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晶析工程基礎試験; 短冷却照射済燃料を用いた晶析試験

Fundamental test of crystallization process; Experience on behavior of FPs in crystallization process by using irradiated MOX fuel

鍛治 直也; 中村 和仁; 野村 和則  ; 柴田 淳広  ; 矢野 公彦 ; 鷲谷 忠博 ; 北嶋 卓史; 小泉 務

Kaji, Naoya; Nakamura, Kazuhito; Nomura, Kazunori; Shibata, Atsuhiro; Yano, Kimihiko; Washiya, Tadahiro; Kitajima, Takafumi; Koizumi, Tsutomu

$$gamma$$分析による短半減期核種の除染係数(DF)のホットデータ取得を目的として、短冷却の高速実験炉「常陽」照射済燃料を用いた晶析基礎試験を実施した。今回測定できたもののうちCs以外の各核種(Pu, Ru-106, Ce-144, Pr-144等)については、U試験等の結果から期待される100程度のDFが得られたほか、これまでのホット試験では除染できなかったCsについても、CsがPuとの複塩を形成せず除染できる条件がありうることが示唆された。

For the purpose of obtaining DFs of the short-life FPs by $$gamma$$ analysis in the hot experiment, fundamental test of crystallization process was carried out using Fast Experimental Reactor "JOYO" irradiated fuel. In this experiment, DFs of nuclides analyzed by $$gamma$$ analysis except Cs (Such as Ru-106, Ce-144, Pr-144) and Pu were evaluated to be about 100. It was suggested that there is the condition in which Pu-Cs double salt does not be formed, although DF of Cs had been very low in the past experiments because of forming Pu-Cs double salt.

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