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論文

Spin dynamics in natural multiferroic pyroxene NaFeSi$$_2$$O$$_6$$

Prokhnenko, O.*; Nikitin, S. E.*; 金子 耕士; 田端 千紘; 廣瀬 雄介; 常盤 欣文; 芳賀 芳範; 藤田 全基; 野尻 浩之*; Anovitz, L. M.*; et al.

Physical Review B, 112(9), p.094402_1 - 094402_7, 2025/09

https://doi.org/10.1103/tb2z-skj1
 被引用回数：0

The spin dynamics in the natural mineral aegirine, NaFeSi$$_2$$O$$_6$$, a member of the pyroxene family, was studied using elastic and inelastic neutron scattering. Magnetization and specific heat measurements as well as single-crystal neutron diffraction maps confirm two successive magnetic transitions at 8.8 and 5.8~K, consistent with previous studies. The observed spin-wave excitations emerge from the incommensurate magnetic Bragg peaks corresponding to the propagation vector $$k_{rm ICM} = (0, 0.77, 0)$$, and extend up to energies of about 1.5 meV. In the low-temperature helical phase, the spin dynamics of the Fe$$^{3+}$$ ions is well described by a simple linear spin-wave model. The observed excitations can be modeled using a spin Hamiltonian that includes three primary exchange interactions. Our results show that no single exchange interaction dominates the spin dynamics. The similar strengths of the intrachain and interchain couplings point to the fact that the magnetic interactions in aegirine are three-dimensional, rather than being confined along one direction. As a result, the system cannot be considered quasi-one-dimensional, as previously suggested, and calls for further investigations.

論文

長期観測結果に基づく防振建物に設置された厚肉積層ゴムのクリープ特性推定の試み

正木 信男*; 室田 伸夫*; 加藤 亨二*; 岡村 茂樹; 山本 智彦; 内田 昌人*; 藤田 聡*

日本建築学会技術報告集, 31(78), p.687 - 692, 2025/06

https://doi.org/10.3130/aijt.31.687

実際の免震建物に55.2年設置された天然ゴム系の厚肉積層ゴムのクリープ特性を、既存測定データと新規測定データを用いて推定した。JIS K6410-2で推奨されている単回帰分析での結果、平均クループ変位特性はべき乗則で説明できることが分かった。その回帰式より、建物に設置された厚肉積層ゴムの平均クリープ量は3.4mmと推定された。その結果から、JIS K6410-2の方法は、クリープ変位の予測に役立つものと考えられる。

論文

Development of a compact ${it in situ}$ $$^{3}$$He neutron spin filter at J-PARC

高橋 慎吾; 鬼柳 亮嗣; 奥平 琢也*; 高田 秀佐*; 小林 龍珠; 奥泉 舞桜; 猪野 隆*; 浅井 寛太*; 土川 雄介; 及川 健一; et al.

Nuclear Instruments and Methods in Physics Research A, 1075, p.170410_1 - 170410_8, 2025/06

https://doi.org/10.1016/j.nima.2025.170410
 被引用回数：0 パーセンタイル：0.00(Instruments & Instrumentation)

This study developed a compact and portable in-situ $$^{3}$$He neutron spin filter (${it in situ}$ $$^{3}$$He NSF) utilizing spin-exchange optical pumping at MLF of J-PARC. Its performance as an incident neutron polarizer was evaluated at MLF, where it achieved a $$^{3}$$He polarization exceeding 0.6, corresponding to a neutron polarization greater than 0.8 at 1.8 ${AA}$. Notably, the ${it in situ}$ $$^{3}$$He NSF demonstrated stable operation for 110 h. These outcomes signify that the developed in-situ $$^{3}$$He NSF facilitates and promotes polarized pulsed neutron experiments at MLF.

論文

Magnetic excitations in the noncentrosymmetric magnet Sr$$_{2}$$MnSi$$_{2}$$O$$_{7}$$

川又 雅広*; Pang, X.*; 村川 寛*; 河村 聖子; 中島 健次; 増田 英敏*; 藤田 全基*; 花咲 徳亮*; 小野瀬 佳文*; 南部 雄亮*

Physical Review Materials (Internet), 9(1), p.014407_1 - 014407_6, 2025/01

https://doi.org/10.1103/PhysRevMaterials.9.014407
 被引用回数：1 パーセンタイル：0.00(Materials Science, Multidisciplinary)

Magnetic excitations in the noncentrosymmetric magnet Sr$$_{2}$$MnSi$$_{2}$$O$$_{7}$$ were investigated through inelastic neutron scattering measurements. Major magnetic excitations are limited up to the energy transfer of 0.5 meV, and two magnon branches under zero magnetic field were well explained in the framework of linear spinwave theory. The magnitudes of the square-lattice in-plane and interplane nearest-neighbor interactions, spin anisotropy term, and the Dzyaloshinskii-Moriya interaction are, respectively, estimated to be J$$_{1}$$ = 45.54(5) $$mu$$eV, J$$_{2}$$ = 0.52(1) $$mu$$eV, = 4.98(11) $$mu$$eV, D$$_{xy}$$ = 0.02(9) $$mu$$eV, and D$$_{z}$$ = 4.10(1) $$mu$$eV, and calculations using these parameters reproduce experimental data quite well. Sr$$_{2}$$MnSi$$_{2}$$O$$_{7}$$ appears to have the smallest energy scale among the melilite-type compounds, and the small J$$_{2}$$/J$$_{1}$$ = 0.0114(2) indicates the strong two dimensionality.

論文

Research and development of three-dimensional isolation system for sodium cooled fast reactor, 9; Evaluating seismic isolation performance through seismic response analysis

深沢 剛司*; 杣木 孝裕*; 湯川 正貴*; 平山 智之*; 渡壁 智祥; 山本 智彦; 岡村 茂樹; 宮崎 真之; 内田 昌人*; 宮川 高行; et al.

Proceedings of ASME 2024 Pressure Vessels & Piping Conference (PVP 2024) (Internet), 10 Pages, 2024/07

https://doi.org/10.1115/PVP2024-121899

This paper elucidates the isolation performance of a newly developed three-dimensional seismic isolation system through seismic response analysis. A novel three-dimensional isolation system was developed and assessed through static loading tests, aiming to unveil the hysteresis loops for each element, labeled Part 1 to Part 6. To ascertain the design feasibility of the isolation system, static loading tests were judiciously conducted, considering a wide array of loading conditions, including the beyond-design basis ground motion. Employing the accumulated test data, a new analytical model was devised, capable of precisely capturing the hysteresis loops for each element. Evaluating the seismic isolation performance based on the static loading results of the entire system posed a notable challenge. Nevertheless, the hysteresis characteristics of the overall system in both horizontal and vertical directions were elucidated using a static loading test with a half-scale model, as detailed in Part 7 and Part 8. The authors conducted a seismic response analysis, leveraging the analytical models identified by the static loading test results obtained from the half-scale model. This paper demonstrates that our isolation system exhibits superior isolation performance against both the design basis and beyond-design basis ground motions when compared to a horizontal isolation system consisting of rubber bearings and oil dampers.

論文

Research and development of three-dimensional isolation system for sodium cooled fast reactor, 7; Development summary of three-dimensional isolation system

渡壁 智祥; 山本 智彦; 岡村 茂樹; 宮崎 真之; 宮川 高行; 内田 昌人*; 平山 智之*; 杣木 孝裕*; 湯川 正貴*; 深沢 剛司*; et al.

Proceedings of ASME 2024 Pressure Vessels & Piping Conference (PVP 2024) (Internet), 10 Pages, 2024/07

ナトリウム冷却高速炉では、薄肉の機械部品や配管の耐震安全性を厳しい設計地震レベルで確保するため、3次元免震装置を開発している。開発成果の進捗をシリーズ(Part7$$sim$$Part9)発表する。Part7では、研究開発の全体概要、各要素を組み立てた状態での3次元免震装置の試験計画、および構成要素の性能について紹介する。Part8では、各要素を組み立てた状態での3次元免震装置の性能を負荷試験を通じて調査した。Part9では、試験結果で得た知見に基づき検証した解析モデルによる3次元免震装置の効果を報告する。

論文

Research and development of three-dimensional isolation system for sodium-cooled fast reactor, 8; Assembly static test results of three-dimensional isolated device by bi-axial loadings

杣木 孝裕*; 湯川 正貴*; 深沢 剛司*; 平山 智之*; 内田 昌人*; 宮川 高行; 岡村 茂樹; 山本 智彦; 渡壁 智祥; 宮崎 真之; et al.

Proceedings of ASME 2024 Pressure Vessels & Piping Conference (PVP 2024) (Internet), 9 Pages, 2024/07

https://doi.org/10.1115/PVP2024-124495

The authors have been developing the three-dimensional isolation system for the Sodium-cooled Fast Reactor. The three-dimensional isolation device consists of the laminated rubber bearing performing the horizontal isolation function, four-disc spring units, the sliding function, strength members such as the horizontal support function, and dampers in the horizontal and vertical directions. We carried out the half-scaled integrated seismic tests under several bi-axial severe conditions from design base loads to significantly exceeding design base loads. The test specimen was assembled elements consisting of Three-Dimensional Seismic Isolation System, but the horizontal and vertical damping devices were not modeled because of the static tests. We report tests results, focusing on the following items. Behavior of smooth operation and ensuring the independency of horizontal isolation and vertical isolation performances. Hypothesis and verification of load transfer mechanism under horizontal and vertical loads superposition. Effect of reinforcing plates on the loading force reduction of horizontal support function. Conditions of the specimen after tests and discussion.

論文

Local atomic displacements and sign of the structural transformation in medium-entropy alloys observed in extended X-ray absorption fine structure spectra

池田 陽一*; 梅本 好日古*; 松村 大樹; 辻 卓也; 橋本 勇輝*; 北澤 崇文*; 藤田 全基*

Materials Transactions, 64(9), p.2254 - 2260, 2023/09

https://doi.org/10.2320/matertrans.MT-M2023043
 被引用回数：4 パーセンタイル：40.61(Materials Science, Multidisciplinary)

Extended X-ray absorption fine structure (EXAFS) and neutron diffraction experiments were carried out to clarify the typical features of the local structure of a family of medium-entropy alloys (CrCoNi, MnCoNi, and FeCoNi). A simple random cluster model was constructed for analyzing EXAFS spectra, and static and dynamic components of the mean-square relative displacement (MSRD) were separately extracted. In our analysis, the static MSRD of the MnCoNi sample was slightly larger than those of the CrCoNi and FeCoNi samples, whereas the dynamic MSRDs of these samples were almost identical. Based on the complementary neutron diffraction data, we argued that the origin of the large static displacement in the MnCoNi alloy can be associated with a short-range structural transformation through long-term structural relaxation.

論文

高速炉向け3次元免震システムの研究開発(1/2縮尺サイズの試験体を用いた静的特性に関する試験的検討)

深沢 剛司*; 平山 智之*; 横井 忍*; 廣田 昭彦*; 杣木 孝裕*; 湯川 正貴*; 宮川 高行; 内田 昌人*; 山本 智彦; 宮崎 真之; et al.

日本機械学会論文集(インターネット), 89(924), p.23-00023_1 - 23-00023_17, 2023/08

https://doi.org/10.1299/transjsme.23-00023

ナトリウム冷却高速炉の耐震性向上の観点で研究開発を進めている3次元免震装置開発に関して、そのシステムの概要を述べるとともに、1/2縮尺試験体を用いた静的載荷試験結果について、その知見を述べる。

論文

Observation of field-induced single-ion magnetic anisotropy in a multiorbital Kondo alloy (Lu,Yb)Rh$$_2$$Zn$$_{20}$$

北澤 崇文; 池田 陽一*; 榊原 俊郎*; 松尾 晶*; 清水 悠晴*; 徳永 陽; 芳賀 芳範; 金道 浩一*; 南部 雄亮*; 池内 和彦*; et al.

Physical Review B, 108(8), p.085105_1 - 085105_7, 2023/08

https://doi.org/10.1103/PhysRevB.108.085105
 被引用回数：0 パーセンタイル：0.00(Materials Science, Multidisciplinary)

We demonstrate field-induced single-ion magnetic anisotropy resulting from the multiorbital Kondo effect on diluted ytterbium alloy (Lu$$_{1-x}$$Yb$$_x$$)Rh$$_2$$Zn$$_{20}$$. Single-ion anisotropic metamagnetic behavior is revealed in low-temperature regions where the local Fermi-liquid state is formed. Specific heat, low-field magnetic susceptibility, and resistivity indicate reproduction of the ground-state properties by the SU($$N$$ = 8) Kondo model with a relatively large $$c$$-$$f$$ hybridization of $$T_{rm K}$$ = 60.9 K. Dynamical susceptibility measurements on YbRh$$_2$$Zn$$_{20}$$ support realizing multiorbital Kondo ground state in (Lu$$_{1-x}$$Yb$$_x$$)Rh$$_2$$Zn$$_{20}$$. The single-ion magnetic anisotropy becomes evident above $$sim$$5 T, which is lower than the isotropic Kondo crossover field of 22.7 T, verifying blurred low-lying crystal field states through the multiorbital Kondo effect.

論文

Cu $$K$$-edge X-ray absorption fine structure study of $$T'$$-type $$RE$$$$_{2}$$CuO$$_{4+alpha-delta}$$ ($$RE$$ = Rare Earth); Toward unified understanding of electronic state of $$T'$$-type cuprate

Chen, Y.*; 浅野 駿*; Wang, T.*; Xie, P.*; 北山 慎之介*; 石井 賢司*; 松村 大樹; 辻 卓也; 谷口 貴紀*; 藤田 全基*

JPS Conference Proceedings (Internet), 38, p.011050_1 - 011050_6, 2023/05

https://doi.org/10.7566/JPSCP.38.011050

To investigate the variation of the electronic state of $$T'$$-type cuprate due to annealing, we performed Cu $$K$$-edge X-ray absorption fine structure measurements on Pr$$_{2}$$CuO$$_{4+alpha-delta}$$ (PCO) and Pr$$_{1.3}$$La$$_{0.7}$$CuO$$_{4+alpha-delta}$$ (PLCO). The induced electrons due to annealing ($$n_{AN}$$) in PCO and PLCO were approximately 2$$delta$$, consistent with a model of electron doping to Mott insulator. Here, $$alpha$$ and $$delta$$ represent the amount of excess oxygen from the stoichiometric composition in the as-sintered compound and that of oxygen loss due to annealing, respectively. Furthermore, the energy of the Einstein oscillator ($$hbaromega_{E}$$) for the Cu-O$$_{p}$$ bond was evaluated by extended X-ray absorption fine structure analysis. (O$$_{p}$$ denotes the in-plane oxygen.) We found a small annealing effect on $$hbaromega_{E}$$ for both PCO and PLCO.

論文

実建物の47年間の観測による厚肉積層ゴムのクリープ挙動

正木 信男*; 加藤 亨二*; 山本 智彦; 宮川 高行*; 藤田 聡*; 岡村 茂樹*

日本建築学会技術報告集, 28(68), p.81 - 84, 2022/02

https://doi.org/10.3130/aijt.28.81

高速炉等の新型炉では機器の耐震性を確保するため、厚肉積層ゴムの採用が検討されているが、厚肉積層ゴムのもつ柔らかな上下剛性は、経年によるゴム物性の変化とクリープに大きく影響されると考える。われわれはゴム物性の変化を考慮できるクリープ評価方法を検討しているが、参照すべき実大かつ実環境下の長期クリープ特性がない。本報告では、厚肉積層ゴムの新たなクリープ評価方法を検討するための第1段階として、この形式の初めての建物である1966年に竣工した厚肉積層ゴム支持の英国防振建物の測定データを集約し厚肉積層ゴムの約47年間のクリープ特性推定の試みについて述べる。

論文

Spin excitations coupled with lattice and charge dynamics in La$$_{2-x}$$Sr$$_{x}$$CuO$$_{4}$$

池内 和彦*; 脇本 秀一; 藤田 全基*; 福田 竜生; 梶本 亮一; 新井 正敏*

Physical Review B, 105(1), p.014508_1 - 014508_7, 2022/01

https://doi.org/10.1103/PhysRevB.105.014508
 被引用回数：4 パーセンタイル：23.19(Materials Science, Multidisciplinary)

Spin excitations of layered copper oxide show various characteristic features, depending on the carrier concentration. In this paper, we conducted inelastic neutron-scattering measurements on La$$_{2-x}$$Sr$$_{x}$$CuO$$_{4}$$ (LSCO) with $$x$$ = 0, 0.075, 0.18, and 0.30 and La$$_{2-x}$$Sr$$_{x}$$NiO$$_{4}$$ (LSNO) with 1/3 to clarify the origin of the intensity enhancement in the excitation spectrum of LSCO at the energy ($$omega$$) of 16-19 meV [Phys. Rev. B $textbf{91}$, 224404 (2015), $textit{ibid.}$ $textbf{93}$, 094416 (2016)]. We confirmed the presence of a peak structure in the $$omega$$ dependence of the local spin susceptibility $$chi''(omega)$$ of superconducting (SC) LSCO with a peak energy of 16-19 meV where the spin excitations intersect optical phonon branches. A comparable peak structure is not observed in the insulating La$$_{2}$$CuO$$_{4}$$, LSNO, and heavily overdoped LSCO with $$x$$ = 0.30. A dome-shaped $$x$$ dependence of the integrated intensity around the peak energies is revealed for the SC phase by summarizing the present and previously reported results. Furthermore, our phonon calculation on LCO shows the existence of two optical branches at $$sim$$19 meV that could stabilize stripe alignment of carriers due to out-of-plane vibrations of Cu or O of the CuO$$_{2}$$ planes. These results indicate the interplay among spin, charge, and lattice dynamics and suggest that the intensity enhancement is associated with their composite excitations.

論文

Distinct variation of electronic states due to annealing in $$T'$$-type La$$_{1.8}$$Eu$$_{0.2}$$CuO$$_{4}$$ and Nd$$_{2}$$CuO$$_{4}$$

浅野 駿*; 石井 賢司*; 松村 大樹; 辻 卓也; 工藤 康太*; 谷口 貴紀*; 齋藤 真*; 春原 稔樹*; 川股 隆行*; 小池 洋二*; et al.

Physical Review B, 104(21), p.214504_1 - 214504_7, 2021/12

https://doi.org/10.1103/PhysRevB.104.214504
 被引用回数：2 パーセンタイル：9.93(Materials Science, Multidisciplinary)

We performed Cu K-edge X-ray absorption fine-structure measurements on $$T'$$-type La$$_{1.8}$$Eu$$_{0.2}$$CuO$$_{4}$$ (LECO) and Nd$$_{2}$$CuO$$_{4}$$ (NCO) to investigate the variation in the electronic state associated with the emergence of superconductivity due to annealing. The X-ray absorption near-edge structure spectra of as-sintered (AS) LECO are quite similar to those of AS NCO, indicating that the ground state of AS LECO is a Mott insulator. The electron density after annealing $$n_{rm AN}$$ was evaluated for both superconducting LECO and nonsuperconducting NCO and was found to be 0.40 and 0.05 electron per Cu atom, respectively. In LECO but not in NCO, extended X-ray absorption fine-structure analysis revealed a reduction in the strength of the Cu-O bond in the CuO$$_{2}$$ plane due to annealing, which is consistent with the screening effect on phonons in the metallic state. The origin of the difference in doping processes due to annealing is discussed in relation to the size of the charge-transfer gap.

論文

Triplon current generation in solids

Chen, Y.*; 佐藤 正寛*; Tang, Y.*; 塩見 雄毅*; 大柳 洸一*; 益田 隆嗣*; 南部 雄亮*; 藤田 全基*; 齊藤 英治

Nature Communications (Internet), 12, p.5199_1 - 5199_7, 2021/08

https://doi.org/10.1038/s41467-021-25494-7
 被引用回数：16 パーセンタイル：68.24(Multidisciplinary Sciences)

A triplon refers to a fictitious particle that carries angular momentum $$S=1$$ corresponding to the elementary excitation in a broad class of quantum dimerized spin systems. Such systems without magnetic order have long been studied as a testing ground for quantum properties of spins. Although triplons have been found to play a central role in thermal and magnetic properties in dimerized magnets with singlet correlation, a spin angular momentum flow carried by triplons, a triplon current, has not been detected yet. Here we report spin Seebeck effects induced by a triplon current: triplon spin Seebeck effect, using a spin-Peierls system CuGeO$$_3$$. The result shows that the heating-driven triplon transport induces spin current whose sign is positive, opposite to the spin-wave cases in magnets. The triplon spin Seebeck effect persists far below the spin-Peierls transition temperature, being consistent with a theoretical calculation for triplon spin Seebeck effects.

論文

島原半島北部の唐比低地における湿地堆積物の形成過程

中西 利典*; 奥野 充*; 山崎 圭二*; Hong, W.*; 藤田 奈津子; 中村 俊夫*; 堀川 義之*; 佐藤 鋭一*; 木村 治夫*; 堤 浩之*

名古屋大学年代測定研究,5, p.38 - 43, 2021/03

雲仙火山の約13km西方にある唐比低地には泥炭層や泥層からなる湿地堆積物が厚く分布しており、それらの堆積物には千々石断層や雲仙火山の活動履歴が記録されていることが期待される。それらの履歴を精度よく検知するために、複数本のボーリングコアを掘削して放射性炭素年代値を測定した。それらの結果を地中レーダ探査断面と対比して湿地堆積物の形成過程を検討した。その結果得られたすべての$$^{14}$$C年代値は層序関係と矛盾がなく、堆積曲線は若干のずれが認められるが概ね一致する結果となった。本研究の年代測定の一部はペレトロン年代測定装置による施設供用利用で行われたものである。

論文

Magnetic excitations of Sr$$_{3}$$Ir$$_{2}$$O$$_{7}$$ observed by inelastic neutron scattering technique

藤田 全基*; 池内 和彦*; 梶本 亮一; 中村 充孝

Journal of the Physical Society of Japan, 90(2), p.025001_1 - 025001_2, 2021/02

https://doi.org/10.7566/JPSJ.90.025001
 被引用回数：1 パーセンタイル：11.14(Physics, Multidisciplinary)

In this short note, we report on the first inelastic neutron scattering (INS) study on high-energy magnetic excitations in Sr$$_{3}$$Ir$$_{2}$$O$$_{7}$$. We observed excitations between $$sim$$80 meV and $$sim$$180 meV. The peak position of the excitations is consistent with the dispersion of a single magnon determined by resonant inelastic X-ray scattering (RIXS) measurement. Thus, our results demonstrate the feasibility of INS for iridates, which has a large neutron absorption cross-section.

論文

Coexistence of two components in magnetic excitations of La$$_{2-x}$$Sr$$_{x}$$CuO$$_{4}$$ ($$x$$ = 0.10 and 0.16)

佐藤 研太朗*; 池内 和彦*; 梶本 亮一; 脇本 秀一; 新井 正敏*; 藤田 全基*

Journal of the Physical Society of Japan, 89(11), p.114703_1 - 114703_7, 2020/11

https://doi.org/10.7566/JPSJ.89.114703
 被引用回数：9 パーセンタイル：53.30(Physics, Multidisciplinary)

To elucidate the spin dynamics of La$$_{2-x}$$Sr$$_{x}$$CuO$$_{4}$$, which couples with the charge degree of freedom, the spin excitations spanning the characteristic energy ($$E_mathrm{cross}$$ $$sim$$ 35-40 meV) are investigated for underdoped $$x$$ = 0.10 and optimally doped (OP) $$x$$ = 0.16 through inelastic neutron scattering measurements. Analysis based on a two-component picture of high-quality data clarified the possible coexistence of upright standing incommensurate (IC) excitations with gapless commensurate (C) excitations in the energy-momentum space. The IC component weakens the intensity toward $$E_mathrm{cross}$$ with increasing energy transfer ($$hbaromega$$), whereas the C component strengthens at high-$$hbaromega$$ regions. The analysis results imply that the superposition of two components with a particular intensity balance forms an hourglass-shaped excitation in appearance. Furthermore, the temperature dependence of the intensity of each component exhibits different behaviors; the IC component disappears near the pseudo-gap temperature ($$T^*$$) upon warming, whereas the C component is robust against temperature. These results suggest the itinerant electron spin nature and the localized magnetism of the parent La$$_{2}$$CuO$$_{4}$$ in IC and C excitations, respectively, similar to the spin excitations in the OP YBa$$_{2}$$Cu$$_{3}$$O$$_{6+delta}$$ and HgBa$$_{2}$$CuO$$_{4+delta}$$ with higher superconducting-transition temperatures.

論文

Observation of magnon polarization

南部 雄亮*; Barker, J.*; 沖野 夕貴*; 吉川 貴史*; 塩見 雄毅*; Enderle, M.*; Weber, T.*; Winn, B.*; Graves-Brook, M.*; Tranquada, J. M.*; et al.

Physical Review Letters, 125(2), p.027201_1 - 027201_6, 2020/07

https://doi.org/10.1103/PhysRevLett.125.027201
 被引用回数：69 パーセンタイル：94.45(Physics, Multidisciplinary)

We measure the mode-resolved direction of the precessional motion of the magnetic order, i.e., magnon polarization, via the chiral term of inelastic polarized neutron scattering spectra. The magnon polarization is a unique and unambiguous signature of magnets and is important in spintronics, affecting thermodynamic properties such as the magnitude and sign of the spin Seebeck effect. However, it has never been directly measured in any material until this work. The observation of both signs of magnon polarization in Y$$_3$$Fe$$_5$$O$$_{12}$$ also gives direct proof of its ferrimagnetic nature. The experiments agree very well with atomistic simulations of the scattering cross section.

論文

Crystal structures of highly hole-doped layered perovskite nickelate Pr$$_{2-x}$$Sr$$_{x}$$NiO$$_{4}$$ studied by neutron diffraction

梶本 亮一; 中島 健次; 藤田 全基*; 石角 元志*; 鳥居 周輝*; 石川 喜久*; Miao, P.*; 神山 崇*

Journal of the Physical Society of Japan, 88(11), p.114602_1 - 114602_6, 2019/11

https://doi.org/10.7566/JPSJ.88.114602
 被引用回数：0 パーセンタイル：0.00(Physics, Multidisciplinary)

A high-resolution time-of-flight powder neutron diffraction study of the layered nickel oxide Pr$$_{2-x}$$Sr$$_{x}$$NiO$$_{4}$$ with $$x = 0.7$$ and $$0.9$$ was performed to characterize the crystal structures of these highly hole-doped nickelates. For the sample with $$x = 0.7$$, the Ni-O bond lengths decrease uniformly with decreasing temperature, and the atomic displacement parameters are similar to those for $$x = 1/3$$. In contrast, for the sample with $$x = 0.9$$, the out-of-plane Ni-O bond length shows a sharp thermal contraction in the high-temperature region, which is suggestive of changes in the orbital occupation accompanied by the development of checkerboard-type charge correlations. Furthermore, the $$x = 0.9$$ sample is characterized by a large atomic displacement parameter for the apical O atoms along the out-of-plane direction, which is interpreted as the existence of two types of Ni$$^{3+}$$ sites with different orbital occupancies. The distinct difference between the $$x = 0.9$$ sample and the lower-concentration compounds should be related to the development of checkerboard-type charge ordering in the metallic matrix and possible orbital ordering at the Ni$$^{3+}$$ sites at $$x sim 1$$ in the hole-doped layered nickel oxides.

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