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長住 達; 松中 一朗*; 藤本 望*; 石井 俊晃; 石塚 悦男

JAEA-Technology 2020-003, 13 Pages, 2020/05




Modeling the processes of hydrogen isotopes interactions with solid surfaces

Chikhray, Y.*; Askerbekov, S.*; Kenzhin, Y.*; Gordienko, Y.*; 石塚 悦男

Fusion Science and Technology, 76(4), p.494 - 502, 2020/05

 被引用回数:0 パーセンタイル:100(Nuclear Science & Technology)

The investigation of the mechanisms and dynamics of hydrogen isotopic interaction with solid surfaces (metals, ceramics, graphites, eutectics) in temperature and pressure ranges is important not only for the correct prediction of each isotope's evolution but also for substantiation of the safe operation of hydrogen-facing structural materials. The interaction of the hydrogen isotopes mix with the surface of solid metal or liquid eutectics is a complicated multistage H-D-T-O-solid interacting process depending on material property, environment, and the solid's surface parameters. To better understand the mechanisms of hydrogen isotopes interchange at a solid surface and to identify the limiting stages in the sorption-desorption processes, a reactor experiment of neutron irradiation was conducted with lithium-containing eutectics as tritium-generating media under the external flow of hydrogen. This work presents the model and results of its application to fitting the experimental results of tritium yield from the lithium-lead eutectics Pb$$_{83}$$Li$$_{17}$$under thermal neutrons irradiation at the IVG.1M reactor in Kazakhstan. The elaborated model and the approach used were also applied to the simulation of high temperature gas cooled reactor graphite corrosion in water vapors.


Promising neutron irradiation applications at the high temperature engineering test reactor

Ho, H. Q.; 本多 友貴*; 濱本 真平; 石井 俊晃; 高田 昌二; 藤本 望*; 石塚 悦男

Journal of Nuclear Engineering and Radiation Science, 6(2), p.021902_1 - 021902_6, 2020/04

High temperature engineering test reactor (HTTR), a prismatic type of the HTGR, has been constructed to establish and upgrade the basic technologies for the HTGRs. Many irradiation regions are reserved in the HTTR to be served as a potential tool for an irradiation test reactor in order to promote innovative basic researches such as materials, fusion reactor technology, and radiation chemistry and so on. This study shows the overview of some possible irradiation applications at the HTTRs including neutron transmutation doping silicon (NTD-Si) and iodine-125 ($$^{125}$$I) productions. The HTTR has possibility to produce about 40 tons of doped Si-particles per year for fabrication of spherical silicon solar cell. Besides, the HTTR could also produce about 1.8$$times$$10$$^{5}$$ GBq/year of $$^{125}$$I isotope, comparing to 3.0$$times$$10$$^{3}$$ GBq of total $$^{125}$$I supplied in Japan in 2016.


Feasibility study of tritium recoil barrier for neutron reflectors

石塚 悦男; 坂本 直樹*

Physical Sciences and Technology, 6(2), p.60 - 63, 2019/12



Conceptual design of direct $$^{rm 99m}$$Tc production facility at the high temperature engineering test reactor

Ho, H. Q.; 石田 大樹*; 濱本 真平; 石井 俊晃; 藤本 望*; 高木 直行*; 石塚 悦男

Nuclear Engineering and Design, 352, p.110174_1 - 110174_7, 2019/10

 被引用回数:0 パーセンタイル:100(Nuclear Science & Technology)

This study proposed a conceptual design of direct $$^{rm 99m}$$Tc production facility from a natural MoO$$_{3}$$ target at the high temperature engineering test reactor (HTTR). $$^{rm 99m}$$Tc is produced by a beta decay of $$^{99}$$Mo, which is formed via the $$^{98}$$Mo(n,$$gamma$$)$$^{99}$$Mo reaction. $$^{rm 99m}$$Tc is then extracted from the MoO$$_{3}$$ target by sublimation method to take advantage of the high temperature of the HTTR core. The foremost advantage of this concept is that the MoO$$_{3}$$ target is heated up inside the reactor without pulling out for external electric heating, and as a result, $$^{rm 99m}$$Tc could be extracted directly during irradiation. With 1 kg of MoO$$_{3}$$ target, the HTTR could produce about 6.8$$times$$10$$^{8}$$ MBq of $$^{rm 99m}$$Tc activity in comparison with 3.0$$times$$10$$^{8}$$ MBq of total $$^{rm 99m}$$Tc supplied in Japan in 2017.


Reactor physics experiment in graphite moderation system for HTGR, 1

深谷 裕司; 中川 繁昭; 後藤 実; 石塚 悦男; 川上 悟; 上坂 貴洋; 守田 圭介; 佐野 忠史*

KURNS Progress Report 2018, P. 148, 2019/08



2018年度夏期休暇実習報告; HTTR炉心を用いた原子力電池に関する予備的検討; 核設計のための予備検討

石塚 悦男; 松中 一朗*; 石田 大樹*; Ho, H. Q.; 石井 俊晃; 濱本 真平; 高松 邦吉; Kenzhina, I.*; Chikhray, Y.*; 近藤 篤*; et al.

JAEA-Technology 2019-008, 12 Pages, 2019/07




Calculation of tritium release from driver fuels into primary coolant of research reactors

Ho, H. Q.; 石塚 悦男

Physical Sciences and Technology, 5(2), p.53 - 56, 2019/00




石塚 悦男; Kenzhina, I.*; 奥村 啓介; Ho, H. Q.; 竹本 紀之; Chikhray, Y.*

JAEA-Technology 2018-010, 33 Pages, 2018/11




Feasibility study of large-scale production of iodine-125 at the high temperature engineering test reactor

Ho, H. Q.; 本多 友貴*; 濱本 真平; 石井 俊晃; 藤本 望*; 石塚 悦男

Applied Radiation and Isotopes, 140, p.209 - 214, 2018/10

 被引用回数:2 パーセンタイル:48.87(Chemistry, Inorganic & Nuclear)

The feasibility of a large-scale iodine-125 production from natural xenon gas at high-temperature gas-cooled reactors was investigated. A high-temperature engineering test reactor, which is located in Japan, was used as a reference HTGR reactor in this study. First, a computer code based on a Runge-Kutta method was developed to calculate the quantities of isotopes arising from the neutron irradiation of natural xenon gas target. This code was verified with a good agreement with a reference result. Next, optimization of irradiation planning was carried out. As results, with 4 days of irradiation and 8 days of decay, the $$^{125}$$I production could be maximized and the $$^{126}$$I contamination was within an acceptable level. The preliminary design of irradiation channels at the HTTR was also optimized. The case with 3 irradiation channels and 20-cm diameter was determined as the optimal design, which could produce approximately 180,000 GBq per year of $$^{125}$$I production.


Feasibility study of new applications at the high-temperature gas-cooled reactor

Ho, H. Q.; 本多 友貴*; 濱本 真平; 石井 俊晃; 高田 昌二; 藤本 望*; 石塚 悦男

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 6 Pages, 2018/10

Besides the electricity generation and hydrogen production, HTGRs have many advantages for thermal neutron irradiation applications such as stable operation in longterm, large space available for irradiation target, and high thermal neutron economy. This study summarized the feasibility of new irradiation applications at the HTGRs including neutron transmutation doping silicon and I-125 productions. The HTTR located in Japan was used as a reference HTGR in this study. Calculation results show that HTTR could irradiate about 40 tons of doped Si particles per year for fabrication of spherical silicon solar cell. Besides, the HTTR could also produce about 1.8x105 GBq in a year of I-125, comparing to 3.0x103 GBq of total I-125 supplied in Japan in 2016.


Study on source of radioactive material in primary coolant of HTTR

石井 俊晃; 島崎 洋祐; 小野 正人; 藤原 佑輔; 石塚 悦男; 濱本 真平

Proceedings of 9th International Topical Meeting on High Temperature Reactor Technology (HTR 2018) (USB Flash Drive), 3 Pages, 2018/10

In the primary cooling system of the High-Temperature Engineering Test Reactor, the highest dose rate was observed at the Helium Gas Circulator filter areas. To find the origin of the radioactive material, the radiation dose rates, and $$gamma$$ ray spectrums were measured. From these results, it is clear that the main radioactive nuclide at the filter is $$^{60}$$Co after 6 years reactor shutdown, and the in-core materials are a low possibility as the candidates of radioactive materials. It is also clear that the mixtures of materials, the contained low-level impurities and other new candidate materials must be considered.


Evaluation of tritium release curve in primary coolant of research reactors

石塚 悦男; Kenzhina, I. E.*

Physical Sciences and Technology, 4(1), p.27 - 33, 2018/06



Proposal of a neutron transmutation doping facility for n-type spherical silicon solar cell at high-temperature engineering test reactor

Ho, H. Q.; 本多 友貴; 元山 瑞樹*; 濱本 真平; 石井 俊晃; 石塚 悦男

Applied Radiation and Isotopes, 135, p.12 - 18, 2018/05

 被引用回数:6 パーセンタイル:16.36(Chemistry, Inorganic & Nuclear)

The p-type spherical silicon solar cell is a candidate for future solar energy with low fabrication cost, however, its conversion efficiency is only about 10%. The conversion efficiency of a silicon solar cell can be increased by using n-type silicon semiconductor as a substrate. This study proposed a new method of neutron transmutation doping silicon (NTD-Si) for producing the n-type spherical solar cell, in which the Si-particles are irradiated directly instead of the cylinder Si-ingot as in the conventional NTD-Si. By using a screw, an identical resistivity could be achieved for the Si-particles without a complicated procedure as in the NTD with Si-ingot. Also, the reactivity and neutron flux swing could be kept to a minimum because of the continuous irradiation of the Si-particles. A high temperature engineering test reactor (HTTR), which is located in Japan, was used as a reference reactor in this study. Neutronic calculations showed that the HTTR has a capability to produce about 40 ton of 10 $$Omega$$ cm resistivity Si-particles for fabrication of the n-type spherical solar cell.


HTTRを用いた崩壊熱最適評価手法の適用性確認試験(非核加熱試験); 原子炉の残留熱除熱特性評価モデルの検証

本多 友貴; 稲葉 良知; 中川 繁昭; 山崎 和則; 小林 正一; 青野 哲也; 柴田 大受; 石塚 悦男

JAEA-Technology 2017-013, 20 Pages, 2017/06





篠原 正憲; 石塚 悦男; 島崎 洋祐; 澤畑 洋明

JAEA-Technology 2016-033, 65 Pages, 2017/01





石塚 悦男; Kenzhina, I. E.*; 奥村 啓介; 竹本 紀之; Chikhray, Y.*

JAEA-Technology 2016-022, 35 Pages, 2016/10


試験研究炉の一次冷却水中へのトリチウム放出機構解明の一環として、ベリリウム炉心構成材からの反跳トリチウム放出率を評価するためPHITSコードを用いた場合の計算方法について検討した。この結果、線源に中性子またはトリトンを用いた場合、両者とも反跳トリチウム放出率は同程となったが、トリトン線源の計算速度が2桁程度速いことが明らかとなった。また、トリトン線源を用いて反跳トリチウム放出率を有効数字2桁の精度で求めるためには、単位体積あたりのヒストリー数が2$$times$$10$$^{4}$$ (cm$$^{-3}$$)程度になるまで計算すれば良いことが明らかとなった。更に、トリトン線源を用いてベリリウム炉心構成材の形状と反跳トリチウム放出率の関係を調べたところ、反跳トリチウム放出率はベリリウムの体積当たりの表面積に対して線形となったが、従来の式を使って求めた値の約半分となった。


Improvement of exchanging method of neutron startup source of high temperature engineering test reactor

澤畑 洋明; 島崎 洋祐; 石塚 悦男; 山崎 和則; 柳田 佳徳; 藤原 佑輔; 高田 昌二; 篠崎 正幸; 濱本 真平; 栃尾 大輔

Proceedings of 24th International Conference on Nuclear Engineering (ICONE-24) (DVD-ROM), 8 Pages, 2016/06



JMTR及び関連施設を活用した実践型オンサイト研修; 2014年度

江口 祥平; 竹本 紀之; 谷本 政隆; 久保 彩子; 石塚 悦男; 中村 仁一; 伊藤 治彦

JAEA-Review 2015-005, 38 Pages, 2015/06


照射試験炉センターでは、発電用原子炉の導入を検討しているアジア諸国をはじめとした海外の原子力人材育成及び将来のJMTRの照射利用拡大を目的とし、海外の若手研究者・技術者を対象に、JMTR等の研究基盤施設を活用した実践的な研修を平成23年度から実施している。一方、国内の若手研究者・技術者を対象とした同様の研修は、平成22年度から実施している。平成26年度は、これらの研修を統合し、国内外の若手研究者・技術者を対象に3週間の研修を 実施した。研修には7か国から19名が参加し、原子力研究の概要、原子力エネルギーの現状と 開発、照射試験研究に係る施設及び技術、原子炉の核特性、原子炉施設の安全管理及び運転管理等について学んだ。また、研修の最後にはエネルギーミックスの現状と将来を題材として参加者間の討論を行い、活発な意見交換がなされた。本報告は、平成26年度に実施した研修の内容と結果についてまとめたものである。


試験研究炉における一次冷却水中へのトリチウム放出源に関する検討; JMTR, JRR-3M及びJRR-4運転データから評価したトリチウム放出率

石塚 悦男; 本橋 純; 塙 善雄; 米田 政夫; 綿引 俊介; Mukanova, A.*; Kenzhina, I. E.*; Chikhray, Y.*

JAEA-Technology 2014-025, 77 Pages, 2014/08


JMTRやJRR-3では、原子炉の運転に伴って一次冷却水中のトリチウム濃度が高くなることが明らかになっている。本報告書では、これらのトリチウム放出源を明らかにするため、JMTR, JRR-3M及びJRR-4の各運転サイクルにおけるトリチウム放出率を実測値から評価した。この結果、炉心構成材にベリリウムを使用していないJRR-4のトリチウム放出率は8Bq/Wd以下であり、運転に伴うトリチウム濃度の上昇は認められなかった。これに対して、炉心構成材にベリリウムを使用しているJMTR及びJRR-3Mでは、トリチウム放出率がそれぞれ約60$$sim$$140及び約10$$sim$$95Bq/Wdで運転に伴ってトリチウム濃度が上昇すること、ベリリウム製炉心構成材を新規製作品と交換するとトリチウム放出率が一時的に低下し、その後、運転サイクルとともに増加する傾向が見られた。

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