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論文

A Lightweight shape-memory alloy with superior temperature-fluctuation resistance

Song, Y.*; Xu, S.*; 佐藤 駿介*; Lee, I.*; Xu, X.*; 大森 俊洋*; 長迫 実*; 川崎 卓郎; 鬼柳 亮嗣; Harjo, S.; et al.

Nature, 638, p.965 - 971, 2025/02

https://doi.org/10.1038/s41586-024-08583-7
 被引用回数：2 パーセンタイル：88.78(Multidisciplinary Sciences)

In advanced applications like aerospace and space exploration, materials must balance lightness, functionality, and extreme thermal fluctuation resistance. Shape-memory alloys show promise with strength, toughness, and substantial strain recovery due to superelasticity, but maintaining low mass and effective operation at cryogenic temperatures is challenging. We hereby introduce a novel shape-memory alloy that adheres to these stringent criteria. Predominantly composed of Ti and Al with a chemical composition of Ti$$_{75.25}$$Al$$_{20}$$Cr$$_{4.75}$$, this alloy 25 is characterized by a low density (4.36$$times$$10$$^{3}$$ kg/m$$^{3}$$) and a high specific strength (185$$times$$10$$^{3}$$ Pa$$cdot$$m$$^{3}$$/kg) at room temperature, while exhibiting excellent superelasticity. The superelasticity, owing to a reversible stress-induced phase transformation from an ordered body-centered cubic parent phase to an ordered orthorhombic martensite, allows for a recoverable strain exceeding 7%. Remarkably, this functionality persists across a broad range of temperatures, from deep cryogenic 4.2 K to above room temperature, arising from an unconventional temperature dependence of transformation stresses. Below a certain threshold during cooling, the critical transformation stress inversely correlates with temperature. We interpret this behavior from the perspective of a temperature-dependent anomalous lattice instability of the parent phase. This alloy holds potential in everyday appliances requiring flexible strain accommodations, as well as components designed for extreme environmental conditions such as deep space and liquefied gases.

論文

Solid-state Alder-ene reaction of 1-hexene under high pressure

Xu, J.*; Lang, P.*; Liang, S.*; Zhang, J.*; Fei, Y.*; Wang, Y.*; Gao, D.*; 服部 高典; 阿部 淳*; Dong, X.*; et al.

Journal of Physical Chemistry Letters (Internet), p.2445 - 2451, 2025/00

https://doi.org/10.1021/acs.jpclett.4c03696
 被引用回数：0 パーセンタイル：0.00(Chemistry, Physical)

アルダー-エン反応は、アルケンとアリル水素との化学反応であり、C-C結合を構築する効率的な方法である。従来、この反応には触媒、高温、あるいは光触媒が必要であった。本研究では、触媒を用いずに室温下で加圧することで成功した1-ヘキセンのアルダー-エン反応を報告する。1-ヘキセンは4.3GPaで結晶化し、18GPaで重合してオレフィンを形成する。ガスクロマトグラフィー-質量分析法により、1-ヘキセンが高圧下でのアルダー-エン反応により二量体を生成することを発見した。その場中性子回折から、この反応過程はトポケミカル則に従わないことがわかった。理論計算により、1つのC-H $$sigma$$結合と2つのアルケン$$pi$$結合を含む6員環遷移状態が示され、そのエネルギーは20GPaまで圧縮すると明らかに減少した。本研究は、触媒を用いずに室温でアルダー-エン反応を実現する新規かつ有望な方法を提供し、この重要な反応の応用を拡大するものである。

論文

Strong low-energy rattling modes enabled liquid-like ultralow thermal conductivity in a well-ordered solid

Liu, P.-F.*; Li, X.*; Li, J.*; Zhu, J.*; Tong, Z.*; 古府 麻衣子*; 楡井 真実; Xu, J.*; Yin, W.*; Wang, F.*; et al.

National Science Review, 11(12), p.nwae216_1 - nwae216_10, 2024/12

https://doi.org/10.1093/nsr/nwae216
 被引用回数：12 パーセンタイル：91.22(Multidisciplinary Sciences)

Crystalline solids exhibiting inherently low lattice thermal conductivity ($$kappa_{rm L}$$) are of great importance in applications such as thermoelectrics and thermal barrier coatings. However, $$kappa_{rm L}$$ cannot be arbitrarily low and is limited by the minimum thermal conductivity related to phonon dispersions. In this work, we report the liquid-like thermal transport in a well-ordered crystalline CsAg$$_5$$Te$$_3$$, which exhibits an extremely low $$kappa_{rm L}$$ value of $$sim$$ 0.18 Wm$$^{-1}$$K$$^{-1}$$. On the basis of first-principles calculations and inelastic neutron scattering measurements, we find that there are lots of low-lying optical phonon modes at $$sim$$ 3.1 meV hosting the avoided-crossing behavior with acoustic phonons. These strongly localized modes are accompanied by weakly bound rattling Ag atoms with thermally induced large amplitudes of vibrations. Using the two-channel model, we demonstrate that coupling of the particle-like phonon modes and the heat-carrying wave-like phonons is essential for understanding the low $$kappa_{rm L}$$, which is heavily deviated from the $$1/T$$ temperature dependence of the standard Peierls theory. In addition, our analysis indicates that the soft structural framework with liquid-like motions of the fluctuating Ag atoms is the underlying cause that leads to the suppression of the heat conduction in CsAg$$_5$$Te$$_3$$. These factors synergistically account for the ultralow $$kappa_{rm L}$$ value. Our results demonstrate that the liquid-like heat transfer could indeed exist in a well-ordered crystal.

論文

$$mu$$SR study on the noncentrosymmetric superconductor NbGe$$_2$$

Jiao, J. C.*; Chen, K. W.*; Hillier, A. D.*; 伊藤 孝; 髭本 亘; Li, Z.*; Lv, B.*; Xu, Z.-A.*; Shu, L.*

Physical Review B, 110(21), p.214516_1 - 214516_9, 2024/12

https://doi.org/10.1103/PhysRevB.110.214516
 被引用回数：0 パーセンタイル：0.00(Materials Science, Multidisciplinary)

We report on a muon spin relaxation ($$mu$$SR) study on the polycrystalline noncentrosymmetric superconductor NbGe$$_2$$ with superconducting transition temperature $$T_c$$ = 2.0-2.1 K. The zero-field $$mu$$SR experiment indicates the absence of a spontaneous magnetic field in the superconducting state, showing the preservation of time-reversal symmetry in the superconducting state. The transverse-field $$mu$$SR experiment is performed to map the phase diagram of NbGe$$_2$$, from which clear evidence of both type-I and type-II superconductivities is obtained. More importantly, we clearly delineate the region in the phase diagram where type-I and type-II superconductivities coexist.

論文

Unique magnetic transition process demonstrating the effectiveness of bond percolation theory in a quantum magnet

Zheng, X.-G.*; 山内 一宏*; 萩原 雅人; 西堀 英治*; 河江 達也*; 渡邊 功雄*; 内山 智貴*; Chen, Y.*; Xu, C.-N.*

Nature Communications (Internet), 15, p.9989_1 - 9989_12, 2024/11

https://doi.org/10.1038/s41467-024-54335-6
 被引用回数：0 パーセンタイル：0.00(Multidisciplinary Sciences)

Like the crystallization of water to ice, magnetic transition occurs at a critical temperature after the slowing down of dynamically fluctuating short-range correlated spins. Here, we report a unique type of magnetic transition characterized by a linear increase in the volume fraction of unconventional static short-range-ordered spin clusters, which triggered a transition into a long-range order at a threshold fraction perfectly matching the bond percolation theory in a new quantum antiferromagnet of pseudo-trigonal Cu$$_{4}$$(OH)$$_{6}$$Cl$$_{2}$$. Static short-range order appeared in its Kagome lattice plane below Ca. 20 K from a pool of coexisting spin liquid, linearly increasing its fraction to 0.492(8), then all Kagome spins transitioned into a stable two-dimensional spin order at $$T$$_${rm N}$$$ = 5.5 K. Inspection on the magnetic interactions and quantum magnetism revealed an intrinsic link to the spin liquid material Herbertsmithite, ZnCu$$_${3}$$$(OH)$$_${6}$$$Cl$$_${2}$$. The unconventional static nature of the short-range order was inferred to be due to a pinning effect by the strongly correlated coexisting spin liquids. This work presents a unique magnetic system to demonstrate a complete bond percolation process toward the critical transition. Meanwhile, the unconventionally developed magnetic order in this chemically clean system should shed new light on spin-liquid physics.

論文

Compound-nucleus and doorway-state decays of $$beta$$-delayed neutron emitters $$^{51,52.53}$$K

Xu, Z. Y.*; Grzywacz, R.*; Andreyev, A. N.; 他49名*

Physical Review Letters, 133(4), p.042501_1 - 042501_7, 2024/07

https://doi.org/10.1103/PhysRevLett.133.042501
 被引用回数：1 パーセンタイル：0.00(Physics, Multidisciplinary)

We investigated decays of $$^{51,52,53}$$K at the ISOLDE Decay Station at CERN in order to understand the mechanism of the $$beta$$-delayed neutron-emission ($$beta$$n) process. The experiment quantified neutron and $$gamma$$-ray emission paths for each precursor. We used this information to test the hypothesis, first formulated by Bohr in 1939, that neutrons in the $$beta$$n process originate from the structureless "compound nucleus". The data are consistent with this postulate for most of the observed decay paths. The agreement, however, is surprising because the compound-nucleus stage should not be achieved in the studied $$beta$$ decay due to insufficient excitation energy and level densities in the neutron emitter. In the $$^{53}$$K $$beta$$n decay, we found a preferential population of the first excited state in $$^{52}$$Ca that contradicted Bohr's hypothesis. The latter was interpreted as evidence for direct neutron emission sensitive to the structure of the neutron-unbound state. We propose that the observed nonstatistical neutron emission proceeds through the coupling with nearby doorway states that have large neutron-emission probabilities. The appearance of "compound-nucleus" decay is caused by the aggregated small contributions of multiple doorway states at higher excitation energy.

論文

Spin and lattice dynamics in the van der Waals antiferromagnet MnPSe$$_{3}$$

Liao, J.*; Huang, Z.*; Shangguan, Y.*; Zhang, B.*; Cheng, S.*; Xu, H.*; 梶本 亮一; 蒲沢 和也*; Bao, S.*; Wen, J.*

Physical Review B, 109(22), p.224411_1 - 224411_10, 2024/06

https://doi.org/10.1103/PhysRevB.109.224411
 被引用回数：0 パーセンタイル：0.00(Materials Science, Multidisciplinary)

Antiferromagnetic van der Waals family $$M$$P$$X_{3}$$ ($$M$$ = Fe, Mn, Co, and Ni; $$X$$ = S and Se) have attracted significant research attention due to the possibility of realizing long-range magnetic order down to the monolayer limit. Here, we perform inelastic neutron scattering measurements on single-crystal samples of MnPSe$$_{3}$$, a member of the $$M$$P$$X_{3}$$ family, to study the spin dynamics and determine the effective spin model. The excited magnon bands are well characterized by a spin model, which includes a Heisenberg term with three intraplane exchange parameters ($$J_{1} = -0.73$$ meV, $$J_{2} = -0.014$$ meV, $$J_{3} = -0.43$$ meV) and one interplane parameter ($$J_{c} = -0.054$$ meV), and an easy-plane single-ion anisotropy term ($$D = -0.035$$ meV). Additionally, we observe the intersection of the magnon and phonon bands but no anomalous spectral features induced by the formation of magnon-phonon hybrid excitations at the intersecting region. We discuss possible reasons for the absence of such hybrid excitations in MnPSe$$_{3}$$.

論文

New isomeric transition in $$^{36}$$Mg; Bridging the $$N = 20$$ and $$N = 28$$ islands of inversion

Madurga, M.*; Christie, J. M.*; Xu, Z.*; Grzywacz, R.*; Poves, A.*; King, T.*; Allmond, J. M.*; Chester, A.*; Cox, I.*; Farr, J.*; et al.

Physical Review C, 109(6), p.L061301_1 - L061301_6, 2024/06

https://doi.org/10.1103/PhysRevC.109.L061301
 被引用回数：2 パーセンタイル：78.45(Physics, Nuclear)

ミシガン州立大学の国立超伝導サイクロトロン研究所にて$$^{48}$$Caからのフラグメンテーション反応によって中性子過剰核$$^{36}$$Mgを生成、分離し、そのアイソマーを探した。その結果、168keVのガンマ線を出して$$2^+$$に半減期約90nsで脱励起するアイソマーを発見した。その性質を議論するため、大規模殻模型計算の結果と比較した。Mg同位体では中性子数20から28領域にかけて広く変形核となることが知られているが、理論的には、前者の領域は$$sd$$殻から2個の中性子が励起することによって変形し、後者の領域は中性子数28の殻ギャップからの中性子励起によって変形する。$$^{36}$$Mgはその中間に位置し、両者の状態が近くに存在することで、励起エネルギーの低い$$0^+$$が出現すると理解される。

論文

Development of an Fe$$^{rm II}$$ complex exhibiting intermolecular proton shifting coupled spin transition

Ji, T.*; Su, S.*; Wu, S.*; 堀 優太*; 重田 育照*; Huang, Y.*; Zheng, W.*; Xu, W.*; Zhang, X.*; 鬼柳 亮嗣; et al.

Angewandte Chemie; International Edition, 63(25), p.e202404843_1 - e202404843_6, 2024/04

https://doi.org/10.1002/anie.202404843
 被引用回数：0 パーセンタイル：0.00(Chemistry, Multidisciplinary)

In this study, we investigated reversible intermolecular proton shifting (IPS) coupled with spin transition (ST) in a novel Fe$$^{rm II}$$ complex. The host Fe$$^{rm II}$$ complex and the guest carboxylic acid anion were connected by intermolecular hydrogen bonds (IHBs). We extended the intramolecular proton transfer coupled ST phenomenon to the intermolecular system. The dynamic phenomenon was confirmed by variable-temperature single-crystal X-ray diffraction, neutron crystallography, and infrared spectroscopy.

論文

Onset of collectivity for argon isotopes close to $$N=32$$

Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G$'o$mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.

Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03

https://doi.org/10.1103/PhysRevC.109.034312
 被引用回数：2 パーセンタイル：58.81(Physics, Nuclear)

理化学研究所RIビームファクトリーにて中性子過剰核$$^{50}$$Arビームからの1中性子ノックアウト反応実験を行い、$$^{49}$$Arのエネルギー準位および分光学的因子を導出した。特に、第一励起状態の$$1/2^-$$への分光学的因子が大きいことから、始状態の$$^{50}$$Arの基底状態において中性子が$$p_{1/2}$$軌道を多く占めていることがわかった。これは、中性子数32がよい魔法数として知られる$$^{52}$$Caとは異なった性質であり、カルシウムからアルゴンへと陽子が2個減ることで閉殻構造が大きく崩れることが明らかになった。

論文

ALTEMIS: Using integrated hydrology and reactive transport modeling to support resilience at the Savannah River Site

Xu, Z.*; Litzinger, A.*; 佐久間 一幸; Arora, B.*; Hazenberg, P.*; Wang, L.*; Gonzalez Raymat, H.*; Fabricatore, E.*; Wainwright, Haruko*; Eddy-Dilek, C.*

Proceedings of Waste Management Symposia 2024 (WM2024) (Internet), 14 Pages, 2024/03

We leverage the Advanced Terrestrial Simulator (ATS), a comprehensive model encompassing overland flow, groundwater processes, canopy and ground evapotranspiration effects. ATS is integrated with reactive transport models, including PFLOTRAN and CrunchFlow, to capture the intricate dynamics of key nuclear-related geochemical species. The Advanced Long-term Environmental Monitoring Systems (ALTEMIS) project extends its efforts across multiple scales: 1) Watershed Scale ATS Model: At the Savannah River Site, we employ a watershed-scale ATS model to quantify the water budget and estimate evapotranspiration fluxes.; 2) Integrated Hydrology Model for Floodplains: Our integrated hydrology model zooms in on the floodplain of Fourmiles Creek, enabling quantification of upwelling groundwater fluxes into wetlands and surface ponds. It also used to assess contaminant migration into Fourmiles Creek; 3) Fully Integrated Reactive Transport Model: Focused on the F-Area seepage basin, one of the largest nuclear waste processing facilities, we develop both 2D transect and 3D basin models. These models estimate the behavior of radioactive elements such as uranium and tritium, as well as non-reactive geochemical species.; 4) Sr-90 Sorption Model: Informed by extensive Sr-90 sorption experiments on minerals and core samples, we parameterize both electrostatic and non-electrostatic sorption models for Sr-90. These models are integrated into multiple reactive transport frameworks, significantly enhancing our ability to accurately predict Sr-90 migration under varying pH conditions.

論文

System of radiological protection; Towards a consistent framework on earth and in space

R$"u$hm, W.*; 伴 信彦*; Chen, J.*; Li, C.*; Dobynde, M.*; Durante, M.*; El-Jaby, S.*; 込山 立人*; 小笹 晃太郎*; 佐藤 達彦; et al.

Journal of Medical Physics - Zeitschrift f$"u$r medizinische Physik -, 34(1), p.4 - 13, 2024/02

https://doi.org/10.1016/j.zemedi.2024.01.004
 被引用回数：0 パーセンタイル：0.00(Radiology, Nuclear Medicine & Medical Imaging)

国際放射線防護委員会(ICRP)は、過去90年間に渡って世界各国や国際的な放射線防護の枠組み作りに貢献してきた。2019年、ICRPは宇宙飛行士の放射線防護に関わる様々な問題に対応したタスクグループ(TG115)を立ち上げ、地上の放射線防護体系と宇宙の放射線防護体系との共通の枠組み作りに取り組んでいる。本論文では、現時点でICRPが定めている宇宙放射線防護体系についてとりまとめて報告する。

論文

Experimental determination of phase equilibria in the Mn-Zn binary system

今富 大介*; 石川 遼典*; 仲田 玲*; 伊東 達矢; Han, K.*; 長迫 実*; Xu, X.*; 大森 俊洋*; 貝沼 亮介*

Journal of Phase Equilibria and Diffusion, 45(1), p.3 - 17, 2024/02

https://doi.org/10.1007/s11669-023-01068-6
 被引用回数：1 パーセンタイル：12.80(Chemistry, Physical)

Mn-Zn二元系における相平衡を、組成分析、結晶構造解析、熱分析により実験的に決定した。これまでの報告と比較し、$$beta$$相、$$varepsilon$$相、$$delta$$相の存在領域に違いが見られた。$$beta$$相の領域から急冷した試料で$$delta$$Mn相と同じ不規則な体心立方構造が確認されたため、$$beta$$-B2の単相域は確認できなかった。先行研究において、$$varepsilon$$相が$$varepsilon$$,$$varepsilon_{1}$$,$$varepsilon_{2}$$相に分離しているかどうかが論争になっていきたが、拡散対といくつかの合金組成の調査により、$$varepsilon$$相、$$varepsilon_{1}$$相、$$varepsilon_{2}$$相は分離しておらず、単一の$$varepsilon$$相となっていることが示された。さらに、熱分析によって対応する不変系反応が検出されなかったことから、$$delta$$相はZn過剰領域には存在しない。

論文

Electromagnetic moments of the antimony isotopes $$^{112-133}$$Sb

Lechner, S.*; 宮城 宇志*; Xu, Z. Y.*; Bissell, M. L.*; Blaum, K.*; Cheal, B.*; Devlin, C. S.*; Garcia Ruiz, R. F.*; Ginges, J. S. M.*; Heylen, H.*; et al.

Physics Letters B, 847, p.138278_1 - 138278_9, 2023/12

https://doi.org/10.1016/j.physletb.2023.138278
 被引用回数：6 パーセンタイル：76.15(Astronomy & Astrophysics)

不安定核を含むアンチモン同位体$$^{112-133}$$Sbの磁気モーメントと電気的四重極モーメントをレーザー分光を用いて測定した。現象論的な相互作用と有効演算子を用いた殻模型計算によって測定値をよく再現することができた。第一原理に基づいたVS-IMSRG法による殻模型計算では、磁気モーメントは現象論的な有効演算子を用いればよく実験値を再現するものの、電気的四重極モーメントについては有効電荷を用いても現象論的な相互作用を用いた計算ほどには実験値を再現することができなかった。

論文

Validation of the $$^{10}$$Be ground-state molecular structure using $$^{10}$$Be($$p,palpha$$)$$^{6}$$He triple differential reaction cross-section measurements

Li, P. J.*; Beaumel, D.*; Lee, J.*; Assi$'e$, M.*; Chen, S.*; Franchoo, S.*; Gibelin, J.*; Hammache, F.*; Harada, T.*; 延与 佳子*; et al.

Physical Review Letters, 131(21), p.212501_1 - 212501_7, 2023/11

https://doi.org/10.1103/PhysRevLett.131.212501
 被引用回数：21 パーセンタイル：93.59(Physics, Multidisciplinary)

$$^{10}$$Beのクラスター構造を($$p,palpha$$)反応を用いて調査した。三重微分断面積が実験的に測定され、Tohsaki-Horiuchi-Schuck-R$"o$pke波動関数の方法や反対称化分子動力学を用いた歪曲波インパルス近似計算と比較した。実験データと理論計算の顕著な一致が確認され、$$^{10}$$Beの比較的コンパクトな分子状態を確認した。

論文

Doubly heavy tetraquarks including one-pion exchange potential

Meng, Q.*; 肥山 詠美子*; 岡 眞*; 保坂 淳; Xu, C.*

Physics Letters B, 846, p.138221_1 - 138221_6, 2023/11

https://doi.org/10.1016/j.physletb.2023.138221
 被引用回数：11 パーセンタイル：93.20(Astronomy & Astrophysics)

2個の重いクォークを含んだテトラクォークの質量スペクトルをパイ中間子交換ポテンシャルをとりいれた構成子クォーク模型によって調べた結果を報告する。

論文

PANDORA Project for the study of photonuclear reactions below $$A=60$$

民井 淳*; Pellegri, L.*; S$"o$derstr$"o$m, P.-A.*; Allard, D.*; Goriely, S.*; 稲倉 恒法*; Khan, E.*; 木戸 英治*; 木村 真明*; Litvinova, E.*; et al.

European Physical Journal A, 59(9), p.208_1 - 208_21, 2023/09

https://doi.org/10.1140/epja/s10050-023-01081-w
 被引用回数：7 パーセンタイル：76.15(Physics, Nuclear)

光核反応は原子核構造の観点からも応用の観点からも重要であるにも関わらず、その反応断面積は未だに不定性が大きい。近年、超高エネルギー宇宙線の起源を探るために、鉄よりも軽い原子核の光核反応断面積を正確に知る必要が指摘されている。この状況を打破するため、原子核物理の実験、理論、宇宙物理の共同研究となるPANDORAプロジェクトが始まった。本論文はその計画の概要をまとめたものである。原子核実験ではRCNP、iThembaによる仮想光子実験とELI-NPによる実光子実験などが計画されている。原子核理論では、乱雑位相近似計算、相対論的平均場理論、反対称化分子動力学、大規模殻模型計算などが計画されている。これらで得られた信頼性の高い光核反応データベースと宇宙線伝搬コードを組み合わせ、超高エネルギー宇宙線の起源の解明に挑む。

論文

A One-third magnetization plateau phase as evidence for the Kitaev interaction in a honeycomb-lattice antiferromagnet

Shangguan, Y.*; Bao, S.*; Dong, Z.-Y.*; Xi, N.*; Gao, Y.-P.*; Ma, Z.*; Wang, W.*; Qi, Z.*; Zhang, S.*; Huang, Z.*; et al.

Nature Physics, 19(12), p.1883 - 1889, 2023/09

https://doi.org/10.1038/s41567-023-02212-2
 被引用回数：19 パーセンタイル：94.19(Physics, Multidisciplinary)

The magnetization of a quantum magnet can be pinned at a fraction of its saturated value by collective effects. One example of such a plateau phase is found in spin-1/2 triangular-lattice antiferromagnets. They feature strong geometrical frustration and the plateau phase therein is often interpreted as arising from an order-by-disorder mechanism driven by quantum fluctuations. Here we observe a one-third magnetization plateau under an applied magnetic field in the spin-1 antiferromagnet Na$$_{3}$$Ni$$_{2}$$BiO$$_{6}$$ with a honeycomb lattice, which, with conventional magnetic interactions, would not be geometrically frustrated. Based on our elastic neutron scattering measurements, we propose the spin structure of the plateau phase to be an unusual partial spin-flop ferrimagnetic order. Our theoretical calculations indicate that bond-anisotropic Kitaev interactions are the source of frustration that produces the plateau. These results suggest that Kitaev interactions provide a different route to frustration and phases driven by quantum fluctuations in high-spin magnets.

論文

Evidence of nonstatistical neutron emission following $$beta$$ decay near doubly magic $$^{132}$$Sn

Heideman, J.*; Grzywacz, R.*; Xu, Z. Y.*; Madurga, M.*; Escher, J. E.*; 河野 俊彦*; Algora, A.*; Andreyev, A. N.; 他41名*

Physical Review C, 108(2), p.024311_1 - 024311_9, 2023/08

https://doi.org/10.1103/PhysRevC.108.024311
 被引用回数：3 パーセンタイル：45.98(Physics, Nuclear)

$$beta$$-delayed neutron emission was observed in the study of the $$beta$$ decay of $$^{134}$$In at ISOLDE CERN. Neutron emission probabilities from the unbound states in $$^{134}$$Sn to known low-lying, single-particle states in $$^{133}$$Sn were measured. The neutron energies were determined using the time-of-flight technique and the decay from excited states in $$^{133}$$Sn was studied by detecting its $$gamma$$ rays. Individual $$beta$$-delayed neutron emission probabilities were determined by correlating the relative intensities and energies of neutrons and $$gamma$$ rays. The new results suggest the violation of the assumption that neutrons are emitted statistically via the intermediate compound nucleus. This impacts the neutron-emission probabilities and other properties of nuclei participating in the $$r$$-process. A model of neutron emission, which links the observed neutron emission probabilities to nuclear shell effects, is proposed.

論文

Level structures of $$^{56,58}$$Ca cast doubt on a doubly magic $$^{60}$$Ca

Chen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; 角田 佑介*; 大塚 孝治*; 茶園 亮樹*; Hagen, G.*; Holt, J. D.*; et al.

Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08

https://doi.org/10.1016/j.physletb.2023.138025
 被引用回数：9 パーセンタイル：85.35(Astronomy & Astrophysics)

$$^{57,59}$$Scからの1陽子ノックアウト反応を用いて、$$^{56}$$Caと$$^{58}$$Caのガンマ崩壊を観測した。$$^{56}$$Caでは1456(12)keVの$$gamma$$線遷移が、$$^{58}$$Caでは1115(34)keVの遷移が観測された。どちらの遷移も暫定的に$$2^{+}_{1} rightarrow 0^{+}_{gs}$$と割り当てられた。有効核子間相互作用をわずかに修正した広い模型空間での殻模型計算では、$$2^{+}_{1}$$準位エネルギー、2中性子分離エネルギー、反応断面積が実験とよく一致し、N=34閉殻の上に新しい殻が形成されていることを裏付けた。その構成要素である$$0_{f5/2}$$と$$0_{g9/2}$$軌道はほぼ縮退しており、これは$$^{60}$$Caが二重魔法核である可能性を排除し、Ca同位体のドリップラインを$$^{70}$$Caあるいはそれ以上にまで広げる可能性がある。

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