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論文

Superzone gap formation induced by ferroic orders

石飛 尊之

Journal of the Physical Society of Japan, 94(7), p.075001_1 - 075001_2, 2025/07

We show that superzone gap formation-phenomena usually attributed to antiferroic ordering-can also arise from ferroic orders in materials featuring sublattice structures. Through an analysis of a $$p$$-orbital tight-binding model on a zigzag chain, we reveal that ferroquadrupolar or ferromagnetic ordering, as well as external magnetic fields, can generate a Su-Schrieffer-Heeger-type gap.

論文

Surface structure and surface state of a tight-binding model on a diamond lattice

久保 勝規

Journal of the Physical Society of Japan, 94(7), p.074701_1 - 074701_5, 2025/07

Surface states of a tight-binding model with nearest-neighbor hopping on a diamond lattice of finite thickness are investigated. We consider systems with (001), (110), and (111) surfaces. Even if the surface direction is fixed, there is freedom to choose the surface structure due to the two-sublattice nature of a diamond lattice. The existence of surface states is governed by the topology of the matrix elements of the bulk Hamiltonian. In this sense, the existence of surface states is determined by the bulk Hamiltonian. However, the matrix elements depend on the choice of the unit cell, which should be chosen to conform to the surface structure. Thus, the surface states depend on the surface structure. We find that for each surface direction, there are two choices of surface structure, and depending on the chosen structure, the corresponding surface states emerge in distinct regions of the surface Brillouin zone.

論文

Three-stage Phase Transitions and Field-induced Phases in CeCoSi; A Landau Theory

石飛 尊之

Journal of the Physical Society of Japan, 94(7), p.073703_1 - 073703_4, 2025/06

We investigate both the nonmagnetic and magnetic ordered phases of CeCoSi using Landau theory. Our analysis predicts that three successive phase transitions occur at zero magnetic field. A quadrupole order parameter that emerges below $$T$$$$_{0}$$ = 12 K acts as a weak symmetry-breaking field on the antiferromagnetic ordering below $$T_{rm N}$$ = 9.4 K, giving rise to two-stage magnetic transitions. In the higher-temperature antiferromagnetic phase in the temperature range in $$T_{rm s2}$$ = 8 K $$<$$ $$T$$ $$<$$ $$T_{rm N}$$, an out-of-plane component of antiferromagnetic moment may be present or absent. If present, magnetic fields applied along the [100] and [110] directions induce additional magnetic phases.

論文

Distinguishing ion dynamics from muon diffusion in muon spin relaxation II; Extension to paramagnetic muons

門野 良典*; 伊藤 孝

Journal of the Physical Society of Japan, 94(6), p.064601_1 - 064601_11, 2025/06

We extend the previously published model that distinguishes between the diffusive motion of diamagnetic muons and the dynamics of ions around the muon in matter, and propose a generalized model for $$paramagnetic$$ $$muons$$ (Mu$$^0$$s, bound states of a muon and an unpaired electron) observed in non-metallic host materials. The new model distinguishes among the independent motion of unpaired electron associated with Mu$$^0$$, the self-diffusive motion of Mu$$^0$$ as single atomic entity, and that of the ions surrounding Mu$$^0$$, where the muon spin relaxation is induced by dynamical fluctuations of the hyperfine (HF) field exerted from the unpaired electron (e.g., due to spin/charge exchange reaction) and/or that of the nuclear hyperfine (NHF) interactions between the unpaired electron and the surrounding ions. We have applied this model to the muonated radicals (Mu$$^0$$s in a polaron state) in conducting polymers, and examined the validity of the interpretations claimed in the earlier literature that the spin relaxation is induced by quasi-one dimensional jump motion of the unpaired electron. The result suggests that experimental support for such a claim is still inadequate and needs to be reexamined, including the possibility of other origins for the fluctuations. It is expected that our model will prove a useful guide for $$mu$$SR studies of various local dynamics involving paramagnetic muon states.

論文

Flat surface state with octupole moment in an $$e_g$$ orbital system on a simple cubic lattice

久保 勝規

Journal of the Physical Society of Japan, 94(5), p.054703_1 - 054703_7, 2025/05

A tight-binding model for $$e_g$$ orbitals on a simple cubic lattice with finite thickness is investigated. The hopping integrals for nearest-neighboring sites are considered. We examine the electronic band structures for systems with (001), (110), and (111) surfaces. Electronic states well localized around the surfaces are found for the (110) and (111) surfaces. In particular, the surface state is flat and extends in the entire Brillouin zone for the (111) surface, provided the bulk band projected onto the surface Brillouin zone is gapped. We also find that these surface states possess octupole moments in both the (110) and (111) surface cases.

論文

Neutron spectroscopy study on crystalline electric field excitations in NdB$$_4$$

山内 宏樹; 目時 直人; 綿貫 竜太*; Hong, T.*; Fernandez-Baca, J. A.*; 萩原 雅人; 益田 隆嗣*; 吉沢 英樹*; 伊藤 晋一*

Journal of the Physical Society of Japan, 94(5), p.054705_1 - 054705_8, 2025/04

The $textit{f}$-electron states of NdB$$_4$$ were determined by observing crystalline electric field (CEF) excitations with inelastic neutron scattering experiments. Our analysis yields CEF excitation energies of 2.8, 12.4, 17.2, and 25.4 meV. The $textit{f}$-electron states are simply described by one of $$J$$-multiplets $$left|pm J_z rightrangle$$ with negligibly small mixing. The ground state is the pseudo-quartet consist of the ground doublet dominated by $$left|pm frac{5}{2} rightrangle$$ and the first excited doublet dominated by $$left|pm frac{7}{2} rightrangle$$ at 2.8 meV, which is consistent with magnetic specific heat and entropy reported in earlier study. The simple $textit{f}$-electron states in NdB$$_4$$ are the consequence of the strong uniaxial and in-plane isotropic CEF potential due to the local structure of Nd$$^{3+}$$ ions with point symmetry $$C_{2v}$$.

論文

Anisotropic magnetic field-temperature phase diagrams in CeCoSi

日高 宏之*; 柳谷 駿*; 小野寺 進太朗*; 柳澤 達也*; 網塚 浩*; 谷田 博司*; 石飛 尊之

Journal of the Physical Society of Japan, 94(3), p.034706_1 - 034706_9, 2025/03

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

We investigated the magnetic-field direction anisotropy of the unknown ordered phase in the tetragonal compound CeCoSi through bulk physical property measurements. The anisotropy in the field direction, previously identified in X-ray diffraction experiments, where a field-induced phase appears along [100] but not along [110], was confirmed in the bulk properties. Combining these experimental results with Landau theory, we infer that the field-induced phase in the [100] direction emerges under an infinitesimally small magnetic field.

論文

The Influence of structural dynamics in two-dimensional hybrid organic-inorganic perovskites on their photoluminescence efficiency; Neutron scattering analysis

Rajeev, H. S.*; Hu, X.*; Chen, W.-L.*; Zhang, D.*; Chen, T.*; 古府 麻衣子*; 梶本 亮一; 中村 充孝; Chen, A. Z.*; Johnson, G. C.*; et al.

Journal of the Physical Society of Japan, 94(3), p.034602_1 - 034602_14, 2025/03

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

Two-dimensional hybrid organic-inorganic perovskites (HOIPs) have emerged as promising materials for light-emitting diode applications. In this study, by using time-of-flight neutron spectroscopy we identified and quantitatively separated the lattice vibrational and molecular rotational dynamics of two perovskites, butylammonium lead iodide (BA)$$_{2}$$PbI$$_{4}$$ and phenethyl-ammonium lead iodide (PEA)$$_{2}$$PbI$$_{4}$$. By examining the corresponding temperature dependence, we found that the lattice vibrations, as evidenced by neutron spectra, are consistent with the lattice dynamics obtained from Raman scattering. We revealed that the rotational dynamics of organic molecules in these materials tend to suppress their photoluminescence quantum yield (PLQY) while the vibrational dynamics did not show predominant correlations with the same. Additionally, we observed photoluminescence emission peak splitting for both systems, which becomes prominent above certain critical temperatures where the suppression of PLQY begins. This study suggests that the rotational motions of polarized molecules may lead to a reduction in exciton binding energy or the breaking of degeneracy in exciton binding energy levels, enhancing non-radiative recombination rates, and consequently reducing photoluminescence yield. These findings offer a deeper understanding of fundamental interactions in 2D HOIPs and could guide the design of more efficient light-emitting materials for advanced technological applications.

論文

Electronic phase diagram of itinerant electron metamagnet UCoAl

前田 瑞穂*; 松田 達磨*; 芳賀 芳範; 白崎 謙次*; 木村 憲彰*

Journal of the Physical Society of Japan, 94(2), p.024707_1 - 024707_6, 2025/01

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

We investigate the pressure dependence of the magnetoresistivity and Hall resistivity for an itinerant-electron metamagnet UCoAl. The first-order metamagnetic transition point varies as a function of hydrostatic pressure and terminates at the critical pressure 2.0 GPa. The electronic system, however, does not show criticality at this pressure but extends to higher pressures, unlike the usual quantum critical behavior.

論文

Self-learning Monte Carlo with equivariant Transformer

永井 佑紀; 富谷 昭夫*

Journal of the Physical Society of Japan, 93(11), p.114007_1 - 114007_8, 2024/11

 被引用回数:1 パーセンタイル:48.32(Physics, Multidisciplinary)

生成AIにおける基幹技術であるTransformerを用いた新しい自己学習モンテカルロ法を提案した。本研究では、文章における距離の離れた単語の関連性を推測することができるTransformerのAttention機構を用いることにより、電子系の相転移で重要となる長距離相関を効率よく取り込める有効模型を構築した。さらに、スピン回転、空間並進など系が満たすべき対称性をネットワークに取り込むことにより、パラメータ数を劇的に減らすことに成功した。また、レイヤー数を増やすにつれてlossが減っていくというスケーリング則を見出した。

論文

Clear reduction in spin susceptibility and superconducting spin rotation for $$H||a$$ in the early-stage sample of spin-triplet superconductor UTe$$_2$$

北川 俊作*; 徳永 陽; 酒井 宏典; 神戸 振作; 他11名*

Journal of the Physical Society of Japan, 93(12), p.123701_1 - 123701_5, 2024/11

 被引用回数:2 パーセンタイル:68.78(Physics, Multidisciplinary)

We report the re-measurement of the $$a$$-axis spin susceptibility component in an early-stage sample of the spin-triplet superconductor UTe$$_2$$ with the transition temperature of $$T_{rm SC}$$ = 1.6 K. Using Knight-shift measurements along the $$b$$ axis and at a 10-degree tilt from the $$b$$ axis towards the $$a$$ axis, we accurately determined the $$a$$-axis component without directly measuring the $$a$$-axis Knight shift. The experiment reveals that the previously reported absence of the reduction in Knight shift is attributed to the missing of signal from the superconducting region and to the detection of residual signals from the non-superconducting region instead.

論文

Improvement of a time-of-flight spectrometer AGNES at JRR-3 using supermirror techniques

秋葉 宙*; 大政 義典*; 古府 麻衣子*; Zhang, M.*; 佐藤 駿*; 山室 修*

Journal of the Physical Society of Japan, 93(9), p.091010_1 - 091010_6, 2024/09

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

AGNES is a direct geometry chopper-type time-of-flight neutron spectrometer installed at the cold neutron guide (C3-1-1) of JRR-3 (Tokai, Japan). This instrument is well-suited for studies on low-energy excitations of powdered and amorphous samples, and quasi-elastic scattering with an energy resolution of 120 $$mu$$eV (standard mode) or 50 $$mu$$eV (high-resolution mode). During the long shutdown period of JRR-3 due to the Great East Japan Earthquake in 2011, AGNES was significantly improved through the installation of supermirror-coated neutron guide tubes and collimator, installation of a new-type top-loading cryo-furnace, and renewal of data acquisition electronics and software. As a result, the neutron intensity has increased by 7.7 times in the standard mode and by 3.2 times in the high-resolution mode. These enhancements facilitate experiments with small amounts of samples, and under special environments, which have previously been challenging.

論文

Chiral gauge field in fully spin-polarized magnetic Weyl semimetal with magnetic domain walls

小沢 耀弘*; 荒木 康史; 野村 健太郎*

Journal of the Physical Society of Japan, 93(9), p.094704_1 - 094704_9, 2024/09

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

磁性ワイル半金属における磁化の変調は、運動量空間におけるワイル点位置のシフトを引き起こし、ワイルフェルミオンに対して実効的なカイラリティ依存のゲージ場として働く。本研究では、完全スピン偏極したワイル強磁性体Co$$_{3}$$Sn$$_{2}$$S$$_{2}$$において、このような磁化誘起カイラルゲージ場の効果を取り扱う。磁化と結合した積層カゴメ格子上で定義したCo$$_{3}$$Sn$$_{2}$$S$$_{2}$$の強束縛模型を用いて、運動量空間におけるワイル点の位置(カイラルゲージ場に相当)の磁化方向依存性を計算した。これを用いて、磁壁構造が存在する場合に、カイラルゲージ場の空間構造から生じるカイラル磁場を評価した。その結果磁壁存在下では、ワイルフェルミオンに対してランダウ量子化を強く引き起こすほどの、数百テスラという巨大なカイラル磁場が生じることが導出された。このような巨大カイラル磁場は、従来の磁性体スピントロニクスにおけるスピン起電力に相当する、磁壁の運動による電荷ポンピングを誘起することも予想される。

論文

Polarized and unpolarized neutron scattering for magnetic materials at the triple-axis spectrometer PONTA in JRR-3

中島 多朗*; 齋藤 開*; 小林 尚暉*; 川崎 卓郎; 中村 龍也; 古川 はづき*; 浅井 晋一郎*; 益田 隆嗣*

Journal of the Physical Society of Japan, 93(9), p.091002_1 - 091002_5, 2024/09

 被引用回数:2 パーセンタイル:68.78(Physics, Multidisciplinary)

Neutron scattering is a powerful tool to study magnetic structures and cross-correlated phenomena originated from symmetry of the magnetic structures in matter. Among a number of neutron scattering techniques, polarized neutron scattering is quite sensitive to the orientations of the magnetic moments, which are essential to understand microscopic mechanisms of the spin-driven emergent phenomena. Here, we present POlarized Neutron Triple-Axis spectrometer PONTA in the Japan Research Reactor 3 (JRR-3), and show the present capabilities of polarized and unpolarized neutron scattering by introducing recent results from the instrument.

論文

Polarized neutron diffraction study on UPt$$_{2}$$Si$$_{2}$$

今 布咲子*; 田端 千紘; 齋藤 開*; 中島 多朗*; 日高 宏之*; 柳澤 達也*; 網塚 浩*

Journal of the Physical Society of Japan, 93(4), p.044701_1 - 044701_11, 2024/04

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

We investigated the magnetic structure of the antiferromagnetic (AFM) ordered state ($$T_{rm N}$$ $$sim$$ 34 K) in tetragonal UPt$$_{2}$$Si$$_{2}$$ using polarized and unpolarized neutron diffraction. Previous neutron scattering studies reported that this system possesses a simple AFM structure with a propagation vector, Q= 0, and the ordered magnetic moments aligned along the c-axis. By contrast, our latest resonant X-ray scattering (RXS) experiments have revealed that the magnetic structure is modulated by the charge-density-wave (CDW) order, which emerges in one of the two Pt atomic layers in the unit cell below $$sim$$320 K. The modulation is characterized by a transverse wave in the c-plane, with the propagation vector of the CDW order, q$$_{rm CDW}$$ = ($$sim$$0.42, 0, 0). In this study using neutron scattering, we observed that the superlattice reflections specified by q$$_{rm CDW}$$ develop below $$T_{rm N}$$, in addition to the magnetic reflections with Q= 0, thereby further confirming the presence of modulation in the AFM structure of this system. From detailed analyses, we revealed that the amplitude of the transverse-wave magnetic modulation is 0.72(2)$$mu$$$$_{rm B}$$/U, which is quantitative information that can not be obtained through RXS experiments. This implies that the CDW drives the ordered magnetic moments to be tilted up to 20$$^{circ}$$ in the AFM state. The observations strongly suggest that the magnetism of UPt$$_{2}$$Si$$_{2}$$ is heavily influenced by the hybridization effects between the $$5f$$ electrons of U and the 5d electrons of Pt.

論文

Distinguishing ion dynamics from muon diffusion in muon spin relaxation

伊藤 孝; 門野 良典*

Journal of the Physical Society of Japan, 93(4), p.044602_1 - 044602_7, 2024/04

 被引用回数:3 パーセンタイル:68.78(Physics, Multidisciplinary)

We propose a model to describe the fluctuations in the internal magnetic field due to ion dynamics observed in muon spin relaxation ($$mu$$SR) by an Edwards-Anderson-type autocorrelation function that separates the quasi-static and dynamic components of the correlation by the parameter $$Q$$ (where $$0leq Qleq 1$$). Our Monte Carlo simulations for this model showed that the time evolution of muon spin polarization deviates significantly from the Kubo-Toyabe function. To further validate the model, the results of simulations were compared with the $$mu$$SR spectra observed in a hybrid organic-inorganic perovskite FAPbI$$_3$$ [with FA referring to HC(NH$$_2$$)$$_2$$], where local field fluctuations associated with the rotational motion of FA molecules and quasi-static fields from the PbI$$_3$$ lattice are presumed to coexist. The least-squares curve fitting showed reasonable agreement with the model with $$Q=0.947(3)$$, and the fluctuation frequency of the dynamical component was obtained. This result opens the door to the possibility of experimentally distinguishing fluctuations due to the dynamics of ions around muons from those due to the self-diffusion of muons. On the other hand, it suggests the need to carefully consider the spin relaxation function when applying $$mu$$SR to the issue of ion dynamics.

論文

Field-induced insulator-metal transition in EuTe$$_2$$

竹内 徹也*; 本多 史憲*; 青木 大*; 芳賀 芳範; 木田 孝則*; 鳴海 康雄*; 萩原 政幸*; 金道 浩一*; 軽部 皓介*; 播磨 尚朝*; et al.

Journal of the Physical Society of Japan, 93(4), p.044708_1 - 044708_10, 2024/04

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

Electrical and magnetic properties of divalent europium antiferromagnet EuTe$$_2$$ are studied on single crystals grown from Te-flux method. Antiferromagnetism occurs at 11 K with an insulating ground state. Application of magnetic field induces a sudden resistance drop leading to a phase transition to metallic state. Energy band calculations reveal the appearance of a Fermi surface pocket with Te-5p character induced by the polarized Eu moments.

論文

Weyl semimetallic state in the Rashba-Hubbard Model

久保 勝規

Journal of the Physical Society of Japan, 93(2), p.024708_1 - 024708_8, 2024/02

 被引用回数:4 パーセンタイル:85.16(Physics, Multidisciplinary)

We investigate the Hubbard model with the Rashba spin-orbit coupling on a square lattice. The Rashba spin-orbit coupling generates two-dimensional Weyl points in the band dispersion. In a system with edges along [11] direction, zero-energy edge states appear, while no edge state exists for a system with edges along an axis direction. The zero-energy edge states with a certain momentum along the edges are predominantly in the up-spin state on the right edge, while they are predominantly in the down-spin state on the left edge. Thus, the zero-energy edge states are helical. By using a variational Monte Carlo method for finite Coulomb interaction cases, we find that the Weyl points can move toward the Fermi level by the correlation effects. We also investigate the magnetism of the model by the Hartree-Fock approximation and discuss weak magnetic order in the weak-coupling region.

論文

Unique band structure of pressure induced semiconducting state in SmS characterized by $$^{33}$$S-nuclear magnetic resonance measurements

吉田 章吾*; 芳賀 芳範; 藤井 拓斗*; 中井 祐介*; 水戸 毅*; 他8名*

Journal of the Physical Society of Japan, 93(1), p.013702_1 - 013702_5, 2024/01

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

In Kondo insulators, a small energy gap evolves only at low temperatures. In this study, $$^{33}$$S-nuclear magnetic resonance measurements under high pressures are performed to clarify the electronic structure of SmS. The spin-lattice relaxation time, consisting of multiple components, was analyzed based on a periodic Anderson model with Bayesian inference, leading to a peculiar small gap state arising from strong hybridization.

論文

Isotopic composition of enriched $$^{100}$$Mo for production of medical $$^{rm 99m}$$Tc by $$^{100}$$Mo($$p,2n$$)$$^{rm 99m}$$Tc

橋本 慎太郎; 永井 泰樹*

Journal of the Physical Society of Japan, 92(12), p.124202_1 - 124202_11, 2023/12

 被引用回数:0 パーセンタイル:0.00(Physics, Multidisciplinary)

$$^{99}$$Moの娘核種であるテクネチウム99m($$^{rm 99m}$$Tc)は6時間の半減期で$$gamma$$線を出す放射性核種(RI)であり、SPECTなどの診断用RIとして世界中で用いられている。親核種の$$^{99}$$Moは原子炉で生成されているが、原子炉施設の老朽化等で安定供給が危ぶまれており、医療用加速器で濃縮$$^{100}$$Mo試料に陽子を照射し、$$^{100}$$Mo($$p,2n$$)$$^{99m}$$Tc反応を通じて生成する方法が提案されている。しかし、試料に微量に含まれる$$^{100}$$Mo以外のMo同位体から、$$^{rm 99m}$$Tc以外のTcが生成される問題がある。そこで本研究では、高純度の$$^{rm 99m}$$Tcを生成できるMo組成を調べるために、天然組成のMoの照射実験データに基づいて、全てのTc同位体生成の反応率を決定し、任意の組成をもつMo試料のTc同位体生成量をPHITSを用いて評価する手法を開発した。本手法の有効性を、濃縮$$^{100}$$Moで生成された各Tcの実測値との比較によって検証するとともに、高純度の$$^{rm 99m}$$Tc生成には$$^{97,96,95}$$Moの各不純物含有量の低減が必須であることを明らかにした。本成果は、照射時間等の施設固有の制約を考慮しながら、高純度の$$^{rm 99m}$$Tcを生成する際に必要なMo原料の組成決定に重要な役割を果たす。

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