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Mochizuki, Akihito; Matsui, Hiroya; Nakayama, Masashi; Sakamoto, Ryo*; Shibata, Masahito*; Motoshima, Takayuki*; Jo, Mayumi*
Case Studies in Construction Materials, 22, p.e04648_1 - e04648_20, 2025/07
Times Cited Count：0The properties of low-pH cement used in the geological disposal of radioactive waste may change through atmospheric carbonation and degradation caused by groundwater during the long-term operation of a repository. In this study, we investigated the effects of atmospheric carbonation and groundwater contact on the chemical, microstructural, and transport properties of shotcrete made from low-pH, high-fly-ash silica-fume cement (HFSC) over a period of 16 years in an underground research laboratory. In both carbonated and degraded zones of the HFSC shotcrete, capillary porosity increased for pores of 
300 nm in diameter, and the total porosity was higher than in undegraded zones. These changes in porosity may be associated with the decalcification of calcium-silicate-hydrate and decomposition of ettringite. Such changes were minor in altered zones of OPC shotcrete, indicating that HFSC shotcrete is less resistant to atmospheric carbonation and groundwater leaching under the studied conditions. However, the hydraulic conductivity in HFSC was low enough to fulfill the specific functional requirements of low-pH cements for geological disposal.
Kinoshita, Junichi; Sakamoto, Yu; Suzuki, Ichiro; Nakajima, Ryota; Morita, Yusuke; Irie, Hirobumi
JAEA-Technology 2024-027, 55 Pages, 2025/05
JAEA-Technology-2024-027.pdf:8.49MB
The Waste Treatment Facility No.2 has equipment that can process solid waste with relatively high radioactive levels generated within the Japan Atomic Energy Agency. This facility had been constructed under the old Building Standards Act. Seismic evaluation based on a new regulatory requirements enforced in December 2013 was executed, thereby, it was found that the seismic resistance requirements was insufficient according to the current Building Standards Act. Therefore, seismic reinforcement works was carried out from November 2018 to February 2020. In this report, seismic reinforcement design, works, test and inspection was complied.
Wilson, J.*; Sasamoto, Hiroshi; Tachi, Yukio; Kawama, Daisuke*
Applied Clay Science, 275, p.107862_1 - 107862_15, 2025/05
Times Cited Count：0High-Level Radioactive Waste (HLW) repositories include iron or steel-based containers/overpack and bentonite buffers. Over the last 25 years or so, research efforts have attempted to elucidate the nature of iron-bentonite interactions, especially the potential for the deleterious alteration of the swelling clay component (smectite), to iron-rich layer silicates, some of which lack the capacity for intracrystalline swelling. This could result in a reduction or loss in swelling pressure in the bentonite buffer which is designed to protect waste containers from shear forces and also acts to restrict water and solute transport, as part of an engineered barrier system. Most data on iron-bentonite interactions come from experimental and geochemical modelling studies, as natural analogue data are lacking. The data suggests that there is the potential for the development of an iron-rich bentonite alteration zone with smectite (generally present as the aluminous montmorillonite type) undergoing alteration to iron-rich solids, including layer silicates and steel corrosion products such as green rust or magnetite. The evidence available is complex, arguably incomplete, with many potential complex couplings. Many uncertainties remain despite efforts taken over the last 25 years, but plausible scenarios for iron-bentonite interactions have been identified and possible implications for buffer properties have been suggested.
Arai, Yoichi; Watanabe, So; Nakahara, Masaumi; Funakoshi, Tomomasa; Hoshino, Takanori; Takahatake, Yoko; Sakamoto, Atsushi; Aihara, Haruka; Hasegawa, Kenta; Yoshida, Toshiki; et al.
Progress in Nuclear Science and Technology (Internet), 7, p.168 - 174, 2025/05
The Japan Atomic Energy Agency (JAEA) has been conducting a project named "Systematic Treatment of RAdioactive liquid waste for Decommissioning (STRAD)" project since 2018 for fundamental and practical studies for treating radioactive liquid wastes with complicated compositions. Fundamental studies have been conducted using genuine liquid wastes accumulated in a hot laboratory of the JAEA called the Chemical Processing Facility (CPF), and treatment procedures for all liquid wastes in CPF were successfully designed on the results obtained. As the next phase of the project, new fundamental and practical studies on primarily organic liquid wastes accumulated in different facilities of JAEA are in progress. This paper reviews the representative achievements of the STRAD project and introduces an overview of ongoing studies.
Nagata, Shohei*; Ichida, Toshiyuki*; Fujieda, Daigo; Aoyagi, Kazuhei
Tunnelling into a Sustainable Future; Methods and Technologies; Proceedings of the ITA-AITES World Tunnel Congress 2025 (WTC 2025), p.3517 - 3524, 2025/05
We performed three-dimensional excavation analysis of three shafts and intersection of horizontal tunnel excavated to 500 m depth at Horonobe URL, and evaluated stress acting on concrete lining under various conditions such as differences in diameter of shafts, lining shape, lining thickness, concrete strength, and installation interval of the lining. The design of the support was determined based on the analysis results, and then the construction of the shafts and horizontal galleries were started. Considering the measured stress acting on the concrete lining of the shaft and sprayed mortar installed at the intersection of shaft and horizontal gallery, we could successfully excavate the shaft to 500 m depth and intersection of horizontal gallery at 420 m depth. We also concluded that appropriate support pattern can be selected based on the measured stress acting on the concrete lining and numerical analysis performed prior to the excavation. This can contribute to enhance the reliability of the appropriate observational construction technology targeting excavation of shaft.
Meigo, Shinichiro; Iwamoto, Hiroki; Sugihara, Kenta*; Hirano, Yukinori*; Tsutsumi, Kazuyoshi*; Saito, Shigeru; Maekawa, Fujio
JAEA-Technology 2024-026, 123 Pages, 2025/03
JAEA-Technology-2024-026.pdf:14.22MB
Based on the design of the ADS Target Test Facility (TEF-T) at the J-PARC Transmutation Experimental Facility, a conceptual study was conducted on the J-PARC proton beam irradiation facility. This research was carried out based on the recommendations of the Nuclear Transmutation Technology Evaluation Task Force of the MEXT. The recommendations state that it is desirable to consider facility specifications that can make the most of the benefits of using the existing J-PARC proton accelerator while also solving the engineering issues of the ADS. We considered facilities that could respond to a variety of needs while reducing the facilities that were not needed in the TEF-T design. In order to clarify these diverse needs, we investigated the usage status of representative accelerator facilities around the world. As a result, it became clear that the main purposes of these facilities were (1) Material irradiation, (2) Soft error testing of semiconductor devices using spallation neutrons, (3) Production of RI for medical use, and (4) Proton beam use, and we investigated the facilities necessary for these purposes. In considering the facility concept, we assumed a user community in 2022 and reflected user opinions in the facility design. This report summarizes the results of the conceptual study of the proton irradiation facility, various needs and responses to them, the roadmap for facility construction, and future issues.
Emori, Tatsuya; Kitatsuji, Yoshihiro; Ban, Yasutoshi
JAEA-Technology 2024-025, 20 Pages, 2025/03
JAEA-Technology-2024-025.pdf:1.65MB
Radioisotope Thermoelectric Generators (RTGs) using the decay heat of Pu-238 has been applied for outer planet missions far from Jupiter, where solar power is limited. However, no facilities are available to produce Pu-238 for space probes in Japan. Moreover, the use of nuclear materials for the space exploration is difficult in term of the regulation. Thus, we focused on Am-241 whose half-life is around 432 years as an alternative heat source for RTGs. This report describes the procedure of separating Am-241 decayed from Pu-241 in aged plutonium oxide. Two experiments were performed: one using solid-liquid extraction and the other combining liquid-liquid extraction and solid-liquid extraction. Packed columns were used in the experiments, with their number reduced by less than one-fifth in the latter experiment compared to the former. Furthermore, the time required for separation in the latter experiment was less than half that of the former. We performed the separation experiments six times, collecting a total of approximately 0.43 g of Am-241 as an oxalate salt.
Asahi, Yoshimitsu; Fukuda, Shigeki; Shiramizu, Daiki; Miyata, Koshi; Tone, Masaya; Katsuoka, Nanako; Maeda, Yuta; Aoyama, Yusuke; Niitsuma, Koichi; Kobayashi, Hidekazu; et al.
JAEA-Technology 2024-024, 271 Pages, 2025/03
JAEA-Technology-2024-024.pdf:33.98MB
JAEA-Technology-2024-024-hyperlink.zip:31.96MB
A glass melter for the vitrification process of highly active liquid waste in the Tokai Reprocessing Plant, TVF's 3rd melter, was built, and the glass of 18 vitrified waste canisters in weight was melted and poured through a cold test operation. The molten glass surface was covered by a cold cap from feeding fiberglass cartridges saturated with non-radioactive simulant liquid waste as raw material, whose components are equivalent to actual waste. Differences in inherent characteristics of the thermal behavior between the 2nd and the 3rd melter due to the difference in design were considered to establish the procedure to control the new melter. The melter's condition was stabilized at a higher glass temperature and the cooling of 1 kW less in each of the two main electrodes, compared to the 2nd one. Under 39 kW joule heating of the main electrodes with 26 Nm3/h coolant flow rate, it showed the capability to finish heating the bottom furnace in 5 hours before pouring, 2 hours shorter than the 2nd melter. Measurements of the temperature distributions in molten glass and casing surface yielded data that is efficient for developing a simulation model. After Platinum Group Elements (PGE) concentration saturates in the molten glass, feeding raw material and discharging glass were suspended to examine a holding state, indicating PGE settling could retard. During the holding test, observation of the melting process of the cold cap declared that the surface was covered by a thin layer with almost non-fluidity. It will be a reason for choosing the no-slip condition of a fluid calculation, even in the hot-top condition. The investigation of PGE discharging behavior by analyzing the elemental composition of poured glass showed the accumulated PGE amount in the 3rd melter is small compared to the 2nd melter. Inspection of the melter inside after draining out concluded that there were neither significant residual glass nor refractory fragments.
Tomioka, Dai; Kochiyama, Mami; Ozone, Kenji; Nakata, Hisakazu; Sakai, Akihiro
JAEA-Technology 2024-023, 38 Pages, 2025/03
JAEA-Technology-2024-023.pdf:1.54MB
Japan Atomic Energy Agency is an implementing organization of near-surface disposal for low-level radioactive wastes generated from research, industrial and medical facilities in Japan. Information on the radioactivity concentration of these radioactive wastes is dispensable for the design and conformity assessment of the waste disposal facilities for the licensing application of the disposal project and its safety review. Radioactive Wastes Disposal Center has been improving the radioactivity evaluation procedure for the dismantling waste generated from the research reactors based on the activation calculation. In order to investigate the applicability of the ORIGEN code (included in SCALE6.2.4), which enables more accurate activation calculations using multigroup neutron spectra, we performed activation calculations with the ORIGEN-code and the ORIGEN-S code (included in SCALE6.0), which has been widely used in the past, for the dismantled wastes from the Rikkyo University Research Reactor, where radioactivity analysis data for the structural materials around the reactor core were compiled. As a result, the calculation time difference between ORIGEN and ORIGEN-S was small and the evaluated radioactivity concentrations of the former were in the range of 0.8-1.0 times those of the latter, which was in good agreement with those of radiochemical analysis in the range of 0.5-3.0 times. The applicability of ORIGEN was confirmed. In addition, activation calculations assuming trace elements in structural materials of nuclear reactor were performed with ORIGEN and ORIGEN-S and the results were compared. The causes of the large differences among 170 nuclides that are important for dose assessment in near-surface disposal were assessed each nuclide.
Kokubu, Yoko; Takeuchi, Ryuji; Nishio, Kazuhisa*; Ikeda, Koki
JAEA-Review 2024-066, 67 Pages, 2025/03
JAEA-Review-2024-066.pdf:8.25MB
The Tono Geoscience Center of the Japan Atomic Energy Agency has undertaken backfilling and restoration activities at the Mizunami Underground Research Laboratory (MIU) site since fiscal year 2020. These activities are being conducted in accordance with "The MIU Project from FY2020 Onwards," outlining the procedures for backfilling, restoration, and environmental monitoring at the MIU site. The backfilling activity was completed in January 2022, and thereafter, the observation of the backfilled shafts was commenced. On November 6, 2023, the settlement of the backfilled surface was observed in the Main Shaft and the Ventilation Shaft. By December 5, 2023, the depth of the settlement reached 12.9 m in the Main Shaft and 27.7 m in the Ventilation Shaft. After an evaluation by the MIU safety confirmation committee, which assessed the settlement condition and recommended countermeasures, the affected areas were backfilled for safety reasons. This report summarizes the observed settlement of the backfilled surface, the subsequent rebackfilling efforts, and the condition of the surface settlement areas. The condition of the backfilled sections has been confirmed up to June 2024.
Taniguchi, Takumi; Matsumoto, Saori; Hiraki, Yoshihisa; Sato, Junya; Fujita, Hideki*; Kaneda, Yoshihisa*; Kuroki, Ryoichiro; Osugi, Takeshi
JAEA-Review 2024-059, 20 Pages, 2025/03
JAEA-Review-2024-059.pdf:1.0MB
The basic performance required for solidifying waste into cement, such as fluidity before curing and strength after curing, is expected to be affected by the chemical effects of substances and components contained in the waste. The fluidity before curing and the strength properties after curing are greatly influenced by the curing speed of the cement. We investigated existing knowledge with a focus on chemical substances that affect the curing speed of cement. In this report, chemical substances that affect fluidity are broadly classified into inorganic substances such as (1) anion species, (2) metal elements such as heavy metals, (3) inorganic compounds as cement admixtures, and (4) organic compounds as cement admixtures. Based on the investigation, we actually added chemicals and measured the setting time. As a result, it was found that there are multiple mechanisms contributing to accelerated hardening. We investigated chemical substances that inhibit the curing reaction of cement, and were able to compile information to consider ingredients that are contraindicated in cement curing.
Ningyo-toge Environmental Engineering Center
JAEA-Review 2024-050, 55 Pages, 2025/03
JAEA-Review-2024-050.pdf:3.57MB
This report outlines some main research and development activities executed by the Ningyo-toge Environmental Engineering Center in FY2023. The Center was working on the development of the nuclear fuel cycle with a focus on its frontend (i.e., uranium exploration, mining, refining, conversion, and enrichment) until 2001, and is now dismantling and removing the facilities and equipment used in the past. In addition, based on the concept of "Uranium and environmental research platform" announced in 2016, we are also working on research and development for the safe processing and disposal of uranium wastes. This research and development can be mainly divided into "Environmental research" and "Uranium waste engineering research"; the former takes advantage of the characteristics of the natural environment in Ningyo-toge, and the latter utilizes our facilities and potentials. Some works are also made on safety and its management as well as radiation effect research in terms of health physics and radiobiology. Regarding the environmental research and environmental conservation, this report describes research on the heterogeneity of groundwater in granitic mountains and the fundamentals and applications of the partitioning of trace elements into minerals. As for the uranium waste engineering research, the laser-based decontamination technique and the corrosion resistance suitable for waste package material are reported. Further, the progress of safeguards activities at the uranium enrichment facility, the construction of safety measures at the mill tailings ponds, and the risk and biological effects of radon are also reported. The achievements of those works have been widely presented through research papers etc.
Nuclear Backend Technology Development
JAEA-Evaluation 2024-002, 86 Pages, 2025/03
JAEA-Evaluation-2024-002.pdf:8.29MB
Japan Atomic Energy Agency (hereinafter referred to as "JAEA") consulted the "Evaluation Committee on Research and Development Activities for Decommissioning" (hereinafter referred to as "Committee") about the in-advance evaluation of research themes which had started after FY2021 of R&D plan for the 4th medium- and long-term objectives period concerning "Decommissioning of nuclear facilities and development of technologies for the treatment of related radioactive waste" project in accordance with the "Guideline for evaluation of government R&D activities". In response, the Committee evaluated to the evaluation points of view made by JAEA.
Nagata, Hiroshi; Kochiyama, Mami; Chinone, Marina; Sugaya, Naoto; Nishimura, Arashi; Ishikawa, Joji; Sakai, Akihiro; Ide, Hiroshi
JAEA-Data/Code 2024-016, 44 Pages, 2025/03
JAEA-Data-Code-2024-016.pdf:3.54MB
The elemental composition of the structural materials of nuclear reactor facilities is used as one of the important parameters in activation calculations that are evaluated when formulating decommissioning plans. Regarding the elemental composition of aluminum alloys and other materials used as structural materials for test and research reactors, sufficient data is not available regarding elements other than the major elements. For this reason, samples were collected from aluminum alloy, beryllium, hafnium, and other materials that have been used as the main structural materials of JMTR (Japan Materials Testing Reactor), and their elemental compositions were analyzed. This report summarizes the elemental composition data of 78 elements obtained in FY2023.
Fujita, Natsuko; Miyake, Masayasu; Matsubara, Akihiro*; Ishii, Masahiro*; Jinno, Satoshi; Watanabe, Takahiro; Nishio, Tomohiro*; Ogawa, Yumi; Omae, Akiomi*; Kimura, Kenji; et al.
Dai-36-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.90 - 92, 2025/03
The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has three accelerator mass spectrometers. We report the present status of the JAEA-AMS-TONO.
Matsubara, Akihiro*; Fujita, Natsuko; Miyake, Masayasu; Ishii, Masahiro*; Omae, Akiomi*; Maeta, Yusuke; Uno, Sadanori*
Dai-36-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.125 - 129, 2025/03
We will report on the maintenance and management of JAEA-AMS-TONO-5MV (NEC 15SDH-2, maximum terminal voltage 5.0 MV) located at the Toki Geochronology Research Institute, Tono Geoscience Center, Japan Atomic Energy Agency; (1) Regarding damage to varistors in beamline equipment and its causes, (2) Phenomena that suggest a vacuum leak in the accelerator tube of a tandem accelerator and its countermeasures.
Kim, M.*; Lee, C.*; Sugita, Yutaka; Kim, J.-S.*; Jeon, M.-K.*
Geomechanics for Energy and the Environment, 41, p.100628_1 - 100628_9, 2025/03
Times Cited Count：0 Percentile：0.00(Energy & Fuels)This study investigates the impact of primary variables selection on the modeling of non-isothermal two-phase flow, by using the numerical work on the full-scale Engineered Barrier System (EBS) experiment conducted at Horonobe URL as part of the DECOVALEX-2023 project. A validated numerical model is employed to simulate the coupled thermo-hydrological behavior of heterogeneous porous media within the EBS. Two different primary variable schemes are compared in discretizing the governing equations, revealing significant difference in results.
Ono, Hirokazu; Takayama, Yusuke*
Geomechanics for Energy and the Environment, 41, p.100636_1 - 100636_14, 2025/03
Times Cited Count：0 Percentile：0.00(Energy & Fuels)Osawa, Hideaki
Gijutsushi "Chubu", (15), p.40 - 47, 2025/03
This paper introduces the history of the development of borehole investigation techniques at the Tono Geoscience Center of the Japan Atomic Energy Agency (JAEA), which started in 1986, as one of the research of geological environmental characteristics.
Masuki, Yuma*; Katsuta, Nagayoshi*; Naito, Sayuri*; Murakami, Takuma*; Umemura, Ayako*; Fujita, Natsuko; Matsubara, Akihiro*; Minami, Masayo*; Niwa, Masakazu; Yoshida, Hidekazu*; et al.
Journal of Hazardous Materials, 485, p.136843_1 - 136843_10, 2025/03
Times Cited Count：0 Percentile：0.00(Engineering, Environmental)Lacustrine deposits have 30-fold higher As abundance than the average crustal deposit. Arsenic is mostly concentrated as discrete horizons deposited in spring and autumn. As-rich layers contain FeAsS, AsS, and As
S
but As-rich hotspots mostly contain FeAsS. As accumulation to sediment is controlled by redox potential with organic matter.
