Challenge for screening of nuclear fuel debris by innovative spectral imaging and its verification by LIBS mapping (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Osaka*

JAEA-Review 2025-040, 111 Pages, 2025/12

JAEA-Review-2025-040.pdf:22.28MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "Challenge for screening of nuclear fuel debris by innovative spectral imaging and its verification by LIBS mapping" conducted in FY2023. The present study aims to develop a remote-sensing technique to identify the in-reactor materials by a combination of Hyper Spectral Imaging (HSI) and Laser Induced Breakdown Spectroscopy (LIBS). HSI analyzes spectral information of more than 100 colors, and is being applied to classify various materials. On the other hand, material composition cannot be directly evaluated by HSI. Therefore, we thought that the combination of HSI and LIBS could be an accurate and wide-ranging visualization technique. In order to demonstrate the HSI and LIBS, it is necessary to prepare standard materials that simulate in-reactor materials, and to acquire and accumulate training data on them. In this study, the University of Osaka is in charge of the preparation of standard materials and HSI data analysis, Nuclear Fuel Development (NFD) is in charge of the preparation of uranium bearing materials and HSI/LIBS measurements, and JAEA is in charge of LIBS development. On the UK side, the Univ. of Strathclyde, National Nuclear Laboratory (NNL), and Lancaster University participate in the joint research project. The compositions of the standard samples were determined from past experiments and thermodynamic calculation results. Several samples such as UO based composites and concrete were prepared. The HSI data were obtained using a hyperspectral camera installed in the NFD. For LIBS, we worked on the automatic optimization of focal distance as part of the development of remote operation technology.

Investigation of effects of nano interfacial phenomena on dissolution aggregation of alpha nanoparticles by using micro nano technologies (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Institute of Science Tokyo*

JAEA-Review 2025-026, 72 Pages, 2025/11

JAEA-Review-2025-026.pdf:7.97MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Investigation of effects of nano interfacial phenomena on dissolution aggregation of alpha nanoparticles by using micro nano technologies" conducted in FY2023. To ensure the safety of retrieval and storage management of nuclear fuel debris generated by the Fukushima-Daiichi Nuclear Power Station accident, understanding of dissolution-denaturation behavior of the fuel debris alpha particles is one of the most crucial issues. This research aims to create novel microfluidic real-time measurement device for elucidating dissolution, aggregation, and denaturation processes of metal oxide nanoparticles under various solution environments, and clarify their nano-size and interfacial effects. In this year, we conducted bulk and micro dissolution tests of simulated fuel debris particles (UO mechanical-treated nanoparticles, UO chemical-treated nanoparticles, and (U,Zr)O nanoparticles), and successfully clarified that the effects of particle sizes, reaction times, and HO concentrations on the dissolution behavior of each nanoparticle. In particular, it was found that (U,Zr)O nanoparticles have different degrees of Zr catalytic reactions depending on HO concentrations, resulting in the generation of different amounts of gas and U. Moreover, we developed a new microfluidic device which enables to instantly react the nanoparticles with HO solutions, and determined dynamic aggregation and dissolution rates of the nanoparticles. The research was carried out in close collaboration with UK researchers, and achieved the expected goal of this year.

An Analytical study on Russia's civilian nuclear energy utilization

Kawasaki, Nobuchika

JAEA-Review 2025-043, 74 Pages, 2025/10

JAEA-Review-2025-043.pdf:2.45MB

Russia is one of the most advanced countries in the civilian use of nuclear energy. However, understanding the internal mechanisms of its nuclear program remains difficult due to various reasons. Therefore, this study presents a historical overview of Russia's nuclear energy utilization, fuel supply, fuel manufacturing capabilities, and concepts regarding reprocessing and the nuclear fuel cycle. From this overview, insights have been extracted and analyzed. These insights are then organized under two strategic perspectives: "Strategic diversity and continuity in developments and demonstrations" and "Diversity in utilizations and deployments," with considerations of implications for Japan, as below. Russia's nuclear energy policy strategically utilizes a variety of reactor types and fuel cycle technologies to expand nuclear power generation both domestically and internationally. Currently, nuclear power, centered on light-water reactors (VVER series), accounts for about 20% of Russia's electricity supply, and there are plans to increase this share to 25% by 2045. A wide range of reactors, from large-scale to medium and small modular reactors, are being constructed in Russia. Russia is also actively developing fast reactor technologies, and focusing on the reprocessing and recycling of spent fuel. Internationally, VVER-1200 reactors are under construction in several countries, and cooperation with China is deepening in the field of fast reactors. Notably, Russia offers an integrated, or selectively customizable, package of nuclear technology services on the international stage. These include not only reactor deployment, but also fuel supply, reprocessing, waste management, and even the provision of radioisotopes. Rather than simply exporting products or technology, Russia fosters long-term relationships and trust by flexibly responding to the conditions and needs of partner countries. For this reason, Russia promotes the technology developments in advance within the country in areas anticipated for future overseas deployment. It carefully selects target technologies and services and systematically rolls them out. This flexible strategy, combining "technological diversity" and "strategic consistency", enables cooperation with countries across various geopolitical contexts. For Japan, this strategic approach offers valuable lessons on how to engage in comprehensive international nuclear cooperation, not merely through technology exports, but through integrated approaches that encompass the entire fuel cycle, and by combining elements such as fast reactors and RI supply.

Influence of steam flow rate on oxidation kinetics of silicon carbide at 1400-1600 C

Pham, V. H.; Kurata, Masaki; Nagae, Yuji; Ishibashi, Ryo*; Sasaki, Masana*

Corrosion Science, 255, p.113098_1 - 113098_9, 2025/10

https://doi.org/10.1016/j.corsci.2025.113098

High-temperature oxidation failure in reactivity-initiated accidents; An Evaluation of failure criteria based on oxygen concentration from the previous NSRR experiments

Luu, V. N.; Taniguchi, Yoshinori; Udagawa, Yutaka; Katsuyama, Jinya

Nuclear Engineering and Design, 442, p.114222_1 - 114222_15, 2025/10

https://doi.org/10.1016/j.nucengdes.2025.114222

Study on water stopping, repair and stabilization of lower PCV by geopolymer, etc. (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2025-008, 134 Pages, 2025/09

JAEA-Review-2025-008.pdf:10.0MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Study on water stopping, repair and stabilization of lower PCV by geopolymer, etc." conducted from FY2021 to FY2023. Since the final year of this proposal was FY2023, the results for 3 fiscal years were summarized. In order to retrieve fuel debris, it is necessary to shut off the water at the bottom of the dry well and repair it in order to control the PCV water level. Therefore, in this study, we evaluated a construction method of stopping the water of the jet deflector with an improved geopolymer and repairing the lower part of the dry well by experiments and simulations. In addition, after understanding the properties of the fuel debris coated with the geopolymer, the long-term life of the waste body was evaluated. As a result, it was predicted that by utilizing geopolymers, it is possible to stop water and repair the lower part of the PCV in consideration of steps from construction to waste management.

Initial benchmark comparison of the open-source Cyclus and NMB fuel cycle simulators

Bachmann, A. M.*; Nishihara, Kenji; Richards, S.*; Abe, Takumi; Feng, B.*

Progress in Nuclear Science and Technology (Internet), 8, p.11 - 16, 2025/09

https://doi.org/10.15669/pnst.8.11

Preliminary criticality analysis of a partially damaged reactor core under different scenarios

Nguyen, H. H.

Annals of Nuclear Energy, 218, p.111361_1 - 111361_9, 2025/08

https://doi.org/10.1016/j.anucene.2025.111361

This study examined the criticality characteristics of a partially damaged reactor model, in which fuels located at the core center melt into fuel debris of varying shapes, while fuels situated at the core edges remain intact. The investigation was conducted using the Serpent code with the JENDL-5 nuclear data library. The results of the calculations indicate that when the volume of fuel debris is small and maintained at a constant level, the shape of the fuel debris does not result in significant alterations in the variation law of k of the system. In contrast, for the scenario in which the volume of the fuel debris is variable, the k variation law can be divided into two groups for the reference case with a system temperature of 300 K and no boron in the water. The first group comprises fuel debris with shapes that are cuboid and cylindrical, while the second group comprises fuel debris with shapes that are spherical, cone-shaped, and truncated cone-shaped.

Characteristics of droplet evaporation on high-temperature porous surfaces for estimating cooling time of fuel debris

Yuki, Kohei*; Horiguchi, Naoki; Yoshida, Hiroyuki; Yuki, Kazuhisa*

Mechanical Engineering Journal (Internet), 12(4), p.24-00451_1 - 24-00451_8, 2025/08

https://doi.org/10.1299/mej.24-00451

Fuel debris at the Fukushima Daiichi nuclear power station is typically cooled under immersion. However, an unexpected significant drop in water level results in coolant contact with high-temperature fuel debris having porous structure. In such scenarios, rapid cooling is essential, yet the thermal behavior at the liquid-solid interface, including capillary phenomena, is not well understood. This paper presents basic research evaluating the evaporation characteristics of droplets upon contact with metallic porous media featuring small pores under 1 mm. We conducted experiments using bronze or stainless steel porous media with pore diameters of 1, 40, or 100 m to derive lifetime curves for droplets. Our findings indicate that Leidenfrost effect is mitigated on porous surfaces as the vapor can escape through the pores. Moreover, in bronze porous media, as the temperature increases, oxide film with a fine structure facilitates capillary action. In contrast, the low wettability of stainless steel porous media prevents capillary action, inhibiting droplet absorption and dispersion into the pores. Consequently, rapid cooling via the capillary action is unlikely if the fuel debris shares similar characteristics with steel porous media. Therefore, for risk management, the cooling system should be established assuming that capillary force does not act in the fuel debris.

Control and irradiation behaviors of oxygen potential of MOX fuel

Hirooka, Shun; Vauchy, R.; Horii, Yuta; Sunaoshi, Takeo*; Saito, Kosuke; Ozawa, Takayuki

Proceedings of Workshop on Fuel Performance Assessment and Behaviour for Liquid Metal Cooled Fast Reactors (Internet), 8 Pages, 2025/07

no abstracts in English