Application of indentation technique to material degradation evaluation in the mercury target vessel for spallation neutron sources

Wakui, Takashi; Saito, Shigeru; Futakawa, Masatoshi

Jikken Rikigaku, 24(4), p.212 - 218, 2024/12

Irradiation damage is one of the main factors determining the lifetime of the mercury target vessel for spallation neutron source in J-PARC. To understand material degradation of the used vessels, it is planned to conduct an evaluation using inverse analyses with indentation tests on the structural materials of the used vessels and numerical experiments. This evaluation technique was applied to two kinds of ion-irradiated materials with different displacement damage doses, in which the irradiation condition was simulated. It could be confirmed that the ultimate strength increased, and the total elongation decreased with increasing irradiation. These trends are like the material degradation behaviors which have been reported by using small specimen's tensile tests.

Development of a hybrid method for evaluating the long-term structural soundness of nuclear reactor buildings using response monitoring and damage imaging technologies (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*

JAEA-Review 2023-048, 151 Pages, 2024/05

JAEA-Review-2023-048.pdf:8.48MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Development of a hybrid method for evaluating the long-term structural soundness of nuclear reactor buildings using response monitoring and damage imaging technologies" conducted in FY2022. The present study aims to develop an evaluation method necessary to obtain a perspective on the long term structural soundness of accident-damaged reactor buildings, where accessibility to work sites is extremely limited due to high radiation dose rate and high contamination. In FY2022, the second year of the three-year plan, some tests and other activities on the following research items were conducted following FY2021, based on the specific research methods and research directions clarified in FY2021.

Aging of fuel-containing materials (fuel debris) in the Chornobyl (Chernobyl) Nuclear Power Plant and its implication for the decommissioning of the Fukushima Daiichi Nuclear Power Station

Kitagaki, Toru; Krasnov, V.*; Ikeda, Atsushi

Journal of Nuclear Materials, 576, p.154224_1 - 154224_14, 2023/04

https://doi.org/10.1016/j.jnucmat.2022.154224

Study on degradation of fuel debris by combined effects of radiological, chemical, and biological functions (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*

JAEA-Review 2022-066, 91 Pages, 2023/03

JAEA-Review-2022-066.pdf:5.88MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Study on degradation of fuel debris by combined effects of radiological, chemical, and biological functions" conducted in FY2021. In the project, radiochemists, nuclear chemists, nuclear physicists, material scientists, and environmental biologists are teamed to elucidate the mechanism of the degradation of fuel debris by combined effects of radiological, chemical, and biological functions. In fiscal year 2021, the members of the project team have conducted on the microbial degradation of the simulated fuel debris under -ray irradiation, complex formation of pentavalent uranium, construction of microchannel system to detect micro-particles and the simulated fuel debris, sorption of tetravalent elements ...

Investigation of environment induced property change and cracking behavior in fuel debris (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2022-036, 115 Pages, 2023/01

JAEA-Review-2022-036.pdf:7.15MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Investigation of environment induced property change and cracking behavior in fuel debris" conducted in FY2021. The present study aims to investigate the environment induced property change and cracking behavior in fuel debris from the viewpoints of materials science. The research objective is cracking behavior in fuel debris which is presumed to be influenced by environment during long-term fuel debris processing period. The degradation models will be established to simulate the oxidation and hydrogenation processes possibly occurred at fuel debris. The evolution of phase constitution and the corresponding property change in the simulated fuel debris under various environmental conditions …

Investigation of environment induced property change and cracking behavior in fuel debris (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2021-058, 75 Pages, 2022/02

JAEA-Review-2021-058.pdf:4.82MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Investigation of environment induced property change and cracking behavior in fuel debris" conducted in FY2020. The present study aims to investigate the environment induced property change and cracking behavior in fuel debris from the viewpoints of materials science. The research objective is cracking behavior in fuel debris which is presumed to be influenced by environment during long-term fuel debris processing period. The degradation models will be established to simulate the oxidation and hydrogenation processes possibly occurred at fuel debris.

Study on degradation of fuel debris by combined effects of radiological, chemical and biological functions (Contract research); FY2019 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*

JAEA-Review 2020-046, 69 Pages, 2021/01

JAEA-Review-2020-046.pdf:4.81MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2019. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Study on Degradation of Fuel Debris by Combined Effects of Radiological, Chemical, and Biological Functions". In the project, radiochemists, nuclear chemists, nuclear physicists, material scientists, and environmental biologists are teamed to elucidate the mechanism of the degradation of fuel debris by combined effects of radiological, chemical, and biological Functions. In FY2019, the members of the project team focused on literature survey, preliminary experiments, and installation of experimental devices for the planned research.

Validation and verification for the melting and eutectic models in JUPITER code

Chai, P.; Yamashita, Susumu; Nagae, Yuji; Kurata, Masaki

Proceedings of 9th Conference on Severe Accident Research (ERMSAR 2019) (Internet), 14 Pages, 2019/03

In order to obtain a precise understanding of molten material behavior inside RPV and to improve the accuracy of the SA code, a new computational fluid dynamics (CFD) code with multi-phase, multi-physics models, which is called JUPITER, was developed. It optimized the algorithms of the multi-phase calculation. Besides, the chemical reactions are also modeled carefully in the code so that the melting process could be treated precisely. A series of verification and validation studies are conducted, which show good agreement with analytical solutions and previous experiments. The capabilities of the multi-physics models in JUPITER code provide us another useful tool to investigate the molten material behaviors in the relevant severe accident scenario.

Performance degradation of candidate accident-tolerant cladding under corrosive environment

Nagase, Fumihisa; Sakamoto, Kan*; Yamashita, Shinichiro

Corrosion Reviews, 35(3), p.129 - 140, 2017/08

https://doi.org/10.1515/corrrev-2017-0014

As the lessons learnt from the accident at the Fukushima Daiichi Nuclear Power Station, advanced cladding materials are being developed to enhance accident tolerance comparing with conventional zirconium alloys. The present paper reviews the progress of the development and summarizes subjects to be solved for the enhanced accident-tolerance fuel cladding, focusing on performance degradation under various corrosive environmental conditions that should be considered in designing the LWR fuel.

Degradation of 2-chlorophenol by -ray irradiation in zeolite/water mixtures

Kumagai, Yuta

Hoshasen Kagaku (Internet), (99), p.53 - 56, 2015/04

Radiation-induced degradation of 2-chlorophenol (2-ClPh) in zeolite/water mixtures was studied in order to consider a possibility of adsorption on zeolites to improve efficiencies of irradiation treatments of water contaminated by organic compounds. The degradation of 2-ClPh by -ray irradiation was investigated as a model compound. The degradation was evaluated by chloride ion (Cl) production. A high concentration of Cl was observed after the irradiation of a mixture with a mordenite-type zeolite (NaMOR), whereas A-type and X-type zeolites showed no significant effect. Therefore, for the mixture with NaMOR, effects of pH of the solution and of the 2-ClPh concentration were examined. At pH 5.7, the excess production of Cl was induced by the addition of NaMOR. Concurrently, adsorption of 2-ClPh on NaMOR was observed. When the mixture contained a higher concentration of 2-ClPh at pH 5.7, the Cl production increased. The adsorption of 2-ClPh also increased with increasing concentration. The results suggest that organics adsorbed on zeolites are decomposed by irradiation effectively at high adsorption concentrations.