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論文

Neutron emission during fission and its impact on fission-fragment mass distribution studied by a Langevin model

高木 慎弥*; 原田 壮太*; 有友 嘉浩*; 廣瀬 健太郎; 西尾 勝久

Physical Review C, 112(4), p.044607_1 - 044607_9, 2025/10

https://journals.aps.org/prc/abstract/10.1103/ml4c-3k8t

Actinide nucleus shows mass-asymmetric fission in low energy due to shell structure. The fission fragment mass distributions at high energy tend to have a symmetric shape due to smearing of the shell. On the other hand, the distribution can be changed by the neutron emission before fission, as it decreases the excitation energy of fissioning nucleus, thus revives the shell structure. In the so called multichance fission, neutron emission is considered at the ground state shape, and competition between fission and neutron emission is determined in the framework of statistical model. In the present work, we describe fission in the Langevin equations, and the neutron emission is treated all over the fission process. The calculation demonstrated experimentally observed mass distribution, characterized by the peak-to-valley ratio, for wide range of initial compound-nucleus excitation energy up to 60MeV. The results show that, while neutron emission dominates at the ground state shape, it occurs along the shape evolution down to the scission point.

論文

Kinetic energy of fission fragments within a dynamical model

高木 慎弥*; 有友 嘉浩*; 中島 滉太*; 岡田 和記; 廣瀬 健太郎; 西尾 勝久

Physical Review C, 112(1), p.014608_1 - 014608_7, 2025/07

https://doi.org/10.1103/8smy-1ls9
 被引用回数：0 パーセンタイル：0.00(Physics, Nuclear)

Kinetic energy of individual fission fragment for actinide nuclei is, for example, important for evaluating the prompt-neutron spectrum in the laboratory system. It is experimentally known that kinetic energy for each fragment is constant at about 100 MeV for light fragments and that for heavy fragments decreases linearly with mass number. Most of the theoretical studies carried out so far attempted to calculate the total kinetic energy of both fragments, i.e. sum of the energies of two fragments, but the kinetic energy of each fragment was not analyzed in detail as far as we recognize. We have calculated them in thermal-neutron induced fission of $$^{239}$$Pu with a dynamical model using Langevin equations within a three-dimensional two-center parametrization. Also fission of $$^{258}$$Fm was investigated. It is calculated from the Coulomb energy at the scission point and the pre-scission kinetic energy. It is found that the pre-scission kinetic energy has about 2-4% contribution in the kinetic energy. The calculated results reproduce the trend of the experimental data.

論文

Competition between mass-symmetric and asymmetric fission modes in $$^{258}$$Md produced in the $$^{4}$$He + $$^{254}$$Es reaction

西尾 勝久; 廣瀬 健太郎; 牧井 宏之; Orlandi, R.; Kean, K. R.*; 塚田 和明; 豊嶋 厚史*; 浅井 雅人; 佐藤 哲也; Chiera, N. M.*; et al.

Physical Review C, 111(4), p.044609_1 - 044609_12, 2025/04

https://doi.org/10.1103/PhysRevC.111.044609
 被引用回数：0 パーセンタイル：0.00(Physics, Nuclear)

In spontaneous fission (SF) it is found that the mass-asymmetric fission of well-known actinides suddenly changes to the symmetric fission when nucleus has a mass number $$A_{c}$$ larger than 257. We have measured for the first time fission-fragment mass and total-kinetic-energy (TKE) distributions of the excited compound nucleus $$^{258}$$Md, populated in the reaction $$^{4}$$He+$$^{254}$$Es, using the rare isotope $$^{254}$$Es with a short half-life, $$T_{1/2}$$=276 days. The fission of $$^{258}$$Md can be interpreted as involving 3 fission modes: an mass-asymmetric mode and two modes of mass-asymmetric fissions, the latter two are manifested by different TKE values. Predominantly symmetric fission was obtained at the excitation energy of 15.0 MeV. By increasing the energy to 18.0 MeV, the asymmetric fission mode dominates. Both such a strong change of fission modes within a small increase of excitation energy and the enhancement of asymmetric split are new phenomena in fission.

論文

Giant dipole resonance photofission and photoneutron reactions in $$^{238}$$U and $$^{232}$$Th

Filipescu, D.*; Gheorghe, I.*; Goriely, S.*; 西尾 勝久; 宇都宮 弘章*; 洲嵜 ふみ; 廣瀬 健太郎; 他10名*

Physical Review C, 109(4), p.044602_1 - 044602_23, 2024/04

https://doi.org/10.1103/PhysRevC.109.044602
 被引用回数：3 パーセンタイル：71.61(Physics, Nuclear)

New measurements of photofission and photoneutron reactions on $$^{238}$$U and $$^{232}$$Th in the Giant Dipole Resonance (GDR) energy region have been performed at the laser Compton-scattering $$gamma$$-ray source of the NewSUBARU synchrotron radiation facility. The photoneutron ($$gamma, in$$) with $$i$$ = 1-3 and photofission ($$gamma, F$$) reactions have been discriminated by considering a Gaussian distribution of prompt-fission-neutron (PFN) multiplicities predicted by the theory of evaporation in sequential neutron emission from excited fission fragments. We report experimental ($$gamma, n$$), ($$gamma, 2n$$), ($$gamma, 3n$$) and ($$gamma, F$$) cross sections, average energies of PFNs and of($$gamma$$, $$in$$) photoneutrons, as well as the mean number of PFNs per fission and the width of the PFNs multiplicity distribution. Based on these primary experimental results and combined with reasonable assumptions, we extract also the first- and second-chance fission contributions.

論文

Search for the 6$$alpha$$ condensed state in $$^{24}$$Mg using the $$^{12}$$C+$$^{12}$$C scattering

Fujikawa, Y.*; Kawabata, T.*; Adachi, S.*; 廣瀬 健太郎; 牧井 宏之; 西尾 勝久; Orlandi, R.; 洲嵜 ふみ; 他13名*

Physics Letters B, 848, p.138384_1 - 138384_6, 2024/01

https://doi.org/10.1016/j.physletb.2023.138384
 被引用回数：8 パーセンタイル：81.51(Astronomy & Astrophysics)

We searched for the 6$$alpha$$-condensed state in $$^{24}$$Mg by measuring the $$^{12}$$C+$$^{12}$$C scattering with the SAKRA Si detector array. By using the invariant-mass method for the detected 3$$alpha$$ particles, the inclusive cross sections for the $$^{12}$$C+$$^{12}$$C $$rightarrow$$ $$^{12}$$C(0$$^{+}_{2}$$) + X and $$^{12}$$C(3$$^{-}_{1}$$) + X reactions were determined. In both the inclusive $$^{12}$$C(0$$^{+}_{2}$$) + X channel and the exclusive $$^{12}$$C(0$$^{+}_{2}$$) + $$^{12}$$C(0$$^{+}_{1}$$) channel, the cross section peaked at E$$_{cm}$$ = 19.4 MeV, which correspond to the excitation energy of E$$_{x}$$ = 33.3 MeV in $$^{24}$$Mg. This 19.4-MeV state is a candidate for the 6$$alpha$$-condensed state

論文

Measurement of double-differential neutron yields for iron, lead, and bismuth induced by 107-MeV protons for research and development of accelerator-driven systems

岩元 大樹; 中野 敬太; 明午 伸一郎; 佐藤 大樹; 岩元 洋介; 杉原 健太*; 西尾 勝久; 石 禎浩*; 上杉 智教*; 栗山 靖敏*; et al.

EPJ Web of Conferences, 284, p.01023_1 - 01023_4, 2023/05

https://doi.org/10.1051/epjconf/202328401023
 被引用回数：0 パーセンタイル：0.00(Nuclear Science & Technology)

加速器駆動システム(ADS)の核特性予測精度の向上と京都大学臨界集合体実験装置(KUCA)におけるADS炉物理実験で用いる中性子源情報の取得を目的として、京都大学の固定磁場強集束(FFAG)加速器を用いた核データ測定実験プログラムを開始した。このプログラムの一環として、鉄,鉛及びビスマスに対する陽子入射二重微分中性子収量(TTNY)及び断面積(DDX)を測定した。測定では、真空チェンバ内に設置された標的試料に107MeVの陽子ビームを照射し、核反応によって標的から発生した粒子の信号を、小型の中性子検出器を用いて検出した。検出信号とFFAGキッカー電磁石の信号の時間差から飛行時間(TOF)を求め、ガンマ線の事象を波形弁別法によって除去して中性子事象をカウントすることで中性子のTOFスペクトルを求めた。得られた中性子のTOFスペクトルから、相対論的運動学によりTTNY及びDDXを求めた。実験で得られたTTNY及びDDXを、モンテカルロ輸送計算コードPHITSによる計算と比較し、PHITSに組み込まれた核反応モデル及び評価済み核データライブラリJENDL-4.0/HEの妥当性を検証するとともに、PHITSによる計算の予測精度を評価した。

論文

Photofission and photoneutron cross sections for $$^{238}$$U and $$^{232}$$Th

Filipescu, D.*; 西尾 勝久; 洲嵜 ふみ; 廣瀬 健太郎; 他12名*

EPJ Web of Conferences, 284, p.04010_1 - 04010_4, 2023/05

https://doi.org/10.1051/epjconf/202328404010

Photofission and photoneutron reactions on $$^{238}$$U and $$^{232}$$Th in the energy range of 5.87 MeV - 20.14 MeV was carried out at the Compton-scattering $$gamma$$-ray source of the NewSUBARU synchrotro radiation facility of SPring-8, Japan. The neutron-multiplicity sorting of high-multiplicity fission neutron coincidence events has been performed using a dedicated energy dependent, multiple firing statistical treatment. The photoneutron ($$gamma$$,xn) and photofission ($$gamma$$,fxn) reactions have been discriminated by considering a Gaussian distribution of prompt-fission-neutrons (PFN) multiplicities predicted by the evaporation theory. We here provide preliminary experimental ($$gamma$$, n), ($$gamma$$, 2n) and ($$gamma$$, F) cross sections, average energies of PFN and of photoneutrons emitted in ($$gamma$$, n) and ($$gamma$$, 2n) reactions, as well as the mean number of PFN per fission.

論文

Measurement of 107-MeV proton-induced double-differential thick target neutron yields for Fe, Pb, and Bi using a fixed-field alternating gradient accelerator at Kyoto University

岩元 大樹; 中野 敬太; 明午 伸一郎; 佐藤 大樹; 岩元 洋介; 杉原 健太; 西尾 勝久; 石 禎浩*; 上杉 智教*; 栗山 靖敏*; et al.

Journal of Nuclear Science and Technology, 60(4), p.435 - 449, 2023/04

https://doi.org/10.1080/00223131.2022.2115423
 被引用回数：4 パーセンタイル：47.14(Nuclear Science & Technology)

加速器駆動核変換システム(ADS)の研究開発及び京都大学臨界実験装置(KUCA)におけるADS未臨界炉物理の基礎研究を目的として、固定磁場強収束(FFAG)加速器を用いて107MeV陽子による鉄、鉛及びビスマス標的に対する二重微分中性子収量(TTNY)を測定した。TTNYは8個の中性子検出器(各検出器は小型のNE213液体有機シンチレータと光電子増倍管より構成される)からなる中性子検出器システムを用いて飛行時間法により得られたものである。測定で得られたTTNYを、粒子・重イオン輸送コードシステム(PHITS)に組み込まれたモンテカルロ法に基づく核破砕反応モデル(INCL4.6/GEM, Bertini/GEM, JQMD/GEM, JQMD/SMM/GEM)及び評価済み高エネルギー核データライブラリ(JENDL-4.0/HE)による計算結果と比較した。JENDL-4.0/HEを含む比較対象のモデルは、検出器角度5度における高エネルギーピークを再現しないなどの特徴的な不一致が見られた。測定で得られたTTNYとPHITSによって評価した20MeV以下のエネルギー及び角度積分中性子収率を比較した結果、INCL4.6/GEMがKUCAにおけるADS炉物理実験のモンテカルロ輸送シミュレーションに適していることが示された。

論文

京都大学FFAG加速器を用いた加速器駆動型核変換システム(ADS)用核データの実験的研究

岩元 大樹; 明午 伸一郎; 中野 敬太*; 佐藤 大樹; 岩元 洋介; 杉原 健太*; 石 禎浩*; 上杉 智教*; 栗山 靖敏*; 八島 浩*; et al.

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (インターネット), p.404 - 409, 2023/01

https://www.pasj.jp/web_publish/pasj2022/proceedings/PDF/TUP0/TUP040.pdf

加速器駆動核変換システム(ADS)の研究開発に資するため、固定磁場強収束(FFAG)加速器を用い、核データを取得する実験的研究プログラムを開始した。ADSの核設計及び京都大学臨界集合体実験装置(KUCA)における未臨界実験体系の解析で重要となる、鉛及びビスマスの陽子入射中性子収量及び核分裂に関する核データを対象とした。中性子の飛行時間(TOF)測定で要求される短パルスビームの技術開発を行い、その要求値となるビーム幅10ns以下を達成するとともに、107MeV陽子入射による厚い標的中性子収量TTNY及び中性子生成二重微分断面積DDXをTOF法により測定した。TTNY及びDDXの測定には、小型シンチレータと光電子増倍管から構成される中性子検出器を用いた。測定で得られた結果をADSの核設計で用いられるPHITSによる解析値と比較した。さらに、マイクロチャンネルプレート(MCP)と多芯線比例計数管(MWPC)を組み合わせにより、107MeV陽子入射の$$^{208}$$Pb核分裂反応から生成される核分裂片の質量数分布を測定した。本プログラムの最終年度となる令和4年度は、$$^{209}$$Biに対する核分裂片の質量数分布と核分裂で生じる核分裂中性子の測定を実施するとともに、$$^{237}$$Np核分裂計数管を用いて、陽子と標的との核反応で形成される中性子場の測定を実施する予定である。

論文

New $$K$$ isomers in $$^{248}$$Cf

Orlandi, R.; 牧井 宏之; 西尾 勝久; 廣瀬 健太郎; 浅井 雅人; 塚田 和明; 佐藤 哲也; 伊藤 由太; 洲嵜 ふみ; 永目 諭一郎*; et al.

Physical Review C, 106(6), p.064301_1 - 064301_11, 2022/12

https://doi.org/10.1103/PhysRevC.106.064301
 被引用回数：5 パーセンタイル：55.72(Physics, Nuclear)

The nuclear structure of $$^{248}$$Cf produced by the $$^{18}$$O+$$^{249}$$Cf multinucleon transfer reaction was investigated using $$gamma$$-ray spectroscopy. Analysis of the $$gamma$$-ray spectrum of $$^{248}$$Cf revealed the presence of multiple long-lived (isomeric) excited states at low excitation energies. The energies and half-lives of the isomers contain information on the proton and neutron orbits in the heavy-element region and the deformation of atomic nuclei, and are important data to predict the properties of nuclei in the "island of stability".

論文

Measurement of 107-MeV proton-induced double-differential neutron yields for iron for research and development of accelerator-driven systems

岩元 大樹; 中野 敬太; 明午 伸一郎; 佐藤 大樹; 岩元 洋介; 石 禎浩*; 上杉 智教*; 栗山 靖敏*; 八島 浩*; 西尾 勝久; et al.

JAEA-Conf 2022-001, p.129 - 133, 2022/11

https://doi.org/10.11484/jaea-conf-2022-001

加速器駆動システム(ADS)の核特性予測精度の向上と京都大学臨界集合体実験装置(KUCA)におけるADS炉物理実験で用いる中性子源情報の取得を目的として、京都大学の固定磁場強集束(FFAG)加速器を用いた核データ測定実験プログラムを開始した。このプログラムの一環として、鉄に対する陽子入射二重微分中性子収量(TTNY)及び断面積(DDX)を測定した。測定では、真空チェンバ内に設置された鉄標的に107MeVの陽子ビームを照射し、核反応によって標的から発生した粒子の信号を、小型の中性子検出器を用いて検出した。検出信号とFFAGキッカー電磁石の信号の時間差から飛行時間(TOF)を求め、ガンマ線の事象を波形弁別法によって除去して中性子事象をカウントすることで中性子のTOFスペクトルを求めた。得られた中性子のTOFスペクトルから、相対論的運動学により鉄標的に対するTTNY及びDDXを求めた。

論文

Angular momentum transfer in multinucleon transfer channels of $$^{18}$$O + $$^{237}$$Np

田中 翔也*; 廣瀬 健太郎; 西尾 勝久; Kean, K. R.*; 牧井 宏之; Orlandi, R.; 塚田 和明; 有友 嘉浩*

Physical Review C, 105(2), p.L021602_1 - L021602_5, 2022/02

https://doi.org/10.1103/PhysRevC.105.L021602
 被引用回数：4 パーセンタイル：48.02(Physics, Nuclear)

The angular momentum of a primary excited compound nucleus produced in multinucleon transfer reaction is an important quantity to evaluate cross sections to synthesize neutron-rich heavy element nuclei as well as for surrogate reaction studies. The mechanism is, however, not enough understood due to the lack of detailed experimental data. In the present study, we determined the angular momentum of primary excited nuclei, $$^{237,238,239}$$Np, $$^{238,239,240}$$Pu, and $$^{239,240,241}$$Am, produced in the multi-nucleon transfer channels of the $$^{18}$$O + $$^{237}$$Np reaction. With this aim, angular distributions of fission fragments with respect to the axis perpendicular to the reaction plane were measured for each compound nucleus. The distributions show an anisotropy exhibiting an enhanced yield on the reaction plane. They are well reproduced by a saddle point model, from which the average angular momentum is derived in the model framework. The angular momentum increases with the compound-nucleus mass, thus the number of nucleons exchanged, but shows a saturating trend toward heavier compound nuclei. These results are the first ones to point to the dependence of the angular momentum on the transfer channels.

論文

The $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross section from the surrogate ratio method and its effect on the $$^{60}$$Fe nucleosynthesis

Yan, S. Q.*; Li, X. Y.*; 西尾 勝久; Lugaro, M.*; Li, Z. H.*; 牧井 宏之; Pignatari, M.*; Wang, Y. B.*; Orlandi, R.; 廣瀬 健太郎; et al.

Astrophysical Journal, 919(2), p.84_1 - 84_7, 2021/10

https://doi.org/10.3847/1538-4357/ac12ce
 被引用回数：6 パーセンタイル：30.23(Astronomy & Astrophysics)

The long-lived $$^{60}$$Fe (with a half-life of 2.62 Myr) is a crucial diagnostic of active nucleosynthesis in the Milky Way galaxy and in supernovae near the solar system. The neutron-capture reaction $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe on $$^{59}$$Fe (half-life=44.5 days) is the key reaction for the production of $$^{60}$$Fe in massive stars. This reaction cross section has been previously constrained by the Coulomb dissociation experiment, which offered partial constraint on the E1 $$gamma$$-ray strength function but a negligible constraint on the M1 and E2 components. In this work, for the first time, we use the surrogate ratio method to experimentally determine the $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe cross sections in which all the components are included. We derived a Maxwellian-averaged cross section of 27.5$$pm$$3.5 mb at $$kT$$ = 30 keV and 13.4$$pm$$1.7 mb at $$kT$$ = 90 keV, roughly 10%-20% higher than previous estimates. We analyzed the impact of our new reaction rates in nucleosynthesis models of massive stars and found that uncertainties in the production of $$^{60}$$Fe from the $$^{59}$$Fe(n,$$gamma$$)$$^{60}$$Fe rate are at most 25$$%$$. We conclude that stellar physics uncertainties now play a major role in the accurate evaluation of the stellar production of $$^{60}$$Fe.

論文

Chemical characterization of a volatile dubnium compound, DbOCl$$_3$$

Chiera, N. M.*; 佐藤 哲也; Eichler, R.*; 富塚 知博; 浅井 雅人; 安達 サディア*; Dressler, R.*; 廣瀬 健太郎; 井上 浩樹*; 伊藤 由太; et al.

Angewandte Chemie; International Edition, 60(33), p.17871 - 17874, 2021/08

https://doi.org/10.1002/anie.202102808
 被引用回数：5 パーセンタイル：22.33(Chemistry, Multidisciplinary)

等温ガスクロマトグラフ法を用いて、105番元素ドブニウム(Db)の単一原子を対象として、揮発性オキシ塩化物を合成し、化学的性質を調べた。同一条件下で同族元素ニオブおよびタンタルの揮発性と比較したところ、NbOCl$$_3 > $$ TaOCl$$_3 geq$$ DbOCl$$_3$$の関係が得られた。これはDb分子中の共有結合性が周期表からの予想よりも強くなっているためと考えられる。本成果により、超アクチノイド元素の化学的性質に関する理論計算に対する信頼できる実験データを与えることができた。

論文

Experimental study of the $$Gamma_{p1}/Gamma_{p0}$$ ratios of resonance states in $$^{8}$$Be for deducing the $$^{7}$$Be($$n$$,$$p_{1}$$)$$^{7}$$Li$$^{*}$$ reaction rate relevant to the cosmological lithium problem

岩佐 直仁*; 石川 竣喜*; 久保野 茂*; 榊原 昂浩*; 小湊 和也*; 西尾 勝久; 松田 誠; 廣瀬 健太郎; 牧井 宏之; Orlandi, R.; et al.

Physical Review C, 103(1), p.015801_1 - 015801_5, 2021/01

https://doi.org/10.1103/PhysRevC.103.015801
 被引用回数：2 パーセンタイル：23.09(Physics, Nuclear)

The $$^{9}$$Be($$^{3}$$He,$$alpha$$)$$^{8}$$Be($$p$$)$$^{7}$$Li reaction was studied at $$E_{rm lab}$$($$^{3}$$He)=30 MeV to deduce the branching ratios of $$Gamma_{p1}/Gamma_{p0}$$ of resonant state at 18.91 - 20.1 MeV in $$^{8}$$Be, which are necessary to extract the $$^{7}$$Be($$n$$, $$p_{1}$$)$$^{7}$$Li$$^{*}$$ reaction rate relevant to the $$^{7}$$Be destruction in the big bang nucleosynthesis, from the $$^{7}$$Li($$p$$,$$n_{0}$$)$$^{7}$$Be reaction cross section. The decay protons from $$^{8}$$Be$$^{*}$$ to the ground and first excited states in $$^{7}$$Li were well-separately measured. The $$Gamma_{p1}/Gamma_{p0}$$ ratio of the 19.235-MeV state was deduced to be 3.4$$pm$$1.9%. The 19.86- and 20.1-MeV states were found to decay dominantly into the first excited and ground states of $$^{7}$$Li, respectively.

論文

Measurement of fission-fragment mass distributions in the multinucleon transfer channels of the $$^{18}$$O+$$^{237}$$Np reaction

Vermeulen, M. J.; 西尾 勝久; 廣瀬 健太郎; Kean, K. R.; 牧井 宏之; Orlandi, R.; 塚田 和明; Tsekhanovich, I.*; Andreyev, A. N.; 石崎 翔馬*; et al.

Physical Review C, 102(5), p.054610_1 - 054610_11, 2020/11

https://doi.org/10.1103/PhysRevC.102.054610
 被引用回数：8 パーセンタイル：57.88(Physics, Nuclear)

Fission fragment mass distributions for 23 nuclei ($$^{234-237}$$U, $$^{236-239}$$Np, $$^{238-241}$$Pu, $$^{240-243}$$Am, $$^{242-245}$$Cm, and $$^{244-246}$$Bk) were measured using the multi-nucleon transfer approach in the reaction of $$^{18}$$O+$$^{237}$$Np, and their excitation-energy dependence was obtained up to a maximum of 70 MeV. Among them, the low energy fission of $$^{236}$$Np, $$^{238}$$Pu, and $$^{245}$$Cm is reported for the first time. The experimental data for all the studied nuclei were compared to the Langevin calculations. The calculation which takes into account the effects of multi-chance fission well reproduced the peak-to-valley ratio and mass-asymmetric peak positions of the distributions. The angular momenta given to the fissioning nucleus is also discussed.

論文

最先端の研究開発,日本原子力研究開発機構,3; 原子科学の最先端を拓く

Orlandi, R.; 廣瀬 健太郎; 矢板 毅; 山上 浩志; 家田 淳一; 神戸 振作; 石川 法人

日本原子力学会誌ATOMO$$Sigma$$, 62(5), p.280 - 284, 2020/05

https://doi.org/10.3327/jaesjb.62.5_280

先端基礎研究センターで行っている研究を紹介する。(1)人工元素アインスタイニウムを用いた実験(安定の島に向かう超重原子核の核分裂と電子軌道のイオン半径)、(2)電子のスピンを駆使した新しいエネルギー変換仕組み、(3)磁場に負けない超伝導、(4)放射線環境中のセラミックスがもつ自己修復能力

論文

New excited 2$$^+$$ and 3$$^-$$ two-proton states in $$_{84}^{210}$$Po$$_{126}$$ populated by two-proton transfer

Dupont, E.*; Astier, A.*; Petrache, C. M.*; Lv, B. F.*; Deloncle, I.*; Kiener, J.*; Orlandi, R.; 牧井 宏之; 西尾 勝久; 廣瀬 健太郎; et al.

Physical Review C, 101(1), p.014309_1 - 014309_6, 2020/01

https://doi.org/10.1103/PhysRevC.101.014309
 被引用回数：2 パーセンタイル：19.13(Physics, Nuclear)

Five new 2$$^+$$ levels and one new 3$$^-$$ level were established in $$^{210}$$Po. The states were populated via the $$^{208}$$Pb($$^{12}$$C, $$^{10}$$Be) two-proton reaction experiment, performed at the JAEA Tandem in Tokai. A setup combining Ge, LaBr$$_3$$, and Si telescopes was used to detect in-beam $$gamma$$-rays and ejectile residues. Two-proton configurations were assigned to all new states. All assignments are strongly supported by shell-model calculations.

論文

Effects of multichance fission on isotope dependence of fission fragment mass distributions at high energies

田中 翔也; 有友 嘉浩*; 宮本 裕也*; 廣瀬 健太郎; 西尾 勝久

Physical Review C, 100(6), p.064605_1 - 064605_6, 2019/12

https://doi.org/10.1103/PhysRevC.100.064605
 被引用回数：16 パーセンタイル：77.68(Physics, Nuclear)

散逸揺動定理を採用した動力学模型を使用し、$$^{234-240}$$U, $$^{236-242}$$Np, $$^{238-244}$$Pu ($$E^{*}$$=15-55MeV)という広い範囲の核種および励起エネルギーにおいて核分裂片質量分布の評価を行った。本研究の特色は、原子核が分裂へ至るまでに中性子を放出するという、マルチチャンス核分裂の概念を理論計算へ導入していることである。その結果、実験データを系統的に再現する計算結果を得られた。特に、励起エネルギーが高い領域においても核分裂片質量分布がふた山構造を維持する傾向や、原子核の初期状態(特に中性子数)に依存するという実験データの傾向を再現することに成功した。またこの傾向が、核分裂前の中性子放出確率を支配している複合核の中性子結合エネルギーと相関を持つことを示した。

論文

Effects of the nuclear structure of fission fragments on the high-energy prompt fission $$gamma$$-ray spectrum in $$^{235}$$U($$n_{rm th},f$$)

牧井 宏之; 西尾 勝久; 廣瀬 健太郎; Orlandi, R.; L$'e$guillon, R.; 小川 達彦; Soldner, T.*; K$"o$ster, U.*; Pollitt, A.*; Hambsch, F.-J.*; et al.

Physical Review C, 100(4), p.044610_1 - 044610_7, 2019/10

https://doi.org/10.1103/PhysRevC.100.044610
 被引用回数：15 パーセンタイル：75.83(Physics, Nuclear)

The prompt fission $$gamma$$-ray energy spectrum for cold-neutron induced fission of $$^{235}$$U was measured in the energy range $$E_{rm gamma}$$ = 0.8 - 20,MeV, by gaining a factor of about 10$$^{5}$$ in statistics compared to the measurements performed so far. The spectrum exhibits local bump structures at $$E_{rm gamma}approx$$4,MeV and $$approx$$6,MeV, and also a broad one at $$approx$$15,MeV. In order to understand the origins of these bumps, the $$gamma$$-ray spectra were calculated using a statistical Hauser-Feshbach model, taking into account the de-excitation of all the possible primary fission fragments. It is shown that the bump at $$approx$$4,MeV is created by the transitions between the discrete levels in the fragments around $$^{132}$$Sn, and the bump at $$approx$$6,MeV mostly comes from the complementary light fragments. It is also indicated that a limited number of nuclides, which have high-spin states at low excitation energies, can contribute to the bump structure around $$E_{rm gamma}approx$$15,MeV, induced by the transition feeding into the low-lying high-spin states.

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