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Huang, Y.-C.*; 吉川 貴史; 他5名*
Applied Physics Letters, 126(9), p.092403_1 - 092403_6, 2025/03
被引用回数：0 パーセンタイル：0.00(Physics, Applied)The application of spin-current volume effect (SVE) with volume magnetostriction of iron gallium (FeGa) films is examined for micro-diaphragm actuation. A silicon diaphragm measuring 1.5
1.5 mm
is coated with Pt (100-nm-thick) and FeGa (100-nm-thick) thin films. An alternating charge current passed through the FeGa/Pt/Si diaphragm under a magnetic field perpendicular to the charge current generates an alternating spin current via the spin Hall effect in the Pt film, transferring angular momentum from the Pt film to the FeGa film. The injected spin current provides energy and changes the effective temperature, thereby varying the thermal fluctuation of the magnetic moments. In a magnetic material with volume magnetostriction, the thermal fluctuation of the magnetic moments affects its volume. When the spin fluctuations change, the volume magnetostriction induces a corresponding expansion or contraction of the material. Both electrodeposited and ion-beam sputter-deposited FeGa films are investigated, and it is observed that the FeGa film exhibits SVE. The force generated by the SVE is evaluated based on the vibration amplitude at the fundamental resonant mode. This study demonstrates that the force generated by the SVE is correlated with the volume magnetostriction and the deposition process.
GeTe
homojunctions小幡 玲二*; 齊藤 英治; 吉川 貴史; 他13名*
Advanced Materials, 37(8), p.2411459_1 - 2411459_11, 2025/02
被引用回数：1 パーセンタイル：0.00(Chemistry, Multidisciplinary)Twistronics, a novel engineering approach involving the alignment of van der Waals (vdW) integrated two-dimensional materials at specific angles, has recently attracted significant attention. Novel nontrivial phenomena have been demonstrated in twisted vdW junctions (the so-called magic angle), such as unconventional superconductivity, topological phases, and magnetism. However, there have been only few reports on integrated vdW layers with large twist angles 
, such as twisted interfacial Josephson junctions using high-temperature superconductors. Herein, vdW homojunctions of the thin-magnetic flakes, Fe
GeTe
(FGT), with large ranging from 0 to 90 deg, without inserting any tunnel barriers are assembled. Nevertheless, these vdW homojunctions exhibit tunnel-magnetoresistance (TMR) like behavior (pseudo-TMR (PTMR) effect) with the ratios highly sensitive to the values, revealing that the vdW gap at the junction interface between the twisted FGT layers behaves like a tunnel barrier and the serves a control parameter for PTMR by drastically varying magnitudes of the lattice-mismatch and the subsequent appearance of antiferromagnetic (AFM) spin alignment. First-principles calculations considering vacuum gaps indicate strong dependence of TMR on the driven by the sixfold screw rotational symmetry of bulk FGT. The present homojunctions hold promise as a platform for novel AFM spin-dependent phenomena and spintronic applications.
小杉 美央子*; 吉川 貴史; 齊藤 英治; 他10名*
ACS Applied Materials & Interfaces, 16(46), p.64190 - 64196, 2024/11
被引用回数：1 パーセンタイル：35.94(Nanoscience & Nanotechnology)Atom-vacancy-defects present in various materials yield numerous interesting physical phenomena, even obstructing high performance in some cases. On the other hand, their valuable applications to novel devices, such as nitrogen vacancy centers in diamond for quantum bits, have gathered significant attention. In particular, these tendencies become more substantial in two-dimensional (2D) (atomically) thin van der Waals layers. However, correlations with various kinds of atom defects are still under exploration. Herein, we find the stochastic behaviors of large hysteresis loops with strong photoresponse in the static electrical properties in few-atom layer semiconductors, molybdenum disulfide (MoS). The temperature dependence and transmission electron microscopy reveal that they arise from pairs of two neighboring in-plane S-vacancy defects, which predominantly present only around the interface at the MoS flake/substrate, with activation energies similar to 0.35 eV. The low-frequency (
) (LF) noise measurements clarify a high f shift in the two 1/ 2-dependent regimes, implying stochastic behaviors of electric charges through the S-vacancy pairs with high-speed charge(spin) transitions across low kinetic energy barriers between narrow discrete states. The shallow energy sates are formed from the highly uniform S-vacancy pairs interacting with Mo atoms, which act like quantum dots. The observed stochastic operation holds promise for various application, particularly for probabilistic neuromorphic computation in artificial intelligence.
GeTe nanomeshes小幡 玲二*; 吉川 貴史*; 齊藤 英治; 他7名*
Nanotechnology, 35(47), p.475601_1 - 475601_9, 2024/11
被引用回数：1 パーセンタイル：40.97(Nanoscience & Nanotechnology)The growth of two-dimensional van der Waals magnetic materials presents attractive opportunities for exploring new physical phenomena and valuable applications. Among these materials, FeGeTe (FGT) exhibits a variety of remarkable properties and has garnered significant attention. Herein, we have for the first time created a nanomesh structure-a honeycomb-like array of hexagonal nanopores-with the zigzag pore-edge atomic structure on thin FGT flakes with and without oxidation of the pore edges. It is revealed that the magnitude of ferromagnetism (FM) significantly increases in both samples compared with bulk flakes without nanomeshes. Critical temperature annealing results in the formation of zigzag pore edges and interpore zigzag-edge nanoribbons. We unveil that the non-oxide (O) termination of the Fe dangling bonds on these zigzag edges enhances FM behavior, while O-termination suppresses this FM by introducing antiferromagnetic behavior through edge O-Fe coupling. FGT nanomeshes hold promise for the creation of strong FM and their effective application in magnetic and spintronic systems.
substrate小幡 玲二*; 齊藤 英治; 吉川 貴史; 他7名*
Advanced Materials, 36(19), p.2311339_1 - 2311339_8, 2024/05
被引用回数：0 パーセンタイル：0.00(Chemistry, Multidisciplinary)SrTiO (STO) substrate, a perovskite oxide material known for its high dielectric constant (epsilon), facilitates the observation of various (high-temperature) quantum phenomena. A quantum Hall topological insulating (QHTI) state, comprising two copies of QH states with antiparallel two ferromagnetic edge-spin overlap protected by the U(1) axial rotation symmetry of spin polarization, has recently been achieved in low magnetic field (B) even as high as approximate to 100 K in a monolayer graphene/thin hexagonal boron nitride (hBN) spacer placed on an STO substrate, thanks to the high epsilon of STO. Despite the use of the heavy STO substrate, however, proximity-induced quantum spin Hall (QSH) states in 2D TI phases, featuring a topologically protected helical edge spin phase within time-reversal-symmetry, is not confirmed. Here, with the use of a monolayer hBN spacer, it is revealed the coexistence of QSH (at B = 0T) and QHTI (at B not equal 0) states in the same single graphene sample placed on an STO, with a crossover regime between the two at low B. It is also classified that the different symmetries of the two nontrivial helical edge spin phases in the two states lead to different interaction with electron-puddle quantum dots, caused by a local surface pocket of the STO, in the crossover regime, resulting in a spin dephasing only for the QHTI state. The results obtained using STO substrates open the doors to investigations of novel QH spin states with different symmetries and their correlations with quantum phenomena. This exploration holds value for potential applications in spintronic devices.
Fe
O
川本 陽*; 吉川 貴史; 齊藤 英治; 他9名*
Applied Physics Letters, 124(13), p.132406_1 - 132406_7, 2024/03
被引用回数：4 パーセンタイル：82.03(Physics, Applied)Magnon spin currents in the ferrimagnetic garnet TbFe
O with 4 electrons were examined through the spin-Seebeck effect and neutron scattering measurements. The compound shows a magnetic compensation, where the spin-Seebeck signal reverses above and below 
= 249.5(4) K. Unpolarized neutron scattering unveils two major magnon branches with finite energy gaps, which are well explained in the framework of spin-wave theory. Their temperature dependencies and the direction of the precession motion of magnetic moments, i.e., magnon polarization, defined using polarized neutrons, explain the reversal at and decay of the spin-Seebeck signals at low temperatures. We illustrate an example that momentum- and energy-resolved microscopic information is a prerequisite to understand the magnon spin current.
layers on SrTiO substrates小杉 美央子*; 齊藤 英治; 吉川 貴史*; 他11名*
APL Materials (Internet), 11(8), p.081106_1 - 081106_6, 2023/08
被引用回数：1 パーセンタイル：13.37(Nanoscience & Nanotechnology)Strontium titanate [SrTiO (STO)], a perovskite oxide with an extremely high gate-tunable dielectric constant (
) due to quantum paraelectric phases, is attracting considerable attention for yielding various physical phenomena when two-dimensional (2D) layers are integrated. Superconductivity is such a typical phenomenon. However, the influence of the STO substrates on enhancing transition temperatures (
) for (atomically) thin 2D flakes attached to them has been rarely investigated. Here, we report gate-tunable and gradual four-terminal resistance drops with critical onset (
) and scanning tunneling spectroscopy (STS) spectra in devices comprising thin TaS flakes attached on monolayer hexagonal boron nitride (hBN) spacer/STO substrates. Observation of STS spectra confirms the presence of local superconducting gaps. (similar to 1.5 meV) with transition (
three-times higher than previous reports of under absent pressure and strong position dependence of 
. Depending on 
on back gate voltages (
) and magnetic fields, there is a strong correlation between and the onset of superconductivity, implying an enhancement of approximately five times compared with the previous highest-onset values without pressure as the applied increases. The high onset and. are discussed based on screening of the long-range Coulomb interaction (CI) due to the high- of SrTiO, while the short-ranged CI remains strong in the 2D limit, causing the superconductivity. Using a monolayer hBN/SrTiO substrate with opens doors to enhancement in thin superconducting layers integrated on it and wide application due to the solid-state high- substrates.
吉川 貴史*; 齊藤 英治
Annual Review of Condensed Matter Physics, 14, p.129 - 151, 2023/03
被引用回数：32 パーセンタイル：69.97(Physics, Condensed Matter)The spin Seebeck effect (SSE) refers to the generation of a spin current as a result of a temperature gradient in a magnetic material, which can be detected electrically via the inverse spin Hall effect in a metallic contact. Since the discovery of the SSE in 2008, intensive studies on the SSE have been conducted to elucidate its origin. SSEs appear in a wide range of magnetic materials including ferro-, ferri-, and antiferromagnets and also paramagnets with classical or quantum spin fluctuation. SSE voltage reflects fundamental properties of a magnet, such as elementary excitation, static magnetic order, spin correlation, and spin transport. In this article, we review recent progress on the SSE in various systems, with particular emphasis on its emerging role as a probe of these magnetic properties in solids. We also briefly discuss the recently discovered nuclear SSE.
前川 禎通; 吉川 貴史*; 中堂 博之; 家田 淳一; 齊藤 英治
Journal of Applied Physics, 133(2), p.020902_1 - 020902_24, 2023/01
被引用回数：24 パーセンタイル：93.17(Physics, Applied)Along with the progress of spin science and spintronics research, the flow of electron spins, i.e., spin current, has attracted interest. New phenomena and electronic states were explained in succession using the concept of spin current. Moreover, as many of the conventionally known spintronics phenomena became well organized based on spin current, it has rapidly been recognized as an essential concept in a wide range of condensed matter physics. In this article, we focus on recent developments in the physics of spin, spin current, and their related phenomena, where the conversion between spin angular momentum and different forms of angular momentum plays an essential role. Starting with an introduction to spin current, we first discuss the recent progress in spintronic phenomena driven by spin-exchange coupling: spin pumping, topological Hall torque, and emergent inductor. We, then, extend our discussion to the interaction/interconversion of spins with heat, lattice vibrations, and charge current and address recent progress and perspectives on the spin Seebeck and Peltier effects. Next, we review the interaction between mechanical motion and electron/nuclear spins and argue the difference between the Barnett field and rotational Doppler effect. We show that the Barnett effect reveals the angular momentum compensation temperature, at which the net angular momentum is quenched in ferrimagnets.
大柳 洸一*; 高橋 三郎*; 吉川 貴史*; 齊藤 英治
Physical Review B, 107(1), p.014423_1 - 014423_8, 2023/01
被引用回数：11 パーセンタイル：82.61(Materials Science, Multidisciplinary)We have theoretically investigated the spin Seebeck effect (SSE) in a normal metal (NM)/paramagnetic insulator (PI) bilayer system. Through a linear response approach, we calculated the thermal spin pumping from PI to NM and backflow spin current from NM to PI, where the spin-flip scattering via the interfacial exchange coupling between conduction-electron spin in NM and localized spin in PI is taken into account. We found a finite spin current appears at the interface under the difference in the effective temperatures between spins in NM and PI, and its intensity increases by increasing the density of the localized spin S. Our model well reproduces the magnetic-field-induced reduction of the paramagnetic SSE in Pt/GdGaO experimentally observed when the Zeeman energy is comparable to the thermal energy, which can be interpreted as the suppression of the interfacial spin-flip scattering. The present finding provides an insight into the mechanism of paramagnetic SSEs and the thermally induced spin-current generation in magnetic materials.
Lee, O.*; 山本 慧; 埋田 真樹; Zollitsch, C. W.*; Elyasi, M.*; 吉川 貴史*; 齊藤 英治; Bauer, G. E. W.*; 紅林 秀和*
Physical Review Letters, 130(4), p.046703_1 - 046703_6, 2023/01
被引用回数：16 パーセンタイル：91.47(Physics, Multidisciplinary)We experimentally and theoretically demonstrate that nonlinear spin-wave interactions suppress the hybrid magnon-photon quasiparticle or "magnon polariton" in microwave spectra of an yttrium iron garnet film detected by an on-chip split-ring resonator. We observe a strong coupling between the Kittel and microwave cavity modes in terms of an avoided crossing as a function of magnetic fields at low microwave input powers, but a complete closing of the gap at high powers. The experimental results are well explained by a theoretical model including the three-magnon decay of the Kittel magnon into spin waves. The gap closure originates from the saturation of the ferromagnetic resonance above the Suhl instability threshold by a coherent back reaction from the spin waves.
Y
FeO films吉川 貴史*; 齊藤 英治; 他6名*
Physical Review Materials (Internet), 6(10), p.104402_1 - 104402_13, 2022/10
被引用回数：7 パーセンタイル：46.06(Materials Science, Multidisciplinary)We have investigated hybridized magnon-phonon excitation (magnon polarons) in spin Seebeck effects (SSEs) in BiYFeO (BixYxIG; x=0, 0.5, and 0.9) films with Pt contact. We observed sharp peak structures in the magnetic field H; dependence of the longitudinal SSE (LSSE) voltages, which appear when the phonon dispersions are tangential to the magnon dispersion curve in BixYIG. By increasing the Bi amount x, the peak fields in the LSSE shift toward lower H values due to the reduction of the sound velocities in BixYIG. We also measured the SSE in a nonlocal configuration and found that magnon-polaron anomalies appear with different signs and intensities. Our result shows composition-tunability of magnon-polaron anomalies and provides a clue to further unravel the physics of magnon-polaron SSEs.
大柳 洸一*; Gomez-Perez, J. M.*; Zhang, X.-P.*; 吉川 貴史*; Chen, Y.*; Sagasta, E.*; Chuvilin, A.*; Hueso, L. E.*; Golovach, V. N.*; Sebastian Bergeret, F.*; et al.
Physical Review B, 104(13), p.134428_1 - 134428_14, 2021/10
被引用回数：18 パーセンタイル：75.12(Materials Science, Multidisciplinary)We report the observation of the spin Hall magnetoresistance (SMR) in a paramagnetic insulator. By measuring the transverse resistance in a Pt/GdGaO (GGG) system at low temperatures, paramagnetic SMR is found to appear with an intensity that increases with the magnetic field aligning GGG's spins. The observed effect is well supported by a microscopic SMR theory, which provides the parameters governing the spin transport at the interface. Our findings clarify the mechanism of spin exchange at a Pt/GGG interface, and demonstrate tunable spin-transfer torque through the field-induced magnetization of GGG. In this regard, paramagnetic insulators offer a key property for future spintronic devices.
吉川 貴史*; Reitz, D.*; 伊藤 宏陽*; 巻内 崇彦*; 杉本 宜陽*; 恒川 翔*; 大門 俊介*; 大柳 洸一*; Ramos, R.*; 高橋 三郎*; et al.
Nature Communications (Internet), 12, p.4356_1 - 4356_7, 2021/07
被引用回数：23 パーセンタイル：84.33(Multidisciplinary Sciences)Thermoelectric effects have been applied to power generators and temperature sensors that convert waste heat into electricity. The effects, however, have been limited to electrons to occur, and inevitably disappear at low temperatures due to electronic entropy quenching. Here, we report thermoelectric generation caused by nuclear spins in a solid: nuclear-spin Seebeck effect. The sample is a magnetically ordered material MnCO having a large nuclear spin 
of 
Mn nuclei and strong hyperfine coupling, with a Pt contact. In the system, we observe low-temperature thermoelectric signals down to 100 mK due to nuclear-spin excitation. Our theoretical calculation in which interfacial Korringa process is taken into consideration quantitatively reproduces the results. The nuclear thermoelectric effect demonstrated here offers a way for exploring thermoelectric science and technologies at ultralow temperatures.
Ramos, R.*; 巻内 崇彦*; 吉川 貴史*; 大門 俊介*; 大柳 洸一*; 齊藤 英治
Applied Physics Letters, 117(24), p.242402_1 - 242402_5, 2020/12
被引用回数：1 パーセンタイル：3.97(Physics, Applied)We investigated the magnetotransport properties of mesoscopic platinum nanostructures (wires and rings) with sub-100 nm lateral dimensions at very low temperatures. Despite the strong spin-orbit interaction in platinum, oscillation of the conductance as a function of the external magnetic field due to quantum interference effects was found to appear. The oscillation was decomposed into Aharonov-Bohm periodic oscillations and aperiodic fluctuations of the conductance due to a magnetic flux piercing the loop of the ring and the metal wires forming the nanostructures, respectively. We also investigated the magnetotransport under different bias currents to explore the interplay between electron phase coherence and spin accumulation effects in strong spin-orbit conductors.
南部 雄亮*; Barker, J.*; 沖野 夕貴*; 吉川 貴史*; 塩見 雄毅*; Enderle, M.*; Weber, T.*; Winn, B.*; Graves-Brook, M.*; Tranquada, J. M.*; et al.
Physical Review Letters, 125(2), p.027201_1 - 027201_6, 2020/07
被引用回数：64 パーセンタイル：94.76(Physics, Multidisciplinary)We measure the mode-resolved direction of the precessional motion of the magnetic order, i.e., magnon polarization, via the chiral term of inelastic polarized neutron scattering spectra. The magnon polarization is a unique and unambiguous signature of magnets and is important in spintronics, affecting thermodynamic properties such as the magnitude and sign of the spin Seebeck effect. However, it has never been directly measured in any material until this work. The observation of both signs of magnon polarization in YFeO also gives direct proof of its ferrimagnetic nature. The experiments agree very well with atomistic simulations of the scattering cross section.
PdSiHirschberger, M.*; 中島 多朗*; Kriener, M.*; 車地 崇*; Spitz, L.*; Gao, S.*; 吉川 明子*; 山崎 裕一*; 佐賀山 基*; 中尾 裕則*; et al.
Physical Review B, 101(22), p.220401_1 - 220401_6, 2020/06
被引用回数：51 パーセンタイル：90.84(Materials Science, Multidisciplinary)For the skyrmion-hosting intermetallic GdPdSi with centrosymmetric hexagonal lattice and triangular net of rare earth sites, we report a thorough investigation of the magnetic phase diagram. Our work reveals a magnetic phase with an isotropic value of the critical field for all orientations, where the magnetic ordering vector 
is depinned from its preferred directions in the basal plane. The bulk nature of the skyrmion lattice and of other magnetic phases was evidenced by specific-heat measurements. Resistivity anisotropy, likely originating from partial gapping of the density of states along in this Ruderman-Kittel-Kasuya-Yoshida magnet, is picked up via the planar Hall effect (PHE). The PHE confirms the single- nature of the magnetic order when the field is in the hexagonal plane, and allows one to detect the preferred directions of . Several scenarios for the depinned phase are discussed on the basis of the data.
FeO小畠 雅明; 吉井 賢資; 福田 竜生; 川崎 郁斗; 岡根 哲夫; 山上 浩志; 矢板 毅; 針井 一哉; 家田 淳一; 岡安 悟; et al.
JPS Conference Proceedings (Internet), 30, p.011192_1 - 011192_6, 2020/03
スピンゼーベック効果を示す系として注目されているPt/YFeO(YIG)系に対し、放射光を用いた硬X線光電子分光(HAXPES)により表面及び界面の電子状態測定を行った。本系ではスピンゼーベック効果のほかに特異な性質を示すことが報告されている。例えば、外部磁場が存在しない状況でもホール効果を発現する。この起源として、YIG中のFe
イオンがPt膜に染み出し、磁性を持つ金属間化合物を生成している可能性が提案されている。そこでHAXPESの分析深さを利用し、界面近傍の鉄イオン等の電子状態を測定した。Ptの厚みが2nm, 5nm, 8nm, 10nmの試料を測定したところ、2nmと5nmの試料において鉄イオンの分析を行うことができた。Fe 1s光電子スペクトルからは、鉄イオンが3+のものと金属的な0価に近い2つの状態が存在することが判明し、上記の可能性を支持する結果が得られた。Pt 4fやO 1sスペクトルなども測定しており、詳しい結果は当日報告する。
大柳 洸一*; 吉川 貴史*; 齊藤 英治
AIP Advances (Internet), 10(1), p.015031_1 - 015031_5, 2020/01
被引用回数：15 パーセンタイル：61.44(Nanoscience & Nanotechnology)We report the nonlocal spin Seebeck effect (nlSSE) in a lateral configuration of Pt/YFeO(YIG)/Pt systems as a function of the magnetic field 
(up to 10 T) at various temperatures (3 K 
300 K). The nlSSE voltage decreases with increasing B in a linear regime with respect to the input power (the applied charge-current squared 
). The reduction of the nlSSE becomes substantial when the Zeeman energy exceeds thermal energy at low temperatures, which can be interpreted as freeze-out of magnons relevant for the nlSSE. Furthermore, we found the nonlinear power dependence of the nlSSE with increasing 
at low temperatures (
20 K), at which the B-induced signal reduction became less visible. Our experimental results suggest that in the nonlinear regime, high-energy magnons are overpopulated compared to those expected from the thermal energy. We also estimate the magnon spin diffusion length as functions of and .
八尋 黎明*; 吉川 貴史*; Ramos, R.*; 大柳 洸一*; 日置 友智*; 大門 俊介*; 齊藤 英治
Physical Review B, 101(2), p.024407_1 - 024407_7, 2020/01
被引用回数：21 パーセンタイル：72.45(Materials Science, Multidisciplinary)We report the observation of anomalous peak structures induced by hybridized magnon-phonon excitation (magnon polarons) in the magnetic field dependence of the spin Peltier effect (SPE) in a LuBi
Fe
GaO (BiGa:LuIG) with Pt contact. The SPE peaks coincide with magnetic fields tuned to the threshold of magnonpolaron formation, consistent with the previous observation in the spin Seebeck effect. The enhancement of SPE is attributed to the lifetime increase in spin current caused by magnon-phonon hybridization in BiGa:LuIG.
