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論文

Temperature-dependent hardening contributions in CrFeCoNi high-entropy alloy

Naeem, M.*; He, H.*; Harjo, S.; 川崎卓郎; Lin, W.*; Kai, J.-J.*; Wu, Z.*; Lan, S.*; Wang, X.-L.*

Acta Materialia, 221, p.117371_1 - 117371_18, 2021/12

https://doi.org/10.1016/j.actamat.2021.117371

We studied the deformation behavior of CrFeCoNi high-entropy alloy by in situ neutron diffraction at room temperature, intermediate low temperature of 140 K, low temperatures of 40 K (no serrated deformation) and 25 K (with massive serrations). The contributions from different deformation mechanisms to the yield strength and strain hardening have been estimated. The athermal contributions to the yield strength were 183 MPa at all temperatures, while the Peierls stress increased significantly at low temperatures (from 148 MPa at room temperature to 493 MPa at 25 K). Dislocations contributed to 94% strain hardening at room temperature. Although the dislocation strengthening remained the major hardening mechanism at very low temperatures, the planar faults contribution increased steadily from 6% at room temperature to 28% at 25 K.

論文

Long decay length of magnon-polarons in BiFeO $_{3}$ /La $_{0.67}$ Sr $_{0.33}$ MnO $_{3}$ heterostructures

Zhang, J.*; Chen, M.*; Chen, J.*; 山本慧; Wang, H.*; Hamdi, M.*; Sun, Y.*; Wagner, K.*; He, W.*; Zhang, Y.*; et al.

Nature Communications (Internet), 12(1), p.7258_1 - 7258_8, 2021/12

https://doi.org/10.1038/s41467-021-27405-2

Magnons can transfer information in metals and insulators without Joule heating, and therefore are promising for low-power computation. The on-chip magnonics however suffers from high losses due to limited magnon decay length. In metallic thin films, it is typically on the tens of micrometre length scale. Here, we demonstrate an ultra-long magnon decay length of up to one millimetre in multiferroic/ferromagnetic BiFeO $_{3}$ (BFO)/La $_{0.67}$ Sr $_{0.33}$ MnO $_{3}$ (LSMO) heterostructures at room temperature. This decay length is attributed to a magnon-phonon hybridization and is more than two orders of magnitude longer than that of bare metallic LSMO. The long-distance modes have high group velocities of 2.5 km $^{-1}$ as detected by time-resolved Brillouin light scattering. Numerical simulations suggest that magnetoelastic coupling via the BFO/LSMO interface hybridizes phonons in BFO with magnons in LSMO. Our results provide a solution to the long-standing issue on magnon decay lengths in metallic magnets and advance the bourgeoning field of hybrid magnonics.

論文

Martensitic transformation in CrCoNi medium-entropy alloy at cryogenic temperature

Naeem, M.*; Zhou, H.*; He, H.*; Harjo, S.; 川崎卓郎; Lan, S.*; Wu, Z.*; Zhu, Y.*; Wang, X.-L.*

Applied Physics Letters, 119(13), p.131901_1 - 131901_7, 2021/09

https://doi.org/10.1063/5.0067268

We investigated the in situ deformation behavior of the CrCoNi medium-entropy alloy at a cryogenic temperature of 140 K and compared it with deformation at room temperature. The sample exhibited higher strength and larger ductility at the cryogenic temperature. The CrCoNi alloy remained single-phase face-centered cubic at room temperature, while deformation at 140 K resulted in a martensitic transformation to the hexagonal close-packed structure. The phase transformation, an additional deformation mechanism to stacking faults, twinning, and dis- location slip, resulted in a higher work hardening at cryogenic temperature. The study addresses the structure metastability in the CrCoNi alloy, which led to the formation of epsilon-martensite from the intrinsic stacking faults.

論文

Phase transition and chemical reactivity of 1H-tetrazole under high pressure up to 100 GPa

Gao, D.*; Tang, X.*; Wang, X.*; Yang, X.*; Zhang, P.*; Che, G.*; Han, J.*; 服部高典; Wang, Y.*; Dong, X.*; et al.

Physical Chemistry Chemical Physics, 23(35), p.19503 - 19510, 2021/09

https://doi.org/10.1039/D1CP02913D

被引用回数：0 パーセンタイル：0.01(Chemistry, Physical)

窒素に富む分子の圧力有機相転移や重合は、環境にやさしい高エネルギー密度材料の開発にとって非常に重要であるため、広く注目されている。本論文では、その場ラマン,IR,X線回折,中性子回折、および理論計算をもちい、100GPaまでの1H-テトラゾールの相転移挙動と化学反応の研究を紹介する。2.6GPa以上での相転移が確認され、その高圧構造は、以前に報告されたユニットセル内に2つの分子をもつものではなく、1つの分子をものであることが分かった。1H-テトラゾールは、おそらく窒素-窒素結合ではなく炭素-窒素結合により、100GPa以下で可逆的に重合する。私たちの研究は、1H-テトラゾールの高圧相の構造モデルを更新し、もっともらしい分子間結合の経路を初めて提示した。これにより、窒素に富む化合物の相転移と化学反応の理解が進み、新しい高エネルギー密度材料の設計に役立つと考えられる。

論文

Stacking fault driven phase transformation in CrCoNi medium entropy alloy

He, H.*; Naeem, M.*; Zhang, F.*; Zhao, Y.*; Harjo, S.; 川崎卓郎; Wang, B.*; Wu, X.*; Lan, S.*; Wu, Z.*; et al.

Nano Letters, 21(3), p.1419 - 1426, 2021/02

https://doi.org/10.1021/acs.nanolett.0c04244

被引用回数：3 パーセンタイル：0(Chemistry, Multidisciplinary)

In CrCoNi, a so-called medium-entropy alloy, an fcc-to-hcp phase transformation has long been anticipated. Here, we report an in situ loading study with neutron diffraction, which revealed a bulk fcc-to-hcp phase transformation in CrCoNi at 15 K under tensile loading. By correlating deformation characteristics of the fcc phase with the development of the hcp phase, it is shown that the nucleation of the hcp phase was triggered by intrinsic stacking faults. The confirmation of a bulk phase transformation adds to the myriads of deformation mechanisms available in CrCoNi, which together underpin the unusually large ductility at low temperatures.

論文

Ultra-fine CeO $_{2}$ particles triggered strong interaction with LaFeO $_{3}$ framework for total and preferential CO oxidation

Zheng, Y.*; Xiao, H.*; Li, K.*; Wang, Y.*; Li, Y.*; Wei, Y.*; Zhu, X.*; Li, H.-W.*; 松村大樹; Guo, B.*; et al.

ACS Applied Materials & Interfaces, 12(37), p.42274 - 42284, 2020/09

https://doi.org/10.1021/acsami.0c10271

被引用回数：4 パーセンタイル：51.8(Nanoscience & Nanotechnology)

Interactions between the active components with the support are one of the fundamentally factors in determining the catalytic performance of a catalyst. In this study, we investigated the interaction between CeO $_{2}$ and LaFeO $_{3}$ , the two important oxygen storage materials in catalysis area, by tuning the sizes of CeO $_{2}$ particles and highlight a two-fold effect of the strong oxide-oxide interaction in determining the catalytic activity and selectivity for preferential CO oxidation in hydrogen feeds. It is found that the anchoring of ultra-fine CeO $_{2}$ particles at the framework of three-dimensional-ordered macroporous LaFeO $_{3}$ surface results in a strong interaction between the two oxides that induces the formation of abundant uncoordinated cations and oxygen vacancy at the interface. This discovery demonstrates that in hybrid oxide-based catalysts, tuning the interaction among different components is essential for balancing the catalytic activity and selectivity.

論文

Comparison of dislocation density, twin fault probability, and stacking fault energy between CrCoNi and CrCoNiFe medium entropy alloys deformed at 293 and 140K

Woo, W.*; Naeem, M.*; Jeong, J.-S.*; Lee, C.-M.*; Harjo, S.; 川崎卓郎; He, H.*; Wang, X.-L.*

Materials Science & Engineering A, 781, p.139224_1 - 139224_7, 2020/04

https://doi.org/10.1016/j.msea.2020.139224

被引用回数：6 パーセンタイル：76.25(Nanoscience & Nanotechnology)

To elucidate deformation behavior behind the exceptional mechanical properties of CrCoNi based medium entropy alloys, the deformation related microstructural parameters were determined by using in situ neutron diffraction and peaks profile analysis methods. Superior tensile strength and elongation of the CrCoNi alloy is relevant to higher twin fault probability ( $P_{tw}$ , up to 3.8%) and dislocation density (, up to 9.7 10 $^{15}$ m $^{-2}$ ) compared to those (1.3% and 3.4 10 $^{15}$ m $^{-2}$ , respectively) of the CrCoNiFe at 293K. Meanwhile, at 140K, the $P_{tw}$ of the CrCoNiFe significantly increased up to 4.4% with the stable of 5.0 10 $^{15}$ m $^{-2}$ and its mechanical properties overwhelm those of the CrCoNi at 273K. Such twinning dominant deformation mechanism at low temperature is also assured by lower stacking fault energy (SFE) of the CrCoNiFe at 140K compared to those of the CrCoNi and CrCoNiFe alloys at 293K.

論文

Clades of huge phages from across Earth's ecosystems

Al-Shayeb, B.*; Sachdeva, R.*; Chen, L.-X.*; Ward, F.*; Munk, P.*; Devoto, A.*; Castelle, C. J.*; Olm, M. R.*; Bouma-Gregson, K.*; 天野由記; et al.

Nature, 578(7795), p.425 - 431, 2020/02

https://doi.org/10.1038/s41586-020-2007-4

被引用回数：83 パーセンタイル：99.63(Multidisciplinary Sciences)

Phage typically have small genomes and depend on their bacterial hosts for replication. We generated metagenomic datasets from many diverse ecosystems and reconstructed hundreds of huge phage genomes, between 200 kbp and 716 kbp in length. Thirty four genomes were manually curated to completion, including the largest phage genomes yet reported. Expanded genetic repertoires include diverse and new CRISPR-Cas systems, tRNAs, tRNA synthetases, tRNA modification enzymes, initiation and elongation factors and ribosomal proteins. Phage CRISPR have the capacity to silence host transcription factors and translational genes, potentially as part of a larger interaction network that intercepts translation to redirect biosynthesis to phage-encoded functions. Some phage repurpose bacterial systems for phage-defense to eliminate competing phage. We phylogenetically define seven major clades of huge phage from human and other animal microbiomes, oceans, lakes, sediments, soils and the built environment. We conclude that large gene inventories reflect a conserved biological strategy, observed across a broad bacterial host range and resulting in the distribution of huge phage across Earth's ecosystems.

論文

Ultralow thermal conductivity from transverse acoustic phonon suppression in distorted crystalline -MgAgSb

Li, X.*; Liu, P.-F.*; Zhao, E.*; Zhang, Z.*; Guide, T.*; Le, M. D.*; Avdeev, M.*; 池田一貴*; 大友季哉*; 古府麻衣子; et al.

Nature Communications (Internet), 11(1), p.942_1 - 942_9, 2020/02

https://doi.org/10.1038/s41467-020-14772-5

被引用回数：15 パーセンタイル：93.25(Multidisciplinary Sciences)

高性能の熱電材料実現には低熱伝導率が必要であり、その機構としてはフォノンの非調和によるもの、あるいは、結晶構造の動的な乱れによるフォノンの散乱によるものがあげられ、どちらも中性子散乱でその現象が明らかにされている。我々は中性子散乱と第一原理計算を組み合わせ、-MgAgSbにおいて、静的な結晶構造の乱れとフォノンの非調和性が組み合わされて極端に低い熱伝導率が実現されているということを見いだしたので、これを報告する。

論文

Fusion reaction $^{48}$ Ca+ $^{249}$ Bk leading to formation of the element Ts (Z=117)

Khuyagbaatar, J.*; Yakushev, A.*; Dllmann, Ch. E.*; Ackermann, D.*; Andersson, L.-L.*; 浅井雅人; Block, M.*; Boll, R. A.*; Brand, H.*; Cox, D. M.*; et al.

Physical Review C, 99(5), p.054306_1 - 054306_16, 2019/05

AA2019-0039.pdf:5.03MB

https://doi.org/10.1103/PhysRevC.99.054306

被引用回数：10 パーセンタイル：88.51(Physics, Nuclear)

$^{48}$ Ca+ $^{249}$ B融合反応を用いて117番元素(Ts)合成実験を行い、117番元素に起因すると思われる4つの崩壊連鎖を観測した。うち2つは長い崩壊連鎖で、 $^{294}$ Tsの崩壊に起因するものと同定された。他の2つは短い崩壊連鎖で、 $^{293}$ Tsの崩壊に起因すると考えると矛盾しない。今回の結果と過去の文献値を比較したところ、今回の我々の結果は過去の文献値をほぼ再現し、117番元素合成の事実を強く再確認する結果となった。

論文

Inverse odd-even staggering in nuclear charge radii and possible octupole collectivity in $^{217,218,219}$ At revealed by in-source laser spectroscopy

Barzakh, A. E.*; Cubiss, J. G.*; Andreyev, A. N.; Seliverstov, M. D.*; Andel, B.*; Antalic, S.*; Ascher, P.*; Atanasov, D.*; Beck, D.*; Biero, J.*; et al.

Physical Review C, 99(5), p.054317_1 - 054317_9, 2019/05

https://doi.org/10.1103/PhysRevC.99.054317

被引用回数：5 パーセンタイル：69.53(Physics, Nuclear)

Hyperfine-structure parameters and isotope shifts for the 795-nm atomic transitions in $^{217,218,219}$ At have been measured at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy technique. Magnetic dipole and electric quadrupole moments, and changes in the nuclear mean-square charge radii, have been deduced. A large inverse odd-even staggering in radii, which may be associated with the presence of octupole collectivity, has been observed. Namely, the radius of the odd-odd isotope $^{218}$ At has been found to be larger than the average.

論文

Coexistence of ferromagnetic and stripe-type antiferromagnetic spin fluctuations in YFe $_{2}$ Ge $_{2}$

Wo, H.*; Wang, Q.*; Shen, Y.*; Zhang, X.*; Hao, Y.*; Feng, Y.*; Shen, S.*; He, Z.*; Pan, B.*; Wang, W.*; et al.

Physical Review Letters, 122(21), p.217003_1 - 217003_5, 2019/05

https://doi.org/10.1103/PhysRevLett.122.217003

被引用回数：2 パーセンタイル：35.62(Physics, Multidisciplinary)

We report neutron scattering measurements of single-crystalline YFe $_{2}$ Ge $_{2}$ in the normal state, which has the same crystal structure as the 122 family of iron pnictide superconductors. YFe $_{2}$ Ge $_{2}$ does not exhibit long-range magnetic order but exhibits strong spin fluctuations. Like the iron pnictides, YFe $_{2}$ Ge $_{2}$ displays anisotropic stripe-type antiferromagnetic spin fluctuations at (). More interesting, however, is the observation of strong spin fluctuations at the in-plane ferromagnetic wave vector (). These ferromagnetic spin fluctuations are isotropic in the () plane, whose intensity exceeds that of stripe spin fluctuations. Both the ferromagnetic and stripe spin fluctuations remain gapless down to the lowest measured energies. Our results naturally explain the absence of magnetic order in YFe $_{2}$ Ge $_{2}$ and also imply that the ferromagnetic correlations may be a key ingredient for iron-based materials.

論文

First ionization potentials of Fm, Md, No, and Lr; Verification of filling-up of 5f electrons and confirmation of the actinide series

佐藤哲也; 浅井雅人; Borschevsky, A.*; Beerwerth, R.*; 金谷佑亮*; 牧井宏之; 水飼秋菜*; 永目諭一郎; 長明彦; 豊嶋厚史; et al.

Journal of the American Chemical Society, 140(44), p.14609 - 14613, 2018/11

https://doi.org/10.1021/jacs.8b09068

被引用回数：16 パーセンタイル：70.21(Chemistry, Multidisciplinary)

第一イオン化エネルギー(IP)は、原子の価電子軌道に関する情報を与える。99番元素アインスタイニウムよりも重いアクチノイドのIPは、一度に一つの原子しか扱うことのできない実験の難しさから、これまでに実験的に測定された例はなかった。我々は表面電離法を応用した新しい測定手法により、103番元素ローレンシウム(Lr)のIP測定に成功し、Lrが弱く束縛された最外殻電子をもつことを強く示唆する結果を得た。一方、Lrとは対象的に、102番元素ノーベリウムは充填された5f軌道および7s軌道をもつために、アクチノイド中最高のIPをもつと考えられている。表面電離法によるIP決定法をNoおよび100番元素フェルミウム, 101番元素メンデレビウムに適用することにより求められた各IPから、5f軌道への電子の充填に伴ってIPが単調に増加し、Noで最も大きくなることを確かめることができた。このことから、f軌道に電子が充填され、アクチノイド系列がLrで終わることを実験的に確かめた。

論文

Deformation of CoCrFeNi high entropy alloy at large strain

Wang, B.*; He, H.*; Naeem, M.*; Lan, S.*; Harjo, S.; 川崎卓郎; Nie, Y.*; Wang, X.-L.*; 他7名*

Scripta Materialia, 155, p.54 - 57, 2018/10

https://doi.org/10.1016/j.scriptamat.2018.06.013

被引用回数：35 パーセンタイル：95.89(Nanoscience & Nanotechnology)

The deformation behavior of an equi-atomic face-centered-cubic CoCrFeNi high entropy alloy was investigated by in-situ neutron diffraction under tensile loading up to 40% applied strain. A three-stage deformation behavior was fully captured by lattice strain and texture evolution. In spite of the chemical complexity, the deformation in CoCrFeNi is dominated by dislocation activities. Analysis of diffraction and microscopy data shows that the deformation progresses from dislocation slip to severe entanglement, where a sharp increase in dislocation density was observed. The neutron diffraction data, corroborated by transmission electron microscopy analysis, provided microscopic insights of the previously reported three-stage hardening behavior.

論文

Liquid-like thermal conduction in intercalated layered crystalline solids

Li, B.; Wang, H.*; 川北至信; Zhang, Q.*; Feygenson, M.*; Yu, H. L.*; Wu, D.*; 尾原幸治*; 菊地龍弥*; 柴田薫; et al.

Nature Materials, 17(3), p.226 - 230, 2018/03

https://doi.org/10.1038/s41563-017-0004-2

被引用回数：71 パーセンタイル：96.98(Chemistry, Physical)

As a generic property, all substances transfer heat through microscopic collisions of constituent particles. A solid conducts heat through both transverse and longitudinal acoustic phonons, but a liquid employs only longitudinal vibrations. As a result, a solid is usually thermally more conductive than a liquid. In canonical viewpoints, such a difference also serves as the dynamic signature distinguishing a solid from a liquid. Here, we report liquid-like thermal conduction observed in the crystalline AgCrSe $_{2}$ . The transverse acoustic phonons are completely suppressed by the ultrafast dynamic disorder while the longitudinal acoustic phonons are strongly scattered but survive, and are thus responsible for the intrinsically ultralow thermal conductivity. This scenario is applicable to a wide variety of layered compounds with heavy intercalants in the van der Waals gaps, manifesting a broad implication on suppressing thermal conduction. These microscopic insights might reshape the fundamental understanding on thermal transport properties of matter and open up a general opportunity to optimize performances of thermoelectrics.

論文

Shape evolution in neutron-rich krypton isotopes beyond N=60; First spectroscopy of $^{98,100}$ Kr

Flavigny, F.*; Doornenbal, P.*; Obertelli, A.*; Delaroche, J.-P.*; Girod, M.*; Libert, J.*; Rodriguez, T. R.*; Authelet, G.*; 馬場秀忠*; Calvet, D.*; et al.

Physical Review Letters, 118(24), p.242501_1 - 242501_6, 2017/06

https://doi.org/10.1103/PhysRevLett.118.242501

被引用回数：27 パーセンタイル：88.56(Physics, Multidisciplinary)

The first -ray spectroscopy of very neutron rich $^{98,100}$ Kr isotopes was carried out at the RIBF at RIKEN Nishina center. Excited states in these isotopes were populated via (p,2p) reactions using radioactive $^{99,101}$ Rb beams accelerated to 220 MeV/nucleon. The new data show a significant increase in deformation beyond N=60, as well as competing configurations (shape-coexistence) at low energy. The data were compared with beyond-mean-field calculations which predict level energies in good agreement with observation, and suggest oblate-prolate shape coexistence.

論文

Identification of the crossing point at = 21 between normal and intruder configurations

Lic, R.*; Rotaru, F.*; Borge, M. J. G.*; Grvy, S.*; Negoita, F.*; Poves, A.*; Sorlin, O.*; Andreyev, A.; Borcea, R.*; Costache, C.*; et al.

Physical Review C, 95(2), p.021301_1 - 021301_6, 2017/02

https://doi.org/10.1103/PhysRevC.95.021301

被引用回数：12 パーセンタイル：79.17(Physics, Nuclear)

The $beta^{-}$ decay of $^{34}$ Mg was used to study the $^{34}$ Al nucleus through spectroscopy at the Isotope Separator On-Line facility of CERN. Previous studies identified two -decaying states in $^{34}$ Al having spin-parity assignments $J^{pi}$ =4 $^{-}$ dominated by the normal configuration (d5/2) $^{-1}$ (f7/2) and $J^{pi}$ = 1 $^{+}$ by the intruder configuration (d5/2) $^{-1}$ (d3/2) $^{-1}$ (f7/2) $^{2}$ . Their unknown ordering and relative energy have been the subject of debate for the placement of $^{34}$ Al inside or outside the = 20 "island of inversion". We report here that the 1 $^{+}$ intruder lies only 46.6 keV above the 4 $^{-}$ ground state. In addition, a new half-life of $T_{1/2}$ =44.9(4)ms, that is twice as long as thepreviously measured 20(10) ms, has been determined for $^{34}$ Mg. Large-scale shell-model calculations with the recently developed SDPF-U-MIX interaction are compared with the new data and used to interpret the mechanisms at play at the very border of the = 20 island of inversion.

論文

Are there signatures of harmonic oscillator shells far from stability?; First spectroscopy of $^{110}$ Zr

Paul, N.*; Corsi, A.*; Obertelli, A.*; Doornenbal, P.*; Authelet, G.*; 馬場秀忠*; Bally, B.*; Bender, M.*; Calvet, D.*; Chteau, F.*; et al.

Physical Review Letters, 118(3), p.032501_1 - 032501_7, 2017/01

https://doi.org/10.1103/PhysRevLett.118.032501

被引用回数：27 パーセンタイル：88.56(Physics, Multidisciplinary)

The first measurement of rays emitted by the very neutron rich nuclei $^{112}$ Mo (Z=42) and $^{110}$ Zr (Z=40) was carried out at the RIBF facility at RIKEN. These data shine light on the postulated N=70 harmonic oscillator shell. If the spin-orbit splitting which gives rise to the N=82 shell gap is reduced in very neutron-rich nuclei, the harmonic oscillator gap at N=70 should open instead. However, both the measured energy of the first excited state $^{112}$ Mo and $^{110}$ Zr, respectively 235(7) keV and 185(11) keV, and their E(4)/E(2) ratio, indicate that these nuclei are good rotors, and exclude the shell stabilization scenario at Z=40 and N=70. These results were compared to state-of-the-art density functional theoretical calculations using Gogny and Skyrme effective interactions.

論文

Recoil--fission and recoil---fission events observed in the reaction $^{48}$ Ca + $^{243}$ Am

Forsberg, U.*; Rudolph, D.*; Andersson, L.-L.*; Di Nitto, A.*; Dllmann, Ch. E.*; Fahlander, C.*; Gates, J. M.*; Golubev, P.*; Gregorich, K. E.*; Gross, C. J.*; et al.

Nuclear Physics A, 953, p.117 - 138, 2016/09

https://doi.org/10.1016/j.nuclphysa.2016.04.025

被引用回数：32 パーセンタイル：93.48(Physics, Nuclear)

$^{48}$ Ca + $^{243}$ Am反応による115番元素合成実験で観測された崩壊連鎖について、最近我々が報告したドイツGSIで測定したデータと過去に報告されたロシアDubna及び米国LBNLで測定されたデータのすべてを使い、その起源を調査した。それらのデータの中に、反跳核--()-核分裂タイプの短い崩壊連鎖が14事象観測されており、そのうちのいくつかは中性子が2個放出されてできる $^{289}$ Mc起源であるとこれまで解釈されてきた。一方、今回我々は、これらの短い崩壊連鎖のほとんどが、中性子が3個放出されてできる $^{288}$ Mc起源であり、崩壊連鎖の途中でEC崩壊して核分裂したものであろうと再同定した。

論文

-delayed fission and decay of $^{196}$ At

Truesdale, V. L.*; Andreyev, A.; Ghys, L.*; Huyse, M.*; Van Duppen, P.*; Sels, S.*; Andel, B.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; et al.

Physical Review C, 94(3), p.034308_1 - 034308_11, 2016/09

https://doi.org/10.1103/PhysRevC.94.034308

被引用回数：9 パーセンタイル：65.08(Physics, Nuclear)

A nuclear-decay spectroscopy study of the neutron-deficient isotope $^{196}$ At is reported where an isotopically pure beam was produced using the selective Resonance Ionization Laser Ion Source and On-Line Isotope Mass Separator (CERN). The fine-structure decay of $^{196}$ At allowed the low-energy excited states in the daughter nucleus $^{192}$ Bi to be investigated. A -delayed fission study of $^{196}$ At was also performed. A mixture of symmetric and asymmetric fission-fragment mass distributions of the daughter isotope $^{196}$ Po (populated by decay of $^{196}$ At) was deduced based on the measured fission-fragment energies. A DF probability $P_{rm beta DF}$ ( $^{196}$ At) = 9(1)10 $^{-5}$ was determined.