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論文

Magnetoferroelectric phase transition induced by latent spin-lattice coupling in the geometrically frustrated magnet $$mathrm{CuFe_{0.95}Al_{0.05}O_{2}}$$

玉造 博夢; 内原 猛*; 満田 節生*; 石井 祐太*; 中尾 裕則*; 竹端 寛治*; 今中 康貴*

Physical Review B, 111(13), p.134403_1 - 134403_9, 2025/04

https://doi.org/10.1103/PhysRevB.111.134403
 被引用回数：0

In multiferroic CuFe$$_{0.95}$$Al$$_{0.05}$$O$$_{2}$$, applying uniaxial pressure $$p$$ generates a magnetoferroelectric phase distinct from the well-studied spin-driven ferroelectric phase associated with helical magnetic ordering in this system. Using a four-circle neutron diffractometer, the magnetic structure of the $$p$$-induced magnetoferroelectric phase is determined as the collinear sinusoidal type, which itself does not break the inversion symmetry in this system. Additionally, synchrotron radiation X-ray diffraction experiments are conducted to investigate how the triangular lattice in CuFe$$_{0.95}$$Al$$_{0.05}$$O$$_{2}$$ is distorted by applied $$p$$. Although lattice distortion during the magnetic phase transition in CuFe$$_{0.95}$$Al$$_{0.05}$$O$$_{2}$$ is mitigated by the substitution of nonmagnetic Al$$^{3+}$$, the application of $$p$$ along the conjugate direction revives the "latent" spin-lattice coupling, causing the triangular lattice to distort during magnetic phase transition. The application of a magnetic filed considerably reduces $$p$$-induced ferroelectric polarization, but does not affect lattice distortion. These results indicate that $$p$$-induced ferroelectric polarization is not a consequence of the piezoelectric effect. Instead, the sinusoidal magnetic structure would contribute to the emergence of $$p$$-induced ferroelectric polarization through spin-lattice coupling.

論文

Single helicity of the triple-$$q$$ triangular skyrmion lattice state in the cubic chiral helimagnet EuPtSi

松村 武*; 田端 千紘; 金子 耕士; 中尾 裕則*; 垣花 将司*; 辺土 正人*; 仲間 隆男*; 大貫 惇睦*

Physical Review B, 109(17), p.174437_1 - 174437_8, 2024/05

https://doi.org/10.1103/PhysRevB.109.174437
 被引用回数：3 パーセンタイル：46.22(Materials Science, Multidisciplinary)

We investigated the magnetic helicity of the triple-$$q$$ magnetic structure of the triangular skyrmion lattice in the A-phase of EuPtSi for a magnetic field along the [111] axis by resonant X-ray diffraction using a circularly polarized beam. We show that all three Fourier components of the triple-$$q$$ structure are perpendicular to the respective $$q$$ vectors and have the same helicity. They are connected by the rotation operations about the [111] axis. The helicity is the same as that of the single-$$q$$ helimagnetic phase at low fields, suggesting that the antisymmetric exchange interaction inherent in the chiral structure supports the formation of the triangular skyrmion lattice. We also observe that the helical plane in the helimagnetic phase is tilted to the magnetic field to form a conical structure before the first-order transition to the skyrmion lattice phase.

論文

Magnetic order in honeycomb layered U$$_2$$Pt$$_6$$Ga$$_{15}$$ studied by resonant X-ray and neutron scattering

田端 千紘; 今 布咲子*; 太田 玖吾*; 日比野 瑠央*; 松本 裕司*; 網塚 浩*; 中尾 裕則*; 芳賀 芳範; 金子 耕士

Physical Review B, 109(13), p.134403_1 - 134403_7, 2024/04

https://doi.org/10.1103/PhysRevB.109.134403
 被引用回数：2 パーセンタイル：46.22(Materials Science, Multidisciplinary)

Antiferromagnetic (AF) order of U$$_2$$Pt$$_6$$Ga$$_{15}$$ with the ordering temperature $$T$$$$_{rm N}$$ = 26 K was investigated by resonant X-ray scattering and neutron diffraction on single crystals. This compound possesses a unique crystal structure in which uranium ions form honeycomb layers and then stacks along the c-axis with slight offset, which gives rise to a stacking disorder. The AF order can be described with the propagation vector of q = (1/6, 1/6, 0) in the hexagonal notation. The ordered magnetic moments orient perpendicular to the honeycomb layers, indicating a collinear spin structure consistent with Ising-like anisotropy. The magnetic reflections are found to be broadened along c$$^{*}$$ indicating that the stacking disorder results in anisotropic correlation lengths. The semiquantitative analysis of neutron diffraction intensity, combined with group theory considerations based on the crystallographic symmetry, suggests a zig-zag type magnetic structure for the AF ground state, in which the AF coupling runs perpendicular to the stacking offset, characterized as q = (1, 0, 0). The realization of the zig-zag magnetic structure implies the presence of frustrating intralayer exchange interactions involving both ferromagnetic (FM) first-neighbor and AF second and third-neighbor interactions in this compound.

論文

Magnetic ordering and structural phase transitions of Nd$$_{3}$$$$T$$$$_{4}$$Sn$$_{13}$$ ($$T$$ = Rh and Ir)

下田 愛海*; 岩佐 和晃*; 桑原 慶太郎*; 佐賀山 基*; 中尾 裕則*; 石角 元志*; 大原 高志; 中尾 朗子*; 星川 晃範*; 石垣 徹*

JPS Conference Proceedings (Internet), 38, p.011091_1 - 011091_6, 2023/05

https://doi.org/10.7566/JPSCP.38.011091

Synchrotron X-ray diffraction study revealed that Nd$$_{3}$$$$T$$$$_{4}$$Sn$$_{13}$$ ($$T$$ = Rh and Ir) undergo structural phase transitions characterized by the wave vector $$q$$$$_{rm L}$$=(1/2,1/2,0). Neutron diffraction study revealed antiferromagnetic ordering below $$T$$$$_{rm N}$$ = 1.65 and 1.42 K for Nd$$_{3}$$Rh$$_{4}$$Sn$$_{13}$$ and Nd$$_{3}$$Ir$$_{4}$$Sn$$_{13}$$, respectively, which is similar to that previously reported for Nd$$_{3}$$Co$$_{4}$$Sn$$_{13}$$. These compounds show a magnetic susceptibility saturation behavior below approximately 3 K. The results indicate emergence of anomalous electronic correlation in Nd$$_{3}$$$$T$$$$_{4}$$Sn$$_{13}$$ ($$T$$ = Co, Rh, and Ir) above $$T$$$$_{rm N}$$.

論文

High-field depinned phase and planar Hall effect in the skyrmion host Gd$$_2$$PdSi$$_3$$

Hirschberger, M.*; 中島 多朗*; Kriener, M.*; 車地 崇*; Spitz, L.*; Gao, S.*; 吉川 明子*; 山崎 裕一*; 佐賀山 基*; 中尾 裕則*; et al.

Physical Review B, 101(22), p.220401_1 - 220401_6, 2020/06

https://doi.org/10.1103/PhysRevB.101.220401
 被引用回数：50 パーセンタイル：90.18(Materials Science, Multidisciplinary)

For the skyrmion-hosting intermetallic Gd$$_2$$PdSi$$_3$$ with centrosymmetric hexagonal lattice and triangular net of rare earth sites, we report a thorough investigation of the magnetic phase diagram. Our work reveals a magnetic phase with an isotropic value of the critical field for all orientations, where the magnetic ordering vector ${bf q}$ is depinned from its preferred directions in the basal plane. The bulk nature of the skyrmion lattice and of other magnetic phases was evidenced by specific-heat measurements. Resistivity anisotropy, likely originating from partial gapping of the density of states along ${bf q}$ in this Ruderman-Kittel-Kasuya-Yoshida magnet, is picked up via the planar Hall effect (PHE). The PHE confirms the single-${bf q}$ nature of the magnetic order when the field is in the hexagonal plane, and allows one to detect the preferred directions of ${bf q}$. Several scenarios for the depinned phase are discussed on the basis of the data.

論文

Successive phase transitions in $$R_{3}$$Ir$$_{4}$$Sn$$_{13}$$ ($$R$$: La and Ce) investigated using neutron and X-ray diffraction

中里 晟也*; 岩佐 和晃*; 橋本 大輔*; 塩澤 真未*; 桑原 慶太郎*; 中尾 裕則*; 佐賀山 基*; 石角 元志*; 大原 高志; 中尾 朗子*; et al.

JPS Conference Proceedings (Internet), 30, p.011128_1 - 011128_6, 2020/03

https://doi.org/10.7566/JPSCP.30.011128

Successive phase transitions of $$R_{3}$$Ir$$_{4}$$Sn$$_{13}$$ ($$R$$: La and Ce) were studied using neutron and X-ray diffraction techniques. A semimetal Ce$$_{3}$$Ir$$_{4}$$Sn$$_{13}$$ undergoes three phase transitions: an antiferromagnetic ordering characterized by a propagation vector $$q_{rm M}$$ = (1/2, 1/2, 2/5) below 0.6 K, a structural transformation with $$q_{rm S2}$$= (1/4, 1/4, 1/4) at 2.0 K, and another structural transformation with $$q_{rm S1}$$ = (1/2, 1/2, 0) above room temperature. La$$_{3}$$Ir$$_{4}$$Sn$$_{13}$$ was confirmed to be a superconductor below 2.5 K under the $$q_{rm S1}$$ = (1/2, 1/2, 0) structure that also appears above room temperature.

論文

Magnetic field induced triple-$$q$$ magnetic order in trillium lattice antiferromagnet EuPtSi studied by resonant X-ray scattering

田端 千紘*; 松村 武*; 中尾 裕則*; 道村 真司*; 垣花 将司*; 稲見 俊哉*; 金子 耕士; 辺土 正人*; 仲間 隆男*; 大貫 惇睦*

Journal of the Physical Society of Japan, 88(9), p.093704_1 - 093704_5, 2019/09

https://doi.org/10.7566/JPSJ.88.093704
 被引用回数：43 パーセンタイル：87.71(Physics, Multidisciplinary)

The magnetic order in the magnetic-fild-induced so-called A phase of cubic chiral antiferromagnet EuPtSi was investigated by resonant X-ray scattering (RXS) near the Eu $$L_{2}$$ edge. The high flux RXS signal under the magnetic field applied along [111] revealed the first and second order satellite magnetic reflections, indicating that the A phase is a triple-$$q$$ magnetic ordered state that is described by three propagation vectors lying in the plane normal to the magnetic field direction; $$q_1$$, $$q_2$$, and $$q_3$$. With the high resolution in the reciprocal space achieved in the RXS measurement, it is suggested that the triple-$$q$$ order strongly couples with the underlying crystal lattice. The triple-$$q$$ magnetic order is discussed in the context of a magnetic skyrmion lattice on which the geometrical frustration may play a crucial role.

論文

Domain structure and electronic state in P3HT:PCBM blend thin films by soft X-ray resonant scattering

久保田 正人; 櫻井 岳暁*; 宮寺 哲彦*; 中尾 裕則*; 杉田 武*; 吉田 郵司*

Journal of Applied Physics, 120(16), p.165501_1 - 165501_5, 2016/10

https://doi.org/10.1063/1.4965988
 被引用回数：0 パーセンタイル：0.00(Physics, Applied)

有機薄膜太陽電池を高効率化するためには、適切なドメイン構造形成、並びにその物性評価が重要である。2成分有機分子凝集系の有機太陽電池薄膜で見られる構造や電子状態の特徴を捉えるために、成膜過程に用いる溶媒を変えた試料の放射光実験を行った。ドメインが成長し、分子自体の配向度が高い方が機能性が高いという特徴があることを明らかにした。

論文

Observation of all-in type tetrahedral displacements in nonmagnetic pyrochlore niobates

鳥越 秀平*; 石本 祐太朗*; 青石 優平*; 村川 寛*; 松村 大樹; 吉井 賢資; 米田 安宏; 西畑 保雄; 樹神 克明; 富安 啓輔*; et al.

Physical Review B, 93(8), p.085109_1 - 085109_5, 2016/02

https://doi.org/10.1103/PhysRevB.93.085109
 被引用回数：6 パーセンタイル：28.00(Materials Science, Multidisciplinary)

We observed all-in type Nb tetrahedral displacement in nonmagnetic pyrochlore niobates A$$_{2}$$Nb$$_{2}$$O$$_{7}$$ (A = Nd$$_{0.5}$$Ca$$_{0.5}$$ and Y$$_{0.5}$$Ca$$_{0.5}$$) through the analysis of the neutron pair distribution function and the extended X-ray absorption function spectroscopy. The all-in type Nb tetrahedral displacement, which has the character of a charge singlet state, is driven by the formation of the bonding orbital. The diffuse scattering in the X-ray diffraction, which has the resonant component in the Nb $$L$$3 edge, indicates that the all-in type Nb tetrahedral displacement has the periodicity with its short-range correlation.

論文

Magnetic and electronic properties of (LaMnO$$_3$$)$$_5$$(SrMnO$$_3$$)$$_5$$ superlattice revealed by resonant soft X-ray scattering

久保田 正人; 山田 浩之*; 中尾 裕則*; 岡本 淳*; 山崎 裕一*; 澤 彰仁*; 村上 洋一*

Japanese Journal of Applied Physics, 53(5S1), p.05FH07_1 - 05FH07_5, 2014/05

https://doi.org/10.7567/JJAP.53.05FH07
 被引用回数：2 パーセンタイル：8.28(Physics, Applied)

We have investigated the magnetic and electronic properties of (LaMnO$$_3$$)$$_5$$(SrMnO$$_3$$)$$_5$$ superlattice fabricated on a lattice-matched La$$_{0.3}$$Sr$$_{0.7}$$Al$$_{0.65}$$Ta$$_{0.35}$$O$$_{3}$$ substrate by resonant soft X-ray scattering. The temperature- and $mbox{boldmath $Q$}$-dependences of the energy spectra were measured around the Mn $$L_{2,3}$$-absorption edges. We successfully observed not only a signal that reflects the valence modulation of Mn ion, but also a magnetic signal reflecting ferromagnetism. Compared with the calculated models, we concluded that the ferromagnetism mainly originates from the magnetic moments at the Mn sites sandwiched by LaO layers.

論文

Antiferromagnetic order of the Co$$^{2+}$$ high-spin state with a large orbital angular momentum in La$$_{1.5}$$Ca$$_{0.5}$$CoO$$_{4}$$

岡本 淳*; 中尾 裕則*; 山崎 裕一*; 和達 大樹*; 田中 新*; 久保田 正人; 堀金 和正*; 村上 洋一*; 山田 和芳*

Journal of the Physical Society of Japan, 83(4), p.044705_1 - 044705_6, 2014/04

https://doi.org/10.7566/JPSJ.83.044705
 被引用回数：9 パーセンタイル：53.70(Physics, Multidisciplinary)

The antiferromagnetic insulator La$$_{1.5}$$Ca$$_{0.5}$$CoO$$_{4}$$ has been investigated by Co L$$_{2,3}$$-edge and O K-edge X-ray absorption spectroscopy (XAS) measurements and Co L$$_{2,3}$$-edge resonant soft X-ray magnetic scattering (RXMS)measurement to determine the Co electronic structures associated with magnetic ordering. Co L$$_{2,3}$$-edge linear-dichroic XAS shows that Co$$^{2+}$$ takes a high-spin (HS) state and Co$$^{3+}$$ takes a low-spin (LS) state. Using Co L$$_{2,3}$$-edge RXMS, we directly determined that an antiferromagnetic order is formed with a HS state of Co$$^{2+}$$ ions. Moreover, the spin and orbital angular momenta of the Co$$^{2+}$$ HS state are quantitatively estimated to be 1.1$$pm$$0.1 and 1.0$$pm$$0.1, respectively, and to align parallel in the ab plane by utilizing the cluster model calculation. The large orbital angular momentum of the Co$$^{2+}$$ HS state originates from the small $$D_{4h}$$-symmetry crystal field splitting of $$t_{2g}$$ levels, which is comparable with the spin-orbit coupling constant of the Co 3$$d$$ orbital.

論文

Spin state of Co$$^{3+} $$ in LaCo$$_{1-x}$$ Rh$$_{x}$$O$$_{3}$$ investigated by structural phenomena

浅井 晋一郎*; 岡崎 竜二*; 寺崎 一郎*; 安井 幸夫*; 小林 航*; 中尾 朗子*; 小林 賢介*; 熊井 玲児*; 中尾 裕則*; 村上 洋一*; et al.

Journal of the Physical Society of Japan, 82(11), p.114606_1 - 114606_6, 2013/11

https://doi.org/10.7566/JPSJ.82.114606
 被引用回数：6 パーセンタイル：42.18(Physics, Multidisciplinary)

LaCo$$_{1-x}$$ Rh$$_{x}$$O$$_{3}$$について中性子および放射光X線回折実験を行い、Co$$^{3+}$$イオンのスピン状態と結晶構造との関連を調べた。10KにおけるLaCo$$_{0.8}$$Rh$$_{0.2}$$O$$_{3}$$では、Co(Rh)O$$_{6}$$八面体のCo(Rh)-O間距離は理論値と一致し、格子体積は温度低下によって減少した。また、この格子体積の減少に伴って高スピン状態の比率は減少した。これらの結果から、Co$$^{3+}$$イオンのスピン状態は高スピン状態と低スピン状態が混在したものであり、高スピン状態は、Rh$$^{3+}$$イオンの置換によって生じたピン止め効果に加え熱励起によって発現することがわかった。

論文

Emergent phenomena in perovskite-type manganites

田口 康二郎*; 酒井 英明*; 奥山 大輔*; 石渡 晋太郎*; 藤岡 淳*; 福田 竜生; 橋爪 大輔*; 賀川 史敬*; 高橋 陽太郎*; 島野 亮*; et al.

Physica B; Condensed Matter, 407(11), p.1685 - 1688, 2012/06

https://doi.org/10.1016/j.physb.2012.01.006
 被引用回数：5 パーセンタイル：22.68(Physics, Condensed Matter)

Perovskite-type manganites exhibit various interesting phenomena arising from complex interplay among spin, charge, orbital, and lattice degrees of freedom. As the respective examples, perovskite-type YMnO$$_3$$ and Sr$$_{1-x}$$Ba$$_x$$MnO$$_3$$ are discussed. In the YMnO$$_3$$, the ferroelectric lattice distortion associated with the $$E$$-type spin order is observed for the first time. Displacement-type ferroelectricity with off-center magnetic ions is discovered for Sr$$_{0.5}$$Ba$$_{0.5}$$MnO$$_3$$, which shows both large polarization value and strong coupling between ferroelectricity and magnetism.

論文

Magnetic phase diagrams of YVO$$_{3}$$ and TbVO$$_{3}$$ under high pressure

備前 大輔*; 中尾 裕則*; 岩佐 和晃*; 村上 洋一*; 長壁 豊隆; 藤岡 淳*; 安江 俊夫*; 宮坂 茂樹*; 十倉 好紀*

Journal of the Physical Society of Japan, 81(2), p.024715_1 - 024715_6, 2012/02

https://doi.org/10.1143/JPSJ.81.024715
 被引用回数：7 パーセンタイル：45.54(Physics, Multidisciplinary)

低温高圧力下の中性子回折実験により、RVO$$_{3}$$(R=Y, Tb)の磁気相図を明らかにした。TbVO$$_{3}$$では、その基底状態が加圧によって${it C}$-タイプのスピン秩序(${it C}$-SO)から${it G}$-タイプのスピン秩序(${it G}$-SO)へと変化することが明らかとなった。これまでに基底状態の軌道秩序は、加圧により${it G}$-タイプの軌道秩序(${it G}$-OO)から${it C}$-タイプの軌道秩序(${it C}$-OO)へと変化することが明らかになっていたが、これと完全に対応している。一方、YVO$$_{3}$$の基底状態は、常圧から今回の最高圧力値6.2GPaまで、${it G}$-SOと${it C}$-OOが同時に存在し、非秩序相-[${it G}$-SO, ${it C}$-OO]相間の相転移が、ペロブスカイト型の遷移元素酸化物RMO$$_{3}$$において初めて観測された。両物質において[${it G}$-SO, ${it C}$-OO]相が加圧とともに安定化していくが、これは共有結合効果と超交換相互作用が重要な役割を果たしていると考えられる。

論文

X-ray photon correlation spectroscopy of structural fluctuations in relaxor ferroelectrics PZN-9%PT

大和田 謙二; 下村 晋*; 中尾 裕則*; 松下 三芳*; 並河 一道*; 水木 純一郎

Journal of Physics; Conference Series, 320, p.012086_1 - 012086_5, 2011/09

https://doi.org/10.1088/1742-6596/320/1/012086
 被引用回数：0 パーセンタイル：0.00(Physics, Condensed Matter)

91$$%$$Pb(Zn$$_{1/3}$$Nb$$_{2/3}$$)O$$_{3}$$-9$$%$$PbTiO$$_{3}$$においてX線光子相関分光を行い、$$T_{rm C}$$近傍において遅い構造揺らぎを見いだした。その遅い構造揺らぎは遅い成分と早い成分からなる。われわれは早い成分を抽出し10秒ほどの緩和時間を得た。これらの揺らぎはマクロな正方晶とミクロな射法対称性の競合によるものであり、低周波誘電率を与えるものであると推測される。

論文

Contribution of intermediate submicrometer structures to physical properties near $$T$$$$_{rm c}$$ in Pb(Zn$$_{1/3}$$Nb$$_{2/3}$$)O$$_{3}$$-9%PbTiO$$_{3}$$PbTiO$$_{3}$$

大和田 謙二; 水木 純一郎; 並河 一道*; 松下 三芳*; 下村 晋*; 中尾 裕則*; 廣田 和馬*

Physical Review B, 83(22), p.224115_1 - 224115_7, 2011/06

https://doi.org/10.1103/PhysRevB.83.224115
 被引用回数：9 パーセンタイル：37.70(Materials Science, Multidisciplinary)

コヒーレントX線回折法,X線散漫散乱法,通常のX線回折法,誘電率測定を相補利用した結果、Pb(Zn$$_{1/3}$$Nb$$_{2/3}$$)O$$_{3}$$-9%PbTiO$$_{3}$$においてマクロスケール,ミクロスケール,ナノスケールといった多重距離スケールを考慮した取り扱いが可能になり、それぞれのスケール階層の物性への寄与が議論できるようになった。

論文

X-ray photon correlation spectroscopy study in valence fluctuation compound Eu$$_{3}$$S$$_{4}$$

中尾 裕則*; 大和田 謙二; 下村 晋*; 落合 明*; 並河 一道*; 水木 純一郎; 三村 秀和*; 山内 和人*; 村上 洋一*

AIP Conference Proceedings 1234, p.935 - 938, 2010/06

https://doi.org/10.1063/1.3463370
 被引用回数：2 パーセンタイル：65.75(Physics, Applied)

X-ray photon correlation spectroscopy (XPCS) is a powerful tool to perform direct measurements of the dynamics of fluctuations in condensed matter systems at atomic resolution. Here we have investigated spatial and time correlations of domains in the valence fluctuated phase in a typical valence fluctuation compound Eu$$_{3}$$S$$_{4}$$ near the charge ordering temperature ($$T_{CO}$$). The spatial correlation was observed at the fundamental reflection (4 4 4) using coherent diffraction techniques, which indicated that the domain size is longer than 200 nm near $$T_{CO}$$. The time correlation of the domain was measured by the XPCS technique, and we found that the slow fluctuation of the order of 10 second exists only near $$T_{CO}$$.

論文

X-ray intensity fluctuation spectroscopy using nanofocused hard X-rays; Its application to study of relaxor ferroelectrics

大和田 謙二; 並河 一道*; 下村 晋*; 中尾 裕則*; 三村 秀和*; 山内 和人*; 松下 三芳*; 水木 純一郎

Japanese Journal of Applied Physics, 49(2), p.020216_1 - 020216_3, 2010/02

https://doi.org/10.1143/JJAP.49.020216
 被引用回数：3 パーセンタイル：14.48(Physics, Applied)

The use of a combination of coherent X-rays from a third-generation synchrotron light source and ultraprecise Kirkpatrick-Baez mirrors enables us to apply nanofocused hard X-rays in solid-state physics. We developed an apparatus for X-ray intensity fluctuation spectroscopy using the nanofocused hard X-rays and applied it to the study of relaxor ferroelectrics. We have successfully detected a large and slow intensity fluctuation of scattered X-rays above cubic-to-tetragonal phase transition temperature with a characteristic time scale on the order of 10 s. We speculated that the intensity fluctuation originates from domain number fluctuation, which is directly related to the dielectric response, particularly the frequency dispersion.

論文

Structural phase transition in the spin gap system YbAl$$_3$$C$$_3$$

松村 武*; 稲見 俊哉; 小坂 昌史*; 加藤 慶顕*; 犬飼 敬希*; 落合 明*; 中尾 裕則*; 村上 洋一*; 片野 進*; 鈴木 博之*

Journal of the Physical Society of Japan, 77(10), p.103601_1 - 103601_4, 2008/10

https://doi.org/10.1143/JPSJ.77.103601
 被引用回数：14 パーセンタイル：62.19(Physics, Multidisciplinary)

The unresolved phase transition at 80K in YbAl$$_3$$C$$_3$$ has been studied by X-ray diffraction. It has been confirmed that the transition is a structural one with atomic displacement. Superlattice reflections that appear below 80K show that the crystal structure changes from hexagonal to orthorhombic. From the reflection conditions, we conclude that the space group in the low temperature phase is Pbca, where all the atoms occupy the general 8c site. By fitting the observed intensities, we present two possible models of atomic displacement. The displacement results in the deformation of the triangular lattice of Yb spins, which is considered to be responsible for the formation of a spin-singlet ground state at low temperatures.

論文

NaV$$_{2}$$O$$_{5}$$の逐次電荷不均化による悪魔の花; 悪魔の花を咲かせるIsingスピンの詳細と競合する相互作用の理解

大和田 謙二; 藤井 保彦; 村岡 次郎*; 中尾 裕則*; 村上 洋一*; 野田 幸男*; 大隅 寛幸*; 池田 直*; 菖蒲 敬久; 礒部 正彦*; et al.

放射光, 21(2), p.87 - 96, 2008/03

http://ci.nii.ac.jp/naid/10020476047

常圧下で電荷不均化を示すNaV$$_{2}$$O$$_{5}$$の温度圧力相図上で「悪魔の花」が観測された。われわれは、X線構造解析的手法と電荷配列に敏感な共鳴X線回折法の相補利用により、低圧側と高圧側に現われる二つの基底状態の構造の関係を電荷配列も含めて明らかにした。その結果、二つの等価な電荷配列パターンがNaV$$_{2}$$O$$_{5}$$におけるIsingスピンに対応し、それに付随する原子変位はIsingスピンに線型に結合したものであることがわかった。このことからNaV$$_{2}$$O$$_{5}$$において、逐次電荷不均化による悪魔の花が実現されていると結論した。またわれわれは、競合する相互作用の起源がIsing spin-phonon結合によるものであると推測した。

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