Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Brumm, S.*; Gabrielli, F.*; Sanchez Espinoza, V.*; Stakhanova, A.*; Groudev, P.*; Petrova, P.*; Vryashkova, P.*; Ou, P.*; Zhang, W.*; Malkhasyan, A.*; et al.
Annals of Nuclear Energy, 211, p.110962_1 - 110962_16, 2025/02
被引用回数:2 パーセンタイル:72.25(Nuclear Science & Technology)The completed Horizon-2020 project on "Management and Uncertainties of Severe Accidents (MUSA)" has reviewed uncertainty sources and Uncertainty Quantification methodology for the purpose of assessing Severe Accidents (SA). The key motivation of the project has been to bring the advantages of the Best Estimate Plus Uncertainty approach to the field of Severe Accident. The applications brought together a large group of participants that set out to apply uncertainty analysis (UA) within their field of SA modelling expertise, in particular reactor types, but also SA code used (ASTEC, MELCOR, etc.), uncertainty quantification tools used (DAKOTA, RAVEN, etc.), detailed accident scenarios, and in some cases SAM actions. This paper synthesizes the reactor-application work at the end of the project. Analyses of 23 partners are sorted into different categories, depending on whether their main goal is/are (i) uncertainty bands of simulation results; (ii) the understanding of dominating uncertainties in specific sub-models of the SA code; (iii) improving the understanding of specific accident scenarios, with or without the application of SAM actions; or, (iv) a demonstration of the tools used and developed, and of the capability to carry out an uncertainty analysis in the presence of the challenges faced. The partners' experiences made during the project have been evaluated and are presented as good practice recommendations. The paper ends with conclusions on the level of readiness of UA in SA modelling, on the determination of governing uncertainties, and on the analysis of SAM actions.
Ren, Q.*; Gupta, M. K.*; Jin, M.*; Ding, J.*; Wu, J.*; Chen, Z.*; Lin, S.*; Fabelo, O.*; Rodriguez-Velamazan, J. A.*; 古府 麻衣子; et al.
Nature Materials, 22(8), p.999 - 1006, 2023/08
被引用回数:65 パーセンタイル:99.32(Chemistry, Physical)Ultralow thermal conductivity and fast ionic diffusion endow superionic materials with excellent performance both as thermoelectric converters and as solid-state electrolytes. Yet the correlation and interdependence between these two features remain unclear owing to a limited understanding of their complex atomic dynamics. Here we investigate ionic diffusion and lattice dynamics in argyrodite AgSnSe
using synchrotron X-ray and neutron scattering techniques along with machine-learned molecular dynamics. We identify a critical interplay of the vibrational dynamics of mobile Ag and a host framework that controls the overdamping of low-energy Ag-dominated phonons into a quasi-elastic response, enabling superionicity. Concomitantly, the persistence of long-wavelength transverse acoustic phonons across the superionic transition challenges a proposed 'liquid-like thermal conduction' picture. Rather, a striking thermal broadening of low-energy phonons, starting even below 50 K, reveals extreme phonon anharmonicity and weak bonding as underlying features of the potential energy surface responsible for the ultralow thermal conductivity (
0.5 Wm
K
) and fast diffusion. Our results provide fundamental insights into the complex atomic dynamics in superionic materials for energy conversion and storage.
山下 恵史朗*; 小松 一生*; Klotz, S.*; Fabelo, O.*; Fernndez-D
az, M. T.*; 阿部 淳*; 町田 真一*; 服部 高典; 入舩 徹男*; 新名 亨*; et al.
Proceedings of the National Academy of Sciences of the United States of America, 119(40), p.e2208717119_1 - e2208717119_6, 2022/10
被引用回数:5 パーセンタイル:23.80(Multidisciplinary Sciences)氷の多形体は、圧力や温度により驚くほど多様な構造を示す。水素結合の乱れは、その構造多様性の重要な要因であるだけでなく、その物性をも支配している。しかし、観測可能な逆格子空間が限られていることや、高圧下で測定されたデータの不確かさにより、高圧下において氷多形体の乱れた構造を明らかにすることは困難であった。今回、単結晶および粉末中性子回折の両方を用いて、2.2GPa, 298Kにおいて主要な高圧氷である氷VIIの乱れた構造を初めて明らかにした。最大エントロピー法を用いることにより3次元的な原子分布を導くことに成功し、水素がこれまで言われていた離散的なサイトではなく、リング状に分布をしていることを発見した。また、274Kでの全散乱実験により、氷VIIの水素秩序相である氷VIIIとは、同じ分子構造を持つにもかかわらず、その分子間構造が異なることを明らかにした。今回の単結晶と粉末回折の相補的な構造解析によって、氷VIIのユニークな無秩序構造が明確に示された。今回の発見は、圧力によって大きく変化するプロトンダイナミクスと関連しており、圧力下における氷VIIの異常な物性の構造的な起源を理解することに役立つと考えられる。
Yakushev, A.*; Lens, L.*; Dllmann, Ch. E.*; Khuyagbaatar, J.*; J
ger, E.*; Krier, J.*; Runke, J.*; Albers, H. M.*; 浅井 雅人; Block, M.*; et al.
Frontiers in Chemistry (Internet), 10, p.976635_1 - 976635_11, 2022/08
被引用回数:17 パーセンタイル:80.63(Chemistry, Multidisciplinary)114番元素フレロビウム(Fl)は現在その化学的性質が研究されている最も重い元素である。Flに関する最初の化学実験では、Flは貴ガス的な性質を持つ元素であると報告された。一方、2番目の研究では、Flは揮発性金属の性質を示すと報告された。より信頼性の高い結論を得るため、我々は更なる実験的研究を行い、二酸化ケイ素と金表面におけるFlの吸着挙動を調べた。その結果、Flは揮発性金属の水銀よりも高い揮発性と低い反応性を示し、一方、貴ガスのラドンよりは反応性が高いことを明らかにした。
Bronis, A.*; Heberger, F. P.*; Antalic, S.*; Andel, B.*; Ackermann, D.*; Heinz, S.*; Hofmann, S.*; Khuyagbaatar, J.*; Kindler, B.*; Kojouharov, I.*; et al.
Physical Review C, 106(1), p.014602_1 - 014602_12, 2022/07
被引用回数:6 パーセンタイル:71.20(Physics, Nuclear)The decay of excited states in No was investigated by applying the evaporation-residue-conversion-electron correlation technique. Two new isomeric states were observed in
No together with the previously known one. Excitation energies of the isomeric states were estimated based on the energies of conversion electrons and
rays from correlation chains. These results were in accord with theoretical calculations based on the mean-field models. A tentative decay scheme of isomeric states in
No is proposed, and their Nilsson configurations are discussed. The energy decrease of the 11/2
[725] Nilsson level for heavy
=153 isotones as a function of increasing proton number is confirmed.
Brumm, S.*; Gabrielli, F.*; Sanchez-Espinoza, V.*; Groudev, P.*; Ou, P.*; Zhang, W.*; Malkhasyan, A.*; Bocanegra, R.*; Herranz, L. E.*; Berda, M.*; et al.
Proceedings of 10th European Review Meeting on Severe Accident Research (ERMSAR 2022) (Internet), 13 Pages, 2022/05
The current HORIZON-2020 project on "Management and Uncertainties of Severe Accidents (MUSA)" aims at applying Uncertainty Quantification (UQ) in the modeling of Severe Accidents (SA), particularly in predicting the radiological source term of mitigated and unmitigated accident scenarios. Within its application part, the project is devoted to the uncertainty quantification of different severe accident codes when predicting the radiological source term of selected severe accident sequences of different nuclear power plant designs, e.g. PWR, VVER, and BWR. Key steps for this investigation are, (a) the selection of severe accident sequences for each reactor design, (b) the development of a reference input model for the specific design and SA-code, (c) the selection of a list of uncertain model parameters to be investigated, (d) the choice of an UQ-tool e.g. DAKOTA, SUSA, URANIE, etc., (e) the definition of the figures of merit for the UA-analysis, (f) the performance of the simulations with the SA-codes, and, (g) the statistical evaluation of the results using the capabilities, i.e. methods and tools offered by the UQ-tools. This paper describes the project status of the UQ of different SA codes for the selected SA sequences, and the technical challenges and lessons learnt from the preparatory and exploratory investigations performed.
佐藤 陽祐*; 関山 剛*; Fang, S.*; 梶野 瑞王*; Qurel, A.*; Qu
lo, D.*; 近藤 裕昭*; 寺田 宏明; 門脇 正尚; 滝川 雅之*; et al.
Atmospheric Environment; X (Internet), 7, p.100086_1 - 100086_12, 2020/10
福島第一原子力発電所(FDNPP)事故により放出されたCsの大気中の挙動を調べるため、第3回大気拡散モデル相互比較が実施された。前回のモデル比較より高い水平格子解像度(1km)が使われた。前回のモデル比較に参加したモデル中9モデルが参加し、全モデルで同一の放出源情報と気象場が使用された。解析の結果、観測された高い
Cs大気中濃度のほとんどが良好に再現され、いくつかのモデルの性能向上によりマルチモデルアンサンブルの性能が向上した。高解像度化によりFDNPP近傍の気象場の再現性が向上したことで、拡散モデルの性能も向上した。風速場の良好な表現によりFDNPP北西の高い沈着量の細い分布が合理的に計算され、FDNPPの南側の沈着量の過大評価が改善された。一方で、中通り地方、群馬県北部、及び首都圏のプルームの再現性能はやや低下した。
佐藤 陽祐*; 滝川 雅之*; 関山 剛*; 梶野 瑞王*; 寺田 宏明; 永井 晴康; 近藤 裕昭*; 打田 純也*; 五藤 大輔*; Qulo, D.*; et al.
Journal of Geophysical Research; Atmospheres, 123(20), p.11748 - 11765, 2018/10
被引用回数:47 パーセンタイル:84.74(Meteorology & Atmospheric Sciences)福島第一原子力発電所事故により放出されたCsの大気中の挙動を理解するため、大気拡散モデル相互比較が実施され、12モデルが参加した。モデルで考慮される過程に起因するモデル間の差異に焦点を当てた解析を行うため、全モデルで同じ気象場、水平分解能、及び放出源情報が使用された。モデルアンサンブルによる観測された大気中
Cs濃度上昇イベントの捕捉率は40%であり、FMSは80を超えた。解析の結果、大気中
Cs濃度上昇イベントの再現には気象場が最も重要な要素であり、気象場の再現性が高い場合のモデル間の差異は、沈着及び拡散過程に起因していることが分かった。また、沈着フラックスが小さいモデル及び拡散が強いモデルは高い性能を示したが、拡散が強いモデルは大気中
Cs濃度を過大評価する傾向を示した。
Bentaib, A.*; Chaumeix, N.*; Grosseuvres, R.*; Bleyer, A.*; Gastaldo, L.*; Maas, L.*; Jallais, S.*; Vyazmina, E.*; Kudriakov, S.*; Studer, E.*; et al.
Proceedings of 12th International Topical Meeting on Nuclear Reactor Thermal-Hydraulics, Operation and Safety (NUTHOS-12) (USB Flash Drive), 11 Pages, 2018/10
In the framework of the French MITHYGENE project, the new highly instrumented ENACCEF2 facility was built at the Institut de Combustion Aerothermique Reactivite et Environnement (ICARE) of the Centre National de la Recherche Scientifique (CNRS) in Orleans (France) to address the flame propagation in hydrogen combustion during a severe accident. The ENACCEF2 facility is a vertical tube of 7.65 m height and 0.23 m inner diameter. In the lower part of the tube, annular obstacles are installed to promote turbulent flame propagation. At the initiative of the MITHYGENE project consortium and the European Technical Safety Organisation Network (ETSON), a benchmark on hydrogen combustion was organised with the goal to identify the current level of the computational tools in the area of hydrogen combustion simulation under conditions typical for safety considerations for NPP. In the proposed paper, the simulation results obtained by participating organizations, using both Computational Fluid Dynamics (CFD) and lumped-parameter computer codes, are compared to experimental results and analysed.
Alexa, P.*; Ramdhane, M.*; Thiamova, G.*; Simpson, G. S.*; Faust, H. R.*; Genevey, J.*; Kster, U.*; Materna, T.*; Orlandi, R.; Pinston, J. A.*; et al.
Physical Review C, 97(3), p.034327_1 - 034327_6, 2018/03
被引用回数:2 パーセンタイル:19.25(Physics, Nuclear)Delayed -ray and conversion-electron spectroscopy was performed on A = 152 fission fragments, at the Lohengrin spectrometer of the Institut Laue-Langevin, Grenoble, France. In this study, a new decay scheme was observed for the odd-odd nuclide
Pr. The low-energy structure of this isotope was analysed by comparison with the quasiparticle phonon model and the particle-rotor model. The main configurations for the (
) ground state and for the 4.7(3)-
s (
) isomer at 115 keV were assigned to, respectively,
3/2[541]
3/2[521] and
3/2[422]
5/2[642].
Samarakoon, A. M.*; 高橋 満*; Zhang, D.*; Yang, J.*; 片山 尚幸*; Sinclair, R.*; Zhou, H. D.*; Diallo, S. O.*; Ehlers, G.*; Tennant, D. A.*; et al.
Scientific Reports (Internet), 7(1), p.12053_1 - 12053_8, 2017/09
被引用回数:10 パーセンタイル:57.09(Multidisciplinary Sciences)Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific challenge. Here, we show that scaling of magnetic memories with time can be used to classify magnetic glassy materials into two distinct classes. The systems studied are high temperature superconductor-related materials, spin-orbit Mott insulators, frustrated magnets, and dilute magnetic alloys. Our bulk magnetization measurements reveal that most densely populated magnets exhibit similar memory behavior characterized by a relaxation exponent of
(1). This exponent is different from
of dilute magnetic alloys that was ascribed to their hierarchical and fractal energy landscape, and is also different from
of the conventional Debye relaxation expected for a spin solid, a state with long range order.
Barbagallo, M.*; Musumarra, A.*; Cosentino, L.*; Maugeri, E.*; Heinitz, S.*; Mengoni, A.*; Dressler, R.*; Schumann, D.*; Kppeler, F.*; 原田 秀郎; et al.
Physical Review Letters, 117(15), p.152701_1 - 152701_7, 2016/10
被引用回数:90 パーセンタイル:94.62(Physics, Multidisciplinary)The energy-dependent cross section of the Be(
He reaction, of interest for the so-called cosmological lithium problem in big bang nucleosynthesis, has been measured for the first time from 10 meV to 10 keV neutron energy. Coincidences between the two alpha particles have been recorded in two Si-
Be-Si arrays placed directly in the neutron beam. The present results are consistent, at thermal neutron energy, with the only previous measurement performed in the 1960s at a nuclear reactor. The energy dependence reported here clearly indicates the inadequacy of the cross section estimates currently used in BBN calculations. Although new measurements at higher neutron energy may still be needed, the n_TOF results hint at a minor role of this reaction in BBN, leaving the long-standing cosmological lithium problem unsolved.
奥村 義和; Gobin, R.*; Knaster, J.*; Heidinger, R.*; Ayala, J.-M.*; Bolzon, B.*; Cara, P.*; Chauvin, N.*; Chel, S.*; Gex, D.*; et al.
Review of Scientific Instruments, 87(2), p.02A739_1 - 02A739_3, 2016/02
被引用回数:8 パーセンタイル:36.72(Instruments & Instrumentation)IFMIFは40MeV/125mAの重水素ビームを発生する2基の線形加速器を用いた核融合材料照射施設である。日欧の幅広いアプローチ活動のもとで、原型加速器(LIPAc)を用いた実証試験が開始されており、その目標は9MeV/125mAの連続重水素ビームを発生することである。フランスで開発された入射器は、既に日本の六ヶ所の国際核融合研究開発センターに搬入され、2014年から運転と試験が開始されている。これまでに、100keV/120mAの連続水素ビームを0.2.mm.mradのエミッタンスのもとで生成することに成功している。
Pikuz, T.*; Faenov, A.*; 松岡 健之*; 松山 智至*; 山内 和人*; 尾崎 典雅*; Albertazzi, B.*; 犬伏 雄一*; 矢橋 牧名*; 登野 健介*; et al.
Scientific Reports (Internet), 5, p.17713_1 - 17713_10, 2015/12
被引用回数:40 パーセンタイル:86.89(Multidisciplinary Sciences)we report, that by means of direct irradiation of lithium fluoride a (LiF) crystal, in situ 3D visualization of the SACLA XFEL focused beam profile along the propagation direction is realized, including propagation inside photoluminescence solid matter. High sensitivity and large dynamic range of the LiF crystal detector allowed measurements of the intensity distribution of the beam at distances far from the best focus as well as near the best focus and evaluation of XFEL source size and beam quality factor M2. Our measurements also support the theoretical prediction that for X-ray photons with energies 10 keV the radius of the generated photoelectron cloud within the LiF crystal reaches about 600 nm before thermalization. The proposed method has a spatial resolution 0.4-2.0 micron for photons with energies 6-14 keV and potentially could be used in a single shot mode for optimization of different focusing systems developed at XFEL and synchrotron facilities.
Lampasi, A.*; Zito, P.*; Coletti, A.*; Novello, L.*; 松川 誠; 島田 勝弘; Burini, F.*; Kuate-Fone, Y.*; Taddia, G.*; Tenconi, S.*
Fusion Engineering and Design, 98-99, p.1098 - 1102, 2015/10
被引用回数:12 パーセンタイル:67.70(Nuclear Science & Technology)In JT-60SA, the first SNU (prototype), consisting of six cubicles, was assembled in 2013. The factory tests on this system, including tests at full current and voltage, are being performed throughout 2014. The manufacturing of the remaining three SNUs will proceed after the success of such tests. The main characteristics of the developed SNU are; (1) Snchronized use of an electronic static circuit breaker (SCB) in parallel with an electromechanical bypass switch (BPS), (2) Nominal voltage of 5 kV, with a specific circuit to limit the transient voltage to 5.5 kV, (3) DC current interruption up to 20 kA, (4) Light BPS with opening and closing times shorter than 15 ms and 65 ms, respectively, (5) Breakdown resistance adaptable from 0.25 to 3.75
by four selectors, (7) Fully electronic making switch (MS) and (8) Breakdown resistors that could dissipate much more than 90 MJ.
奥村 義和; Ayala, J.-M.*; Bolzon, B.*; Cara, P.*; Chauvin, N.*; Chel, S.*; Gex, D.*; Gobin, R.*; Harrault, F.*; Heidinger, R.*; et al.
Proceedings of 12th Annual Meeting of Particle Accelerator Society of Japan (インターネット), p.203 - 205, 2015/09
日欧協力のもと、国際核融合中性子照射施設(IFMIF)の工学設計工学実証活動(EVEDA)が2007年から開始されている。IFMIFにおける最大の開発課題は、40MeV/250mA/CWの重水素イオンビームを発生できる大電流加速器であり、現在、その原型加速器(9MeV/125mA/CW)の試験を六ヶ所村の国際核融合研究センターにおいて段階的に実施している。試験は日欧の事業チームメンバーと、入射器を担当したフランスサクレー研究所などの欧州ホームチーム,日本ホームチームのメンバーから構成される原型加速器統合チームが担当している。入射器については、2014年から試験を開始し、現在までに100keV/120mA/CWの水素イオンビームを0.3mm.mrad以下のエミッタンスで生成することに成功している。2015年には、高周波四重極加速器(RFQ)用高周波電源の搬入据付が開始され、入射器の試験の終了とともにRFQ本体の据付も開始される予定である。本稿では、入射器の実証試験の結果とともに、RFQ,超伝導リニアック,高周波電源,ビームダンプ等の現状について報告する。
Taprogge, J.*; Jungclaus, A.*; Grawe, H.*; 西村 俊二*; Doornenbal, P.*; Lorusso, G.*; Simpson, G. S.*; Sderstr
m, P.-A.*; 炭竃 聡之*; Xu, Z. Y.*; et al.
Physical Review C, 91(5), p.054324_1 - 054324_11, 2015/05
被引用回数:24 パーセンタイル:80.70(Physics, Nuclear)The decay of
Cd, produced in relativistic fission of a
U beam, was studied at the RIKEN Nishina Center. From the
-ray analysis, 31 excited states and 69
ray transitions were established in the level scheme of
In, and compared with state-of-the-art shell-model calculations. It was found that the
decay of
Cd is dominated by Gamow teller transitions, but a non-negligible contribution to the
decay is also made by first-forbidden transitions. To estimate the contribution of first-forbidden transitions is important for calculations of the
-decay half-lives of nuclei in this region.
Taprogge, J.*; Jungclaus, A.*; Grawe, H.*; 西村 俊二*; Xu, Z. Y.*; Doornenbal, P.*; Lorusso, G.*; Ncher, E.*; Simpson, G. S.*; S
derstr
m, P.-A.*; et al.
Physics Letters B, 738, p.223 - 227, 2014/11
被引用回数:23 パーセンタイル:78.70(Astronomy & Astrophysics)The decay of an isomeric state in the neutron-rich nucleus Cd was observed via the detection of internal conversion and Compton electrons. This measurement provided the first experimental information on excited states in this nucleus. The isomer was populated in the projectile fission of a
U beam at the RIBF facility at RIKEN. From the measured yields of
rays and internal conversion electrons, E3 multipolarity was tentatively assigned to the isomeric transition. A half-life of 3.6(2) ms was determined for this new state which, by comparison with shell-model calculations, was tentatively assigned a spin of (21/2
).
Burini, F.*; Kuate-Fone, Y.*; Taddia, G.*; Tenconi, S.*; Lampasi, A.*; Zito, P.*; 松川 誠; 島田 勝弘; Coletti, A.*; Novello, L.*
Proceedings of 40th Annual Conference of the IEEE Industrial Electronics Society (IECON 2014), p.5035 - 5040, 2014/10
This paper describes the design and implementation of the Switching Network Unit (SNU) for the superconducting Central Solenoid coils of the international nuclear fusion experiment JT-60SA to be built in Naka, Japan. The SNU can interrupt a current up to 20 kA in less than 1 ms to create a voltage up to 5 kV. It is realized with a hybrid switch integrating an electro-mechanical device and a solid state Static Circuit Breaker, parallel connected. SNU resistance can be pre-arranged and dynamically reduced by a solid state making switch. Preliminary test results confirmed the current balance of the multiple parallel branches constituting the solid state switch and proper behavior of the devices, confirming simulations results. Further applications could be medium voltage DC networks (either naval or land based); higher DC voltages are practicable.
Taprogge, J.*; Jungclaus, A.*; Grawe, H.*; 西村 俊二*; Doornenbal, P.*; Lorusso, G.*; Simpson, G.*; Sderstr
m, P.-A.*; 炭竃 聡之*; Xu, Z. Y.*; et al.
Physical Review Letters, 112(13), p.132501_1 - 132501_6, 2014/04
被引用回数:53 パーセンタイル:88.39(Physics, Multidisciplinary)A low-lying state in In, the one-proton hole nucleus with respect to double magic
Sn, was observed by its
decay to the beta emitting isomer. The new state, which was populated both in the beta decay of
Cd and after beta-delayed neutron emission from
Cd, was identified, at an excitation energy of 1353 keV, as the previously unknown single-hole state with respect to the
Sn core. Exploiting this crucial new experimental information, shell-model calculations were performed to study the structure of experimentally inaccessible
=82 isotones below
Sn. The results evidence a surprising absence of proton subshell closures along the chain of
=82 isotones. This finding bears consequences on the evolution of the
=82 shell gap along the r-process path.