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論文

Electronic structure in heavy fermion compound UPd$$_2$$Al$$_3$$ through directional Compton profile measurement

小泉 昭久*; 久保 康則*; 山本 悦嗣; 芳賀 芳範; 櫻井 吉晴*

Journal of the Physical Society of Japan, 88(3), p.034714_1 - 034714_6, 2019/03

 パーセンタイル:100(Physics, Multidisciplinary)

Directional Compton profiles of a heavy fermion compound UPd$$_2$$Al$$_3$$ are measured in the basal plane of the hexagonal lattice. A remarkable change of the two-dimensional electron occupation number densities has been observed between 20 K and 100 K. Obtained results are attributed to the modification of the 5$$f$$ electronic states.

論文

Novel critical behavior of magnetization in URhSi; Similarities to the uranium ferromagnetic superconductors UGe$$_2$$ and URhGe

立岩 尚之; 芳賀 芳範; 山本 悦嗣

Physical Review B, 99(9), p.094417_1 - 094417_12, 2019/03

 パーセンタイル:100(Materials Science, Multidisciplinary)

ウラン系強磁性物質URhSiについて、強磁性転移温度$$T_{rm C}$$近辺で磁気測定を行い、臨界現象の研究を行った。自発磁化の温度依存に関する臨界指数$$beta$$、磁化率の指数$$gamma$$$$T_{rm C}$$における磁化に関する指数$$delta$$を、修正アロットプロットとスケーリング理論等を用いて決定した。URhSiの強磁性状態は一軸磁気異方性が大きいものの、臨界指数は三次元イジングモデルから期待されるもの($$beta$$ = 0.325, $$gamma$$ = 1.241, and $$delta$$ = 4.82)とは異なることが明らかにされた。URhSiの臨界指数($$beta$$ = 0.300 $$pm$$ 0.002, $$gamma$$ = 1.00 $$pm$$ 0.02, and $$delta$$ = 4.32 $$pm$$ 0.04)は、ウラン系強磁性超伝導物質UGe$$_2$$とURhGeと類似している。URhSiの静的磁性と動的磁性をウラン系強磁性超伝導物質と対比させ議論する。

論文

Unique helical magnetic order and field-induced phase in trillium lattice antiferromagnet EuPtSi

金子 耕士; Frontzek, M. D.*; 松田 雅昌*; 中尾 朗子*; 宗像 孝司*; 大原 高志; 垣花 将司*; 芳賀 芳範; 辺土 正人*; 仲間 隆男*; et al.

Journal of the Physical Society of Japan, 88, p.013702_1 - 013702_5, 2019/01

 被引用回数:1 パーセンタイル:100(Physics, Multidisciplinary)

Magnetic transitions in chiral antiferromagnet EuPtSi were investigated by means of single crystal neutron diffraction. In the ground state, magnetic peaks emerge at positions represented by $$q_{1}$$=$$(0.2, 0.3, 0)$$. Upon heating, an additional magnetic peak splitting around 2.5 K was uncovered, indicating a presence of a first-order transition with $$q^*_{1}$$=$$(0.2, 0.3, {delta})$$. An half-polarized neutron scattering for polarization parallel to Q reveled that polarization antiparallel to Q has stronger intensity in both magnetic phases. This feature clarifies single chiral character of helical structure with moments normal to the ordering vector in both ordered states. Under vertical magnetic field along [1,1,1] in the $$A$$ phase, magnetic peaks form hexagonal patterns in the equatorial scattering plane around nuclear. An ordering vector $$q_{A}$$ of the $$A$$-phase has the similar size in the periodicity to $$q_{1}$$, and could be a hallmark of a formation of skyrmion lattice in EuPtSi.

論文

Manifestation of electron correlation effect in 5$$f$$ states of uranium compounds revealed by 4$$d$$-5$$f$$ resonant photoelectron spectroscopy

藤森 伸一; 小畠 雅明; 竹田 幸治; 岡根 哲夫; 斎藤 祐児; 藤森 淳; 山上 浩志; 芳賀 芳範; 山本 悦嗣; 大貫 惇睦*

Physical Review B, 99(3), p.035109_1 - 035109_5, 2019/01

 パーセンタイル:100(Materials Science, Multidisciplinary)

In the present study, we have elucidated the nature of the electron correlation effect in uranium compounds by imaging the partial $$mathrm{U}~5f$$ density of states (pDOS) of typical itinerant, localized, and heavy fermion uranium compounds by using the $$mathrm{U}$$ 4$$d$$-5$$f$$ resonant photoemission spectroscopy. Obtained $$mathrm{U}~5$$ pDOS exhibit a systematic trend depending on the physical properties of compounds: Although the coherent peak at the Fermi level can be explained by the band-structure calculation, an incoherent peak emerges on the higher binding energy side ($$lesssim 1~mathrm{eV}$$) in the cases of localized and heavy fermion compounds. The intensity and energy position of the incoherent peak is increased and shifted to a higher binding energy as the localization of the $$mathrm{U}~5$$ state increases. These behaviors are consistent with the prediction of the Mott metal-insulator transition, suggesting that the Hubbard-$$U$$ type mechanism takes an essential role in the $$5f$$ electronic structure of actinide materials.

論文

Magnetic and electrical properties of the ternary compound U$$_2$$Ir$$_3$$Si$$_5$$ with one-dimensional uranium zigzag chains

Li, D. X.*; 本多 史憲*; 三宅 厚志*; 本間 佳哉*; 芳賀 芳範; 仲村 愛*; 清水 悠晴*; Maurya, A.*; 佐藤 芳樹*; 徳永 将史*; et al.

Physical Review B, 99, p.054408-1 - 054408-9, 2019/01

Physical properties of the single-crystalline U$$_2$$Ir$$_3$$Si$$_5$$, a new ternary uranium compound with U$$_2$$Co$$_3$$Si$$_5$$-type orthorhombic structure, are investigated by means of magnetic susceptibility, specific heat and electrical resistivity. This compound undergoes an antiferromagnetic transition followed by a first-order phase transition at lower temperature. A possible mechanism of the first-order transition is the occurrence of a magnetic magnetic quadrupolar order, resulting from the quasi-one-dimensional uranium zigzag chain.

論文

Strong correlation between ferromagnetic superconductivity and pressure-enhanced ferromagnetic fluctuations in UGe$$_2$$

立岩 尚之; 芳賀 芳範; 山本 悦嗣

Physical Review Letters, 121(23), p.237001_1 - 237001_6, 2018/12

 被引用回数:1 パーセンタイル:47.22(Physics, Multidisciplinary)

ウラン系強磁性超伝導物質UGe$$_2$$の高圧下磁化測定を行い、データをTakahashiによるスピンのゆらぎ理論を用いて解析した。強磁性相FM1とFM2の相境界$$P_x$$で、スピンゆらぎスペクトルの分布幅$$T_0$$に明確な異常が現れた。$$P_x$$では、超伝導転移温度$$T_{rm sc}$$が最大値を示す。このことは、$$P_x$$近辺で発達する強磁性スピンのゆらぎが超伝導出現に役割を果たすことを示唆する。また、パラメーター$${T_{rm Curie}}/{T_0}$$(ここで、$${T_{rm Curie}}$$は強磁性転移温度)の圧力変化から、局在性の強いFM2から遍歴性の強いFM1へ基底状態は転移することが示唆された。$$T_0$$$$T_{rm sc}$$の関係について、銅酸化物超伝導体等、他の超伝導物質と議論された。

論文

Phenomenological approach to study the degree of the itinerancy of the 5$$f$$ electrons in actinide ferromagnets with spin fluctuation theory

立岩 尚之; Posp$'i$$v{s}$il, J.*; 芳賀 芳範; 酒井 宏典; 松田 達磨*; 山本 悦嗣

Progress in Nuclear Science and Technology (Internet), 5, p.104 - 107, 2018/12

ウラン系強磁性超伝導物質UGe$$_2$$, URhGe, UCoGeについて盛んに研究が行われてきた。最近、我々は69個のウラン化合物、7個のネプツニウム化合物、4個のプルトニウム化合物について、スピンゆらぎ理論の適用性を検討した。その結果、アクチノイド5$$f$$電子の遍歴性を示唆する結果が得られた。会議では全強磁性化合物の解析結果と、UGe$$_2$$のスピンのゆらぎパラーメーターの圧力依存を議論する。

論文

Localized 5$$f^2$$ states in UPd$$_5$$Al$$_2$$ and valence crossover in the Vicinity of Heavy-Fermion superconductivity

目時 直人; 芳賀 芳範; 山本 悦嗣; 松田 雅昌*

Journal of the Physical Society of Japan, 87(11), p.114712_1 - 114712_9, 2018/11

 パーセンタイル:100(Physics, Multidisciplinary)

ウラン金属間化合物UPd$$_5$$Al$$_2$$は、四価イオンU$$^{4+}$$の局在5$$f^2$$($$^3H_4$$)電子状態を伴うことを中性子散乱による結晶場スペクトルから明らかにした。この電子状態は、最近研究した$$f$$電子数と結晶構造が同じ希土類参照物質PrPd$$_5$$Al$$_2$$と同一であり、c軸方向に大きな磁気モーメントを伴う平べったい形状の軌道が、縦長の体心正方晶の持つ二次元結晶場ポテンシャルによって安定化されていることがわかった。ウランの5$$f$$電子が金属状態において局在的な性格を持つことは非常に珍しい発見であり、やはり、結晶構造の特殊性に起因する。ウランが四価イオンであることは、三価のNpPd$$_5$$Al$$_2$$との間に価数転移が存在することを意味し、この価数転移が結晶格子の異常や電気抵抗の増加によって観察されることを明らかにした。また、価数が不安定な領域で超伝導や磁気転移、重い電子系状態など多体効果の存在を示す数多くの現象が生じていることがわかった。

論文

Electronic structure of URu$$_2$$Si$$_2$$ studied by photoelectron spectroscopy (INVITED)

藤森 伸一; 竹田 幸治; 岡根 哲夫; 斎藤 祐児; 藤森 淳; 山上 浩志; 芳賀 芳範; 山本 悦嗣; 大貫 惇睦*

Progress in Nuclear Science and Technology (Internet), 5, p.82 - 85, 2018/11

One of the most remarkable properties of actinide compounds is the coexistence of superconductivity and magnetic ordering which has been realized in several strongly-correlated uranium based compounds. In these compounds, both superconductivity and magnetic ordering originate from U 5f states. To understand the origin of the coexistence as well as the mechanism of the superconductivity, it is essential to reveal their U 5f electronic structures. In this presentation, the U 5f electronic structures of heavy Fermion superconductors UPd$$_2$$Al$$_3$$ and URu$$_2$$Si$$_2$$ studied by photoelectron spectroscopy using soft X-rays from SPring-8 BL23SU are presented. For UPd$$_2$$Al$$_3$$, U 4d-5f resonant photoemission experiment was performed, and its partial U 5f spectrum was revealed experimentally. Furthermore, we have applied the three-dimentional ARPES to the hidden order compound URu$$_2$$Si$$_2$$, and revealed its complete 3D electronic structure in the paramagnetic phase. Their electronic structures are discussed based on these results.

論文

Magnetization study on the Ising ferromagnet URhGe with high-precision angle-resolved magnetic field near the hard axis

中村 翔太*; 榊原 俊郎*; 清水 悠晴*; 橘高 俊一郎*; 河野 洋平*; 芳賀 芳範; Pospisil, J.; 山本 悦嗣

Progress in Nuclear Science and Technology (Internet), 5, p.123 - 127, 2018/11

Dc magnetization measurements have been performed on the orthorhombic Ising ferromagnet Urge. We observed a clear first-order reorientation transition with a small hysteresis and estimated the tricritical point to be around 4 K. The magnetization and the thermal expansion data indicate the presence of a characteristic temperature of about 1 K.

論文

Anomalous Hall effect in a triangular-lattice antiferromagnet UNi$$_4$$B

小山田 明*; 猪原 崇生*; 山本 悦嗣; 芳賀 芳範

Progress in Nuclear Science and Technology (Internet), 5, p.128 - 131, 2018/11

We report the Hall effect measurements on a triangular-lattice antiferromagnet UNi$$_4$$B in the context of the proposed relevance of the ferroic order. Our measurements show that the Hall voltage is proportional to the square of the electric current and its coefficient increases significantly below the transition temperature, which supports the theoretical prediction.

論文

Crystal structure and magnetic properties of new ternary uranium compound U$$_3$$TiBi$$_9$$

本山 岳*; 芳賀 芳範; 山口 明*; 川崎 郁斗*; 住山 昭彦*; 山村 朝雄*

Progress in Nuclear Science and Technology (Internet), 5, p.157 - 160, 2018/11

The crystal structure of the newly discovered compound U$$_3$$TiBi$$_9$$ was determined from single-crystal X-ray diffraction data. This compound shows an antiferromagnetic ordering at 31.5 K. A clear anomaly was observed at the transition temperature on the temperature dependence of magnetic susceptibility and electrical resistivity.

論文

Soft X-ray magnetic circular dichroism study on UGe$$_{2}$$

竹田 幸治; 岡根 哲夫; 斎藤 祐児; 山上 浩志; 山本 悦嗣; 芳賀 芳範

Progress in Nuclear Science and Technology (Internet), 5, p.171 - 174, 2018/11

In order to investigate the electronic and magnetic states of UGe$$_{2}$$ element-specifically, we have performed soft X-ray magnetic circular dichroism experiments at the U N$$_{4,5}$$ and Ge L$$_{2,3}$$ absorption edges. We have detected the XMCD signals at both the U and Ge sites and observed clear hysteresis loops in the ferromagnetic (FM) state at T = 5.5 K. From the branching ratio B, it is found that the occupation number of 5f electrons (n$$^{5f}$$) in UGe$$_{2}$$ is close to 3. In addition, applying the magneto-optical sum rules analysis to the XMCD spectrum at the U N$$_{4,5}$$ edges, the ratio of orbital magnetic moment to the spin magnetic moment (-M$$_{L}$$/M$$_{S}$$) is estimated to be 2.17. These values of B and -M$$_{L}$$/M$$_{S}$$ are comparable compared with the results of other FM superconductors: URhGe and UCoGe

論文

Effects of magnetic field and pressure on the valence-fluctuating antiferromagnetic compound EuPt$$_2$$Si$$_2$$

竹内 徹也*; 屋良 朝之*; 安次富 洋介*; 伊覇 航*; 垣花 将司*; 中島 美帆*; 天児 寧*; 本多 史憲*; 本間 佳哉*; 青木 大*; et al.

Journal of the Physical Society of Japan, 87(7), p.074709_1 - 074709_14, 2018/07

 被引用回数:2 パーセンタイル:27.52(Physics, Multidisciplinary)

Effects of magnetic field and pressure on the Kondo-like behavior in the valence-fluctuating antiferromagnetic compound EuPt$$_2$$Si$$_2$$ were studied using single-crystalline samples. Anomalous features in EuPt$$_2$$Si$$_2$$ are due to valence fluctuation and/or valence change of the Eu ions at low temperatures.

論文

Magnetic field induced phenomena in UIrGe in fields applied along the $$b$$ axis

Posp$'i$$v{s}$il, J.*; 芳賀 芳範; 小濱 芳允*; 三宅 厚志*; 神戸 振作; 立岩 尚之; Vali$v{s}$ka, M.*; Proschek, P.*; Prokle$v{s}$ka, J.*; Sechovsk$'y$, V.*; et al.

Physical Review B, 98(1), p.014430_1 - 014430_7, 2018/07

 被引用回数:1 パーセンタイル:55.95(Materials Science, Multidisciplinary)

The metamagnetic transition between the antiferromagnetic and paramagnetic state in UIrGe has been studied at various temperatures by magnetization, heat capacity, and magnetocaloric effect measurements on a single crystal in static and pulsed magnetic fields applied along the orthorhombic $$b$$ axis. The first-order transition is accompanied by a dramatic increase of the Sommerfeld coefficient. A tentative scenario explaining these anomalies by antiferromagnetic correlations or short-range order in the paramagnetic state is discussed.

論文

Electronic states in EuCu$$_2$$(Ge$$_{1-x}$$Si$$_x$$)$$_2$$ based on the doniach phase diagram

伊覇 航*; 屋良 朝之*; 安次富 洋介*; 垣花 将司*; 竹内 徹也*; 本多 史憲*; 仲村 愛*; 青木 大*; 郷地 順*; 上床 美也*; et al.

Journal of the Physical Society of Japan, 87(6), p.064706_1 - 064706_14, 2018/06

 被引用回数:2 パーセンタイル:27.52(Physics, Multidisciplinary)

We succeeded in growing single crystals of the series of EuCu$$_2$$(Ge$$_{1-x}$$Si$$_x$$)$$_2$$ compounds.Physical property measurements demonstrate a maximum of the antiferromagnetic transition temperature appears at $$x = 0.5$$. Antiferromagnetism then disappears around $$x = 0.7$$ followed by a heavy-fermion formation at higher concentrations. These observations follow the Doniach phase diagram as a function of $$x$$.

論文

Odd-parity electronic multipolar ordering in URu$$_2$$Si$$_2$$; Conclusions from Si and Ru NMR measurements

神戸 振作; 徳永 陽; 酒井 宏典; 服部 泰佑; 比嘉 野乃花; 松田 達磨*; 芳賀 芳範; Walstedt, R. E.*; 播磨 尚朝*

Physical Review B, 97(23), p.235142_1 - 235142_10, 2018/06

 被引用回数:4 パーセンタイル:22.8(Materials Science, Multidisciplinary)

We report $$^{29}$$Si and $$^{101}$$Ru NMR measurements on high-quality, single-crystal URu$$_2$$Si$$_2$$ samples with a residual resistivity ratio RRR$$sim$$70. Our results show that the Si and Ru sites exhibit 4-fold electronic symmetry around the $$c$$-axis in the hidden-order state. A previously observed 2-fold contribution of Si NMR linewidth is concluded to be due to extrinsic magnetic centers. Since the U and Si sites are aligned along the $$c$$-axis, we conclude further that the electronic state shows 4-fold symmetry around the U site below the hidden-order transition. From this observed local symmetry, possible space groups for the hidden-order state are $$P4/nnc$$ or $$I4/m$$, based on group theoretical considerations. Since the order vector is considered to be $$Q=(001)$$, the hidden-order state is then found to be $$P4/nnc$$ with rank 5 odd-parity, i.e. electric dotriacontapolar order.

論文

Inelastic X-ray scattering of $$RT$$Al$$_3$$ ($$R$$ = La, Ce, $$T$$ = Cu, Au)

筒井 智嗣*; 金子 耕士; Pospisil, J.; 芳賀 芳範

Physica B; Condensed Matter, 536, p.24 - 27, 2018/05

 パーセンタイル:100(Physics, Condensed Matter)

Inelastic X-ray scattering (IXS) experiments of RTAl$$_3$$ ($$R$$ = La Ce, $$T$$ = Cu, Au) were carried out at 300 and 5.5 K. The spectra between LaCuAl$$_3$$ and CeCuAl$$_3$$ (LaAuAl$$_3$$ and CeAuAl$$_3$$) are nearly identical at both temperatures except for temperature factors such as temperature dependence of Bose factor in IXS spectra and effect on thermal expansion. This means that no evident temperature dependence of IXS spectra was observed in CeTAl$$_3$$ ($$T$$ = Cu, Au).

論文

Element-specific observation of the ferromagnetic ordering process in UCoAl via soft X-ray magnetic circular dichroism

竹田 幸治; 斎藤 祐児; 岡根 哲夫; 山上 浩志; 松田 達磨*; 山本 悦嗣; 芳賀 芳範; 大貫 惇睦*

Physical Review B, 97(18), p.184414_1 - 184414_7, 2018/05

 パーセンタイル:100(Materials Science, Multidisciplinary)

We have performed soft X-ray magnetic circular dichroism (XMCD) experiments on the itinerant-electron metamagnet UCoAl at the U 4$$d$$-5$$f$$ ($$N_mathrm{4, 5}$$) and Co 2$$p$$-3$$d$$ ($$L_mathrm{2, 3}$$) absorption edges in order to investigate the magnetic properties of the U 5$$f$$ and Co 3$$d$$ electrons separately. From the line shape of the XMCD spectrum, it is deduced that the orbital magnetic moment of the Co 3$$d$$ electrons is unusually large. Through the systematic temperature ($$T$$)- and magnetic field ($$H$$)-dependent XMCD measurements, we have obtained two types of the magnetization curve as a function of $$H$$ and $$T$$ (M-H curve and M-T curve, respectively). The metamagnetic transition from a paramagnetic state to a field-induced ferromagnetic state was observed clearly under 15 K at $$H_mathrm{M}$$. The value of the $$H_mathrm{M}$$ and its $$T$$-dependence agree well between the U and Co sites, and the bulk magnetization. Whereas, we have discovered the remarkable differences in the M-H and M-T curves between the U and Co sites. The present findings show clearly that the role of the Co 3$$d$$ electrons should be considered more carefully in order to understand the origin of the magnetic ordering in UCoAl.

論文

Ruderman-Kittel interaction between Si in URu$$_{2}$$Si$$_{2}$$

神戸 振作; 服部 泰佑; 徳永 陽; 酒井 宏典; 松田 達磨*; 芳賀 芳範; Walstedt, R. E.*

Journal of Physics; Conference Series, 969(1), p.012033_1 - 012033_6, 2018/03

NMR核である$$^{29}$$Si同位体を52%濃縮した高品質のURu$$_{2}$$Si$$_{2}$$を作成した。$$^{29}$$Si同位体の自然存在比は、4%程度なので、この濃縮により測定積算時間を100分の1程度に短縮できる。この単結晶試料を用いた隠れた秩序相のSi-NMR線幅の結果は、既に報告した。今回は、この線幅の磁場、温度、角度依存に関するより詳細な解析について報告する。RKKYモデルによる2回対称の磁化率の分布の可能性に関しても議論する。

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