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Smallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Muir, D.*; Prchniak, L.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; et al.
Physical Review C, 110(2), p.024318_1 - 024318_16, 2024/08
被引用回数:1 パーセンタイル:0.00(Physics, Nuclear)In the selenium isotopes various shape phenomena are present, in particular the emergence of a dominant oblate deformation in the most neutron-deficient isotopes has been observed. The scenario of shape coexisting oblate and prolate bands has been proposed across the isotopic chain, with the crossing point of such bands being located near Se, where no coexistence has yet been identified. To determine the presence or absence of any low-lying
state in
Se, confirm the level structure, and interpret the nuclear deformation with theoretical models. A combined internal conversion electron and
-ray spectroscopy study was undertaken with the SPICE and TIGRESS spectrometers at the TRIUMF-ISAC-II facility. Nuclear models were provided by the Generalised Triaxial Rotor Model (GTRM) and the collective Generalised Bohr Hamiltonian (GBH). Despite a comprehensive search, no evidence was found for the existence of a
state below 2 MeV in
Se. Significant discrepancies to the previously established positive parity level scheme were found. GBH calculations using UNEDF1 mass parameters were found to reproduce the revised low-lying level structure well.
Se does not have a well defined axial shape. The 2
state at 1601 keV resembles a quasi-
excitation rather than a member of a shape coexisting band; the presence of such a band is all but ruled out.
Martel, I.*; Acosta, L.*; Aguado, J. L.*; Smallcombe, J.; 他68名*
Nuclear Instruments and Methods in Physics Research B, 541, p.176 - 179, 2023/08
被引用回数:3 パーセンタイル:46.61(Instruments & Instrumentation)The ISOLDE Scientific Infrastructure at CERN offers a unique range of post-accelerated radioactive beams. The scientific program can be improved with the Isolde Superconducting Recoil Separator (ISRS), an innovative spectrometer able to deliver unprecedented (A, Z) resolution. In this paper we present an overview of the physics and ongoing technical developments.
Yates, D.*; Krcken, R.*; Dillmann, I.*; Garrett, P. E.*; Smallcombe, J.; 他44名*
Physical Review C, 107(6), p.064309_1 - 064309_20, 2023/06
被引用回数:0 パーセンタイル:0.00(Physics, Nuclear)Detailed spectroscopy of neutron-rich, heavy, deformed nuclei is of broad interest for nuclear astrophysics and nuclear structure. Nuclei in the -process path and following freeze-out region impact the resulting
-process abundance distribution, and the structure of nuclei midshell in both proton and neutron number helps to understand the evolution of subshell gaps and large deformation in these nuclei.
Sun, L. J.*; Fry, C.*; Davids, B.*; Esker, N.*; Wrede, C.*; Smallcombe, J.; 他27名*
Physics Letters B, 839, p.137801_1 - 137801_8, 2023/04
被引用回数:2 パーセンタイル:45.98(Astronomy & Astrophysics)Motivated primarily by the large uncertainties in the thermonuclear rate of the 30PS reaction that limit our understanding of classical novae, we carried out lifetime measurements of S excited states using the Doppler Shift Lifetimes (DSL2) facility at the TRIUMF Isotope Separator and Accelerator (ISAC-II) facility.
Smallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; Barton, C. J.*; Bhattacharjee, S. S.*; et al.
Physical Review C, 106(1), p.014312_1 - 014312_9, 2022/07
被引用回数:5 パーセンタイル:61.57(Physics, Nuclear)The selenium isotopes lie at the heart of a tumultuous region of the nuclear chart where shape coexistence effects grapple with neutron-proton pairing correlations, triaxiality, and the impending proton dripline. In this work a study of Se by internal conversion electron and
-ray spectroscopy was undertaken with the SPICE and TIGRESS arrays. New measurements of the branching ratio and lifetime of the
state were performed yielding a determination of
milliunits. Two state mixing calculations were performed that highlighted the importance of interpretation of such
strength values in the context of shape-coexistence.
Xiao, Y.*; Go, S.*; Grzywacz, R.*; Orlandi, R.; Andreyev, A. N.; 浅井 雅人; Bentley, M. A.*; de Angelis, G.*; Gross, C. J.*; Hausladen, P.*; et al.
Physical Review C, 100(3), p.034315_1 - 034315_8, 2019/09
被引用回数:19 パーセンタイル:83.66(Physics, Nuclear)A search for super-allowed decay of N=Z nuclei
Te and
Xe was carried out using a novel recoil-decay scintillator detector at the tandem accelerator facility at Japan Atomic Energy Agency. Inorganic crystal scintillation material of YAP:Ce (Yttrium Aluminium Perovskite) coupled to position-sensitive photo-multiplier tube (PSPMT) was implemented for the first time in a radioactive decay experiment. Residues from the fusion-evaporation reaction
Ni+
Fe
Xe
were separated by the JAEA Recoil Mass Separator (RMS) and implanted into the YAP:Ce crystal.
decays of neutron-deficient tellurium isotopes were identified and proton-emission of
I was observed. No conclusive evidence was found for the decay chain
Xe
Te
Sn within 3 days experiment. The cross section limit of 130 pb was obtained for production of two events of
Xe, about an order of magnitude below the expectation based on earlier cross section measurements and HIVAP calculations.
廣瀬 健太郎; 西尾 勝久; 田中 翔也*; Lguillon, R.*; 牧井 宏之; 西中 一朗*; Orlandi, R.; 塚田 和明; Smallcombe, J.*; Vermeulen, M. J.; et al.
Physical Review Letters, 119(22), p.222501_1 - 222501_6, 2017/12
被引用回数:59 パーセンタイル:91.48(Physics, Multidisciplinary)JAEAタンデム加速器施設で行ったO+
U反応における多核子移行チャンネルを用いた実験により、
U,
Np、および
Puの核分裂質量分布を励起エネルギー10
60MeVにおいて測定した。これらのうち、
U,
Npのデータは本実験により初めて観測された。原子核の殻効果の減衰によって対称分裂すると予想されていた高励起エネルギーにおいても、質量分布が非対称を示すことがわかった。搖動散逸定理に基づく動力学モデル計算との比較から、この振る舞いはマルチチャンス核分裂によるものであることを明らかにした。
西尾 勝久; 廣瀬 健太郎; Lguillon, R.*; 牧井 宏之; Orlandi, R.; 塚田 和明; Smallcombe, J.*; 千葉 敏*; 有友 嘉浩*; 田中 翔也*; et al.
Proceedings of 6th International Conference on Fission and Properties of Neutron-rich Nuclei (ICFN-6), p.590 - 597, 2017/11
We are promoting a fission study using multi-nucleon transfer reactions, where excited states in neutron-rich actinide nuclei, which cannot be accessed by particle capture and/or fusion reactions, are populated. This allows us to study fission in the new region of chart of nuclei. Also, the excited states in the fissioning nucleus are widely populated in the reactions, thus the effects of excitation energy on fission can be investigated. Experiments were carried out at the JAEA tandem facility in Tokai, Japan. We studied reactions using the O beam (
9MeV/u) and several actinide target nuclei such as
Th,
U,
Np,
Cm. Ejectile nuclei and thus the transfer channels were identified by a newly developed silicon
E-E detectors. The produced nuclei in one experiment reached more than fifteen. Fission fragment mass distributions (FFMDs) were measured for each isotopes. Measured FFMDs are reproduced by a calculation based on the fluctuation-dissipation model (Langevin-type calculation), where effects of multi-chance fission were included. We also started to measure the prompt neutrons accompanied by fission.
西尾 勝久; 廣瀬 健太郎; Lguillon, R.*; 牧井 宏之; Orlandi, R.; 塚田 和明; Smallcombe, J.*; 千葉 敏*; 有友 嘉浩*; 田中 翔也*; et al.
EPJ Web of Conferences, 146, p.04009_1 - 04009_6, 2017/09
被引用回数:3 パーセンタイル:83.66(Nuclear Science & Technology)The objective of this work is to extend fission data for actinide nuclei not investigated so far in order to understand the fission mechanism, especially for neutron-rich nuclei. Multi-nucleon transfer reactions were used to populate the compound nuclei which cannot be accessed by particle capture or fusion reactions. The experiment was carried out at the tandem facility of Japan Atomic Energy Agency. In the multi-nucleon transfer reactions using O beam, a wide variety of nuclei around a target nucleus was produced. By identifying transfer channels, fission data of nuclei more than fifteen compound nuclei were generated in one experiment. Another feature of transfer reaction is that the excitation energies of a compound nucleus can be populated continuously from the ground state up to several tens MeV, allowing us to study the excitation energy dependence of fission properties. From the excitation function of fission probabilities, fission-barrier heights of neutron-rich actinide nuclei were obtained. Experiments were carried out in the reactions of
O +
U,
Th,
Cm,
Np. The obtained fission fragment mass distributions were reproduced by a model calculation based on a fluctuation dissipation model.
Lguillon, R.; 西尾 勝久; 廣瀬 健太郎; 牧井 宏之; 西中 一朗*; Orlandi, R.; 塚田 和明; Smallcombe, J.*; 千葉 敏*; 有友 嘉浩*; et al.
Physics Letters B, 761, p.125 - 130, 2016/10
被引用回数:45 パーセンタイル:92.51(Astronomy & Astrophysics)It is shown that the multinucleon transfer reactions is a powerful tool to study fission of exotic neutron-rich actinide nuclei, which cannot be accessed by particle-capture or heavy-ion fusion reactions. In this work, multinucleon transfer channels of the O +
Th reaction are used to study fission of fourteen nuclei
Th,
Pa, and
U. Identification of fissioning nuclei and of their excitation energy is performed on an event-by-event basis, through the measurement of outgoing ejectile particle in coincidence with fission fragments. Fission fragment mass distributions are measured for each transfer channel, in selected bins of excitation energy. In particular, the mass distributions of
Th and
Pa are measured for the first time. Predominantly asymmetric fission is observed at low excitation energies for all studied cases, with a gradual increase of the symmetric mode towards higher excitation energy. The experimental distributions are found to be in general agreement with predictions of the fluctuation-dissipation model.
西尾 勝久; 廣瀬 健太郎; Lguillon, R.; Orlandi, R.; 西中 一朗; Smallcombe, J.*; 千葉 敏; 荒木 祥平*; 渡辺 幸信*; 立澤 遼太郎*; et al.
no journal, ,
A recent development of fission study using multi-nucleon transfer reaction at the JAEA tandem facility will be presented. Using multi-nucleon transfer reactions, a wide variety of nuclei around a target nucleus is produced. By identifying transfer channels, fission data of several compound nuclei can be studied in one experiment. Another feature of transfer reaction is that excitation energy of a compound nucleus can be populated widely from the ground state up to several tens MeV, allowing us to study the excitation energy dependence of fission properties. The experiments were carried out in the reactions of O +
U,
Th,
Cm. Results for fission fragment mass distributions and their excitation energy dependence are compared with a model calculation based on a fluctuation dissipation model. Also, experimental data of prompt neutron multiplicity in fission and angular distribution of fission fragments will be discussed.
牧井 宏之; 西尾 勝久; 廣瀬 健太郎; Orlandi, R.; Yan, S. Q.*; Lguillon, R.; Smallcombe, J.*; Vermeulen, M. J.; 西中 一朗*; 塚田 和明; et al.
no journal, ,
原子力機構タンデム加速器施設で進行中の、中性子反応核データを間接的に導出する代理反応の研究について紹介する。我々は重イオン核子移行反応で生成された複合核を同定するためのシリコンE-E検出器、核分裂片を検出するための多芯線比例計数管(MWPC)、複合核からの
線を観測するためのコンプトン抑止型LaBr
(Ce)シンチレータ、及び核分裂即発中性子を検出するための液体シンチレータから構成された測定装置の開発を行ってきた。得られた結果のうち、代理反応法で導出した核分裂断面積, 中性子捕獲断面積について議論する。
廣瀬 健太郎; 西尾 勝久; 田中 翔也*; Leguillon, R.*; 牧井 宏之; 西中 一朗*; Orlandi, R.; 塚田 和明; Smallcombe, J.*; Vermeulen, M. J.*; et al.
no journal, ,
The multi-nucleon transfer reaction is very useful way to populate a multitude of nuclides in a wide excitation energy range. We have developed a measurement system at the JAEA tandem accelerator facility to obtain fission observables such as fission-fragment mass distributions (FFMD), prompt fission neutron multiplicities and so on. By identifying the ejectile, the initial compound nucleus is also identified. At high excitation energies, fission of nuclides produced via neutron emission from the initial compound nucleus also contribute to FFMD. In the present study, effects of the multi-chance fission on FFMDs were successfully separated by a combination of a systematic data set obtained from experiments using O beams and actinide targets and a dynamical fission calculation based on the fluctuation-dissipation model.
洲嵜 ふみ; 西尾 勝久; 牧井 宏之; 廣瀬 健太郎; Orlandi, R.; Smallcombe, J.
no journal, ,
Multinucleon transfer (MNT) reaction has attracted attention in the fields of nucleosynthesis and the production of superheavy elements because they can produce nuclei with a large neutron number. To produce desired nuclei efficiently and investigate their nuclear properties, it is necessary to determine the optimal beam and target combination and reaction energy, as well as detection angle. The objective of this study is to measure ER cross sections by changing various experimental conditions in order to establish a reliable theoretical model. We have started a program to study MNT reaction using the JAEA Recoil Mass Separator (JAEA-RMS). In contrast to kinematic separators dedicated for fusion reaction, the RMS is advantageous as it can rotate around the target chamber, essential for the study of MNT reactions. As a first attempt, we performed the experiment in the reaction of Si +
Bi. The production rate as a function of recoil angle, recoil energy (thus excitation energy), and incident beam-energy dependence were studied. The alpha-decay of the implanted ERs in the focal plane Si detector was observed online. The result is the first to realize the decay measurement in correlated with ERs, produce in the MNT reaction at a finite angle.
Smallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*; Ali, F. A.*; Andreoiu, C.*; Ansari, S.*; Ball, G. C.*; Barton, C. J.*; Bhattacharjee, S. S.*; et al.
no journal, ,
The phenomenon of shape coexistence is prevalent in the Z34 region, with isotopes of neutron-deficient even Ge, Se and Kr each exhibiting the characteristic low-lying coexisting 0+ bands which display quadrupole deformation different to that of the ground states. In the selenium isotopes,
Se seem to show a prolate ground structure with shape coexisting oblate excitation, while in
Se the oblate structure appears to have become the ground state. The exact nature of the low-lying structure
Se and any shape coexistence remains uncertain. Combining the Spectrometer for Internal Conversion Electrons (SPICE) with the TIGRESS HPGe Array, a full electron and gamma-ray experimental study of
Se,
Se was undertaken at the TRIUMF ISAC-II facility to unveil the low-lying structure of these nuclei. Details of the device and experiment will be presented, alongside the experimental results and possible structural interpretations for both isotopes.
Smallcombe, J.; Garnsworthy, A. B.*; Korten, W.*; Singh, P.*
no journal, ,
The phenomenon of shape coexistence is prevalent in the Z~34 region, with isotopes of neutron-deficient even Ge, Se and Kr each exhibiting the characteristic low-lying coexisting 0 bands which display quadrupole deformation different to that of the ground states. In the selenium isotopes,
Se seem to show a prolate ground structure with shape coexisting oblate excitation, while in
Se the oblate structure appears to have become the ground state. The exact nature of the low-lying structure
Se and any shape coexistence remains uncertain. Combining the Spectrometer for Internal Conversion Electrons (SPICE) with the TIGRESS HPGe Array, a full electron and gamma-ray experimental study of
Se was undertaken at the TRIUMF ISAC-II facility to unveil the low-lying structure of these nuclei. Details of the device and experiment will be presented, alongside the experimental results and possible structural interpretations for both isotopes.
Smallcombe, J.
no journal, ,
In the Z=34 region of the atomic chart a pattern of shape coexistence has been observed, with oblate and prolate bands apparently coexisting and switching order as neutron number changes. With recent spectroscopic developments the question of where such an inversion occurs has been drawn into question. Following a detailed electron and gamma ray spectroscopic study of 70Se previous theoretical descriptions of the nucleus have been invalidated and a new picture of the region has emerged.
西尾 勝久; 岩本 修; 牧井 宏之; 廣瀬 健太郎; Orlandi, R.; 洲嵜 ふみ; 塚田 和明; 浅井 雅人; Smallcombe, J.
no journal, ,
長寿命マイナーアクチノイド(MA)原子核を核変換する加速器駆動炉など次世代の原子炉システムを設計するためには高エネルギーまでの中性子入射断面積が必要である。本発表では、実験データがほとんどない非弾性散乱断面積に加え、核分裂断面積、捕獲断面積、(n,2n)断面積を同時に測定する技術開発の計画を示す。
Smallcombe, J.
no journal, ,
Recent developments in nuclear physics have elucidated exotic nuclear structure such as new magic numbers and exotic clustering. Even near stable nuclei, state-of-the-art theories provide new interpretations for well-known nuclear-structure problems like the nature of the side bands. To establish such an interesting scenario, direct reactions play a crucial role as a unique tool to access the characteristics of those states. The importance of direct reactions is becoming more evident in the study of exotic nuclei, which can only be accessed by few available methods. Hence it is a good time for specialists in nuclear structure and nuclear reactions to get together and to consider future collaboration schemes.
Smallcombe, J.
no journal, ,
In the Z=34 region of the atomic chart a pattern of shape coexistence has been observed, with oblate and prolate bands apparently coexisting and switching order as neutron number changes. With recent spectroscopic developments the question of where such an inversion occurs has been drawn into question. Following a detailed electron and gamma ray spectroscopic study of Se previous theoretical descriptions of the nucleus have been invalidated and a new picture of the region has emerged.