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Sb
uncovered by soft X-ray magnetic circular dichroismSaito, Yuji; Fujiwara, Hidenori*; Yasui, Akira*; Kadono, Toshiharu*; Sugawara, Hitoshi*; Kikuchi, Daisuke*; Sato, Hideyuki*; Suga, Shigemasa*; Yamasaki, Atsushi*; Sekiyama, Akira*; et al.
Physical Review B, 102(16), p.165152_1 - 165152_8, 2020/10
Nagai, Takayuki; Okamoto, Yoshihiro; Akiyama, Daisuke*; Uehara, Akihiro*; Fujii, Toshiyuki*; Sekimoto, Shun*
KURNS Progress Report 2019, P. 257, 2020/08
To understand the influence of glass structural change by neutron irradiation and boron isotope composition, glass samples were made from enrichment boric acid reagents and neutron irradiation of those samples was carried out in Pn-2 of KUR. The structural change of glass sample after the irradiation will be estimated in 2020FY. Before neutron irradiation test of glass samples, the Si-O bridging structure difference by boron isotope composition compared by using a Raman spectrometry.
Si
O
Suzuki, Eriko; Nakajima, Kunihisa; Osaka, Masahiko; Oishi, Yuji*; Muta, Hiroaki*; Kurosaki, Ken*
Journal of Nuclear Science and Technology, 57(7), p.852 - 857, 2020/07
Times Cited Count：0 Percentile：100(Nuclear Science & Technology)The low temperature heat capacity of CsSiO, which is one of the cesium chemisorbed compounds onto stainless steel during severe accident of the light water nuclear reactor, was experimentally determined for the first time in the temperature range of 1.9 - 302 K. The experimentally determined heat capacity, 
(298.15K), and the standard entropy, 
(298.15K), were 249.4 
1.1 J K
mol and 322.1 1.3 J K mol, respectively. The standard Gibbs energy of formation of CsSiO at high temperatures, 
(
), were reevaluated by using the presently obtained (298.15K) and the previously reported experimental results of the standard enthalpy of formation, 
(298.15K), and the standard enthalpy increments at high temperatures, ()- (298.15K).
and EuAu with the characteristic hexagonal structureMatsuda, Shinya*; Ota, Joji*; Nakaima, Kenri*; Iha, Wataru*; Gochi, Jun*; Uwatoko, Yoshiya*; Nakashima, Miho*; Amako, Yasushi*; Honda, Fuminori*; Aoki, Dai*; et al.
Philosophical Magazine, 100(10), p.1244 - 1257, 2020/04
Times Cited Count：1 Percentile：100(Materials Science, Multidisciplinary)
Si single crystal grown by the flux methodTakeuchi, Tetsuya*; Haga, Yoshinori; Taniguchi, Toshifumi*; Iha, Wataru*; Ashitomi, Yosuke*; Yara, Tomoyuki*; Kida, Takanori*; Tahara, Taimu*; Hagiwara, Masayuki*; Nakashima, Miho*; et al.
Journal of the Physical Society of Japan, 89(3), p.034705_1 - 034705_15, 2020/03
Times Cited Count：0 Percentile：100(Physics, Multidisciplinary)Kim, J.*; Yamanaka, Satoru*; Murayama, Ichiro*; Kato, Takanori*; Sakamoto, Tomokazu*; Kawasaki, Takuro; Fukuda, Tatsuo; Sekino, Toru*; Nakayama, Tadachika*; Takeda, Masatoshi*; et al.
Sustainable Energy & Fuels (Internet), 4(3), p.1143 - 1149, 2020/03
Times Cited Count：2 Percentile：32.54(Chemistry, Physical)Collaborative Laboratories for Advanced Decommissioning Science; Osaka University*
JAEA-Review 2019-029, 36 Pages, 2020/02
JAEA-Review-2019-029.pdf:2.33MB
JAEA/CLADS, had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. The Project aims to contribute to solving problems in nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of Gel Filler that Facilitates Fuel Debris Retrieval". When gel materials such as polymer, silicate and clay minerals with adjusted viscosity are used in the process of debris retrieval, the gel would not leak down from the damaged parts, resulting in the reduction of surrounding air dose rate. In addition, gel materials can reduce the diffusion and scattering of dust that is produced by cutting. For these reasons, we propose a method where inside of a containment vessel is filled by gel materials in order to simplify the debris retrieval.
Onuki, Yoshichika*; Kakihana, Masashi*; Iha, Wataru*; Nakaima, Kenri*; Aoki, Dai*; Nakamura, Ai*; Honda, Fuminori*; Nakashima, Miho*; Amako, Yasushi*; Gochi, Jun*; et al.
JPS Conference Proceedings (Internet), 29, p.012001_1 - 012001_9, 2020/02
Collaborative Laboratories for Advanced Decommissioning Science; Osaka University*
JAEA-Review 2019-025, 36 Pages, 2020/01
JAEA-Review-2019-025.pdf:2.57MB
CLADS, JAEA, had been conducting the Center of World Intelligence Project for Nuclear Science/Technology and Human Resource Development (hereafter referred to "the Project") in FY2018. The Project aims to contribute to solving problems in nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of Technology to Simultaneously Measure Viscosity and Surface Tension of Molten Materials in Reactor Core". Since (U,Zr)O and boride, molten materials in reactor core, exist at extremely high temperature, chemical reactions between the vessel and these molten materials are unavoidable. Therefore, it is difficult to measure the thermophysical property of these materials. In the present study, droplets are produced by heating and melting the samples levitated by a gas levitation method, then the droplets are collided with a substrate. From the instant behavior of the collision, a new technology to simultaneously derive the viscosity and surface tension will be developed.
Murai, Naoki; Fukuda, Tatsuo; Nakajima, Masamichi*; Kawamura, Mitsuaki*; Ishikawa, Daisuke*; Tajima, Setsuko*; Baron, A. Q. R.*
Physical Review B, 101(3), p.035126_1 - 035126_6, 2020/01
Times Cited Count：0 Percentile：100(Materials Science, Multidisciplinary)We report an inelastic X-ray scattering investigation of phonons in FeSe superconductor. Comparing the experimental phonon dispersion with density functional theory (DFT) calculations in the non-magnetic state, we found a significant disagreement between them. A better overall agreement was obtained by allowing for spin-polarization in DFT calculations, despite the absence of magnetic order in FeSe. This calculation gives a realistic approximation, at DFT level, of the disordered paramagnetic state of FeSe, in which strong spin fluctuations are present.
K
FeAsIdeta, Shinichiro*; Murai, Naoki; Nakajima, Masamichi*; Kajimoto, Ryoichi; Tanaka, Kiyohisa*
Physical Review B, 100(23), p.235135_1 - 235135_7, 2019/12
Times Cited Count：0 Percentile：100(Materials Science, Multidisciplinary)Nagai, Takayuki; Kobayashi, Hidekazu; Okamoto, Yoshihiro; Akiyama, Daisuke*; Sato, Nobuaki*; Uehara, Akihiro*; Fujii, Toshiyuki*; Sekimoto, Shun*
KURNS Progress Report 2018, P. 105, 2019/08
To understand this structural change of a borosilicate glass by a neutron irradiation in detail, the irradiation test was carried out in KUR in 2017FY. The glass structure was estimated by using Raman spectrometry in 2018FY. Comparing with the Raman spectra of glass samples before and after irradiation, it could be observed the change of peak height of Si-O bridging structure by the irradiation.
mesons as a probe of Casimir effect for chiral symmetry breakingIshikawa, Tsutomu*; Nakayama, Katsumasa*; Suenaga, Daiki*; Suzuki, Kei
Physical Review D, 100(3), p.034016_1 - 034016_14, 2019/08
Times Cited Count：0 Percentile：100(Astronomy & Astrophysics)We propose mesons as probes to investigate finite-volume effects for chiral symmetry breaking at zero and finite temperatures. By using the 2+1-flavor linear sigma model with constituent light quarks, we analyze the Casimir effects for the 
mean fields; the chiral symmetry is rapidly restored by the antiperiodic boundary for light quarks, and the chiral symmetry breaking is catalyzed by the periodic boundary. We also show the phase diagram of the mean fields on the volume and temperature plane. For mesons, we employ an effective model based on the chiral-partner structure, in which the volume dependence of mesons is induced by the mean fields. We find that 
mesons are less sensitive to finite volume than mesons, which is caused by the insensitivity of 
mean fields. An anomalous mass shift of mesons at high temperature with the periodic boundary will be useful in examinations with lattice QCD simulations. The dependence on the number of compactified spatial dimensions is also studied.
Iha, Wataru*; Kakihana, Masashi*; Matsuda, Shinya*; Honda, Fuminori*; Haga, Yoshinori; Takeuchi, Tetsuya*; Nakashima, Miho*; Amako, Yasushi*; Gochi, Jun*; Uwatoko, Yoshiya*; et al.
Journal of Alloys and Compounds, 788, p.361 - 366, 2019/06
Times Cited Count：2 Percentile：49.74(Chemistry, Physical)-based simulated fuel containing CsITakamatsu, Yuki*; Ishii, Hiroto*; Oishi, Yuji*; Muta, Hiroaki*; Yamanaka, Shinsuke*; Suzuki, Eriko; Nakajima, Kunihisa; Miwa, Shuhei; Osaka, Masahiko; Kurosaki, Ken*
Nippon Genshiryoku Gakkai Wabun Rombunshi, 17(3/4), p.106 - 110, 2018/12
In order to establish the synthesis method of simulated fuel contacting Cesium (Cs) which is required for the evaluation of physical/chemical characteristics in fuel and release behavior of Cs, sintering tests of the cerium dioxide (CeO) based simulated fuels containing Cesium iodide (CsI) are performed by using spark plasma sintering (SPS) method. The sintered CeO pellets with homogeneous distribution of several micro meter of CsI spherical precipitates were successfully obtained by optimizing SPS conditions.
Kim, J.*; Yamanaka, Satoru*; Nakajima, Akira*; Kato, Takanori*; Kim, Y.*; Fukuda, Tatsuo; Yoshii, Kenji; Nishihata, Yasuo; Baba, Masaaki*; Takeda, Masatoshi*; et al.
Advanced Sustainable Systems (Internet), 2(11), p.1800067_1 - 1800067_8, 2018/11
Times Cited Count：1 Percentile：82.92(Green & Sustainable Science & Technology)Moro, Takuya*; Kim, J.*; Yamanaka, Satoru*; Murayama, Ichiro*; Kato, Takanori*; Nakayama, Tadachika*; Takeda, Masatoshi*; Yamada, Noboru*; Nishihata, Yasuo; Fukuda, Tatsuo; et al.
Journal of Alloys and Compounds, 768, p.22 - 27, 2018/11
Times Cited Count：7 Percentile：35.32(Chemistry, Physical)Hiyama, Emiko; Hosaka, Atsushi; Oka, Makoto; Richard, J.-M.*
Physical Review C, 98(4), p.045208_1 - 045208_8, 2018/10
Times Cited Count：12 Percentile：8.77(Physics, Nuclear)A quark model, which reproduces the ground-state mesons and baryons, i.e., the threshold energies, is applied to the 
configurations, where 
is a light quark and 
the charmed quark. In the calculation, several open channels are explicitly included such as 
, 
, 
, etc. To distinguish genuine resonances and estimate their width, we employ Gaussian Expansion Method supplemented by the real scalingmethod (stabilization). No resonance is found at the energies of the 
and 
pentaquarks. On the other hand, there is a sharp resonant state at 4690 MeV with 
state and another one at 4920 MeV with 
state, which have a compact structure.
symmetry in CeCuGe; Soft X-ray absorption and hard X-ray photoemission spectroscopyAratani, Hidekazu*; Nakatani, Yasuhiro*; Fujiwara, Hidenori*; Kawada, Moeki*; Kanai, Yuina*; Yamagami, Kohei*; Fujioka, Shuhei*; Hamamoto, Satoru*; Kuga, Kentaro*; Kiss, Takayuki*; et al.
Physical Review B, 98(12), p.121113_1 - 121113_6, 2018/09
Times Cited Count：3 Percentile：63.29(Materials Science, Multidisciplinary)Koizumi, Mitsuo; Goto, Jun*; Matsuki, Seishi*
Journal of Semiconductors, 39(8), p.082001_1 - 082001_5, 2018/08
Dynamic nuclear self-polarization (DYNASP) is a phenomenon observed in III-V semiconductors. When electrons of the valence band of a semiconductor are optically excited to the conduction band, a relaxation process of the conduction electrons induces a large nuclear polarization to suddenly occur below a critical temperature. Extending the original theoretical work of Dyakonov et al., we examined the effect of spin distribution of valence electrons excited by the circularly polarized light and the effect of external magnetic field on the phenomenon of the nuclear self-polarization. We found that the nuclear polarization is achieved even above the critical temperatures by the effect of electron polarization and of the external magnetic field. To investigate the phenomenon experimentally, we constructed an apparatus for low-temperature experiments.
