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BaCo(PO
)Sheng, J.*; Wang, L.*; Candini, A.*; Jiang, W.*; Huang, L.*; Xi, B.*; Zhao, J.*; Ge, H.*; Zhao, N.*; Fu, Y.*; et al.
Proceedings of the National Academy of Sciences of the United States of America, 119(51), p.e2211193119_1 - e2211193119_9, 2022/12
被引用回数：3 パーセンタイル：28(Multidisciplinary Sciences)Although considerable progress has been made in the theoretical understanding of the low-dimensional frustrated quantum magnets, experimental realizations of a well-established scaling analysis are still scarce. This is particularly true for the two-dimensional antiferromagnetic triangular lattices. Owing to the small exchange strength, the newly discovered compound NaBaCo(PO) provides a rare opportunity for clarifying the quantum criticality in an ideal triangular lattice with quantum spin S=1/2. In addition to the establishment of the complete phase diagrams, the spin Hamiltonian with a negligible interplane interaction has been determined through the spin wave dispersion in the polarized state, which is consistent with the observation of a two-dimensional quantum critical point with the Bose-Einstein condensation of diluted free bosons.
Wei, D.*; Wang, L.*; Zhang, Y.*; Gong, W.; 都留 智仁; Lobzenko, I.; Jiang, J.*; Harjo, S.; 川崎 卓郎; Bae, J. W.*; et al.
Acta Materialia, 225, p.117571_1 - 117571_16, 2022/02
被引用回数：59 パーセンタイル：99.75(Materials Science, Multidisciplinary)Recently-developed high-entropy alloys (HEAs) containing multiple principal metallic elements have ex-tended the compositional space of solid solutions and the range of their mechanical properties. Here we show that the realm of possibilities can be further expanded through substituting the constituent metals with metalloids, which are desirable for tailoring strength/ductility because they have chemical interactions and atomic sizes distinctly different from the host metallic elements. Specifically, the metalloid substitution increases local lattice distortion and short-range chemical inhomogeneities to elevate strength, and in the meantime reduces the stacking fault energy to discourage dynamic recovery and encourage defect accumulation via partial-dislocation-mediated activities. These impart potent dislocation storage to improve the strain hardening capability, which is essential for sustaining large tensile elongation. As such, metalloid substitution into HEAs evades the normally expected strength-ductility trade-off, enabling an unusual synergy of high tensile strength and extraordinary ductility for these single-phase solid solutions.
clusters in dilute neutron-rich matter田中 純貴*; Yang, Z.*; Typel, S.*; 足立 智*; Bai, S.*; van Beek, P.*; Beaumel, D.*; 藤川 祐輝*; Han, J.*; Heil, S.*; et al.
Science, 371(6526), p.260 - 264, 2021/01
被引用回数：48 パーセンタイル：99.12(Multidisciplinary Sciences)ノックアウト反応を用いることで、中性子過剰な錫同位体の核表面でのクラスター形成を実験的に確かめた。実験で得られた、質量数とともに単調に減少するノックアウト断面積は理論による予言と非常に良く一致し、クラスター形成率と中性子スキン厚との関係を示唆している。
Lai, W.-H.*; Wang, H.*; Zheng, L.*; Jiang, Q.*; Yan, Z.-C.*; Wang, L.*; 吉川 浩史*; 松村 大樹; Sun, Q.*; Wang, Y.-X.*; et al.
Angewandte Chemie; International Edition, 59(49), p.22171 - 22178, 2020/12
被引用回数：77 パーセンタイル：95.81(Chemistry, Multidisciplinary)Herein, we report a comprehensive strategy to synthesize a full range of single-atom metals on carbon matrix, including V, Mn, Fe, Co, Ni, Cu, Ge, Mo, Ru, Rh, Pd, Ag, In, Sn, W, Ir, Pt, Pb, and Bi. The extensive applications of various single-atom catalysts (SACs) are manifested via their ability to electro-catalyze typical hydrogen evolution reactions (HER) and conversion reactions in novel room-temperature sodium sulfur batteries (RT-Na-S). The enhanced performances for these electrochemical reactions arisen from the ability of different single active atoms on local structures to tune their electronic configuration. Significantly, the electrocatalytic behaviors of diverse SACs, assisted by density functional theory calculations, are systematically revealed by in situ synchrotron X-ray diffraction and in situ transmission electronic microscopy, providing a strategic library for the general synthesis and extensive applications of SACs in energy conversion and storage.
decay of 
USun, M. D.*; Liu, Z.*; Huang, T. H.*; Zhang, W. Q.*; Andreyev, A. N.; Ding, B.*; Wang, J. G.*; Liu, X. Y.*; Lu, H. Y.*; Hou, D. S.*; et al.
Physics Letters B, 800, p.135096_1 - 135096_5, 2020/01
被引用回数：11 パーセンタイル：79.42(Astronomy & Astrophysics)Fine structure in the decay of U was observed in the fusion-evaporation reaction 
Re(
Ar,p3n) by using fast digital pulse processing technique. Two -decay branches of U feeding the ground state and 244 keV excited state of 
Th were identified by establishing the decay chain U
Th
Ra
Rn. The -particle energy for the ground-state to ground-state transition of U was determined to be 8993(17) keV, 213 keV higher than the previous value, the half-life was updated to be 62
s. Evolution of nuclear structure for 
=131 even-
isotones from Po to U was discussed in the frameworks of nuclear mass and reduced -decay width, a weakening octupole deformation in the ground state of U relative to its lighter isotones Ra and Th was suggested.
fungal cells; A pH-dependent contribution of phosphoryl functional groupJiang, M. Y.*; 大貫 敏彦; 山崎 信哉; 田中 万也*; 宇都宮 聡*
Journal of Radioanalytical and Nuclear Chemistry, 295(3), p.2283 - 2287, 2013/03
被引用回数：3 パーセンタイル：25.73(Chemistry, Analytical)イッテルビウムの酵母への吸着についてXAFSによる化学種同定により検討した。その結果、リン酸官能基に配位したYbの割合はpH3-5でほぼ一定であった。この結果は、解離していないリン酸基への配位を示唆している。
Jiang, M. Y.*; 大貫 敏彦; 田中 万也*; 香西 直文; 上石 瑛伍; 宇都宮 聡*
Geochimica et Cosmochimica Acta, 93, p.30 - 46, 2012/09
被引用回数：31 パーセンタイル：63.8(Geochemistry & Geophysics)酵母表面におけるYbリン酸塩鉱物化機構を実験により検討した。細胞表面に吸着したYbが細胞から排出されたリン酸と結合してナノ粒子化することをTEMやEXAFSによる分析から明らかにした。
中村 一男*; Jiang, Y.*; Liu, X.*; 御手洗 修*; 栗原 研一; 川俣 陽一; 末岡 通治; 長谷川 真*; 徳永 和俊*; 図子 秀樹*; et al.
Fusion Engineering and Design, 86(6-8), p.1080 - 1084, 2011/10
被引用回数：4 パーセンタイル：32.59(Nuclear Science & Technology)CCS (Cauchy Condition Surface) method is a numerical approach to reproduce plasma shape, which has good precision in conventional tokamak. In order to apply it in plasma shape reproduction of ST (Spherical Tokamak), the calculation precision of the CCS method in CPD (
= 0.25 T, 
= 0.3 m, 
= 0.2 m) has been analyzed. The precision was confirmed also in ST and decided to be applied to QUEST ( = 0.25 T, = 0.68 m, = 0.40 m). In present stage from the magnetic measurement, it is known that the eddy current effect is large in QUEST experiment, and there are no special magnetic measurements for eddy current now, so some proper model should be selected to evaluate the eddy current effect. The eddy current density by not only CS (Center Solenoid) coil but also plasma current is calculated using EDDYCAL (JAEA), the eddy currents are taken as unknown variables and solved together with plasma shape reconstruction. The result shows that the CCS method with eddy current adjustment achieves stable, accurate reconstruction of plasma shape in application to QUEST.
末田 敬一*; 栗田 隆史*; 川嶋 利幸*; 山川 考一; 河仲 準二*; 関根 尊史*; Zhao, B.*; Jiang, Y.*; 松本 修*; 藤田 雅之*; et al.
no journal, ,
レーザー光に空間的・時間的光波制御を加味することによって物質との相互作用、特に非線形相互作用における新現象の発現を目指し、搬送波包絡線位相を制御した数サイクルマルチテラワットレーザーの開発を進めている。今回、超広帯域光パルメトリックチャープパルス(OPCPA)増幅器の励起光源として、半導体レーザー励起Nd:ガラスレーザー増幅器の開発を行い、OPCPA励起用のピコ秒パルスに必要なスペクトル幅(3.7nm)を達成し、出力として2.4J/パルスを10Hzの繰り返しで実証した。
