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Journal Articles

Analysis of dissolved radionuclides trapped into corrosion products formed on carbon steel and the corresponding increase in radioactivity

Aoyama, Takahito; Ueno, Fumiyoshi; Sato, Tomonori; Kato, Chiaki; Sano, Naruto; Yamashita, Naoki; Otani, Kyohei; Igarashi, Takahiro

Annals of Nuclear Energy, 214, p.111229_1 - 111229_6, 2025/05

Journal Articles

Evaluation of the distribution accuracy of radioactivity from a gamma-ray source using an omnidirectional detector for radiation imaging with fractal geometry

Sasaki, Miyuki; Abe, Yuki*; Sanada, Yukihisa; Torii, Tatsuo*

Nuclear Instruments and Methods in Physics Research A, 1072, p.170207_1 - 170207_12, 2025/03

We have developed an omnidirectional radiation imager with fractal geometry named the FRIE system. This paper presents the development and evaluation of the FRIE system, designed to accurately estimate radioactivity distribution within decommissioning environments, such as the Fukushima Daiichi Nuclear Power Station. The FRIE system is a unit of tetrahedral radiation sensors; 16 sensors are arranged in a Sierpinski tetrahedron shape, and the space between the sensors is filled with tungsten-based alloy for radiation shielding. This study assessed the performance of the FRIE system in estimating radiation distribution through simulations and actual measurement tests. From the results of the simulations and experimental data, it was confirmed that by maintaining a measurement density of at least 2 points/m$$^{2}$$, limiting the positional error to within $$pm$$10 cm, and the angular error to within $$pm$$10 degrees, it is possible to estimate the source location with an angular resolution of approximately 30 degrees. Future improvements in the arrangement of the FRIE system's crystals and shielding should enhance the performance metrics. This research signifies a pioneering implementation of fractal-based radiation imaging technology, offering a new direction in radiation measurement.

Journal Articles

Unusual low-temperature ductility increase mediated by dislocations alone

Naeem, M.*; Ma, Y.*; Tian, J.*; Kong, H.*; Romero-Resendiz, L.*; Fan, Z.*; Jiang, F.*; Gong, W.; Harjo, S.; Wu, Z.*; et al.

Materials Science & Engineering A, 924, p.147819_1 - 147819_10, 2025/02

 Times Cited Count:0

Journal Articles

Characterization of neutrons emitted by an expected small amount of fuel debris in a trial retrieval from Fukushima Daiichi Nuclear Power Station

Matsumura, Taichi; Okumura, Keisuke; Sakamoto, Masahiro; Terashima, Kenichi; Riyana, E. S.; Kondo, Kazuhiro*

Nuclear Engineering and Design, 432, p.113791_1 - 113791_9, 2025/02

 Times Cited Count:0

JAEA Reports

Annual Report of Nuclear Human Resource Development Center (April 1, 2023 - March 31, 2024)

Nuclear Human Resource Development Center

JAEA-Review 2024-048, 69 Pages, 2025/01

JAEA-Review-2024-048.pdf:3.5MB

This annual report summarizes the activities of Nuclear Human Resource Development Center(NuHRDeC) of Japan Atomic Energy Agency (JAEA) in the fiscal year (FY) 2023. In FY 2023, in addition to the regular training programs at NuHRDeC, we actively organized special training courses responding to the external training needs, cooperated with universities, offered international training courses for Asian countries, and promoted activities of the Japan Nuclear Human Resource Development Network (JN-HRD.net) and the human resource development concierge. Regular domestic training programs; training courses for radioisotopes and radiation engineers, nuclear energy engineers and national qualification examinations, were conducted as scheduled inthe annual plan. We also delivered training for other organizations outside the JAEA. We continued cooperative activities with universities, such as acceptance of postdoctoral researchers, and activities in line with the cooperative graduate school system, including the acceptance of students from Nuclear Professional School, the University of Tokyo. Furthermore, joint course among seven universities was successfully held by utilizing remote education system. The joint course and the intensive summer course and nuclear fuel cycle training were conducted as part of the collaboration network with universities. The Instructor Training Program (ITP) under the contract with Ministry of Education, Culture, Sports, Science and Technology, was continually offered to the ITP participating countries. As part of the ITP, the Instructor Training courses such as "Reactor Engineering Course", advanced instructor training course, and the nuclear technology seminar "Basic Radiation Knowledge for School Education" were conducted at NuHRDeC. As joint secretariat of JN-HRD.net, we steadily facilitated the network and actively held seminar, training, and facility tours for students.

JAEA Reports

Annual report for FY2022 on the activities of Naraha Center for Remote Control Technology Development (April 1, 2022 - March 31, 2023)

Naraha Center for Remote Control Technology Development

JAEA-Review 2024-046, 52 Pages, 2025/01

JAEA-Review-2024-046.pdf:3.6MB

Naraha Center for Remote Control Technology Development (NARREC) was established in Japan Atomic Energy Agency to promote a decommissioning work of Fukushima Daiichi Nuclear Power Station (Fukushima Daiichi NPS). NARREC consists of a Full-scale Mock-up Test Building and Research Management Building. Various test facilities are installed in these buildings for the decommissioning work of Fukushima Daiichi NPS. These test facilities are intended to be used for various users, such as companies engaged in the decommissioning work, research and development institutions, educational institutions and so on. The number of NARREC facility uses was 113 in FY2022. We participated booth exhibitions and presentations on the decommissioning related events. Moreover, we also contributed to the development of human resources by supporting the 7th Creative Robot Contest for Decommissioning. As a new project, "Narahakko Children's Classroom" was implemented for elementary school students in Naraha Town. This report summarizes the activities of NARREC in FY2022, such as the utilization of facilities and equipment of NARREC, arrangement of the remote-control machines for emergency response, and training for operators by using the machines.

Journal Articles

Simulation of excavation and long-term permeability test at 350 m gallery in Horonobe Underground Research Laboratory based on large-scale three-dimensional coupled analysis

Suetake, Koya*; Ogata, Sho*; Yasuhara, Hideaki*; Aoyagi, Kazuhei; Inui, Toru*; Kishida, Kiyoshi*

Dai-16-Kai Iwa No Rikigaku Kokunai Shimpojiumu Koen Rombunshu (Internet), p.304 - 309, 2025/01

It is very important to predict the extent of EDZ (excavation disturbed zone) and the behavior of hydraulic conductivity after excavation of shafts and tunnels for geological disposal of radioactive waste. In this study, we attempted to reproduce the in-situ tunnel excavation test and the subsequent permeability test at the Horonobe Underground Research Laboratory (URL) using a three-dimensional tunnel excavation simulator. As a result, similar results to the in-situ tests were obtained for the extent of EDZ propagation by excavation and the results of permeability tests. The simulator is effective in predicting the mechanical effects of excavation, coupled phenomena such as deformation and seepage, and hydraulic conductivity in deep mudstones in Japan.

Journal Articles

Chemical interaction of CsOH vapor with UO$$_{2}$$ and Fe-Zr melt

Nakajima, Kunihisa; Takano, Masahide

Journal of Nuclear Science and Technology, 62(1), p.78 - 85, 2025/01

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

At TEPCO's Fukushima Daiichi Nuclear Power Station, it is estimated that considerable amounts of cesium still remain in the reactors from the analysis results using the severe accident analysis codes and the reverse analysis from contaminated water. Since cesium is known to form stable compounds with uranium and zirconium, chemisorption experiments with uranium dioxide pellets and iron-zirconium melts for cesium hydroxide vapor were carried out. As the results, formations of cesium uranate, Cs$$_{2}$$UO$$_{4}$$, and cesium zirconate, Cs$$_{2}$$ZrO$$_{3}$$, were confirmed, indicating that cesium was chemisorbed on both of the uranium dioxide pellets and the iron-zirconium melts in an Ar-H$$_{2}$$-H$$_{2}$$O flow and an Ar-H$$_{2}$$ flow, respectively. Therefore, it was considered that cesium released from fuel might be trapped by chemisorption with fuels and/or iron-zirconium melts during light water reactor severe accidents.

Journal Articles

Development of a dissolution method for analyzing the elemental composition of fuel debris using sodium peroxide fusion technique

Nakamura, Satoshi; Ishii, Sho*; Kato, Hitoshi*; Ban, Yasutoshi; Hiruta, Kenta; Yoshida, Takuya; Uehara, Hiroyuki; Obata, Hiroki; Kimura, Yasuhiko; Takano, Masahide

Journal of Nuclear Science and Technology, 62(1), p.56 - 64, 2025/01

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

A dissolution method for analyzing the elemental composition of fuel debris using the sodium peroxide (Na$$_{2}$$O$$_{2}$$) fusion technique has been developed. Herein, two different types of simulated debris materials (such as solid solution of (Zr,RE)O$$_{2}$$ and molten core-concrete interaction products (MCCI)) were taken. At various temperatures, these debris materials were subsequently fused with Na$$_{2}$$O$$_{2}$$ in crucibles, which are made of different materials, such as Ni, Al$$_{2}$$O$$_{3}$$, Fe, and Zr. Then, the fused samples are dissolved in nitric acid. Furthermore, the effects of the experimental conditions on the elemental composition analysis were evaluated using inductively coupled plasma-atomic emission spectroscopy (ICP-AES), which suggested the use of a Ni crucible at 923 K as an optimum testing condition. The optimum testing condition was then applied to the demonstration tests with Three Mile Island unit-2 (TMI-2) debris in a shielded concrete cell, thereby achieving complete dissolution of the debris. The elemental composition of TMI-2 debris revealed by the proposed dissolution method has good reproducibility and has an insignificant contradiction in the mass balance of the sample. Therefore, this newly developed reproducible dissolution method can be effectively utilized in practical applications by dissolving fuel debris and estimating its elemental composition.

Journal Articles

In-situ detection of high-energy beta ray emitter $$^{90}$$Sr/$$^{90}$$Y inside the Fukushima Daiichi Nuclear Power Station Unit 3 reactor building using a liquid light guide Cherenkov counter

Terasaka, Yuta; Sato, Yuki; Furuta, Yoshihiro*; Kubo, Shin*; Ichiba, Yuta*

Nuclear Instruments and Methods in Physics Research A, 1070(2), p.170021_1 - 170021_9, 2025/01

 Times Cited Count:0 Percentile:0.00(Instruments & Instrumentation)

Journal Articles

Environmental geochemistry of radionuclides (Environmental radiochemistry)

Takahashi, Yoshio*; Yamaguchi, Akiko; Yomogida, Takumi

Treatise on Geochemistry, 3rd edition, Vol.6, 46 Pages, 2025/00

With the recent development of measurement techniques, new approaches to the environmental geochemistry of radionuclides have been applied for various research targets. In this review article, several topics within the last 10-15 years in the field of environmental geochemistry of radionuclides have been discussed. In particular, this article mainly focused on two topics, (i) studies on the migration of radionuclides emitted by the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident in 2011 and (ii) the development of X-ray absorption fine structure (XAFS) spectroscopy and its application to the geochemical processes of radionuclides.

JAEA Reports

Proceedings of the 9th "Conference for R&D Initiative on Nuclear Decommissioning Technology by the Next Generation"

Usami, Hiroshi; Ito, Rintaro; Tagawa, Akihiro

JAEA-Review 2024-045, 49 Pages, 2024/12

JAEA-Review-2024-045.pdf:13.38MB

The decommissioning of the TEPCO's Fukushima Daiichi Nuclear Power Station is a long-term project, and the training of young engineers and researchers who will be responsible for future decommissioning is a necessary and urgent task. Since 2016, Collaborative Laboratories for Advanced Decommissioning Science has been continuously organizing "Conferences for R&D Initiative on Nuclear Decommissioning Technology by the Next Generation (NDEC)" for students who are engaged in research activities for decommissioning. NDEC is a forum for students to present their research for the purpose of human resource development and networking among young researchers, and to increase their motivation for decommissioning research. NDEC-9 was held at "Manabi-no-Mori" in Tomioka-machi, Fukushima Prefecture, from March 21-22, 2024. This proceeding compiles the contents of report papers in the conference.

JAEA Reports

Development of a high-resolution imaging camera for alpha dust and high-dose rate monitor (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*

JAEA-Review 2024-016, 61 Pages, 2024/12

JAEA-Review-2024-016.pdf:2.88MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Development of a high-resolution imaging camera for alpha dust and high-dose rate monitor" conducted in FY2022. The present study aims to develop a high-resolution imaging camera for alpha dust and a high-dose rate monitor. To realize the high-resolution imaging camera for alpha dust, we have developed novel scintillation materials with emission bands of 500-800 nm. Moreover, we have prepared several materials for the camera and software. We have also developed novel scintillation materials with emission bands of 650-1,000 nm, and simulation studies have been conducted for the high-dose-rate monitor system consisting of optical fiber.

JAEA Reports

Data report of ROSA/LSTF experiment SB-PV-03; 0.2% pressure vessel bottom break LOCA with SG depressurization and gas inflow

Takeda, Takeshi

JAEA-Data/Code 2024-014, 76 Pages, 2024/12

JAEA-Data-Code-2024-014.pdf:4.0MB

An experiment denoted as SB-PV-03 was conducted on November 19, 2002 using the Large Scale Test Facility (LSTF) in the Rig of Safety Assessment-V (ROSA-V) Program. The ROSA/LSTF experiment SB-PV-03 simulated a 0.2% pressure vessel bottom small-break loss-of-coolant accident in a pressurized water reactor (PWR). The test assumptions included total failure of high pressure injection system of emergency core cooling system (ECCS) and noncondensable gas (nitrogen gas) inflow to the primary system from accumulator (ACC) tanks of ECCS. Secondary-side depressurization of both steam generators (SGs) as an accident management (AM) action to achieve the depressurization rate of 55 K/h in the primary system was initiated 10 min after the generation of a safety injection signal, and continued afterwards. Auxiliary feedwater injection into the secondary-side of both SGs was started for 30 min with some delay after the onset of the AM action. The AM action was effective on the primary depressurization until the ACC tanks began to discharge nitrogen gas into the primary system. The core liquid level recovered in oscillative manner because of intermittent coolant injection from the ACC system into both cold legs. Therefore, the core liquid level remained at a small drop. The pressure difference between the primary and SG secondary sides became larger after nitrogen gas ingress. Core uncovery occurred by core boil-off during reflux condensation in the SG U-tubes under nitrogen gas influx. When the maximum cladding surface temperature of simulated fuel rods exceeded the pre-determined value of 908 K, the core power was automatically reduced to protect the LSTF core. After the automatic core power reduction, coolant injection from low pressure injection (LPI) system of ECCS into both cold legs led to the whole core quench. After the continuous core cooling was confirmed through the actuation of the LPI system, the experiment was terminated.

Journal Articles

Study on the specifications of the basic core configurations of the modified STACY

Gunji, Satoshi; Araki, Shohei; Izawa, Kazuhiko; Suyama, Kenya

Annals of Nuclear Energy, 209, p.110783_1 - 110783_7, 2024/12

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Since the compositions and properties of the fuel debris are uncertain, critical experiments are required to validate calculation codes and nuclear data used for the safety evaluation. For this purpose, the Japan Atomic Energy Agency (JAEA) has been modifying a critical assembly called "STACY." The first criticality of the modified STACY is scheduled for spring 2024. This paper reports the consideration results of the specifications of the basic core configurations of the modified STACY at the first criticality. We prepared two types of gird plates with different neutron moderation conditions (their intervals are 1.50 cm and 1.27 cm). However, there is a limitation on the number of available UO$$_{2}$$ fuel rods. The core configurations for the first criticality satisfying these experimental constraints were designed by computational analysis. A cylindrical core configuration with a 1.50 cm grid plate close to the optimum moderation condition needs 253 fuel rods to reach criticality. As to the 1.27 cm grid plate, we considered core configurations with 2.54 cm intervals by using doubled pitches of the grid plate. It will need 213 fuel rods for the criticality. In addition, we considered the experimental core configuration with steel/concrete simulant rods to simulate fuel debris conditions. This paper shows these core configurations and their evaluated specifications.

Journal Articles

New insight on the thermal impact on cementitious materials due to high-temperature with water supply; Continuous expansive spalling in water

Miura, Taito*; Miyamoto, Shintoro*; Maruyama, Ippei*; Aili, A.*; Sato, Takumi; Nagae, Yuji; Igarashi, Go*

Case Studies in Construction Materials, 21, p.e03571_1 - e03571_14, 2024/12

 Times Cited Count:0 Percentile:0.00(Construction & Building Technology)

Journal Articles

Assessment of individual external exposure doses based on environmental radiation in areas affected by the Fukushima Daiichi Nuclear Power Station accident

Sato, Rina; Yoshimura, Kazuya; Sanada, Yukihisa; Mikami, Satoshi; Yamada, Tsutomu*; Nakasone, Takamasa*; Kanaizuka, Seiichi*; Sato, Tetsuro*; Mori, Tsubasa*; Takagi, Marie*

Environmental Science & Technology, 194, p.109148_1 - 109148_8, 2024/12

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Assessment of individual external doses from ambient dose equivalents is used for predictive and retrospective assessments where personal dosimeters are not applicable. However, it tends to contain more errors than assessment by personal dosimetry due to various parameters. Therefore, in order to accurately assess the individual dose from ambient dose equivalents, a model that estimates effective doses considering life patterns and the shielding effects by buildings and vehicles, were developed in this study. The model parameters were examined using robust datasets of environmental radiation measured in the areas affected by the Fukushima Daiichi Nuclear Power Station accident in 2020 to 2021. The accuracy of the model was validated by comparison with 106 daily personal doses measured in Fukushima Prefecture in 2020. The measured personal dose was well reproduced by the model-estimated effective dose, showing that the model can be used to assess the individual exposure dose, similar to personal dosimetry. Furthermore, this model is an effective tool for radiation protection, as it can estimate the individual dose predictively and retrospectively by using environmental radiation data.

Journal Articles

Current status and future prospects of the Horonobe International Project (HIP), 4; Task C: Full-scale Engineering Barrier System (EBS) dismantling experiment

Ono, Hirokazu

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 31(2), p.140 - 143, 2024/12

In the geological disposal of high-level radioactive waste, after emplacement of an EBS, the near-field environment is affected by processes such as heat release from the waste, groundwater infiltration into the EBS, swelling and deformation of the buffer material, and chemical reactions between groundwater and minerals. It is crucial to develop simulation codes to evaluate such coupled thermal-hydraulic-stress-chemical (THMC) processes for safety assessment of geological disposal. The full-scale vertical-emplacement EBS experiment (Horonobe EBS experiment) has been undertaken in the 350 m gallery of the Horonobe Underground Research Laboratory (URL) with the Horonobe geological environment. In the Horonobe EBS experiment, various sensors were installed in the buffer and backfill material to obtain the data required to evaluate coupled THMC processes in near-field. In Task C of the Horonobe International Project (HIP), the dismantling experiment of the Horonobe EBS experiment will be carried out and the data obtained from this experiment will be used to understand the coupled processes and to evaluate the simulation code.

Journal Articles

Effective porosity in groundwater flow analysis for fractured sedimentary rocks; Case studies of the Koetoi and Wakkanai formations in Horonobe, Hokkaido, Japan

Miyakawa, Kazuya; Ishii, Eiichi; Imai, Hisashi*; Hirai, Satoru*; Ono, Hirokazu; Nakata, Kotaro*; Hasegawa, Takuma*

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 31(2), p.82 - 95, 2024/12

no abstracts in English

Journal Articles

Role of retained austenite and deformation-induced martensite in 0.15C-5Mn steel monitored by ${it in situ}$ neutron diffraction measurement during tensile deformation

Yamashita, Takayuki*; Morooka, Satoshi; Gong, W.; Kawasaki, Takuro; Harjo, S.; Hojo, Tomohiko*; Okitsu, Yoshitaka*; Fujii, Hidetoshi*

ISIJ International, 64(14), p.2051 - 2060, 2024/12

12938 (Records 1-20 displayed on this page)