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Electronic structure of ThPd$$_2$$Al$$_3$$; Impact of the U $$5f$$ states on the electronic structure of UPd$$_2$$Al$$_3$$

ThPd$$_2$$Al$$_3$$の電子状態; UPd$$_2$$Al$$_3$$の電子状態におけるU $$5f$$状態の影響

藤森 伸一  ; 竹田 幸治  ; 山上 浩志; Posp$'i$$v{s}$il, J.*; 山本 悦嗣 ; 芳賀 芳範 

Fujimori, Shinichi; Takeda, Yukiharu; Yamagami, Hiroshi; Posp$'i$$v{s}$il, J.*; Yamamoto, Etsuji; Haga, Yoshinori

The electronic structure of $$mathrm{ThPd_2Al_3}$$, which is isostructural to the heavy fermion superconductor $$mathrm{UPd_2 Al_3}$$, was investigated by photoelectron spectroscopy. The band structure and Fermi surfaces of $$mathrm{ThPd_2Al_3}$$ were obtained by angle-resolved photoelectron spectroscopy (ARPES), and the results were well-explained by the band-structure calculation based on the local density approximation. The comparison between the ARPES spectra and the band-structure calculation suggests that the Fermi surface of $$mathrm{ThPd_2Al_3}$$ mainly consists of the $$mathrm{Al}~3p$$ and $$mathrm{Th}~6d$$ states with a minor contribution from the $$mathrm{Pd}~4d$$ states. The comparison of the band structures between $$mathrm{ThPd_2Al_3}$$ and $$mathrm{UPd_2Al_3}$$ argues that the $$mathrm{U}~5f$$ states form Fermi surfaces in $$mathrm{UPd_2Al_3}$$ through hybridization with the $$mathrm{Al}~3p$$ state in the $$mathrm{Al}$$ layer, suggesting that the Fermi surface of $$mathrm{UPd_2Al_3}$$ has a strong three-dimensional nature.

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