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Concept for the single cycle process based on mutual separation by reverse extraction of actinides and fission products

アクチノイドと核分裂生成元素の逆抽出による相互分離を基礎とする単サイクルプロセス概念

佐々木 祐二; 津幡 靖宏; 白数 訓子; 森田 圭介; 鈴木 智也

Sasaki, Yuji; Tsubata, Yasuhiro; Shirasu, Noriko; Morita, Keisuke; Suzuki, Tomoya

高レベル廃液の新しい分離プロセス概念が検討された。このプロセスはアクチノイドと核分裂生成元素を一括で抽出し、逆抽出で相互分離する方法である。単独の抽出剤と幾つかの逆抽出剤が必要となり、白金族元素,アクチノイド,酸素酸の陰イオンを同時に抽出する抽出剤が望まれる。NTAアミドは有望な抽出剤の一つである。次に逆抽出剤の検討が必要であり、水溶性のハードドナー,ソフトドナーによる効果を調査中であり、結果を報告する。

The concept for the new partitioning method of high-level radioactive waste (HLW) by single-cycle extraction process has been investigated. This process is based on extraction of actinides (An) and fission products (FP), and mutual separation by reverse extraction. Solo extractant and several stripping reagents will be utilized in this process. The extractant employed in this process is required to extract soft (platinum metals), hard acid metals(An), and oxonium anions (Mo, Tc) simultaneously. NTAamide is one of the candidate extractants. After extraction of An and FP by NTAamide(C8), the mutual separation among these metals by reverse extraction will be followed using the suitable water-miscible reagents. The extraction of An and FP, and the masking effect by some water-miscible reagents has been studied.

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