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Journal Articles

Simple pretreatment method for tritium measurement in environmental water samples using a liquid scintillation counter

Nakasone, Shunya*; Yokoyama, Sumi*; Takahashi, Tomoyuki*; Ota, Masakazu; Kakiuchi, Hideki*; Sugihara, Shinji*; Hirao, Shigekazu*; Momoshima, Noriyuki*; Tamari, Toshiya*; Shima, Nagayoshi*; et al.

Plasma and Fusion Research (Internet), 16, p.2405035_1 - 2405035_5, 2021/02

Removal of impurities such as organic and other types of dissolved matters from environmental water samples is required for precise analysis of tritium with a liquid scintillation counting method. In general, a distillation method is a conventional one for tritium analysis in environmental water samples, but is a time-consuming process that takes 24 hours for removal of impurities. We have proposed a rapid pretreatment method for tritium analysis, that uses ion exchange resins. In this study, we performed batch experiments, to evaluate the effectiveness of the ion exchange resins on the tritium measurement. The results obtained demonstrated that removal of impurities in the sample water by ion exchange resins can be achieved during a short period of time (i.e., in 5 min).

Journal Articles

Preliminary investigation of pretreatment methods for liquid scintillation measurements of environmental water samples using ion exchange resins

Nakasone, Shunya*; Yokoyama, Sumi*; Takahashi, Tomoyuki*; Ota, Masakazu; Kakiuchi, Hideki*; Sugihara, Shinji*; Hirao, Shigekazu*; Momoshima, Noriyuki*; Tamari, Toshiya*; Shima, Nagayoshi*; et al.

Plasma and Fusion Research (Internet), 15, p.2405027_1 - 2405027_3, 2020/05

A quick preprocessing system for tritium analysis of environmental samples is important to judge environmental influence of tritium releases due to accident or tritium-handling facilities. Analysis of tritium in water samples with liquid scintillation counting method requires removal of impurities such as organic matter and ion species from water samples. Generally, a distillation method is adopted as a pretreatment of analysis for tritium; however, the distillation method is a time-consuming process. The aim of this study is to evaluate a rapid pretreatment method for tritium analysis with ion exchange resin. From batch and column experiments that used inland water and ion exchange resin, we confirmed removals of impurities of the water sample and that the removal of impurities was possible for a short time (by 5 minutes).

Journal Articles

Development of field estimation technique and improvement of environmental tritium behavior model

Yokoyama, Sumi*; Takahashi, Tomoyuki*; Ota, Masakazu; Kakiuchi, Hideki*; Sugihara, Shinji*; Hirao, Shigekazu*; Momoshima, Noriyuki*; Tamari, Toshiya*; Shima, Nagayoshi*; Atarashi-Andoh, Mariko; et al.

Plasma and Fusion Research (Internet), 14(Sp.2), p.3405099_1 - 3405099_4, 2019/06

The Large Helical Device of the National Institute for Fusion Science started D-D experiments in 2017. To ensure the safety of the facility, it is important to develop evaluation methods for environmental tritium transfer. Tritiated water (HTO) in atmosphere and soil is transferred to plants, and organically bound tritium (OBT) is formed by photosynthesis. Prediction of OBT formation is important, because OBT accumulates in plants and causes dose through ingestion. The objective of this study is to estimate environmental tritium transfer using a simple compartment model and practical parameters. We proposed a simple compartment model consisting of air-soil-plant components, and tried to validate the model by comparison with a sophisticated model, SOLVEG. In this study, we plan to add wet deposition to the model and obtain parameters from measurements of soil permeability and tritium concentrations in air, soil and plants. We also establish rapid pretreatment methods for OBT analysis.

Journal Articles

Formation and retention of organically bound deuterium in rice in deuterium water release experiment

Atarashi-Andoh, Mariko; Amano, Hikaru; Kakiuchi, Hideki; Ichimasa, Michiko*; Ichimasa, Yusuke*

Health Physics, 82(6), p.863 - 868, 2002/06

 Times Cited Count:6 Percentile:39.48(Environmental Sciences)

As a substitute of tritium, deuterium water (D2O) vapor release experiments were performed to estimate the difference of formation and subsequent retention of organically bound deuterium (OBD) in rice plants between daytime and nighttime exposure. Potted plants were exposed to deuterium water vapor in a greenhouse for 8 hours, under day and night conditions. Deuterium concentrations in free water and organic matter in rice leaves and ears were investigated until the harvest time. Data analysis was carried out using a model in which different generating processes of organic matter were considered. The calculated results agreed with the measured value.

Journal Articles

Results of D$$_{2}$$O release experiement; Transfer of deutrium and Carbon-13 from air to plant

Atarashi-Andoh, Mariko; Amano, Hikaru; Porntepkasemsan, B.; Kakiuchi, Hideki; Ichimasa, Michiko*; Ichimasa, Yusuke*

KURRI-KR-53, p.18 - 21, 2000/10

no abstracts in English

JAEA Reports

Research and considerations of radiation control in decommissioning

Goda, Tadashi; Ando, Hideki

JNC TN9420 2000-001, 54 Pages, 1999/09

JNC-TN9420-2000-001.pdf:2.8MB

In O-arai Engineering Center of Japan Nuclear Cycle Development Institute, dccommissioning of nuclear facilities will be expected in future. The results of preceding JPDR decommissioning were researched and the radiation control in decommisioning was examined. The principles and technology necessaly for radiation control in decommissioning were arranged. The radiation control in decommissioning seems to be on extension line of daily radiological work control. Noticing points all the control of exposure dose with disassembly of high radiological equipment, the surface contamination measurement of building disassembly waste which large arises and the radioactivity measurement of activated material. When high radiological equipment is disassembled, the measures which reduce the exposure in the remote manipulation are taken. The total adiation protection program including the control of exposure dose in preparedness stage must be decided. Much time and personnel are required, when surface contamination of waste arisen in the building disassembly was measured by surveymeters. Therefore, it is necessaly to rationalize the measurement using automatic inspection equipment with large detection area. This type equipment has results which effectively fulfilled the function in the decommissioning of JPDR. It is possible to product the equipment in the combination of existing technology.

JAEA Reports

Development of NRESP98 Monte Carlo codes for the calculation of neutron response functions of neutron detectors; Calculation of the response function of spherical BF$$_{3}$$ proportional counter

Hashimoto, Makoto; Saito, Kei; Ando, Hideki

PNC TN9410 98-061, 59 Pages, 1998/05

PNC-TN9410-98-061.pdf:2.58MB

The method to calculate the response function of spherical BF$$_{3}$$ proportional counter; which is commonly used as neutron dose rate meter and neutron spectrometer with multi moderator system, is developed. As the calculation code for evaluating the response function, the existing code series NRESP, the Monte Carlo code for the calculation of response function of neutron detectors, is selected. However, the application scope of the existing NRESP is restricted, the NRESP98 is tuned as generally applicable code, with expansion of the geometrical condition, the applicable element, ete. The NRESP98 is tested with the response function of the spherical BF$$_{3}$$ proportional counter. Including the effect of the distribution of amplification factor, the detailed evaluation of the charged particle transportation and the effect of the statistical distribution, the result of NRESP98 calculation fit the experience within $$pm$$ 10%.

JAEA Reports

Report of radiation exposure control on the 11th periodic inspection at experimental fast reactor JOYO; Reported by radiation control section

; ; ; Ando, Hideki

PNC TN9410 97-094, 27 Pages, 1997/10

PNC-TN9410-97-094.pdf:0.85MB

The 11th periodic inspection had been executed at the experimental fast reactor JOYO from May 10,1995 to March 24,1997. Because the inspection had been extended several times, the time span of external exposure control was divided into two period. The result of collective dose equivalent in the previous term(from May 10,1995 to December 7,1996: about seventeen months) was 243.34 man*mSv, whereas, the expected collective dose equivalent was about 280man*mSv. The result of collective dose equivalent in the latter term (from December 8,1996 to March 24,1997: about three months) was 44.73 man*mSv, whereas, the expected collective dose equivalent was about 85man*mSv. The collective dose equivalent in the whole period of this inspection was 288.07 man*mSv. It was confirmed that this inspection was carried out with the suitable radiation protection programmes. In this report, the method for the control of external exposure and the reduction of external exposure, provided in 11th periodic inspection, were described with taking the results of the past periodic inspections into consideration.

Journal Articles

None

Takada, Chie; Nozaki, Tatsuo; Torii, Tatsuo; Ando, Hideki; Hashimoto, Makoto

P23(PROGRAM AND ABST, P. 23, 1997/00

None

JAEA Reports

Development of a radioactive gas monitor using plastic scintillation fibers

Nozaki, Tatsuo; Torii, Tatsuo; Takada, Chie; Tobita, Kazunori; Ando, Hideki

PNC TN9410 96-262, 96 Pages, 1996/09

PNC-TN9410-96-262.pdf:3.27MB

The basic research on large electron linear accelerator is under current investigation at Quantum Technology Development Facility in O-arai Engineering Center, Power Reactor and Nuclear Fuel Development Corporation. The result of this, the transmutation of fission products would be incorporated In the future demonstrative stage of the transmission of fission products, Nitrogen-13 and Oxygen-15 will be produced by the interaction between high energy bremsstrahlung and air during operation of the linac. The detection limits of conventional monitors are not sufficient for the limits of the concentration of Nitrogen-13 (6$$times$$10$$^{-4}$$ Bq/cm$$^{3}$$) and Oxygen-15 (6$$times$$10$$^{-4}$$ Bq/cm$$^{3}$$) in exhaust air. Therefore we have developed a new type of gas monitor detector that is packed with plastic scintillation fibers as the detection elements to detect the limits of concentration of Nitrogen-13 and Oxygen-15 in exhaust air. On designing the gas monitor detectors, the sensitivities of the detectors were simulated to optimize the shape and the volume of detector by using EGS4, the Monte-Carlo code for electrons and photons. Based on the results of the simulations, the detectors were composed and the characteristic examinations of sensitivities were carried out by using beta-ray checking sources and Krypton-85 gas. Main points are as follows : (1) The detection limit of the developed torus-type detector for Krypton-85 is 5.4$$times$$10$$^{-4}$$ Bq/cm$$^{3}$$ based on the results of the experiments. (2) The counting efficiency of a detector for Nitrogen-13 is 40 percent higher than the counting efficiency for Krypton-85 based on the results of simulations. This indicates that the detection limit of the detector for Nitrogen-13 is about 3.9 $$times$$10$$^{-4}$$ Bq/cm$$^{3}$$. (3) The beta-ray energy of Oxygen-15 is higher than the beta-ray energy of Nitrogen-13. This theoretically reaches the conclusion that the detection limit of the detector for Oxygen-15 is lower than the ...

JAEA Reports

Experimental measurement of dose-rate distribution with scintillation fiber detector

Emoto, Takehiko; Torii, Tatsuo; Nozaki, Tatsuo; Saito, Kei; Emori, Shuichi; Ando, Hideki

PNC TN9410 96-299, 74 Pages, 1996/08

PNC-TN9410-96-299.pdf:3.06MB

The technique has been developed to measure the dose-rate distribution of radiation easily. The detector is made of plastic scintillation fibers (of following PSFs). The technique is based on the time of flight method, that is to measure the time difference of scintillation reaching from a incidence position to both ends of fibers. Measuring devices were built as trials. The position resolution was measured with collimated $$gamma$$ ray. The dose-rate linearity and the energy response were measured with an irradiation equipment of $$gamma$$ ray. Then, the devices were applied to the dose-rate distribution measurements in facilities. The tests were carried out to turn the technique into practicable use. Main results are as follows; (1) The continuos dose-rate distribution of $$gamma$$ ray can be measured with a single detector. The result of a measurement is illustrated on the screen of a device immediately. (2) The upper limit of counting rate measuring range is 10$$^{6}$$ cps. The upper limit of $$gamma$$ ray dose-rate measuring range is 1 mSv/h (calculated value) for a detector of "0.25 mm $$phi$$ $$times$$ 1 peace, 10 m length". (3) The detection efficiency does not depend on the $$gamma$$ ray energy between 500 keV and 1.5 MeV. (4) The practical length of PSFs is up to about 10 m for the dose-rate distribution measurement. (5) When the dose-rate distribution has sharp peaks, the output distribution of measurement is slightly flattened against the actual distribution based on the detector characteristic of position resolution. The unfolding method can correct this effect. (6) It is possible to discriminate the energy and type of radiation, if the pulse height output of a photomultiplire is corrected in each incidence position with the multi-parameter measuring method.

JAEA Reports

Realistic contamination control methods at $$alpha$$ and $$beta$$($$gamma$$) nuclide coexistence facilities

Ando, Hideki;

PNC TN9100 96-007, 32 Pages, 1996/03

PNC-TN9100-96-007.pdf:1.09MB

At the light water reactors with no fuel failure, radioactive contamination control is needed for $$beta$$($$gamma$$) nuclides such as $$^{60}$$Co and $$^{54}$$Mn. On the other hand, at the nuclear facilities where irradiated fuels (spent fuels) are handred, contamination control is needed for many kinds of $$alpha$$ and $$beta$$($$gamma$$) nuclides. There are three facilities where destructive testing of irradiated fuels and materials is done at Oarai Engineering Center. The ratios of the nuclidc composition are considerably stable at these facilities. Therefore, daily contamination control is cxecuted by measuring total (gross) $$beta$$($$gamma$$) activity with paying attention to the representative nuclides such as $$^{239}$$Pu, $$^{241}$$Pu and $$^{90}$$Sr. The investigation about the ratios of the nuclide composition, the basic idea of the contamination control, and the reality of the contamination control in the facilities are reported.

JAEA Reports

Radiological work control at nuclear facilities

Ando, Hideki;

PNC TN9100 96-006, 23 Pages, 1996/02

PNC-TN9100-96-006.pdf:2.19MB

None

JAEA Reports

Development of compound neutron dose meter

Hashimoto, Makoto; Torii, Tatsuo; Ando, Hideki

PNC TN9410 95-189, 69 Pages, 1995/08

PNC-TN9410-95-189.pdf:2.88MB

The new radiation weighting factors for neutron are introduced in ICRP 1990 Recommendations instead of the former quality factor. The contribution of intermediate energy neutron to the dose estimated with the new factors is more serious than with the former factors. Therefore, it indicates that the neutron dose evaluated by the former factors sometimes underestimates the dose evaluated by the new factors. Accordingly, to develop the neutron dose meter adjusted to the new recommendations, the new neutron detector has been cxperimented. In this study, instead of moderated detectors usually used as a neutron dose rate meter, the compound detector based on the multidetector method was employed. To understand the characteristic of this detector, we simulated the energy response and carried out the characteristic cxamination with neutron sources and accelerators. As a result of energy response simulation, in the region of interest, it can apply the multidetector method. As a result of characteristic examination, the detector can be used for measuring the neutron dose. Furthermore, in processes of the examination, this detector can discriminate the average energy of neutrons of $$^{241}$$Am-Be from that of $$^{239}$$Pu-Be. It is very sensitive to the neutron cnergy difference at intermediate energy. In future, it will be made improvement to make more practical dose estimation, and it will be made investigation to apply the ability of energy resolution.

Journal Articles

Measurement of Spatial Dose-Rate Distribution Using Scintillating Optical Fiber

Emoto, Takehiko; Torii, Tatsuo; Nozaki, Tatsuo; Ando, Hideki

Hoshasen, 21(3), p.49 - 58, 1995/07

None

JAEA Reports

Research and tests of position sensitive radiation detector

Emoto, Takehiko; ; Ando, Hideki

PNC TN9410 93-186, 65 Pages, 1993/09

PNC-TN9410-93-186.pdf:2.24MB

From the viewpoint of radiation protection and radiation shielding evaluation, the needs to know the positions that are irradiated by radiation are increasing, because measuring irradiated positions is useful for detecting local streaming at working areas in nuclear facilities and evaluating beam-loss from accelerators. We have investigated and experimented the characteristics of plastic scintillating fiber(PSF), that has been recently developed one of most popular position sensitive particle detectors in high energy physics, for purpose of that we can apply them to the radiation measurements as a position sensitive radiation detector. First, we referred to the results of the committed research performed in last year and to relative works. And, to aim for improvement of efficiency of gamma-ray and for stretch of the detector, we investigated efficiency and resolution of the detectors giving priorities to (a) variation of length and bundle of PSFs hamess, and (b) variation of the irradiated positions. As the results of referring to the works and the experiments on the detectors, we got the followings, (1)The method using the difference of reaching time between the scintillation photons from both ends of PSF is hopeful as position sensitive radiation detecting, because PSF has good time resolution and the time measurements have been recently developed to be rather easy and accurate methods. (2)Position resolution is 20cm to 30cm for collimated gamma-ray of $$^{137}$$Cs. And, the detectors bundled of ten PSFs have better characteristics of both efficiency and resolution. (3)When the detector is irradiated at near one of the ends, the efficiency and resolution will be 10% to 30% worse than irradiated at middle of it.

Journal Articles

Development of a 240mm bore-13T superconducting coil for large scale conductor testing

Nishi, Masataka; Ando, Toshinari; Isono, Takaaki; Sugimoto, Makoto; Koizumi, Norikiyo; Yoshida, Kiyoshi; Kawano, Katsumi; Takahashi, Yoshikazu; *; Tsuji, Hiroshi; et al.

IEEE Transactions on Magnetics, 28(1), p.597 - 600, 1992/01

 Times Cited Count:5 Percentile:52.28(Engineering, Electrical & Electronic)

no abstracts in English

Journal Articles

None

Ando, Hideki

Hoken Butsuri, , 

None

Oral presentation

Results of winding trial for ITER TF coil

Matsui, Kunihiro; Yamane, Minoru; Hemmi, Tsutomu; Kajitani, Hideki; Takano, Katsutoshi; Ando, Shinji; Koizumi, Norikiyo

no journal, , 

no abstracts in English

Oral presentation

Results of heat treatment trial of ITER toroidal field coil

Yamane, Minoru; Matsui, Kunihiro; Kajitani, Hideki; Hemmi, Tsutomu; Takano, Katsutoshi; Ando, Shinji; Koizumi, Norikiyo

no journal, , 

no abstracts in English

32 (Records 1-20 displayed on this page)