkaido, north Japan. In 2021 fiscal year (2021/2022), JAEA continue to conduct research on "Demonstration of EBS in geological environment", "Demonstration of disposal concept", and "Validation of buffer capacity of the sedimentary rock to tectonism", which are the important issues shown in the Horonobe underground research plan after 2020 fiscal year. The main studies to be conducted in 2021 fiscal year are as follows. As "Demonstration of EBS in geological environment", we will shift to the test under the condition that the influence of heating is eliminated in the full scale EBS experiment. As "Demonstration of disposal concept", as a demonstration of the closure techniques, it details the conditions under which long-term transitions in the tunnel and surrounding bedrock have a significant impact on safety assessments. And we will continue engineering scale experiment to confirm the workability and performance of plugs and laboratory tests to examine the interaction between backfilling materials and buffer materials. As "Validation of buffer capacity of the sedimentary rock to tectonism", we will analyze the results of the hydraulic disturbance test and continue to study the hydraulic disconnection of faults/fissures in the Wakkanai Formation. As an advancement of technology for investigating and evaluating areas where the flow of groundwater is extremely slow, a boring exploration will be conducted to confirm the three-dimensional distribution of the fossil seawater area.

Journal Articles

The Impact of cement on argillaceous rocks in radioactive waste disposal systems; A Review focusing on key processes and remaining issues

Wilson, J.*; Bateman, K.; Tachi, Yukio

Applied Geochemistry, 130, p.104979_1 - 104979_19, 2021/07

 Times Cited Count:1 Percentile:0.56(Geochemistry & Geophysics)

The concept of deep geological disposal will include the multiple use of cement-based materials. In the case of argillaceous host rocks, the presence of hyperalkaline cement porefluid results in the destabilization of primary minerals in the argillite, resulting in the development of a zone of alteration at cement-rock interfaces. The process understanding gained from experimental, analogue, and modelling studies has been reviewed, and remaining areas of uncertainty identified. Although there is a reasonably good understanding of the mineral assemblages that are likely to occur due to cement-rock interactions, there are still some areas where a degree of uncertainty remains, in particular: the evolution of cement-argillite interfaces at T $$>$$ 25$$^{circ}$$C; the rates at which secondary minerals form; the extent of pore clogging due to secondary mineral precipitation; the implications of alteration for radionuclide transport.

Journal Articles

Density functional study on Am(III)/Eu(III) selectivity using crown ether type ligands

Fukasawa, Yuto*; Kaneko, Masashi; Nakashima, Satoru*

Journal of Radioanalytical and Nuclear Chemistry, 329(1), p.77 - 84, 2021/07

 Times Cited Count:0 Percentile:0.01(Chemistry, Analytical)

Density functional theory calculations were applied to understand the selectivity between Am$$^{3+}$$ and Eu$$^{3+}$$ ions with the crown ethers type ligands. 18C6 is predicted to form the most stable complex with Eu$$^{3+}$$ and show the higher stability for Am$$^{3+}$$ over Eu$$^{3+}$$, being consistent with previously reported Am$$^{3+}$$/Eu$$^{3+}$$ selectivity. We modeled N- and S-donor complexes by using framework of 18C6 complex and analyzed the complexation Gibbs energies, indicating that 18C6 with N-donor atoms is suitable for both complexation and higher Am$$^{3+}$$ stability over Eu$$^{3+}$$ due to the stronger covalent interaction.

Journal Articles

Analysis and mapping of detailed inner information of crystalline grain by wavelength-resolved neutron transmission imaging with individual Bragg-dip profile-fitting analysis

Sakurai, Yosuke*; Sato, Hirotaka*; Adachi, Nozomu*; Morooka, Satoshi; Todaka, Yoshikazu*; Kamiyama, Takashi*

Applied Sciences (Internet), 11(11), p.5219_1 - 5219_17, 2021/06

 Times Cited Count:1 Percentile:76.99(Chemistry, Multidisciplinary)

JAEA Reports

A Numerical simulation study of the desaturation and oxygen infusion into the sedimentary rock around the tunnel in the Horonobe Underground Research Laboratory

Miyakawa, Kazuya; Aoyagi, Kazuhei; Akaki, Toshifumi*; Yamamoto, Hajime*

JAEA-Data/Code 2021-002, 26 Pages, 2021/05

JAEA-Data-Code-2021-002.pdf:2.14MB
JAEA-Data-Code-2021-002-appendix(CD-ROM).zip:40.99MB

Investigations employing numerical simulation have been conducted to study the mechanisms of desaturation and oxygen infusion into sedimentary formations. By mimicking the conditions of the Horonobe underground research laboratory, numerical simulations aided geoscientific investigation of the effects of dissolved gas content and rock permeability on the desaturation (Miyakawa et al., 2019) and mechanisms of oxygen intrusion into the host rock (Miyakawa et al., 2021). These simulations calculated multi-phase flow, including flows of groundwater and exsolved gas, and conducted sensitivity analysis changing the dissolved gas content, rock permeability, and humidity at the gallery wall. Only the most important results from these simulations have been reported previously, because of publishers' space limitations. Hence, in order to provide basic data for understanding the mechanisms of desaturation and oxygen infusion into rock, all data for 27 output parameters (e.g., advective fluxes of heat, gas, and water, diffusive fluxes of water, CH$$_{4}$$, CO$$_{2}$$, O$$_{2}$$, and N$$_{2}$$, saturation degree, water pressure, and mass fraction of each component) over a modeling period of 100 years are presented here.

Journal Articles

Evaluation of high-energy delayed gamma-ray spectra dependence on interrogation timing patterns

Rodriguez, D.; Bogucarska, T.*; Koizumi, Mitsuo; Lee, H.-J.; Pedersen, B.*; Rossi, F.; Takahashi, Toon; Varasano, G.*

Nuclear Instruments and Methods in Physics Research A, 997, p.165146_1 - 165146_13, 2021/05

 Times Cited Count:1 Percentile:0.03(Instruments & Instrumentation)

Journal Articles

Effect of interlayer cations on montmorillonite swelling; Comparison between molecular dynamic simulations and experiments

Yotsuji, Kenji*; Tachi, Yukio; Sakuma, Hiroshi*; Kawamura, Katsuyuki*

Applied Clay Science, 204, p.106034_1 - 106034_13, 2021/04

 Times Cited Count:4 Percentile:97.52(Chemistry, Physical)

JAEA Reports

Investigation and consideration on evaluation of radiation doses to residents in the case of a nuclear emergency

Hashimoto, Makoto; Kinase, Sakae; Munakata, Masahiro; Murayama, Takashi; Takahashi, Masa; Takada, Chie; Okamoto, Akiko; Hayakawa, Tsuyoshi; Sukegawa, Masato; Kume, Nobuhide*; et al.

JAEA-Review 2020-071, 53 Pages, 2021/03

JAEA-Review-2020-071.pdf:2.72MB

In the case of a nuclear accident or a radiological emergency, the Japan Atomic Energy Agency (JAEA), as a designated public corporation assigned in the Disaster Countermeasures Basic Act and the Armed Attack Situation Response Law, undertakes technical supports to the national government and local governments. The JAEA is requested to support to evaluate radiation doses to residents in a nuclear emergency, which is specified in the Basic Disaster Management Plan and the Nuclear Emergency Response Manual. For the dose evaluation, however, its strategy, target, method, structure and so on have not been determined either specifically or in detail. This report describes the results of investigation and consideration discussed in the "Working Group for Radiation Dose Evaluation at a Nuclear Emergency" established within the Nuclear Emergency Assistance and Training Center to discuss technical supports for radiation dose evaluation to residents in the case of a nuclear emergency, and aims at contributing to specific and detailed discussion and activities in the future for the national government and local governments, also within the JAEA.

JAEA Reports

Effective dose coefficients for internal exposure dose assessment in accordance with ICRP 2007 recommendations (Contract research)

Takahashi, Fumiaki; Manabe, Kentaro; Sato, Kaoru

JAEA-Review 2020-068, 114 Pages, 2021/03

JAEA-Review-2020-068.pdf:2.61MB

Radiation safety regulations have been currently established based on the 1990Recommendation by the International Commission on Radiological Protection (ICRP) in Japan. Meanwhile, ICRP released the 2007 Recommendation that replaces the 1990 Recommendation. Thus, the Radiation Council, which is established under the Nuclear Regulation Authority (NRA), has made discussions to incorporate the purpose of the 2007 Recommendation into Japanese regulations for radiation safety. As ICRP also has published effective dose coefficients for internal exposure assessment in accordance with the 2007recommendation, the technical standards are to be revised for the internal exposure assessment method in Japan. Currently, not all of the effective doses have been published to revise concentration limits for internal exposure protections of workers and public. The published effective dose coefficients are applied to radionuclides which are important in radiation protection for internal exposure of a worker. Thus, we review new effective dose coefficients as well as basic dosimetry models and data based upon Occupational Intakes of Radionuclides (OIR) parts 2, 3 and 4 that have been published from 2016 to 2019 by ICRP. In addition, issues are sorted out to provide information for revision of the technical standards for internal exposure assessment based on the 2007 Recommendations in future.

JAEA Reports

Interim activity status report of "the group for investigation of reasonable safety assurance based on graded approach" (from September, 2019 to September, 2020)

Yonomoto, Taisuke; Nakashima, Hiroshi*; Sono, Hiroki; Kishimoto, Katsumi; Izawa, Kazuhiko; Kinase, Masami; Osa, Akihiko; Ogawa, Kazuhiko; Horiguchi, Hironori; Inoi, Hiroyuki; et al.

JAEA-Review 2020-056, 51 Pages, 2021/03

JAEA-Review-2020-056.pdf:3.26MB

A group named as "The group for investigation of reasonable safety assurance based on graded approach", which consists of about 10 staffs from Sector of Nuclear Science Research, Safety and Nuclear Security Administration Department, departments for management of nuclear facility, Sector of Nuclear Safety Research and Emergency Preparedness, aims to realize effective graded approach (GA) about management of facilities and regulatory compliance of JAEA. The group started its activities in September, 2019 and has had discussions through 10 meetings and email communications. In the meetings, basic ideas of GA, status of compliance with new regulatory standards at each facility, new inspection system, etc were discussed, while individual investigation at each facility were shared among the members. This report is compiled with expectation that it will help promote rational and effective safety management based on GA by sharing contents of the activity widely inside and outside JAEA.

JAEA Reports

Analysis of the radioactivity concentrations in low-level radioactive waste generated from JRR-3 and JPDR facilities

Tsuchida, Daiki; Haraga, Tomoko; Tobita, Minoru*; Omori, Hiroyuki*; Omori, Takeshi*; Murakami, Hideaki*; Mitsukai, Akina; Aono, Ryuji; Ishimori, Kenichiro; Kameo, Yutaka

JAEA-Data/Code 2020-022, 34 Pages, 2021/03

JAEA-Data-Code-2020-022.pdf:1.74MB

Radioactive wastes generated from nuclear research facilities in Japan Atomic Energy Agency are planning to be buried in the near surface disposal field. Therefore, it is required to establish the method to evaluate the radioactivity concentrations of radioactive wastes until the beginning of disposal. In order to contribute to this work, we collected and analyzed concrete samples generated from JRR-3 and JPDR. In this report, we summarized the radioactivity concentrations of 22 radionuclides($$^{3}$$H, $$^{14}$$C, $$^{36}$$Cl, $$^{41}$$Ca, $$^{60}$$Co, $$^{63}$$Ni, $$^{90}$$Sr, $$^{94}$$Nb, $$^{rm 108m}$$Ag, $$^{133}$$Ba, $$^{137}$$Cs, $$^{152}$$Eu, $$^{154}$$Eu, $$^{rm 166m}$$Ho, $$^{234}$$U, $$^{238}$$U, $$^{238}$$Pu, $$^{239+240}$$Pu, $$^{241}$$Am, $$^{243}$$Am, $$^{244}$$Cm) which were obtained from radiochemical analysis of the samples.

JAEA Reports

JAEA-TDB-RN in 2020; Update of JAEA's thermodynamic database for solubility and speciation of radionuclides for performance assessment of geological disposal of high-level and TRU wastes

Kitamura, Akira

JAEA-Data/Code 2020-020, 164 Pages, 2021/03

JAEA-Data-Code-2020-020.pdf:3.11MB
JAEA-Data-Code-2020-020-appendix(DVD-ROM).zip:0.56MB

Part of JAEA's Thermodynamic Database (JAEA-TDB) for solubility and speciation of radionuclides (JAEA-TDB-RN) for performance assessment of geological disposal of high-level radioactive and TRU wastes has been updated with subsuming the database for geochemical calculations (JAEA-TDB-GC). This report has focused to update JAEA-TDB-RN after selecting change in standard Gibbs free energy of formation ($$Delta_{rm f}$$$$G^{circ}_{rm m}$$), change in standard enthalpy change of formation ($$Delta$$$$H$$$$^{circ}$$$$_{rm m}$$), standard molar entropy ($$S^{circ}$$$$_{rm m}$$) and, heat capacity ($$C^{circ}_{rm p}$$), change in standard Gibbs free energy of reaction ($$Delta_{rm r}G^{circ}$$$$_{rm m}$$), change in standard enthalpy change of reaction ($$Delta$$$$_{rm r}$$$$H$$$$^{circ}$$$$_{rm m}$$) and standard entropy change of reaction ($$Delta_{rm r}S^{circ}_{rm m}$$) as well as logarithm of equilibrium constant (log$$_{10}$$$$K^{circ}$$) at standard state. The extent of selection of these thermodynamic data enables to evaluate solubility and speciation of radionuclides at temperatures other than 298.15 K. Furthermore, the latest thermodynamic data for iron which have been critically reviewed, selected and compiled by the Nuclear Energy Agency within Organisation for Economic Co-operation and Development (OECD/NEA) have been accepted. Most of previously selected log$$_{10}$$$$K^{circ}$$ have been refined to confirm internal consistency with JAEA-TDB-GC. Text files of the updated JAEA-TDB have been provided for geochemical calculation programs of PHREEQC and Geochemist's Workbench.

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