検索対象:     
報告書番号:
※ 半角英数字
 年 ~ 
 年

Defect chemistry and basic properties of non-stoichiometric PuO$$_{2}$$

不定比性PuO$$_{2}$$の欠陥化学と基礎特性

加藤 正人   ; 中村 博樹  ; 渡部 雅  ; 松本 卓; 町田 昌彦  

Kato, Masato; Nakamura, Hiroki; Watanabe, Masashi; Matsumoto, Taku; Machida, Masahiko

PuO$$_{2-x}$$の実験データをレビューし、酸素ポテンシャル、電気伝導率及び第一原理計算結果を用いて欠陥濃度を評価した。欠陥濃度を評価する式を導出し、様々な基礎特性の間の整合性を確認するとともに、熱物性を評価するための機構論的モデルを導出した。

The basic properties of PuO$$_{2-x}$$ were reviewed, and the equilibrium defects in PuO$$_{2-x}$$ were evaluated from the experimental data of the oxygen potential and electrical conductivity as well as the Ab-initio calculation results. Consistency among various properties was confirmed, and the mechanistic models for thermal property representations were derived.

Access

:

- Accesses

InCites™

:

Altmetrics

:

[CLARIVATE ANALYTICS], [WEB OF SCIENCE], [HIGHLY CITED PAPER & CUP LOGO] and [HOT PAPER & FIRE LOGO] are trademarks of Clarivate Analytics, and/or its affiliated company or companies, and used herein by permission and/or license.