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Journal Articles

Investigation on multi-dimensional short-term behaviour through benchmark analysis of a large-volume sodium combustion experiment

Sonehara, Masateru; Okano, Yasushi; Uchibori, Akihiro; Oki, Hiroshi*

Journal of Nuclear Science and Technology, 62(5), p.403 - 414, 2025/05

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

For sodium-cooled fast reactors, understanding sodium combustion behaviour is crucial for managing sodium leakage accidents. In this study, we perform benchmark analyses of the Sandia National Laboratories (SNL) T3 experiment using the multi-dimensional thermal hydraulic code AQUA-SF. Conducted in an enclosed space with a large vessel volume of 100 m$$^3$$ and a sodium mass flow rate of 1 kg/s, the experiment highlighted the multi-dimensional effects of local temperature increase shortly after sodium injection. This study aims to extend the capabilities of AQUA-SF by focusing on the simulation of these multi-dimensional temperature variations, in particular the formation of high temperature regions at the bottom of the vessel. The proposed models include the temporary stopping of sodium droplet ignition and spray combustion of sodium splash on the floor. Furthermore, it has been shown that additional heat source near the floor is essential to enhance the reproduction of the high temperature region at the bottom. Therefore, case studies including sensitivity analyses of spray cone angle and prolonged combustion of droplets on the floor are conducted. This comprehensive approach provides valuable insights into the dynamics of sodium combustion and safety measures in sodium-cooled fast reactors.

Journal Articles

Adsorption isotherm and kinetics of diffusion of water accumulated between polypropylene thin film and Si substrate; Neutron reflectivity investigation

Miyazaki, Tsukasa*; Miyata, Noboru*; Arima-Osonoi, Hiroshi*; Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Takenaka, Mikihito*; Nakanishi, Yohei*; Shibata, Motoki*; Aoki, Hiroyuki; Yamada, Norifumi*; et al.

Colloids and Surfaces A; Physicochemical and Engineering Aspects, 701, p.134928_1 - 134928_8, 2024/11

 Times Cited Count:0 Percentile:0.00(Chemistry, Physical)

JAEA Reports

Development of the versatile reactor analysis code system, MARBLE3

Yokoyama, Kenji; Hazama, Taira; Taninaka, Hiroshi; Oki, Shigeo

JAEA-Data/Code 2024-007, 41 Pages, 2024/10

JAEA-Data-Code-2024-007.pdf:1.1MB

The third version of the versatile reactor analysis code system, MARBLE3, has been developed. In the development of the former version of MARBLE, object-oriented scripting language Python (Python2) had been used and then the latest version of Python (Python3) was released. However, due to its backward incompatibility, MARBLE no longer worked with Python3. For this reason, MARBLE3 has been fully modified and maintained to work with Python3. In MARBLE3, newly developed analysis codes and newly proposed calculation methods were incorporated, and the user interface was extended and solvers were reimplemented for maintainability, extensibility, and flexibility. In MARBLE3, the three-dimensional hexagonal/triangular transport code MINISTRI Ver.7 (MINISTRI7) and the three-dimensional hexagonal/triangular diffusion code D-MINISTRI are available as the new analysis codes. These codes can be used in the neutronics analysis system SCHEME and the fast reactor burnup analysis system OPRHEUS, which are the subsystems of MARBLE. In addition, the user interface of CBG, a core analysis system embedded in MARBLE, was extended so that the diffusion and transport calculation solvers for the 2-dimensional RZ system of CBG can be used on SCHEME. On the other hand, MARBLE3 has extended the functionality of the burnup calculation solver so that it can use the numerical methods proposed in the papers on the improvement of the Chebyshev rational function approximation method and the minimax polynomial approximation method. From the viewpoint of maintainability, the point reactor kinetics solver POINTKINETICS, which was introduced in MARBLE2, has been newly reworked as the KINETICS solver in MARBLE3.

Journal Articles

Influence of MC carbides on pitting corrosion resistance of weld metal in austenitic stainless steels

Kadoi, Kota*; Kanno, Yudai*; Aoki, So; Inoue, Hiroshige*

ISIJ International, 64(9), p.1450 - 1456, 2024/07

 Times Cited Count:0 Percentile:0.00(Metallurgy & Metallurgical Engineering)

The influence of the chemical composition on the pitting corrosion in the weld metal of austenitic stainless steel were investigated. The specimens containing higher content of chromium and molybdenum showed the lower the reactivation rate. The addition of titanium drastically deteriorated the pitting corrosion resistance. The chromium depleted region was formed near the carbide such as M$$_{23}$$C$$_{6}$$ and TiC. Besides, TiC phase which formed during solidification acted as nucleation sites for M$$_{23}$$C$$_{6}$$ precipitation. The depleted region caused by chromium diffusion because of the M$$_{23}$$C$$_{6}$$ precipitation, induced to deteriorate the pitting corrosion resistance.

Journal Articles

Model integration of the ex-vessel modules for the SFR safety analysis code SPECTRA

Aoyagi, Mitsuhiro; Makino, Toru*; Oki, Hiroshi*; Uchibori, Akihiro; Okano, Yasushi

Mechanical Engineering Journal (Internet), 11(2), p.23-00459_1 - 23-00459_12, 2024/04

Journal Articles

Development of a D$$_2$$O/H$$_2$$O vapor generator for contrast-variation neutron scattering

Arima-Osonoi, Hiroshi*; Takata, Shinichi; Kasai, Satoshi*; Ouchi, Keiichi*; Morikawa, Toshiaki*; Miyata, Noboru*; Miyazaki, Tsukasa*; Aoki, Hiroyuki; Iwase, Hiroki*; Hiroi, Kosuke; et al.

Journal of Applied Crystallography, 56(6), p.1802 - 1812, 2023/12

 Times Cited Count:6 Percentile:77.05(Chemistry, Multidisciplinary)

Journal Articles

Transient analyses of hydraulic head in the fault slip experiments in fracture zones of Shionohira and Kuruma Faults

Wakahama, Hiroshi*; Nojo, Haruka*; Aoki, Kazuhiro; Imai, Hirotaro; Guglielmi, Y.*; Cook, P.*; Soom, F.*

Oyo Chishitsu, 64(5), p.236 - 254, 2023/12

Upon the Hamadori earthquake (Mw 6.7) of 11 April 2011, coseismic surface deformation of 14 km running NNW to SSE in southeast Fukushima Prefecture occurred and was newly named the Shionohira Fault. However, no surface deformation was observed along the Kuruma Fault which is a southern extension of the Shionohira Fault. Fault injection tests using SIMFIP method at the Shionohira site on the former active segment and the Minakamikita site on the latter inactive segment were conducted to evaluate the activity of the two faults. Based on hydraulic responses to water injection into the fault rupture zone in the monitoring boreholes at the two sites, hydraulic properties of the area across the fault zone were estimated using the GRF model (Barker, 1988). The results obtained on hydraulic conductivity, specific storage and flow dimension were consistent with those in the domestic and international literature. The hydraulic conductivity and specific storage were larger in Shionohira than in Minakamikita. The flow dimension of Shionohira was three-dimensional, while that of Minakamikita was found to be a two-dimensional fractional flow. In addition, it is understood that the volumetric expansion occurs in the former site in the triaxial direction and the latter in the uniaxial with the comparison between the uniaxial expansion coefficient calculated from the results of SIMFIP displacement measurements and the specific storage in the hydraulic analysis. The difference in the hydraulic parameters between the two sites corresponded to the difference in the spatial development of fractures considered to be the "water passway," indicating the possibility of a correlation between the parameters and the different possible causes for fault activity at the two sites.

Journal Articles

Impact of the Ce$$4f$$ states in the electronic structure of the intermediate-valence superconductor CeIr$$_3$$

Fujimori, Shinichi; Kawasaki, Ikuto; Takeda, Yukiharu; Yamagami, Hiroshi; Sasabe, Norimasa*; Sato, Yoshiki*; Shimizu, Yusei*; Nakamura, Ai*; Maruya, A.*; Homma, Yoshiya*; et al.

Electronic Structure (Internet), 5(4), p.045009_1 - 045009_7, 2023/11

Journal Articles

Development of the ex-vessel modules for the integrated SFR safety analysis code SPECTRA

Aoyagi, Mitsuhiro; Makino, Toru*; Oki, Hiroshi*; Uchibori, Akihiro; Okano, Yasushi

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 7 Pages, 2023/05

JAEA Reports

On-site training using JMTR and related facilities in FY2019

Nakano, Hiroko; Nishikata, Kaori; Nagata, Hiroshi; Ide, Hiroshi; Hanakawa, Hiroki; Kusunoki, Tsuyoshi

JAEA-Review 2022-073, 23 Pages, 2023/01

JAEA-Review-2022-073.pdf:2.02MB

A practical training course using the JMTR (Japan Materials Testing Reactor) and other research infrastructures was held from July 24th to July 31st in 2019 for Asian young researchers and engineers. This course was adopted as Japan-Asia Youth Exchange Program in Science (SAKURA Exchange Program in Science) which is the project of the Japan Science and Technology Agency, and this course aims to enlarge the number of high-level nuclear researchers/engineers in Asian countries which are planning to introduce a nuclear power plant, and to promote the use of facilities in future. In this year, 12 young researchers and engineers joined the course from 6 countries. This course consists of lectures, which are related to irradiation test research, safety management of nuclear reactors, nuclear characteristics of the nuclear reactors, etc., practical training such as practice of research reactor operation using simulator and technical tour of nuclear facilities on nuclear energy. The content of this course in FY 2019 is reported in this paper.

Journal Articles

Weyl-Kondo semimetal behavior in the chiral structure phase of Ce$$_{3}$$Rh$$_{4}$$Sn$$_{13}$$

Iwasa, Kazuaki*; Suyama, Kazuya*; Kawamura, Seiko; Nakajima, Kenji; Raymond, S.*; Steffens, P.*; Yamada, Akira*; Matsuda, Tatsuma*; Aoki, Yuji*; Kawasaki, Ikuto; et al.

Physical Review Materials (Internet), 7(1), p.014201_1 - 014201_11, 2023/01

 Times Cited Count:4 Percentile:42.21(Materials Science, Multidisciplinary)

Journal Articles

Neutron reflectivity study on the suppression of interfacial water accumulation between a polypropylene thin film and Si substrate using a silane-coupling agent

Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Miyata, Noboru*; Arima-Osonoi, Hiroshi*; Nakanishi, Yohei*; Takenaka, Mikihito*; Shibata, Motoki*; Yamada, Norifumi*; Seto, Hideki*; Aoki, Hiroyuki; et al.

Langmuir, 38(41), p.12457 - 12465, 2022/10

 Times Cited Count:2 Percentile:13.50(Chemistry, Multidisciplinary)

Journal Articles

Radiation exposure to the lens of the eye for Japanese nuclear power plant workers

Yokoyama, Sumi*; Tatsuzaki, Hideo*; Tanimura, Yoshihiko; Yoshitomi, Hiroshi; Hirao, Shigekazu*; Aoki, Katsunori; Tachiki, Shuichi*; Ezaki, Iwao*; Hoshi, Katsuya; Tsujimura, Norio

Journal of Radiological Protection, 42(3), p.031504_1 - 031504_17, 2022/09

 Times Cited Count:2 Percentile:29.47(Environmental Sciences)

In Japan, the radiation-dose limit for the lens of the eye was revised in April 2021. Consequently, for workers, the numerical values of the equivalent dose to the lens of the eye are equal to those of the effective dose. Radiation workers, radiation safety officers and licensees must comply with regulations related to radiation protection and optimize protection. The new guidelines on dose monitoring of the lens of the eye developed by the Japan Health Physics Society recommend for the dose to be estimated near the eye for accurate estimation, when the dose to the lens approaches or exceeds the management criteria. However, there is limited information regarding the non-uniform exposure of nuclear power plant workers. In this study, the dose equivalents of high-dose-rate workplaces and the personal doses of 88 workers were estimated at four Japanese commercial nuclear power plant sites (RWR: 3 units and BWR: 3 units) and the dose to the lens of the eye and the exposure situations of the workers were analyzed.

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

JAEA Reports

Development of the unified cross-section set ADJ2017R

Yokoyama, Kenji; Maruyama, Shuhei; Taninaka, Hiroshi; Oki, Shigeo

JAEA-Data/Code 2021-019, 115 Pages, 2022/03

JAEA-Data-Code-2021-019.pdf:6.21MB
JAEA-Data-Code-2021-019-appendix(CD-ROM).zip:435.94MB

In JAEA, several versions of unified cross-section set for fast reactors have been developed so far; we have developed a new unified cross-section set ADJ2017R, which is an improved version of the unified cross-section setADJ2017 for fast reactors. The unified cross-section set is used for reflecting information of C/E values (analysis / experiment values) obtained by integral experiment analyses in reactor core design via the cross-section adjustment methodology; the values are stored in the standard database for FBR core design. In the methodology, the cross-section set is adjusted by integrating the information such as uncertainty (covariance) of nuclear data, uncertainty of integral experiment / analysis, sensitivity of integral experiment with respect to nuclear data. ADJ2017R basically has the same performance as ADJ2017, but we conducted an additional investigation on ADJ2017 and revised the following two points. The first is to unify the evaluation method of the correlation coefficient of uncertainty caused by experiments (hereinafter referred to as the experimental correlation coefficient). Because it was found that the common uncertainty used in the evaluation of the experimental correlation coefficient was evaluated by two different methods, the experimental correlation coefficients were revised for all experimental data, and the evaluation method was unified. The second is the review of the integral experiment data used for the cross-section adjustment calculation. It was found that one of the experimental values of composition ratio after irradiation of the Am-243 sample has a problem in uncertainty evaluation because its experimental uncertainty is extremely small compared to the others. The cross-section adjustment calculation was, therefore, redone by excluding the experimental value. In the creation of ADJ2017, a total of 719 data sets were analyzed and evaluated, and eventually adopted 620 integral experimental data sets. In contrast, a total of 61

JAEA Reports

Study on the evaluation method to determine the radioactivity concentration in radioactive waste on Oarai Research and Development Institute (FY2020)

Asakura, Kazuki; Shimomura, Yusuke; Donomae, Yasushi; Abe, Kazuyuki; Kitamura, Ryoichi; Miyakoshi, Hiroyuki; Takamatsu, Misao; Sakamoto, Naoki; Isozaki, Ryosuke; Onishi, Takashi; et al.

JAEA-Review 2021-020, 42 Pages, 2021/10

JAEA-Review-2021-020.pdf:2.95MB

The disposal of radioactive waste from the research facility need to calculate from the radioactivity concentration that based on variously nuclear fuels and materials. In Japan Atomic Energy Agency Oarai Research and Development Institute, the study on considering disposal is being advanced among the facilities which generate radioactive waste as well as the facilities which process radioactive waste. This report summarizes a study result in FY2020 about the evaluation method to determine the radioactivity concentration in radioactive waste on Oarai Research and Development Institute.

Journal Articles

Layered structure in the crystalline adsorption layer and the leaching process of poly(vinyl alcohol) revealed by neutron reflectivity

Miyazaki, Tsukasa*; Miyata, Noboru*; Arima, Hiroshi*; Kira, Hiroshi*; Ouchi, Keiichi*; Kasai, Satoshi*; Tsumura, Yoshihiro*; Aoki, Hiroyuki

Langmuir, 37(32), p.9873 - 9882, 2021/08

 Times Cited Count:7 Percentile:35.84(Chemistry, Multidisciplinary)

JAEA Reports

Manufacture of substitutive assemblies for MONJU reactor decommissioning

Sakakibara, Hiroshi; Aoki, Nobuhiro; Muto, Masahiro; Otabe, Jun; Takahashi, Kenji*; Fujita, Naoyuki*; Hiyama, Kazuhiko*; Suzuki, Hirokazu*; Kamogawa, Toshiyuki*; Yokosuka, Toru*; et al.

JAEA-Technology 2020-020, 73 Pages, 2021/03

JAEA-Technology-2020-020.pdf:8.26MB

The decommissioning is currently in progress at the prototype fast breeder reactor Monju. Fuel assemblies will be taken out of its core for the first step of the great task. Fuel assemblies stand on their own spike plugged into a socket on the core support plate and support with adjacent assemblies through their housing pads each other, resulting in steady core structure. For this reason, some substitutive assemblies are necessary for the purpose of discharging the fuel assemblies of the core. Monju side commissioned, therefore, Plutonium Fuel Development Center to manufacture the substitutive assemblies and the Center accepted it. This report gives descriptions of design, manufacture, and shipment in regard to the substitutive assemblies.

Journal Articles

Core-level photoelectron spectroscopy study of UTe$$_{2}$$

Fujimori, Shinichi; Kawasaki, Ikuto; Takeda, Yukiharu; Yamagami, Hiroshi; Nakamura, Ai*; Homma, Yoshiya*; Aoki, Dai*

Journal of the Physical Society of Japan, 90(1), p.015002_1 - 015002_2, 2021/01

 Times Cited Count:21 Percentile:82.58(Physics, Multidisciplinary)

The valence state of $$mathrm{UTe}_2$$ was studied by core-level photoelectron spectroscopy. The main peak position of the $$mathrm{U}~4f$$ core-level spectrum of $$mathrm{UTe}_2$$ coincides with that of $$mathrm{UB}_2$$, which is anitinerant compound with a nearly $$5f^3$$ configuration. However, the main peak of $$mathrm{UTe}_2$$ is broader than that of $$mathrm{UB}_2$$, and satellite structures are observed in the higher binding energy side of the main peak, which are characteristics of mixed-valence uranium compounds. These results suggest that the $$mathrm{U}~5f$$ state in $$mathrm{UTe}_2$$ isin a mixed valence state with a dominant contribution from the itinerant$$5f^3$$ configuration.

Journal Articles

Eco-friendly carboxymethyl cellulose nanofiber hydrogels prepared via freeze cross-linking and their applications

Sekine, Yurina; Nankawa, Takuya; Yunoki, Shunji*; Sugita, Tsuyoshi; Nakagawa, Hiroshi; Yamada, Teppei*

ACS Applied Polymer Materials (Internet), 2(12), p.5482 - 5491, 2020/12

 Times Cited Count:63 Percentile:94.22(Materials Science, Multidisciplinary)

We developed a cross-linking method using freeze concentration and used it to synthesize a new type of carboxymethyl cellulose nanofiber (CMCF) hydrogel with high compressive strength ($$>$$ 80 MPa) and high compressive recoverability. The hydrogels were prepared by adding an aqueous solution of citric acid (CA) to a frozen CMCF sol and then thawing the sol. The reaction between the freeze-concentrated CMCF and CA created a rigid porous structure that reflected the ice crystal structure. Their cross-linked structure has a high stability to compressive stress. Bentonite was immobilized on a CMCF hydrogel by adding bentonite to the CMCF sol before freeze cross-linking. The CMCF-bentonite hydrogel showed high adsorptivity for chemical dyes. The physically cross-linked CMCF hydrogels are non-toxic, metal-free, and simple to prepare, and thus they may be useful as sustainable materials in various fields.

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