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JAEA Reports

High-speed 3D modeling for nuclear reactor environment based on feature extraction results from video images (Contract research); FY2024 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Sapporo University*

JAEA-Review 2026-020, 81 Pages, 2026/09

JAEA-Review-2026-020.pdf:6.0MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), has been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") from FY2019. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "High-speed 3D modeling for nuclear reactor environment based on feature extraction results from video images" conducted in FY2024. The present study aims to develop a methodology for 3D modeling of workspaces using video footage captured during surveys of the reactor containment vessel and reactor building at 1F. Based on features extracted from the video within a specified timeframe, the method selects a high-information-content 3D reconstruction approach while augmenting the surrounding contextual information. In fiscal year 2024, we developed a methodology to achieve high-precision photogrammetry-based 3D reconstruction within a specified time limit, using a single video sequence obtained from simulation as input. We also devised a 3D modeling algorithm based on structural grouping and concurrently implemented an optimization algorithm to reduce computation time for 3D reconstruction, thereby accelerating the overall modeling process. Furthermore, we quantitatively evaluated the generation accuracy of moving image data using generative models and continued to enhance both hardware construction and software development to further improve computational efficiency.

Journal Articles

A Study for establishment of passive creep-fatigue test techniques using the difference of thermal expansion coefficients of materials

Wakai, Takashi; Ando, Masanori; Okajima, Satoshi; Toyota, Kodai; Ishigami, Katsuo*; Onuma, Terumitsu*; Takahashi, Ryoya*; Asayama, Tai

Nihon Kikai Gakkai Rombunshu (Internet), 92(961), p.26-00004_1 - 26-00004_12, 2026/09

This paper describes current efforts within the Japan Atomic Energy Agency to develop a new materials surveillance technology for sodium-cooled fast reactors that aims at raising the confidence levels in operating reactors' structural integrity to the ones which could otherwise be achieved only by a vast amount of long-term material test data that needs decades to accumulate. The technology would allow for monitoring on-going materials degradation processes in an actual reactor, namely fatigue and creep-fatigue, by inserting a newly developed specimen for this purpose into the reactor and establishing procedures to observe and evaluate the specimen to get desired information such as the extent of degradation and residual life. To establish the test procedure, a passive creep-fatigue test model was developed in the framework of the "Civil Nuclear Energy Research and Development Working Group (CNWG)", a collaboration agreement between the US and Japan, and a demonstration test was performed under cyclic thermal loads using an electric furnace. Temperature conditions had been determined based on finite element analyses. As a result, the test specimen failed by several hundred thermal cycles. Macroscopic inspection of the specimen after the test showed the test had been performed successfully without buckling. Fracture surface observations suggested that the failure caused probably by fatigue or creep-fatigue.

JAEA Reports

Radioactive Materials Analysis and Research Facility Laboratory-1 construction report

Shindo, Ryuji; Ichimura, Takahito; Nozawa, Yoshihiko; Komori, Tsuyoshi; Rachi, Reona; Kitahara, Katsumi*; Nakamura, Tomoki*; Koike, Akihiro*

JAEA-Technology 2026-005, 379 Pages, 2026/08

JAEA-Technology-2026-005.pdf:45.42MB

Laboratory-1 of the Radioactive Material Analysis and Research Facility (Laboratory-1) is a facility for analyzing and testing the properties of low and medium radiation dose debris, logging, incinerator ash, and secondary wastes from the decommissioning of the TEPCO HD Fukushima Daiichi Nuclear Power Station (1F) to obtain technical prospects for treatment and disposal measures and their safety. In addition, the ALPS treated water was analyzed by a third party independent of TEPCO HD prior to its discharge into the sea. Laboratory-1 was constructed by the Japan Atomic Energy Agency from January 2017 to June 2022 as part of the 1F Specific Nuclear Facility. The construction work of Laboratory-1 is classified into "building work" for construction of the building by architectural work, electrical equipment work, and mechanical equipment work, and "interior equipment work" for the maintenance of analysis facilities such as iron cells, glove boxes, hoods, etc. This report is a compilation of construction records related to the "building work" that Okuma Construction Office was in charge of. This report is a compilation of construction records and other information related to "building construction" handled by Okuma Construction Office. This report comprehensively summarizes the experience and knowledge from a technical perspective on construction management related to the construction of nuclear facilities, including quality control and construction status for each type of building work, composite coordination, implementation systems and methods for safety and construction quality management, and permits and approvals (such as changes to implementation plans, building permit applications, and forest land development permits). The report also includes a summary of the specific management details such as radiation control for construction in special environments such as construction on the 1F site and construction in a difficult-to-return zone. In the future, we hope that this report will be used as a reference for the development of nuclear facilities such as Laboratory-1, contributing to the identification of issues and rational facility planning.

JAEA Reports

Development of a radiation resistant laser scanner and 3D modeling method using AI and image processing (Contract research); FY2024 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Osaka*

JAEA-Review 2026-009, 81 Pages, 2026/07

JAEA-Review-2026-009.pdf:5.42MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), has been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") from FY2019. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2024, this report summarizes the research results of the "Development of a radiation resistant laser scanner and 3D modeling method using AI and image processing" conducted in FY2024. This research focuses on developing a radiation-resistant 3D laser scanner and technologies to enhance the quality of point cloud data. A new scanner system was designed with a laser scanning head composed only of radiation-tolerant electrical and mechanical components, excluding semiconductors, and a control unit placed remotely in a low-radiation zone. The system aims to enable stable scanning in high-radiation environments. Its performance will be evaluated in comparison with commercial scanners. To address the sparsity of acquired point clouds, we are developing two complementary systems: one uses machine learning to complete and enhance point clouds through processes such as denoising, normalization, and interpolation; the other uses photogrammetry to reconstruct 3D data from image sets and integrate it with scanner-derived data. In FY2024, (1) Optical and electronic circuits were designed and assembled, and waveform collection and analysis software was developed to prepare for scanner detection efficiency evaluation. (2) A point cloud completion system incorporating AI was implemented, and methods for point cloud densification and completion were investigated. (3) A processing environment and workflow were established to integrate point clouds with photogrammetry, and 3D surface models were constructed. (4) Efficient scanning strategies under high-radiation conditions were analyzed, and a methodology for accuracy evaluation was studied. (5) The project was advanced through close coordination among research components and related institutions.

Journal Articles

Observation of the structure and dynamics of water in aqueous alkaline chloride solutions under gigapascal pressure by neutron scattering

Jing, Z.*; Yamaguchi, Toshio*; Hattori, Takanori; Yamada, Takeshi*; Tamatsukuri, Hiromu; Matsuura, Masato*; Zhou, Y.*

Journal of Physical Chemistry Letters (Internet), 17(29), p.8419 - 8428, 2026/07

 Times Cited Count:0 Percentile:0.00(Chemistry, Physical)

We conducted high-pressure neutron diffraction and quasielastic neutron scattering on a series of aqueous alkaline chloride solutions and clarified that the pressure- and ion-induced modifications to the water structure and diffusion originate from distinct physical mechanisms. Applying gigapascal pressure transforms the tetrahedral hydrogen-bonded network structure of water into a dense random packing, due to the collapse of the second and third coordination shells and an increase in the number of interstitial water molecules, regardless of the ion species. On the contrary, dissolved ions disturb the second shell but preserve the inherent tetrahedral network structure of water at ambient pressure. The anomalous trend of water diffusion from Li$$^+$$ to Cs$$^+$$ under the ambient conditions disappears under the gigapascal pressure, and all the ions show a behavior of structure-making ions.

JAEA Reports

Reports on research activities and evaluation of advanced computational science in FY2024

Center for Computational Science & e-Systems

JAEA-Evaluation 2026-003, 41 Pages, 2026/06

JAEA-Evaluation-2026-003.pdf:1.08MB

Research on advanced computational science for nuclear applications, based on "the plan to achieve the medium- and long-term goal of the Japan Atomic Energy Agency", has been performed by Center for Computational Science & e-Systems (CCSE), Japan Atomic Energy Agency. CCSE established a committee consisting of external experts and authorities which evaluates and advises toward the future research and development. This report summarizes the results of the R&D performed by CCSE in FY2024 (April 1st, 2024 - March 31st, 2025) and their evaluation by the committee.

JAEA Reports

Annual report for FY2024 on the activities of radiation safety in Nuclear Science Research Institute and so on (April 1, 2024 - March 31, 2025)

Department of Radiation Protection, Nuclear Science Research Institute; Nuclear Facilities Management Section, Aomori Research and Development Center

JAEA-Review 2025-055, 107 Pages, 2026/03

JAEA-Review-2025-055.pdf:2.26MB

This annual report describes the activities in the 2024 fiscal year of Department of Radiation Protection at Nuclear Science Research Institute, Harima Synchrotron Radiation Radioisotope Laboratory, and Nuclear Facilities Management Section at Aomori Research and Development Center. The activities described in this report are environmental monitoring, radiation protection practices in workplaces, individual monitoring, maintenance of monitoring instruments, and research and development of radiation protection. At these institutes, the occupational exposures did not exceed the dose limits. The radioactive gaseous and liquid discharges from the facilities were well below the prescribed limits. The research and development activities in the field of radiological protection were continued.

JAEA Reports

Ultrasonic analysis of columnar crystal propagation echo in acoustically anisotropic weld metals; Targeting intergranular cracking of stainless-steel piping in pressurized water reactor primary system "FY2024 Nuclear Regulation Research Technology Infrastructure Construction Project Subsidy 'The Grant to Establish Technology Bases for Enhancement of Nuclear Regulation Research'"

Matsui, Tetsuya; Shimodaira, Masaki; Yamaguchi, Yoshihito; Toyama, Takeshi; Katsuyama, Jinya

JAEA-Research 2025-017, 41 Pages, 2026/03

JAEA-Research-2025-017.pdf:4.52MB

The JAEA Safety Research Center has been conducting fundamental research on advanced inspection and structural integrity assessment technologies since FY2024, including the development of a machine-learning-based ultrasonic flaw detection method using an ultrasonic simulator. To assess the simulator's applicability, phased array ultrasonic testing (PAUT) results produced by the simulator were compared with actual measurement data. Due to limited publicly available datasets, an intergranular crack in the pressurizer spray line piping of Kansai Electric Power Co. Inc.'s Ohi Nuclear Power Station Unit 3 was selected as the reference case. PAUT linear scanning analysis at a 45$$^{circ}$$ incident angle detected the crack's corner and edge echoes. Strong columnar-crystal propagation echoes were also observed within the weld metal, with their intensity showing dependence on the symmetric axis angle. Analysis at a 31$$^{circ}$$ incident angle similarly identified strong columnar-crystal propagation echoes, which connected to the crack's corner echoes and propagated into the weld region. These results align with actual measurements, indicating that the observed weld-metal echoes are likely attributable to columnar-crystal propagation.

Journal Articles

Effects of irradiation parameters on $$alpha$$' phase precipitation in FeCrAl alloys

Yamashita, Shinichiro; Abe, Yosuke; Okubo, Nariaki; Ukai, Shigeharu; Sasaki, Taisuke*

QST-M-56; QST Takasaki Annual Report 2024, P. 28, 2026/02

Journal Articles

Effect of nanoscale cellular structure on the mechanical properties of Inconel 718 with unique hierarchical structure fabricated by laser powder bed fusion

Cho, K.*; Yamashita, Kippei*; Kakutani, Shinnosuke*; Saito, Takuma*; Sasaki, Taisuke*; Sawaizumi, Katsuhiko*; Okugawa, Masayuki*; Koizumi, Yuichiro*; Mayama, Tsuyoshi*; Kikukawa, Taichi*; et al.

Acta Materialia, 303, p.121696_1 - 121696_18, 2026/01

 Times Cited Count:21 Percentile:95.69(Materials Science, Multidisciplinary)

Journal Articles

Application of the spectral determination method to unified $$gamma$$-ray singles and coincidence spectra

Oshima, Masumi*; Hayakawa, Takehito*; Asai, Masato; Goto, Jun*; Shinohara, Hirofumi*

Journal of Nuclear Science and Technology, 11 Pages, 2026/00

 Times Cited Count:0

To analyze radioactive spectra, we developed a simple algorithmic method of the Spectral Determination Method (SDM), which analyzes the entire spectrum, including continuum backgrounds and peaks. This method was successfully applied to $$gamma$$-ray singles spectra and liquid scintillation $$beta$$ and X-ray spectra. To further extend the applicability of this method, we have newly applied this method to $$gamma$$-$$gamma$$ coincidence spectra, which demonstrated the superiority of the SDM analysis even for the $$gamma$$-$$gamma$$ coincidence spectra.

Journal Articles

None

Koizumi, Mitsuo; Yogo, Akifumi*

Isotope News, (802), p.11 - 14, 2025/12

no abstracts in English

JAEA Reports

Development of inspection technology for pipes in high background radiation environments (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; University of Fukui*

JAEA-Review 2025-036, 88 Pages, 2025/11

JAEA-Review-2025-036.pdf:6.36MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "Development of inspection technology for pipes in high background radiation environments" conducted in FY2023. The following two studies are being conducted with the aim of comprehensively developing technologies to address the three needs indicated in the hearing with TEPCO regarding observation of the inside of piping: (1) Hydrogen content, (2) Presence of precipitates, (3) Presence or absence of $$alpha$$/$$beta$$ radiation emitting nuclides. First, by downsizing existing nondestructive inspection equipment and developing a dedicated radiation detector capable of nondestructively imaging the inside of piping, we aim to obtain information on the inside of piping by nondestructive inspection using lasers, etc., and to clarify the presence or absence of $$alpha$$-nuclides in piping and the internal conditions of piping, etc. In addition, we will develop equipment to visualize $$alpha$$-nuclides and discriminate $$beta$$-nuclides in high dose rate environments, as well as technology to investigate the contents of the piping. Deployment of the developed technology is expected to be put into practical use by TEPCO and private companies.

JAEA Reports

High-speed 3D modeling for nuclear reactor environment based on feature extraction results from video images (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Sapporo University*

JAEA-Review 2025-033, 71 Pages, 2025/11

JAEA-Review-2025-033.pdf:4.48MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "High-speed 3D modeling for nuclear reactor environment based on feature extraction results from video images" conducted in FY2023. The present study aims to develop a 3D model for a workspace that maximizes the amount of information based on the features extracted from video, which is taken when surveying the primary containment vessel and inside the reactor building as part of the decommissioning of 1F, considering within a specified time. In FY2023, we verified extracting effective shooting conditions for obtaining 3D reconstruction based on photogrammetry and the method extracting feature values that can generate 3D restoration results from a small amount of data within a specified time based on deep learning. In addition, we applied point cloud data extracted from video to segmentation and classified it into parts with instance labels.

JAEA Reports

An Analytical study on Russia's civilian nuclear energy utilization

Kawasaki, Nobuchika

JAEA-Review 2025-043, 74 Pages, 2025/10

JAEA-Review-2025-043.pdf:2.45MB

Russia is one of the most advanced countries in the civilian use of nuclear energy. However, understanding the internal mechanisms of its nuclear program remains difficult due to various reasons. Therefore, this study presents a historical overview of Russia's nuclear energy utilization, fuel supply, fuel manufacturing capabilities, and concepts regarding reprocessing and the nuclear fuel cycle. From this overview, insights have been extracted and analyzed. These insights are then organized under two strategic perspectives: "Strategic diversity and continuity in developments and demonstrations" and "Diversity in utilizations and deployments," with considerations of implications for Japan, as below. Russia's nuclear energy policy strategically utilizes a variety of reactor types and fuel cycle technologies to expand nuclear power generation both domestically and internationally. Currently, nuclear power, centered on light-water reactors (VVER series), accounts for about 20% of Russia's electricity supply, and there are plans to increase this share to 25% by 2045. A wide range of reactors, from large-scale to medium and small modular reactors, are being constructed in Russia. Russia is also actively developing fast reactor technologies, and focusing on the reprocessing and recycling of spent fuel. Internationally, VVER-1200 reactors are under construction in several countries, and cooperation with China is deepening in the field of fast reactors. Notably, Russia offers an integrated, or selectively customizable, package of nuclear technology services on the international stage. These include not only reactor deployment, but also fuel supply, reprocessing, waste management, and even the provision of radioisotopes. Rather than simply exporting products or technology, Russia fosters long-term relationships and trust by flexibly responding to the conditions and needs of partner countries. For this reason, Russia promotes the technology developments in advance within the country in areas anticipated for future overseas deployment. It carefully selects target technologies and services and systematically rolls them out. This flexible strategy, combining "technological diversity" and "strategic consistency", enables cooperation with countries across various geopolitical contexts. For Japan, this strategic approach offers valuable lessons on how to engage in comprehensive international nuclear cooperation, not merely through technology exports, but through integrated approaches that encompass the entire fuel cycle, and by combining elements such as fast reactors and RI supply.

Journal Articles

Nanostructural analysis of composite materials by spin-contrast variation small-angle neutron scattering and neutron reflectometry

Kumada, Takayuki

For the Future of Hydrogen Science and Technology, 3(1), p.2 - 6, 2025/10

Journal Articles

Mechanistic insights into deformation, load redistribution, and stress partitioning in high-strength dual-phase medium-entropy alloys

Gu, G. H.*; Ha, H.*; Harjo, S.; Gong, W.; Louzguine-Luzgin, D. V.*; Kim, H. S.*

Materials Science & Engineering A, 943, p.148818_1 - 148818_10, 2025/10

 Times Cited Count:4 Percentile:61.57(Nanoscience & Nanotechnology)

JAEA Reports

Clarification of debris formation conditions on the basis of the sampling data and experimental study using simulated fuel debris and reinforcement of the analytical results of severe accident scenario (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; University of Fukui*

JAEA-Review 2025-007, 120 Pages, 2025/09

JAEA-Review-2025-007.pdf:8.13MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Clarification of debris formation conditions on the basis of the sampling data and experimental study using simulated fuel debris and reinforcement of the analytical results of severe accident scenario" conducted from FY2021 to FY2023. The present study aims to clarify the debris formation mechanism and utilize the results to refine the accident scenario. In the backward analysis of oxide debris formation, we prepared simulated fuel particles by the aerodynamic levitation method and ejection of melted oxides from a tungsten pipe with a small hole and summarized the relationship between preparation conditions and the properties of the particles. We also demonstrated the formation of simulated fuel debris obtained by the sampling in 1F and clarified the difference between the experimental results and thermodynamic calculation. From the estimation of mixing, melting and solidified states of metallic debris, it was found that the formation of thin reaction layer suppresses the damage of SUS in spite of Zr content around 1000 $$^{circ}$$C, and we quantify the elution rate of B$$_{4}$$C and Zircaloy to the melted SUS. We extended reaction rate data between various pressure vessel with SUS and Zr and welding parts and suggested reaction rate equation for large scale experiment. We also estimated the failure behavior of lower plenum of pressure vessel and outflow behavior of melt. Furthermore, we estimated transition behavior of Uranium melt to metallic debris melt in the re-melting process of predropped metallic debris. As the experimental techniques in the future, we prepared the semi-melted debris from oxide and metals and analyzed the reaction products and discussed the formation of simulated debris with a small amount of uranium oxide using a CCIM furnace and the aerodynamic levitation method.

Journal Articles

Phase transitions and relaxor behavior of lead-free ferroelectric bismuth potassium titanate

Saito, Kotaro*; Matsuo, Hiroki*; Yoneda, Yasuhiro; Ye, Z.-G*; Noguchi, Yuji*

Journal of Applied Physics, 138(9), p.094102_1 - 094102_9, 2025/09

 Times Cited Count:2 Percentile:40.34(Physics, Applied)

Journal Articles

Particle arrangements and optical changes induced by the water swelling of melanin-like polydopamine layers

Watanabe, Taku*; Maejima, Yui*; Ueda, Yuki; Motokawa, Ryuhei; Takabatake, Ai*; Takeda, Shinichi*; Fudoji, Hiroshi*; Kishikawa, Keiki*; Koori, Michinari*

Langmuir, 41(34), p.22762 - 22773, 2025/09

 Times Cited Count:5 Percentile:57.35(Chemistry, Multidisciplinary)

The assembled structures of melanin particles, i.e., colloidal particles coated with a melanin-like polydopamine (PDA) layer, create vivid structural colors. While the thickness of the PDA layer influences the particle arrangement and optical properties, the underlying mechanism has remained controversial. We demonstrate that the water swelling characteristics of PDA are crucial factors governing the dispersion and aggregation of these particles in solution. Detailed comparisons between dry and wet conditions revealed that the PDA layer readily absorbs water molecules, which leads to significant swelling in the thicker layers. The swelling of the PDA layers determined whether the particles remained dispersed or partially aggregated in the water, ultimately controlling the particle arrangement in the dry state once the water evaporated. These findings provide insights into the self-assembly of colloidal particles and offer a strategy for tuning the periodic particle order. This feature is pivotal for various applications in optical and sensing technologies.

1316 (Records 1-20 displayed on this page)