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Observation of adsorbed hydrogen species on supported metal catalysts by inelastic neutron scattering

吉田 寿雄*; 山本 旭*; 細川 三郎*; 山添 誠司*; 吉川 聡一*; 原 賢二*; 中村 充孝; 蒲沢 和也*; 田中 庸裕*

Topics in Catalysis, 64(9-12), p.660 - 671, 2021/08

 被引用回数:0 パーセンタイル:0.01(Chemistry, Applied)

Inelastic neutron scattering (INS) enables direct and selective observation of H species due to the extremely large incoherent neutron scattering cross section of a hydrogen atom. In the present study, the adsorbed H species on some heterogeneous precious metal catalysts supported by alumina and carbon black were investigated by in situ INS spectroscopy with a newly designed sample cell. Three alumina-supported metal catalysts having Pt, Pd, and Rh metal nanoparticles with different particle sizes exhibited different INS spectra in intensities and band distribution. Observation of the H species on the metal nanoparticles and the alumina surface revealed their properties. In addition, the H atoms stored in Pd nanoparticles were observed as palladium hydride. In contrast, the H species on a Pt catalyst supported by carbon black were found to be strongly adsorbed on the carbon support.


Energy-dependent angular distribution of individual $$gamma$$ rays in the $$^{139}$$La($$n, gamma$$)$$^{140}$$La$$^{ast}$$ reaction

奥平 琢也*; 遠藤 駿典; 藤岡 宏之*; 広田 克也*; 石崎 貢平*; 木村 敦; 北口 雅暁*; 古賀 淳*; 新實 裕大*; 酒井 健二; et al.

Physical Review C, 104(1), p.014601_1 - 014601_6, 2021/07

 被引用回数:0 パーセンタイル:0.03(Physics, Nuclear)

Neutron energy-dependent angular distributions were observed for individual $$gamma$$ rays from the 0.74 eV $$p$$-wave resonance of $$^{139}$$La+$$n$$ to several lower excited states of $$^{140}$$La. The $$gamma$$-ray signals were analyzed in a two dimensional histogram of the $$gamma$$-ray energy, measured with distributed germanium detectors, and neutron energy, determined with the time-of-flight of pulsed neutrons, to identify the neutron energy dependence of the angular distribution for each individual $$gamma$$ rays. The angular distribution was also found for a photopeak accompanied with a faint $$p$$-wave resonance component in the neutron energy spectrum. Our results can be interpreted as interference between $$s$$- and $$p$$-wave amplitudes which may be used to study discrete symmetries of fundamental interactions.


Study of neutron-nuclear spin correlation term with a polarized Xe target

酒井 健二; 奥 隆之; 奥平 琢也; 甲斐 哲也; 原田 正英; 廣井 孝介; 林田 洋寿*; 加倉井 和久*; 清水 裕彦*; 広田 克也*; et al.

JPS Conference Proceedings (Internet), 33, p.011116_1 - 011116_6, 2021/03

中性子基礎物理学において、パリティ非保存(PNC)項や時間反転非保存項と干渉する中性子スピン$${bf s}$$と標的核スピン$${bf I}$$の相関項$${bf s}cdot{bf I}$$は重要な研究テーマである。中性子共鳴ピーク付近でPNC項の増大が測定され、スピン交換光ポンピング(SEOP)法により$$sim 10^{-1}$$の偏極が得られるキセノン(Xe)は、本研究にとって興味深い原子核である。我々は小型SEOPシステムを用いた偏極Xe標的を開発し、核破砕中性子源で得られる大強度の熱外中性子ビームを利用した$${bf s}cdot{bf I}$$項の研究を計画している。その第一段階として、我々は$$^{129}$$Xeの9.6eV共鳴ピーク付近でのXe偏極時と非偏極時の中性子透過率比の変化$$Delta R$$を捕らえることで、$${bf s}cdot{bf I}$$項に起因する中性子偏極能力の測定をJ-PARC物質・生命科学実験施設(MLF)のBL10で試みた。実験では、本測定系がドップラーブロードニングの影響($$Delta R_{rm DB} , {approx},10^{-2}$$)を検知できることを実証した上で、初期結果として有意な$$Delta R$$の値を得ている。現在は$$Delta R$$をより詳細に評価するために、核磁気・電子スピン共鳴法によるXe偏極度の導出を進めている。


Freezable and unfreezable hydration water; Distinct contributions to protein dynamics revealed by neutron scattering

山本 直樹*; 古府 麻衣子; 中島 健次; 中川 洋; 柴山 修哉*

Journal of Physical Chemistry Letters (Internet), 12(8), p.2172 - 2176, 2021/03

 被引用回数:0 パーセンタイル:0.01(Chemistry, Physical)



Observation of Coulomb-assisted nuclear bound state of $$Xi^-$$-$$^{14}$$N system

早川 修平; 藤田 真奈美; 長谷川 勝一; 橋本 直; 細見 健二; 市川 裕大; 今井 憲一*; 七村 拓野; 成木 恵; 佐甲 博之; et al.

Physical Review Letters, 126(6), p.062501_1 - 062501_6, 2021/02

 被引用回数:6 パーセンタイル:97.77(Physics, Multidisciplinary)

In an emulsion-counter hybrid experiment performed at J-PARC, a $$Xi^-$$ absorption event was observed which decayed into twin single-$$Lambda$$ hypernuclei. Kinematic calculations enabled a unique identification of the reaction process as $$Xi^{-} + ^{14}$$N$$ rightarrow ^{10}_Lambda$$Be + $$^5_Lambda$$He. For the binding energy of the $$Xi^{-}$$ hyperon in the $$Xi^-$$-$$^{14}$$N system a value of $$1.27 pm 0.21$$ MeV was deduced. The energy level of $$Xi^-$$ is likely a nuclear $$1p$$ state which indicates a weak $${Xi}N$$-$$LambdaLambda$$ coupling.


Identification of hydrogen species on Pt/Al$$_{2}$$O$$_{3}$$ by ${it in situ}$ inelastic neutron scattering and their reactivity with ethylene

山添 誠司*; 山本 旭*; 細川 三郎*; 福田 良一*; 原 賢二*; 中村 充孝; 蒲沢 和也*; 佃 達哉*; 吉田 寿雄*; 田中 庸裕*

Catalysis Science & Technology, 11(1), p.116 - 123, 2021/01

 被引用回数:3 パーセンタイル:81.22(Chemistry, Physical)

Hydrogen (H) species adsorbed on catalyst surfaces are key intermediates in catalytic hydrogenation reactions over supported metal catalysts. However, individual identification of H species on the metal catalysts has not been established to date. Here, we elucidated the H species on Pt/Al$$_{2}$$O$$_{3}$$ by the combination of ${it in situ}$ inelastic neutron scattering (INS) and density functional theory (DFT). Several H species in the presence of H$$_{2}$$ were successfully identified at different sites on the Pt surface and Al$$_{2}$$O$$_{3}$$ support. The ${it in situ}$ INS and FT-IR measurements revealed that the hydride/atop Pt-H, bridged perimeter/terrace Pt-H-Pt, and threefold Pt$$_{3}$$-H are active intermediates in the C$$_{2}$$H$$_{4}$$ hydrogenation reaction, whereas the edge Pt-H-Pt is a rather inert species. In addition, the ${it in situ}$ measurements indicate that the Al$$_{2}$$O$$_{3}$$ itself acts as hydrogen storage material by mediating AlO-H and Al-H-Al species, which serve H species in the C$$_{2}$$H$$_{4}$$ hydrogenation reaction.


Development of a Gd$$_{2}$$Si$$_{2}$$O$$_{7}$$ (GPS) scintillator-based alpha imaging detector for rapid plutonium detection in high-radon environments

森下 祐樹; 井崎 賢二; 金子 純一*; 山本 誠一*; 樋口 幹雄*; 鳥居 建男

IEEE Transactions on Nuclear Science, 67(10), p.2203 - 2208, 2020/10

 被引用回数:2 パーセンタイル:62.87(Engineering, Electrical & Electronic)



Development and application of a $$^3$$He neutron spin filter at J-PARC

奥平 琢也; 奥 隆之; 猪野 隆*; 林田 洋寿*; 吉良 弘*; 酒井 健二; 廣井 孝介; 高橋 慎吾*; 相澤 一也; 遠藤 仁*; et al.

Nuclear Instruments and Methods in Physics Research A, 977, p.164301_1 - 164301_8, 2020/10

 被引用回数:4 パーセンタイル:76.41(Instruments & Instrumentation)

We are developing a neutron polarizer with polarized $$^3$$He gas, referred to as a $$^3$$He spin filter, based on the Spin Exchange Optical Pumping (SEOP) for polarized neutron scattering experiments at Materials and Life Science Experimental Facility (MLF) of Japan Proton Accelerator Research Complex (J-PARC). A $$^3$$He gas-filling station was constructed at J-PARC, and several $$^3$$He cells with long spin relaxation times have been fabricated using the gas-filling station. A laboratory has been prepared in the MLF beam hall for polarizing $$^3$$He cells, and compact pumping systems with laser powers of 30 W and 110 W, which can be installed onto a neutron beamline, have been developed. A $$^3$$He polarization of 85% was achieved at a neutron beamline by using the pumping system with the 110 W laser. Recently, the first user experiment utilizing the $$^3$$He spin filter was conducted, and there have been several more since then. The development and utilization of $$^3$$He spin filters at MLF of J-PARC are reported.


Weak-coupling mean-field theory of magnetic properties of NiGa$$_{2}$$S$$_{4}$$

野村 拓司*; 山本 裕史*; 吉井 賢資

Journal of the Physical Society of Japan, 89(2), p.024704_1 - 024704_10, 2020/02

 被引用回数:0 パーセンタイル:0(Physics, Multidisciplinary)

三角格子上のスピン系の磁性は物性物理の分野で古くから取り扱われている。スピン間に反強磁性的相互作用が存在する場合は、フラストレーションにより複雑な磁気状態が発生すること等から、様々な系の性質が調べられている。本系では、このような系の一つであるNiGa$$_{2}$$S$$_{4}$$の性質を平均場近似により調べた。バンド計算で求まった電子状態を基にしたHatree-Fock法により、中性子回折で観測されているインコメンシュレートなスピン秩序状態を再現することができた。Ni 3d電子間のクーロン相互作用は2eV程度と小さく、Niスピンの値もS=1.1ボーア磁子程度と小さいことから、弱相関系でありNi-Sの共有結合が強いことも判明した。スピン間の相関関数を求めたところ、中性子非弾性散乱の結果と矛盾しない結果も得られた。


Measurement of the angular distribution of $$gamma$$-rays after neutron capture by $$^{139}$$La for a T-violation search

奥平 琢也; 清水 裕彦*; 北口 雅暁*; 広田 克也*; Haddock, C. C.*; 伊藤 維久也*; 山本 知樹*; 遠藤 駿典*; 石崎 貢平*; 佐藤 匠*; et al.

EPJ Web of Conferences, 219, p.09001_1 - 09001_6, 2019/12

原子核が熱外中性子を共鳴吸収する反応において、弱い相互作用起因のパリティ対称性の破れが核子間相互作用の最大10$$^{6}$$倍増幅される現象が観測されている。この反応では時間反転対称性の破れにも同様の増幅効果があることが理論的に予言されており、全く新しい手法で未知の時間反転対称性の破れを世界最高感度で探索できる可能性がある。しかし、その増幅率は全ての核種で未知であり、この手法がもつ可能性を具体的に議論できていなかった。本研究ではJ-PARC, MLF, BL04のGe検出器群を用いて、$$^{139}$$La(n,$$gamma$$)反応の角度分布測定を行い、世界で初めて$$^{139}$$Laで時間反転対称性の破れの増幅率を求めることに成功した。この結果を用いて、実験に必要な測定時間を見積もると、偏極率40%のLa核偏極技術、偏極率70%, 79atm・cmの$$^3$$He Spin Filterを用意すれば、1.4日の測定で世界最高感度で時間反転対称性の破れ探索実験が可能であることが判明した。現在原子力機構では高性能な$$^3$$He Spin Filterの開発を行なっており、本発表では$$gamma$$線の角度分布測定の結果、及び共用ビームラインに適用するための$$^3$$He Spin Filterの開発の現状について発表する。


Development of the neutron polarizer for the T-violation search using compound nuclei

奥平 琢也; 奥 隆之; 酒井 健二; 猪野 隆*; 林田 洋寿*; 廣井 孝介; 篠原 武尚; 加倉井 和久*; 相澤 一也; 清水 裕彦*; et al.

Proceedings of Science (Internet), 356, 5 Pages, 2019/12



A $$Sigma p$$ scattering experiment at J-PARC and the analysis status

中田 祥之*; 長谷川 勝一; 早川 修平*; 細見 健二; 市川 裕大; 今井 憲一; 七村 拓野*; 成木 恵*; 佐甲 博之; 佐藤 進; et al.

JPS Conference Proceedings (Internet), 26, p.023024_1 - 023024_5, 2019/11

J-PARC E40 aims to measure the differential cross sections of the $$Sigma^{pm}p$$ elastic scatterings and the $$Sigma^-p to Lambda n$$ conversion. A clear peak of $$Sigma^-$$ was observed in a missing mass spectrum of the $$pi^-pto K^+X$$ reaction and recoil protons from the $$pi p$$ elastic scattering were successfully observed in the data taken in the summer 2018. The rest of data taking is coming in the spring 2019.


First $$gamma$$-ray spectroscopy of an $$sd$$-shell hypernucleus, $$^{19}_{Lambda}$$F

Yang, S. B.*; 長谷川 勝一; 早川 修平*; 細見 健二; 市川 裕大; 今井 憲一; 佐甲 博之; 佐藤 進; 田村 裕和*; 谷田 聖; et al.

JPS Conference Proceedings (Internet), 26, p.023015_1 - 023015_5, 2019/11

We performed a gamma-ray spectroscopy of $$({}_{Lambda}^{19}{rm F})$$ at J-PARC Hadron Experimental Facility in 2015. It is the first measurement of $$gamma$$ rays emitted from $$sd$$-shell hypernuclei. In this experiment, we determined the energy spacing between the ground state spin doublet, $$3/2^+$$ and $$1/2^+$$ states, as 316 keV. The excitation energies of $$5/2^+$$ and $$1/2^+$$ states are also determined to be 895 and 1266 keV, respectively. The energy spacing is found to be well reproduced by shell-model calculations which describe $$s$$- and $$p$$-shell $$Lambda$$ hypernuclei well. The results show that the present theories of the $$Lambda N$$ interaction describe not only the light hypernuclei but also a heavier hypernucleus.


Study of $$Y^*$$ in nuclei through C$$(K^-, pi^+)X$$ spectrum at 1.8 GeV/$$c$$ in the J-PARC E05 experiment

本多 良太郎*; 長谷川 勝一; 早川 修平; 細見 健二; 今井 憲一; 市川 裕大; 七村 拓野; 成木 恵; 佐甲 博之; 佐藤 進; et al.

JPS Conference Proceedings (Internet), 26, p.023014_1 - 023014_4, 2019/11

We measured the $$(K^-,pi^+)$$ reaction spectra at 1.8 GeV/$$c$$ for the graphite and the polyethylene targets in the J-PARC E05 pilot experiment. By comparing the spectra for these two targets, it was found that $$Sigma^{*-}(1385)$$ in the $$^{11}$$B nucleus is quite broadened. Furthermore, we also compared broadness of $$Sigma^{*-}(1385)$$ with $$K^*(892)$$ obtained in the $$(K^-,p)$$ spectrum. $$Sigma^{*-}(1385)$$ seems to be much more broadened in nuclei than $$K^*(892)$$. We gave a possible interpretation, which is related to compositeness of decuplet baryons, for this situation.


Search for excited state of $$_{Sigma }^{4}{rm He}$$ hypernucleus in the J-PARC E13 experiment

中川 真菜美*; 長谷川 勝一; 早川 修平; 細見 健二; 市川 裕大; 今井 憲一; 佐甲 博之; 佐藤 進; 田村 裕和; 谷田 聖; et al.

JPS Conference Proceedings (Internet), 26, p.023005_1 - 023005_3, 2019/11

The $$Sigma N$$ interaction is not much studied than the $$Lambda N$$ interaction. To understand the $$Sigma N$$ interaction, we study $$Sigma$$ hypernuclei. As for the $$Sigma$$ hypernucleus, only the ground state of $$_{Sigma }^{4}{rm He}$$ has been observed. To obtain more information about the $$Sigma N$$ interaction, the excited state should be studied. Therefore, we measure the missing-mass of the $$^4$$He$$(K^-,pi^-)$$ reaction at $$p_{K^-} = 1.5$$ GeV/$$c$$ and $$theta_{rm Lab} =$$ 2-14$$^{circ}$$ at the J-PARC K1.8 beam line. The ground state of $$_{Sigma }^{4}{rm He}$$ is observed whereas a peak of the excited states is not observed. We also observe suppression of the $$Sigma$$ quasi-free process at smaller angles.


Gamma-ray spectroscopy of single $$Lambda$$-hypernuclei at J-PARC; Results and perspective

小池 武志*; 長谷川 勝一; 早川 修平*; 細見 健二; 市川 裕大; 今井 憲一; 佐甲 博之; 佐藤 進; 杉村 仁志; 田村 裕和; et al.

AIP Conference Proceedings 2130, p.020011_1 - 020011_9, 2019/07

 被引用回数:1 パーセンタイル:65.18

Experimental results from the J-PARC E13 experiments are summarized. A new experimental set up of E13 has established a platform for the future $$gamma$$-ray hypernuclear spectroscopy at J-PARC using kaon beams. New $$gamma$$ rays are identified in $$^4_{Lambda}$$He and $$^{19}_{Lambda}$$F. The energy of 1.406 MeV for the $$^4_{Lambda}$$He$$(1^+ to 0^+)$$ transition confirmed a sizable effect of Charge Symmetry Breaking (CSB) in $$Lambda N$$ interaction in the $$A=4$$ hypernuclear system. The identification of four $$gamma$$ rays in $$^{19}_{Lambda}$$F is made for the first time in $$sd$$ shell hypernuclei. Especially, energy spacing of the ground state doublet is found to be 315.5 keV. A good agreement with two theoretical calculations suggests that the theoretical formalism used in $$p$$ shell hypernuclei is also applicable to heavier hypernuclei. Lastly, an overview of the future J-PARC E63 experiment is given.


Observation of a $$Xi$$ bound state in the $$^{12}$$C$$(K^-, K^+)$$ reaction at 1.8 GeV/$$c$$

永江 知文*; 江川 弘行; 長谷川 勝一; 早川 修平; 細見 健二; 市川 裕大; 今井 憲一; 金原 慎二; 七村 拓野*; 成木 恵; et al.

AIP Conference Proceedings 2130, p.020015_1 - 020015_9, 2019/07

For the full understanding of baryon-baryon interactions in flavor $$SU(3)$$, the $$Xi N$$ interaction is the last missing piece of information. So far, we have revealed the $$Lambda N$$ interaction to be attractive ($$U_{Lambda} cong 30$$ MeV), and $$Sigma N$$ interaction to be repulsive in the medium to heavy mass-number region. The $$Lambda Lambda$$ bonding energy is weakly attractive. While we have a few experimental observations suggesting the $$Xi N$$ interaction would be attractive, there still exist large theoretical ambiguities weather it is attractive or not. Experimental determinations on the existence of bound states of $$Xi$$ hypernuclei by observing bound-state peaks are strongly awaited. In this report, a new preliminary result on the missing-mass spectrum of a $$^{12}$$C$$(K^-, K^+)$$ reaction, which strongly suggests the existence of $$Xi$$-hypernuclear bound states, is presented.


Localized magnetic excitations in the fully frustrated dimerized magnet Ba$$_{2}$$CoSi$$_{2}$$O$$_{6}$$Cl$$_{2}$$

栗田 伸之*; 山本 大輔*; 金坂 拓哉*; 古川 信夫*; 河村 聖子; 中島 健次; 田中 秀数*

Physical Review Letters, 123(2), p.027206_1 - 027206_6, 2019/07

 被引用回数:2 パーセンタイル:35.62(Physics, Multidisciplinary)

Magnetic excitations of the effective spin $$S$$ =1/2 dimerized magnet Ba$$_{2}$$CoSi$$_{2}$$O$$_{6}$$Cl$$_{2}$$ have been probed directly via inelastic neutron scattering experiments. We observed five types of excitation, which are all dispersionless within the resolution limits. The scattering intensities of the three low-lying excitations were found to exhibit different $$Q$$-dependences. Detailed analysis has demonstrated that Ba$$_{2}$$CoSi$$_{2}$$O$$_{6}$$Cl$$_{2}$$ is a two dimensional spin dimer system described only by a single dimer site, where the triplet excitations are localized owing to the almost perfect frustration of the interdimer exchange interactions and the undimerized spins, even in small concentration, make an essential contribution to the excitation spectrum.


Observation of a Be double-Lambda hypernucleus in the J-PARC E07 experiment

江川 弘行; 足利 沙希子; 長谷川 勝一; 橋本 直; 早川 修平; 細見 健二; 市川 裕大; 今井 憲一; 金原 慎二*; 七村 拓野; et al.

Progress of Theoretical and Experimental Physics (Internet), 2019(2), p.021D02_1 - 021D02_11, 2019/02

 被引用回数:13 パーセンタイル:85.21(Physics, Multidisciplinary)

A double-$$Lambda$$ hypernucleus, $${}_{LambdaLambda}mathrm{Be}$$, was observed by the J-PARC E07 collaborationin nuclear emulsions tagged by the $$(K^{-},K^{+})$$ reaction. This event was interpreted as a production and decay of $$ {}_{LambdaLambda}^{;10}mathrm{Be}$$,$${}_{LambdaLambda}^{;11}mathrm{Be}$$, or $${}_{LambdaLambda}^{;12}mathrm{Be}^{*}$$ via $$Xi^{-}$$ capture in $${}^{16}mathrm{O}$$.By assuming the capture in the atomic 3D state, the binding energy of two $$Lambda$$ hyperons$$,$$($$B_{LambdaLambda}$$)of these double-$$Lambda$$ hypernuclei are obtained to be$$15.05 pm 0.11,mathrm{MeV}$$, $$19.07 pm 0.11,mathrm{MeV}$$, and $$13.68 pm 0.11,mathrm{MeV}$$, respectively. Based on the kinematic fitting, $${}_{LambdaLambda}^{;11}mathrm{Be}$$ is the most likely explanation for the observed event.


Optimization of thickness of GAGG scintillator for detecting an alpha particle emitter in a field of high beta and gamma background

森下 祐樹; 山本 誠一*; 井崎 賢二; 金子 純一*; 星 勝也; 鳥居 建男

Radiation Measurements, 112, p.1 - 5, 2018/05

 被引用回数:7 パーセンタイル:77.16(Nuclear Science & Technology)

高線量$$beta$$$$gamma$$バックグランド下でプルトニウム同位体を検出するため、低$$beta$$$$gamma$$感度の$$alpha$$線検出器が必要となる。そこで、$$alpha$$線検出器のためのGAGGシンチレータの厚みの最適化を行った。0.05mm, 0.07mm, 0.1mmの厚みのシンチレータを用い、角厚みのシンチレータに対し$$alpha$$, $$beta$$, $$gamma$$線をそれぞれ照射し、波高スペクトルを得た。$$alpha$$線のエネルギー分解能は0.05mm厚のGAGGシンチレータが最も良かった。0.05mm、0.07mm、0.1mm、全ての厚みで$$gamma$$感度は問題とならなかった。$$beta$$感度は0.05mm厚のGAGGシンチレータを用いることで、0.1mm厚のGAGGシンチレータに対し1/100に減少した。したがって、0.05mm厚のGAGGシンチレータを用いた$$alpha$$線検出器は、高線量$$beta$$$$gamma$$バックグランド下でのプルトニウム同位体に検出に期待できる。

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