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CPham, V. H.; Kurata, Masaki; Nagae, Yuji; Ishibashi, Ryo*; Sasaki, Masana*
Corrosion Science, 255, p.113098_1 - 113098_9, 2025/10
Luu, V. N.; Taniguchi, Yoshinori; Udagawa, Yutaka; Katsuyama, Jinya
Nuclear Engineering and Design, 442, p.114222_1 - 114222_15, 2025/10
Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2024-064, 118 Pages, 2025/06
JAEA-Review-2024-064.pdf:6.73MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Development of extremely small amount analysis technology for fuel debris analysis" conducted from FY2019 to FY2023. Understanding the properties of fuel debris is necessary for handling, criticality control, storage control, etc. A key technique is the chemical analysis of actinide nuclides. We developed sample pretreatment technology and separation / analysis process required for chemical analysis. The purpose of this study is to streamline future planned fuel debris analysis. To promote 1F decommissioning, we will train human resources through on-the-job training. In particular, we applied the extremely small amount analysis (ICP-MS/MS), which has recently been successful in the fields of analytical chemistry and radiochemistry, to the nuclear field. This method allows high-accuracy analysis without pretreatment to isolate the nuclide to be measured. The separation pretreatment can be skipped and a rapid analysis process can be established.
Birkholzer, J. T.*; Graupner, B. J.*; Harrington, J.*; Jayne, R.*; Kolditz, O.*; Kuhlman, K. L.*; LaForce, T.*; Leone, R. C.*; Mariner, P. E.*; McDermott, C.*; et al.
Geomechanics for Energy and the Environment, 42, p.100685_1 - 100685_17, 2025/06
Nagatani, Taketeru; Kosuge, Yoshihiro*; Sagara, Hiroshi*; Nakaguki, Sho; Nomi, Takayoshi; Okumura, Keisuke
Progress in Nuclear Science and Technology (Internet), 7, p.41 - 46, 2025/05
Abe, Takumi; Oizumi, Akito; Nishihara, Kenji; Nakase, Masahiko*; Asano, Hidekazu*; Takeshita, Kenji*
Progress in Nuclear Science and Technology (Internet), 7, p.299 - 304, 2025/05
Currently, much research continues on stable energy sources that do not emit CO
in order to achieve a carbon-neutral and sustainable society. Nuclear energy is one of the such sources, and various new reactors and reprocessing technologies are being developed. In order to implement the nuclear fuel cycle with these technologies, a nuclear fuel cycle simulator is required to quantitatively evaluate various quantities, such as the distribution of nuclear fuel materials and the scale of waste loading. For this purpose, NMB4.0 was developed in collaboration with Tokyo Institute of Technology and Japan Atomic Energy Agency. This code calculates the material balance of 179 nuclides including actinides and fission products (FPs) from the front-end to the back-end and simulates the nuclear fuel cycle in an integrated manner. Unlike other nuclear fuel cycle simulators, the code is capable of performing precise back-end analyses such as the number of radioactive wastes and the scale of the geological repository considering heat generation of waste package under diverse nuclear energy scenario, and is an open source code that runs on Microsoft Excel. By these features, it is possible to quantitatively study nuclear energy utilization strategies with various stakeholders. The presentation will detail the numerical model used in NMB4.0.
Np, 
Am, and 
Am reaction rates in highly enriched uranium fuel cores at Kyoto University Critical AssemblyPyeon, C. H.*; Oizumi, Akito; Katano, Ryota; Fukushima, Masahiro
Nuclear Science and Engineering, 199(3), p.429 - 444, 2025/03
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Experimental analyses of neptunium-237 (Np), americium-241 (Am), and Am fission and Np capture reaction rates are conducted by the Serpent 2 code together with ENDF/B-VIII.0 and JENDL-5, using experimental data at neutron spectra of thermal and intermediate regions obtained in the solid-moderated and solid-reflected cores with highly-enriched uranium fuel at the Kyoto University Critical Assembly. Also, uncertainty quantification of fission and capture reaction rate ratios of test samples of Np, Am and Am with reference samples of uranium-235 (
U) and gold-197 (
Au) are evaluated by the MARBLE code system. In terms of fission reaction rate ratios of Np/U, Am/U and Am/U, a comparison between experiments and Serpent 2 calculations shows an accuracy about 5, 15 and 10%, respectively, together with ENDF/B-VIII.0 and JENDL-5. For capture reaction rate ratios of Np/Au, Serpent 2 calculations reveal a fairly good accuracy at the thermal neutron spectrum. The total uncertainties of Np/U, Am/U and Am/U fission reaction rate ratios by MARBLE with the covariance data of ENDF/B-VIII.0 and JENDL-5 are found to be about 4% at most in all cores, except for about 8% of Am/U with ENDF/B-VIII.0 at the intermediate neutron spectrum.
Aihara, Jun; Ueta, Shohei; Honda, Masaki*; Kasahara, Seiji; Okamoto, Koji*
JAEA-Research 2024-012, 98 Pages, 2025/02
JAEA-Research-2024-012.pdf:32.24MB
Concept of Pu-burner high temperature gas-cooled reactor (HTGR) was proposed for the purpose of more safely reducing amount of recovered Pu. In Pu-burner HTGR concept, coated fuel particle (CFP), with ZrC coated yttria stabilized zirconia (YSZ) containing PuO (PuO-YSZ) small particle and with tri-structural isotropic (TRISO) coating, is employed for very high burn-up and high nuclear proliferation resistance. ZrC layer is oxygen getter. In research project of Pu-burner HTGR carried out from fiscal year of 2014 to fiscal year of 2017, simulated CFPs were fabricated using Ce to simulate Pu. Moreover, simulated fuel compacts were fabricated using fabricated simulated CFPs. In this report, results of microstructural observation of CeO-YSZ and ZrC layer at each fabrication step are reported.
Matsumura, Taichi; Okumura, Keisuke; Sakamoto, Masahiro; Terashima, Kenichi; Riyana, E. S.; Kondo, Kazuhiro*
Nuclear Engineering and Design, 432, p.113791_1 - 113791_9, 2025/02
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Calabrese, R.*; Hirooka, Shun
Progress in Nuclear Energy, 178, p.105516_1 - 105516_11, 2025/01
Thermal creep is one of the key properties of mixed oxide (MOX) fuel for innovative fast reactors. Thermal creep of fuel affects markedly the interaction between the fuel and the cladding. A review of correlations available in the literature is presented. The effect of porosity, plutonium concentration, and stoichiometry are discussed also in the light of recent numerical results. Our analysis pointed out some inconsistencies concerning the modelling of the effect of porosity on diffusional creep and a re-evaluation of the effect of plutonium concentration. The discussion suggested that Evans's findings on the effect of stoichiometry should be better assessed as well as the level of increase in creep moving towards stoichiometry. Typical operating conditions of fast breeder reactors confirmed the need for an extension of porosity and temperature correlations' domains. Besides this, a new correlation based on a separate-effect approach has been proposed for fuel performance codes.
Sakamoto, Masahiro; Okumura, Keisuke; Kanno, Ikuo; Matsumura, Taichi; Terashima, Kenichi; Riyana, E. S.; Kaneko, Junichi*; Mizokami, Masato*; Mizokami, Shinya*
Journal of Nuclear Science and Technology, 10 Pages, 2025/00
Times Cited Count：0 Percentile：0.00(Nuclear Science & Technology)Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*
JAEA-Review 2024-021, 126 Pages, 2024/11
JAEA-Review-2024-021.pdf:6.51MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Study on water stopping, repair and stabilization of lower PCV by geopolymer, etc" conducted in FY2022. The present study aims to propose a construction method to stop jet deflectors by improved geopolymer and ultra-heavy muddy water, and to repair the lower part of the dry well. In addition, in order to increase the options for on-site construction in unknown situations such as deposition conditions, we will examine a wide range of construction outside the pedestal, and evaluate the feasibility of the construction method by the latest thermal flow simulation method.
Batsaikhan, M.; Oba, Hironori; Karino, Takahiro; Akaoka, Katsuaki; Wakaida, Ikuo
Optics Express (Internet), 32(24), p.42626 - 42638, 2024/11
Times Cited Count：0 Percentile：0.00(Optics)Yuki, Kohei*; Horiguchi, Naoki; Yoshida, Hiroyuki; Yuki, Kazuhisa*
Proceedings of 31st International Conference on Nuclear Engineering (ICONE31) (Internet), 4 Pages, 2024/11
Fuel debris in the Fukushima Nuclear Power Station is cooled under immersion condition. However, in the event of an unexpected decrease in water level, coolant contacts high-temperature fuel debris having porous structure. In this event, although fuel debris needs to be cooled rapidly, thermal behavior at liquid-solid contact, such as capillary phenomenon, remains unclear. In this paper, as basic research, we evaluate droplet evaporation characteristics after contact with metal porous media with small pores less than 1 mm. In experiment, to obtain life time curve of a droplet, bronze or stainless steel porous media having 1, 40, or 100 
m pore diameter are utilized. Experimental results show that Leidenfrost phenomenon is suppressed on the porous surfaces because generated vapor can be discharged from the pores. Further, for bronze porous media, capillary phenomenon is observed as the temperature of the porous media increase because of generation of oxide film having fine structure. On the other hand, due to low wettability of stainless steel porous media, capillary phenomenon does not occur, and the droplet was not sucked and spread into pore. This indicates that rapid cooling by the capillary phenomenon can not be expected if fuel debris has the same characteristics as the stainless steel porous media.
Miyazawa, Takeshi; Uwaba, Tomoyuki; Yano, Yasuhide; Tanno, Takashi; Otsuka, Satoshi; Onizawa, Takashi; Ando, Masanori; Kaito, Takeji
JAEA-Technology 2024-009, 140 Pages, 2024/10
JAEA-Technology-2024-009.pdf:8.03MB
For the purpose of enhancing the reliability of fast reactor fuel designing using modified type 316 steel, the out-of-pile and in-pile mechanical data of modified type 316 steel cladding tubes and wrapper tubes were statistically analyzed with the knowledge on material science and engineering; the high-temperature strength equations of modified type 316 steel, which can be applied to high-dose neutron irradiation environment, were derived. The out-of-pile high-temperature tensile and creep data of modified type 316 steel cladding tubes and wrapper tubes were derived up to 900C, which is higher than the upper limit temperature of anticipated transient event of fast reactor. Using the extended database, the best-fit equation and the lower limit equation were derived for out-of-pile 0.2% proof strength, ultimate tensile strength and creep rupture strength while the best-fit equation and the upper and lower limit equations for creep strain. Furthermore, the degradation factors for tensile and creep strength, which will be produced by in-reactor environment (i.e., neutron irradiation in liquid sodium), were evaluated using the existing neutron irradiation data of modified type 316 steel, which were derived using the experimental fast reactor Joyo, the French proto-type fast reactor Phenix, the American experimental fast reactor FFTF. The derived equations were validated by the comparison with the experimental data.
Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*
JAEA-Review 2024-026, 80 Pages, 2024/10
JAEA-Review-2024-026.pdf:1.96MB
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Study on degradation of fuel debris by combined effects of radiological, chemical, and biological functions" conducted from FY2019 to FY2022. In the project, radiochemists, nuclear chemists, nuclear physicists, material scientists, and environmental biologists are teamed to elucidate the mechanism of the degradation of fuel debris by combined effects of radiological, chemical, and biological functions.
Rochman, D.*; Minato, Futoshi; Watanabe, Tomoaki; 52 of others*
EPJ Nuclear Sciences & Technologies (Internet), 10, p.9_1 - 9_83, 2024/10
Vauchy, R.; Hirooka, Shun; Horii, Yuta; Ogasawara, Masahiro*; Sunaoshi, Takeo*; Yamada, Tadahisa*; Tamura, Tetsuya*; Murakami, Tatsutoshi
Journal of Nuclear Materials, 599, p.155233_1 - 155233_11, 2024/10
Times Cited Count：0 Percentile：0.00(Materials Science, Multidisciplinary)The fluorite exsolution/recombination in U
Pu
O
(y = 0.30 and 0.45) and PuO was investigated using differential scanning calorimetry. The results are in relatively good agreement with the literature data, except for plutonia. Our values indicate that the critical temperature of the miscibility gap in Pu-O is 30
50 K lower than previously reported. Finally, the systematic experimental procedure allowed us refining the locus of the solvus existing in hypostoichiometric U
0Pu
O, U
Pu
O, and PuO dioxides.
Bachmann, A. M.*; Richards, S.*; Feng, B.*; Nishihara, Kenji; Abe, Takumi
Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10
This work demonstrates the value of code verification as an initial step in utilizing fuel cycle simulation. Cyclus and NMB are open-source fuel cycle simulators that provide computational modeling of nuclear fuel cycle alternatives and were chosen by Argonne National Laboratory and Japan Atomic Energy Agency (JAEA), respectively, for a multi-year collaboration on fuel cycle benchmarks. Both are relatively new and can be improved after conducting a rigorous code-to-code comparison. Initial verification of these simulators was performed using a set of hypothetical scenarios for once-through and multi-recycle fuel cycles. The results of this work identify how differences in scenario definitions and the modeling methodologies of the two simulators lead to differences in results in material inventories, mass flows, and other important metrics for fuel cycle assessments.
Nakashima, Shinsuke*; Moro, A.*; Komatsu, Ren*; Faragasso, A.*; Matsuhira, Nobuto*; Woo, H.*; Kawabata, Kuniaki; Yamashita, Atsushi*; Asama, Hajime*
Proceedings of International Topical Workshop on Fukushima Decommissioning Research 2024 (FDR2024) (Internet), 4 Pages, 2024/10
