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Neutron scattering study of antiferromagnet U$$_{2}$$Pt$$_{6}$$Al$$_{15}$$

U$$_{2}$$Pt$$_{6}$$Al$$_{15}$$の中性子散乱

太田 玖吾*; 松本 裕司*; 渡部 悠貴*; 金子 耕士   ; 田端 千紘; 芳賀 芳範   

Ota, Kyugo*; Matsumoto, Yuji*; Watabe, Yuki*; Kaneko, Koji; Tabata, Chihiro; Haga, Yoshinori

ハニカム格子を持つ反強磁性体U$$_{2}$$Pt$$_{6}$$Al$$_{15}$$の磁気構造を決定するために中性子散乱実験を行った。U$$_{2}$$Pt$$_{6}$$Al$$_{15}$$$$T_{rm m1}$$=9Kと$$T_{rm m2}$$=26Kで二つの相転移を示す。$$T_{rm m1}$$ $$<$$ $$T$$ $$<$$ $$T_{rm m2}$$の第一相では、$$kappa$$$$_{rm I}$$=(1/3, 0, 0)の伝搬ベクトルで記述される磁気反射が観測された。$$T$$$$<$$$$T_{rm m1}$$のフェーズIIでは、$$kappa$$$$_{rm I}$$=(1/3, 0, 0)と$$kappa$$$$_{rm II}$$=(1/2, 0, 0)の磁気反射が観測され、$$kappa$$$$_{rm I}$$=(1/3, 0, 0)の磁気反射強度は弱いが有限であった。温度依存強度のヒステリシスは$$T_{rm m1}$$での相転移にまたがって観測され、$$T_{rm m1}$$での転移が1次転移であることを示唆している。

We have performed the neutron scattering study of antiferromagnet U$$_{2}$$Pt$$_{6}$$Al$$_{15}$$ with the honeycomb lattice to determine the magnetic structure. U$$_{2}$$Pt$$_{6}$$Al$$_{15}$$ exhibits two phase transitions at $$T_{rm m1}$$ = 9 K and $$T_{rm m2}$$ = 26 K. In phase I at $$T_{rm m1}$$ $$<$$ $$T$$ $$<$$ $$T_{rm m2}$$, the magnetic reflections described by a propagation vector $$kappa$$$$_{rm I}$$ = (1/3, 0, 0) were observed. In phase II at $$T$$ $$<$$ $$T_{rm m1}$$, magnetic reflections of $$kappa$$$$_{rm I}$$ = (1/3, 0, 0) and $$kappa$$$$_{rm II}$$ = (1/2, 0, 0) were observed and the magnetic reflection intensity of $$kappa$$$$_{rm I}$$ = (1/3, 0, 0) is weak but finite. The hysteresis in the temperature dependent intensities is observed across the phase transition at $$T_{rm m1}$$, suggesting that the transition at $$T_{rm m1}$$ is of first order.

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