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Takeuchi, Tetsuya*; Honda, Fuminori*; Aoki, Dai*; Haga, Yoshinori; Kida, Takanori*; Narumi, Yasuo*; Hagiwara, Masayuki*; Kindo, Koichi*; Karube, Kosuke*; Harima, Hisatomo*; et al.
Journal of the Physical Society of Japan, 93(4), p.044708_1 - 044708_10, 2024/04
Motegi, Kosuke; Shibamoto, Yasuteru; Kukita, Yutaka
Annals of Nuclear Energy, 184, p.109679_1 - 109679_10, 2023/05
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)Kitaori, Aki*; Kanazawa, Naoya*; Kida, Takanori*; Narumi, Yasuo*; Hagiwara, Masayuki*; Kindo, Koichi*; Takeuchi, Tetsuya*; Nakamura, Ai*; Aoki, Dai*; Haga, Yoshinori; et al.
Journal of the Physical Society of Japan, 92(2), p.024702_1 - 024702_6, 2023/02
Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)Motegi, Kosuke; Shibamoto, Yasuteru; Kukita, Yutaka
Journal of Nuclear Science and Technology, 59(8), p.1037 - 1046, 2022/08
Times Cited Count:3 Percentile:68.71(Nuclear Science & Technology)Inagawa, Jun; Kitatsuji, Yoshihiro; Otobe, Haruyoshi; Nakada, Masami; Takano, Masahide; Akie, Hiroshi; Shimizu, Osamu; Komuro, Michiyasu; Oura, Hirofumi*; Nagai, Isao*; et al.
JAEA-Technology 2021-001, 144 Pages, 2021/08
Plutonium Research Building No.1 (Pu1) was qualified as a facility to decommission, and preparatory operations for decommission were worked by the research groups users and the facility managers of Pu1. The operation of transportation of whole nuclear materials in Pu1 to Back-end Cycle Key Element Research Facility (BECKY) completed at Dec. 2020. In the operation included evaluation of criticality safety for changing permission of the license for use nuclear fuel materials in BECKY, cask of the transportation, the registration request of the cask at the institute, the test transportation, formulation of plan for whole nuclear materials transportation, and the main transportation. This report circumstantially shows all of those process to help prospective decommission.
Okutani, Akira*; Onishi, Hiroaki; Kimura, Shojiro*; Takeuchi, Tetsuya*; Kida, Takanori*; Mori, Michiyasu; Miyake, Atsushi*; Tokunaga, Masashi*; Kindo, Koichi*; Hagiwara, Masayuki*
Journal of the Physical Society of Japan, 90(4), p.044704_1 - 044704_9, 2021/04
Times Cited Count:3 Percentile:30.35(Physics, Multidisciplinary)Takeuchi, Tetsuya*; Haga, Yoshinori; Taniguchi, Toshifumi*; Iha, Wataru*; Ashitomi, Yosuke*; Yara, Tomoyuki*; Kida, Takanori*; Tahara, Taimu*; Hagiwara, Masayuki*; Nakashima, Miho*; et al.
Journal of the Physical Society of Japan, 89(3), p.034705_1 - 034705_15, 2020/03
Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)Takeuchi, Tetsuya*; Yara, Tomoyuki*; Ashitomi, Yosuke*; Iha, Wataru*; Kakihana, Masashi*; Nakashima, Miho*; Amako, Yasushi*; Honda, Fuminori*; Homma, Yoshiya*; Aoki, Dai*; et al.
Journal of the Physical Society of Japan, 87(7), p.074709_1 - 074709_14, 2018/07
Times Cited Count:12 Percentile:64.96(Physics, Multidisciplinary)Iha, Wataru*; Yara, Tomoyuki*; Ashitomi, Yosuke*; Kakihana, Masashi*; Takeuchi, Tetsuya*; Honda, Fuminori*; Nakamura, Ai*; Aoki, Dai*; Gochi, Jun*; Uwatoko, Yoshiya*; et al.
Journal of the Physical Society of Japan, 87(6), p.064706_1 - 064706_14, 2018/06
Times Cited Count:19 Percentile:75.67(Physics, Multidisciplinary)Kobayashi, Fuyumi; Sumiya, Masato; Kida, Takashi; Kokusen, Junya; Uchida, Shoji; Kaminaga, Jota; Oki, Keiichi; Fukaya, Hiroyuki; Sono, Hiroki
JAEA-Technology 2016-025, 42 Pages, 2016/11
A preliminary test on MOX fuel dissolution for the STACY critical experiments had been conducted in 2000 through 2003 at Nuclear Science Research Institute of JAEA. Accordingly, the uranyl / plutonium nitrate solution should be reconverted into oxide powder to store the fuel for a long period. For this storage, the moisture content in the oxide powder should be controlled from the viewpoint of criticality safety. The stabilization of uranium / plutonium solution was carried out under a precipitation process using ammonia or oxalic acid solution, and a calcination process using a sintering furnace. As a result of the stabilization operation, recovery rate was 95.6% for uranium and 95.0% for plutonium. Further, the recovered oxide powder was calcined again in nitrogen atmosphere and sealed immediately with a plastic bag to keep its moisture content low and to prevent from reabsorbing atmospheric moisture.
Sugiyama, Kiyohiro*; Hirose, Yusuke*; Enoki, Kentaro*; Ikeda, Shugo*; Yamamoto, Etsuji; Tateiwa, Naoyuki; Haga, Yoshinori; Kida, Takanori*; Hagiwara, Masayuki*; Kindo, Koichi*; et al.
Journal of the Physical Society of Japan, 80(Suppl.A), p.SA104_1 - SA104_3, 2011/07
Times Cited Count:3 Percentile:27.54(Physics, Multidisciplinary)Ishii, Junichi; Kobayashi, Fuyumi; Uchida, Shoji; Sumiya, Masato; Kida, Takashi; Shirahashi, Koichi; Umeda, Miki; Sakuraba, Koichi
JAEA-Technology 2009-068, 20 Pages, 2010/03
At Nuclear Fuel Cycle Safety Engineering Research Facility, the cerium mediated electrolytic oxidation method which is a decontamination technique to decrease the radioactivity of TRU wastes to the clearance-level has been developed for the effective reduction of TRU wastes generated from the decommissioning of a nuclear fuel reprocessing facility and so on. This method corrodes the oxide layer and the surface of metallic TRU metal wastes by the strong oxidation power of Ce in nitric acid. In this study, parameter tests were conducted to optimize the solution condition of Ce initial concentrations and nitric acid concentrations. The target corrosion rate of metallic TRU wastes set to be 24m/h for the practical use of this method. Under the optimized solution condition, a dissolution test of stainless steel simulating wastes was carried out. From the result of the dissolution test, the average corrosion rate was 3.3 m/h during the test time of 90 hours. Based on the supposition that the corrosion depth of metallic TRU wastes was 20 m enough to achieve the clearance-level, the treatment time for the decontamination was about 6 hours. It was confirmed from the result that the decontamination could be performed within one day and the decontamination solution could repeatedly reuse 15 times.
Sugikawa, Susumu; Nakazaki, Masato; Kimura, Akihiro; Kida, Takashi*; Kihara, Takehiro*; Akabori, Mitsuo; Minato, Kazuo; Suda, Kazuhiro*; Chikazawa, Takahiro*
Nihon Genshiryoku Gakkai Wabun Rombunshi, 6(4), p.476 - 483, 2007/12
A one-step simple extraction chromatography method using TODGA (-tetraoctyl-diglycolamide) adsorbent column has been developed to separate the americium from plutonium-solvent extraction raffinate. The raffinate contained Am(620 mg/), Np(107 mg/), Ag(2000 mg/), Fe(290 mg/), Cr(38 mg/), Ni(52 mg/) and trace of TBP. Small-scale and scale-up tests for separation of americium and conversion to americium oxide were carried out in NUCEF. Efforts were made to increase yield and purity of americium. The americium was separated with 83-92% yields and 97-98% purities by small-scale tests and 85-95% yields and 98-99% purities by scale-up tests. The yields for conversion of americium nitrate solution to americium oxide were 89-100% by small-scale tests and 85-96 % by scale-up tests. Approximately 1.8 gram americium oxide was recovered from 6 litres of the raffinate and supplied for the research on the high-temperature chemistry of TRU.
Kokusen, Junya; Seki, Masakazu; Abe, Masayuki; Nakazaki, Masato; Kida, Takashi; Umeda, Miki; Kihara, Takehiro; Sugikawa, Susumu
JAERI-Tech 2005-004, 53 Pages, 2005/03
This report presents operating records of dissolution of uranium dioxide and concentration of uranyl nitrate solution and acid removal, which have been performed from 1994 through 2003, for the purpose of feeding 10% and 6% enriched uranyl nitrate solution fuel to Static Experimental Critical Facility(STACY) and Transient Experimental Critical Facility(TRACY) in Nuclear Fuel Safety Engineering Facility(NUCEF).
Kida, Takashi; Sugikawa, Susumu
JAERI-Tech 2004-019, 30 Pages, 2004/03
It is known that hydrazine nitrate used in nuclear fuel reprocessing plants is an unstable substance thermochemically like hydroxylamine nitrate. In order to take the basic data regarding the reaction of hydrazine nitrate with nitric acid, initiation temperatures and heats of this reaction, effect of impurity on initiation temperature and self-accelerating reaction when it holds at constant temperature for a long time were measured by the pressure vessel type reaction calorimeter etc. In this paper, the experimental data and evaluation of the safe handling of hydrazine nitrate in nuclear fuel reprocessing plants are described.
Haga, Katsuhiro; Kinoshita, Hidetaka; Kaminaga, Masanori; Hino, Ryutaro; Tagawa, Hisato*; Kukita, Yutaka*
Proceedings of 11th International Conference on Nuclear Engineering (ICONE-11) (CD-ROM), 8 Pages, 2003/04
The cross-flow type mercury target, in which mercury flows crossing the proton beam path, has been developed as the spallation target of the material and life science facility in the high intensity proton accelerator project. As a part of design optimization, we proposed a mercury target using perforated plates aiming to simplify the inner structure, to make the target assembling easier, and to decrease the assembling cost. Then, the effectiveness of the target structure was investigated by no-heat water experiments and computational analyses. A mockup model of the cross-flow type mercury target using perforated plates was fabricated with plexi-glass and the water flow field was measured using PIV technique and the results were compared with the analytical results. The cross-flow field was realized by perforated plates and the analytical results corresponded well with the experimental results in the proton beam path where the cooling of heat generation is important.
Umeda, Miki; Nakazaki, Masato; Kida, Takashi; Sato, Kenji; Kato, Tadahito; Kihara, Takehiro; Sugikawa, Susumu
JAERI-Tech 2003-024, 23 Pages, 2003/03
MOX dissolution with silver mediated electrolytic oxidation method is planned for the preparation of plutonium nitrate solution to be used for criticality safety experiments at Nuclear Fuel Cycle Safety Engineering Research Facility (NUCEF). Silver mediated electrolytic oxidation method uses the strong oxidisation ability of Ag(II) ion. This method is thought to be effective for the dissolution of MOX, which is difficult to be dissolved with nitric acid.In this paper, the results of experiments on dissolution with 100 g of MOX are described. It was confirmed by the results that the MOX powder to be used at NUCEF was completely dissolved by silver mediated electrolytic oxidation method and that Pu(VI) ion in the obtained solution was reduced to tetravalent by means of NO purging.
Kida, Takashi; Umeda, Miki; Sugikawa, Susumu
JAERI-Data/Code 2003-001, 29 Pages, 2003/03
MOX dissolution using silver-mediated electrochemical method will be employed for the preparation of plutonium nitrate solution in the criticality safety experiments in NUCEF. A simulation code for the MOX dissolution has been developed for the operating support. In this report an outline of the simulation code is proposed and a comparison with the experimental data and a parameter study on the MOX dissolution rate are described.The principle of this code is based on Zundelevich's model for PuO dissolution using Ag. The influence of nitrous acid on the material balance of Ag and the surface area of MOX powder on the basis of particle size distribution are taken into consideration in this model. A comparison with experimental data was carried out to confirm a validity of this model. It was confirmed that the behavior of MOX dissolution could adequately be simulated using the appropriate MOX dissolution rate constant. The parameters affecting the dissolution rate were studied, it was found that MOX particle size was major governing factor on the dissolution rate.
Yonomoto, Taisuke; *; *; Anoda, Yoshinari; Kukita, Yutaka; ; Ito, Hideo; Osaki, Hideki; ; Nishikizawa, Tomotoshi; et al.
JAERI-M 94-069, 145 Pages, 1994/03
no abstracts in English
Kukita, Yutaka; Nakamura, Hideo; *; *; *; Anoda, Yoshinari; Kumamaru, Hiroshige; Suzuki, Mitsuhiro; ; Yonomoto, Taisuke; et al.
JAERI-M 91-040, 122 Pages, 1991/03
no abstracts in English