Role of solute hydrogen on mechanical property enhancement in Fe-24Cr-19Ni austenitic steel; An neutron diffraction study

Ito, Tatsuya; Ogawa, Yuhei*; Gong, W.; Mao, W.*; Kawasaki, Takuro; Okada, Kazuho*; Shibata, Akinobu*; Harjo, S.

Acta Materialia, 287, p.120767_1 - 120767_16, 2025/04

https://doi.org/10.1016/j.actamat.2025.120767

Crystal structures of ReO under hydrostatic pressure; A Combined neutron, X-ray, Raman, and first-principles calculation study

Efthimiopoulos, I.*; Klotz, S.*; Kunc, K.*; Baptiste, B.*; Chauvigne, P.*; Hattori, Takanori

Physical Review B, 111(13), p.134103_1 - 134103_13, 2025/04

https://doi.org/10.1103/PhysRevB.111.134103

We present a comprehensive study of the high pressure behaviour of ReO using X-ray and neutron diffraction, Raman scattering and first-principles calculations to 15 GPa. We show that the ambient pressure structure converts at 0.7 GPa in a continuous phase transition directly to a cubic phase with space group and rhombohedral structures in this pressure range are an artifact due to an alteration of the sample by high-flux synchrotron X-ray radiation. The structural pressure dependence of the O samples are presented. The data shed light onto the unusual transition and densification mechanism due to progressive tilting of essentially rigid ReO octahedra.

Robustness of ferromagnetism in van der Waals magnet FeGeTe to hydrostatic pressure

Wang, Y.*; Zeng, X.-T.*; Li, B.*; Su, C.*; Hattori, Takanori; Sheng, X.-L.*; Jin, W.*

Chinese Physics B, 34(4), p.046203_1 - 046203_6, 2025/03

https://doi.org/10.1088/1674-1056/adb26f

Two-dimensional van der Waals ferromagnet FeGeTe (FGT) holds a great potential for applications in spintronic devices, due to its high Curie temperature, easy tunability, and excellent structural stability in air. In this study, we have performed high-pressure neutron powder diffraction (NPD) up to 5 GPa, to investigate the evolution of its structural and magnetic properties with hydrostatic pressure. The NPD data clearly reveal the robustness of the ferromagnetism in FGT, despite of an apparent suppression by hydrostatic pressure. As the pressure increases from 0 to 5 GPa, the Curie temperature is found to decrease monotonically from 225(5) K to 175(5) K, together with a dramatically suppressed ordered moment of Fe, which is well supported by the first-principles calculations. Although no pressure-driven structural phase transition is observed up to 5 GPa, quantitative analysis on the changes of bond lengths and bond angles indicate a significant modification of the exchange interactions, which accounts for the pressure-induced suppression of the ferromagnetism in FGT.

Development of on-site detection system for concealed nuclear materials

Tanabe, Kosuke*; Komeda, Masao; Toh, Yosuke; Kitamura, Yasunori*; Misawa, Tsuyoshi*

Nihon Genshiryoku Gakkai-Shi ATOMO, 67(3), p.198 - 202, 2025/03

https://doi.org/10.3327/jaesjb.67.3_198

no abstracts in English

Evaluation report for sludge measurement by nondestructive assay (Plutonium Scrap Multiplicity Counter)(Joint research)

Tanigawa, Masafumi; Seya, Kazuhito*; Asakawa, Naoya*; Hayashi, Hiroyuki*; Horigome, Kazushi; Mukai, Yasunobu; Kitao, Takahiko; Nakamura, Hironobu; Henzlova, D.*; Swinhoe, M. T.*; et al.

JAEA-Technology 2024-014, 63 Pages, 2025/02

JAEA-Technology-2024-014.pdf:3.02MB

The liquid waste treatment process generated sludge items at the plutonium conversion development facility. They are highly heterogeneous and contain large amounts of impurities (Na, Fe, Ni etc.). Therefore, the sludge items have very large sampling uncertainty and so the total measurement uncertainty is very large (approximately 24%). The plutonium scrap multiplicity counter (PSMC) measurement technique for sludge items was developed by joint research between the Japan Atomic Energy Agency (JAEA) and Los Alamos National Laboratory (LANL). The technical validity for sludge items using the PSMC was evaluated using various types of sample measurements and Monte Carlo N-Particle transport code calculations. The PSMC measurement parameters were found to be valid for use with sludge items and the validity of multiplicity analysis was confirmed and demonstrated through comparisons with standard MOX powder and a standard sludge. As a result, the PSMC measurement values were shown to be consistent and reasonable and the large amount of impurity (Fe, Ni etc.) did not impact the results. Therefore, the measurement uncertainty of the improved nuclear material accountancy (NMA) procedure by combined PSMC and high-resolution gamma spectrometry was shown to be 6.5%. In addition, an acceptance test was conducted using PSMC/HRGS and IAEA benchmark equipment. Measured Pu mass by both equipment agrees within the measurement uncertainty of each method, and so the validity for Pu mass measurement by PSMC/HRGS was confirmed. The above results confirm the applicability of PSMC/HRGS as an additional NMA method for sludge and a newly designed NDA procedure based on this study is applied to sludge for NMA in PCDF.

Verification of direct coupling code system using FRENDY version 2 and GENESIS for light water reactor lattices

Fujita, Tatsuya; Yamamoto, Akio*

Journal of Nuclear Science and Technology, 62(2), p.179 - 196, 2025/02

https://doi.org/10.1080/00223131.2024.2410918

This study newly established a direct coupling code system consisting of the nuclear data processing code FRENDY version 2, and the three-dimensional heterogeneous transport code GENESIS (FRENDY-V2/GENESIS) for easy implementation of the random-sampling-based uncertainty quantification considering the implicit effect due to nuclear cross-section (XS) perturbations. The multi-group macroscopic XSs prepared for GENESIS were generated by FRENDY version 2, where the Dancoff factor was calculated by the neutron current method. Then the background XSs were evaluated based on the Carlvik two-term rational approximation. The infinite multiplication factor (k-infinity) and the fission reaction rate distribution in UO and MOX lattice geometries were compared with MVP3 to verify the calculation accuracy of FRENDY-V2/GENESIS. The sensitivity analyses on the discretization conditions such as the ray tracing of the method of characteristics were also carried out. Through several comparisons between FRENDY-V2/GENESIS and MVP3, FRENDY-V2/GENESIS with the SHEM 361-group structure calculates the k-infinity within approximately 50 pcm and the fission reaction rate distribution within approximately 0.1% by the root mean square, respectively. Consequently, the applicability of FRENDY-V2/GENESIS was verified, and FRENDY-V2/GENESIS can be used to discuss the implicit effect due to multi-group XS perturbations.

Measurements of neutron capture cross-section for nuclides of interest in decommissioning (III); Er(n,)Er and Hf(n,)Hf reactions

Nakamura, Shoji; Shibahara, Yuji*; Endo, Shunsuke; Rovira Leveroni, G.; Kimura, Atsushi

Journal of Nuclear Science and Technology, 14 Pages, 2025/00

https://doi.org/10.1080/00223131.2025.2457589

Possible criticality scenario and its mechanism of the Windscale Works criticality accident in 1970 analyzed by computational fluid dynamics and Monte Carlo neutron transport

Fukuda, Kodai

Annals of Nuclear Energy, 208(1), p.110748_1 - 110748_10, 2024/12

https://doi.org/10.1016/j.anucene.2024.110748

Application of indentation technique to material degradation evaluation in the mercury target vessel for spallation neutron sources

Wakui, Takashi; Saito, Shigeru; Futakawa, Masatoshi

Jikken Rikigaku, 24(4), p.212 - 218, 2024/12

Irradiation damage is one of the main factors determining the lifetime of the mercury target vessel for spallation neutron source in J-PARC. To understand material degradation of the used vessels, it is planned to conduct an evaluation using inverse analyses with indentation tests on the structural materials of the used vessels and numerical experiments. This evaluation technique was applied to two kinds of ion-irradiated materials with different displacement damage doses, in which the irradiation condition was simulated. It could be confirmed that the ultimate strength increased, and the total elongation decreased with increasing irradiation. These trends are like the material degradation behaviors which have been reported by using small specimen's tensile tests.

Development of a nondestructive assay technique using a laser-driven neutron source

Koizumi, Mitsuo; Ito, Fumiaki*; Lee, J.; Hironaka, Kota; Takahashi, Tone; Suzuki, Satoshi*; Arikawa, Yasunobu*; Abe, Yuki*; Wei, T.*; Yogo, Akifumi*; et al.

Dai-45-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2024/11