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-ray beam measurementsOmer, M.; Shizuma, Toshiyuki*; Koizumi, Mitsuo; Taira, Yoshitaka*; Zen, H.*; Ogaki, Hideaki*; Hajima, Ryoichi*
Radiation Physics and Chemistry, 240, p.113467_1 - 113467_8, 2026/03
Miyahara, Shinya*; Koie, Ryusuke*; Uno, Masayoshi*; Kawaguchi, Munemichi*; Sato, Rika; Seino, Hiroshi
Nuclear Engineering and Design, 446(Part A), p.114523_1 - 114523_14, 2026/01
Yoneyama, Kai; Nitta, Ayako; Tanaka, Yasuyuki; Kodaka, Noriyasu; Kikuchi, Riku; Sakano, Takuma; Furuse, Takahiro; Sato, Soichi; Sambongi, Mitsuru; Tanaka, Kosuke
JAEA-Technology 2025-008, 44 Pages, 2025/12
At the TEPCO's Fukushima Daiichi Nuclear Power Station (1F), an investigation inside the reactors has been carried out. In order to safely carry out the decommissioning work such as fuel debris retrieval and building demolition, it is important to estimate the contamination in primary containment vessel for control the decommissioning planning and the worker radiation exposure levels. Therefore, the analysis of the deposit inside the penetration for the 1F Unit 2 primary containment vessel ("X-6 penetration") was performed to clarify the components and activity. The smears from the deposit were used for the analysis. Non-destructive analysis such as gamma-ray spectrometry, X-ray Fluorescence (XRF) and Scanning Electron Microscope-Energy dispersive X-ray spectroscopy (SEM-EDX) for the smear-samples were performed to determine the gamma-nuclides and the morphology of elements in the deposit. Furthermore, in order to evaluate the nuclides and nuclide composition of the deposit in detail, the smear-samples were dissolved and the quantitative analysis of gamma-nuclides, Sr-90, alpha-nuclides in the dissolved solution were conducted. The results (non-destructive analysis and quantitative analysis) were compared with the results of samples collected at different locations in the X-6 penetration in 2020. In the gamma-ray spectrometry as non-destructive analysis where the smears were analyzed directly, Co-60, Sb-125, Cs-134, Cs-137, Eu-154, Eu-155 and Am-241 were detected. In XRF results, Fe originating from construction material was detected as a major element and small amount of U and Zr originating from the fuel and fuel cladding were also detected. In SEM-EDX results, O and Fe were found as a major element of the deposit and U particles coexisting with Fe, Si, Cr, Ni and Zr were also found. These results were consistent with the SEM-EDX results of the samples collected in 2020. In radioactivity analysis, quantitative values for gamma-nuclides (Co-60, Sb-125, Cs-134, Cs-137, Eu-154, Eu-155), Sr-90, Pu-238, Pu-239+240, Am-241, Cm-244, U-235 and U-238 were obtained. Using the results, the ratios of radioactivity based on Cs-137 and U-238 were calculated. Both sets of the ratios were compared to the calculated value of the Unit 2 fuel composition from ORIGEN.
Nakayama, Masashi; Ishii, Eiichi; Aoyagi, Kazuhei; Hayano, Akira; Murakami, Hiroaki; Ono, Hirokazu; Takeda, Masaki; Fukatsu, Yuta; Mochizuki, Akihito; Ozaki, Yusuke; et al.
JAEA-Review 2025-042, 136 Pages, 2025/12
The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant technologies for geological disposal of high-level radioactive waste through investigating the deep geological environment within the host sedimentary rocks at Horonobe-cho in Hokkaido, north Japan. In the fiscal year 2024, we continued R&D on "Study on near-field system performance in geological environment", "Demonstration of repository design options", and "Understanding of buffering behaviour of sedimentary rock to natural perturbations". These are identified as key R&D on challenges to be tackled in the Horonobe underground research plan for the fiscal year 2020 onwards. Specifically, "full-scale engineered barrier system (EBS) performance experiment" and "solute transport experiment with model testing" were carried out as part of "Study on nearfield system performance in geological environment". "Demonstration of engineering feasibility of repository technology" and "evaluation of EBS behaviour over 100
C" were addressed for "Demonstration of repository design options". The validation of a method for assessing permeability using the Ductility Index and a method for estimating the state of in-situ ground pressure from hydraulic perturbation tests were investigated as part of the study "Understanding of buffering behaviour of sedimentary rock to natural perturbations". In FY2024, we continued construction of the East Access Shaft and the Ventilation Shaft, and construction of these shafts were completed to a depth of 500 m. After the completion of the East Access Shaft, excavation of the West Access Shaft and 500 m gallery has began. As of the end of FY2024, excavation progress is as follows, the East Access Shaft and the Ventilation Shaft were 500 m depth, the West Access Shaft was 472 m depth, 500 m gallery was 112.9 m, respectively. In the Horonobe International Project (HIP), Management Board and Joint Task Meeting was held at the Horonobe URL in June 2024 to review the progress of construction of galleries and preparations of experiments. Task Meetings to review the implementation plan for in-situ testing and analysis were also held. HIP will be implemented in two phases: Phase 1 (from FY2022 to FY2024) and Phase 2 (from FY2025 to FY2028), the research results of Phase 1 were compiled in FY2024.
Collaborative Laboratories for Advanced Decommissioning Science; Tokai National Higher Education and Research System*
JAEA-Review 2025-023, 63 Pages, 2025/11
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Development and evaluation of a real-time 3D positioning embedded system combining wireless UWB and camera image analysis" conducted in FY2023. The present study aims to realize an embedded system that combines two of the latest popular technologies, "wireless UWB (Ultra Width Band)" and "multi-camera object recognition" with the goal of simple real-time 3D positioning with less than 10 cm accuracy by a human or robot for measuring air doses in nuclear reactor buildings. In this research, Gifu Univ. and National Institute of Technology, Fukushima College have developed an embedded system with camera shooting function, camera analysis function, and wireless communication function, in order to realize real-time 3D positioning based on the analysis of camera images by using these multiple devices. The Univ. of Tokyo and LocationMind Inc. will apply UWB real-time positioning technology to the inside of nuclear reactor buildings and attempt to develop technology to improve stability. Nagoya Univ. will be in charge of verifying wireless UWB stability from the hardware side by using electromagnetic wave absorbing materials. The radiation resistance evaluation will be conducted in cooperation with the JAEA and National Institute of Technology, Fukushima College.
vapor-liquid transfer model in the chemical behavior analysis code SCHERN for accident of evaporation to dryness by boiling of reprocessed high level liquid wasteYoshida, Kazuo; Hiyama, Mina*; Tamaki, Hitoshi
JAEA-Research 2025-011, 25 Pages, 2025/11
An accident of evaporation to dryness by boiling of high-level radioactive liquid waste (HLLW) is postulated as one of the severe accidents caused by the loss of cooling function at a fuel reprocessing plant. In this case, volatile radioactive materials, such as ruthenium (RuO
) are released from the tanks with water and nitric-acid mixed vapor into the atmosphere. Accurate quantitative estimation of released Ru is one of the important issues for risk assessment of those facilities. RuO
is expected to be absorbed chemically into water dissolving nitrous acid (HNO
). This behavior has been experimentally confirmed and plays an important role in the migration of Ru in the facility. A new model has been proposed as a chemical and physical absorption model based on the experimental results of the migration of RuO
into nitric acid-water mixtures. In this study, to improve the analytical performance of SCHERN, these new analytical models have been incorporated and attempted to analyze the behavior of RuO
in each phase. As a result, it has been observed a tendency that HNO
in the liquid phase increases rapidly during the late boiling phase, when RuO
release increases rapidly, and confirmed that this HNO
concentration change significantly affects the subsequent migration behavior of RuO
. These results indicate that it is essential to improve the analytical accuracy of the chemical behavior of HNO
in each phase.
Yanagisawa, Hiroshi; Motome, Yuiko
JAEA-Research 2025-010, 197 Pages, 2025/11
For understandings of nuclear criticality risks of TRIGA fuel rods and review of safety measures for handling them, nuclear criticality characteristics for infinite and finite heterogeneous lattice systems composed of the NSRR fuel rods were re-evaluated with the use of a detailed computational model for the fuel rod. The MVP version 3 code was used with the JENDL libraries including the latest version, JENDL-5, for the re-evaluation. As the criticality characteristics, variations of neutron multiplication factors of the infinite and water-reflected finite systems were examined in detail with parameters of the lattice pitch and density of moderator water. From the results of the re-evaluated criticality characteristics, the minimum critical number of fuel rods for the water-reflected hexagonal shaped lattice system was obtained to be 46.8
0.2 using the JENDL-5 library. Moreover, the attainability of criticality without the water as moderator and reflector was examined because the zirconium hydride moderator and graphite reflector are equipped with the TRIGA fuel rod. It was found that the criticality is possible to be attained by 115.7
0.6 of the number of fuel rods, which is the smaller number of fuel rods than loaded in the NSRR standard core, even though no water exists.
Be nuclear magnetic resonance in UBe
; Itinerant-localized duality and possible Fermi surface reconstruction at high magnetic fieldMatsuki, Rintaro*; Minami, Shoko*; Kotegawa, Hisashi*; Harima, Hisatomo*; Haga, Yoshinori; Yamamoto, Etsuji; Onuki, Yoshichika*; To, Hideki*
Journal of the Physical Society of Japan, 94(12), p.124702_1 - 124702_8, 2025/11
Hagiwara, Hiroki; Watanabe, Yusuke; Konishi, Hiromi*; Funaki, Hironori; Fujiwara, Kenso; Iijima, Kazuki
Applied Geochemistry, 190, p.106490_1 - 106490_10, 2025/10
Times Cited Count:0 Percentile:0.00Nakayama, Masashi; Ishii, Eiichi; Hayano, Akira; Aoyagi, Kazuhei; Murakami, Hiroaki; Ono, Hirokazu; Takeda, Masaki; Mochizuki, Akihito; Ozaki, Yusuke; Kimura, Shun; et al.
JAEA-Review 2025-027, 80 Pages, 2025/09
The Horonobe Underground Research Laboratory Project is being pursued by the Japan Atomic Energy Agency to enhance the reliability of relevant technologies for geological disposal of high-level radioactive waste through investigating the deep geological environment within the host sedimentary rocks at Horonobe Town in Hokkaido, north Japan. In the fiscal year 2025, we continue R&D on "Study on near-field system performance in geological environment" and "Demonstration of repository design options". These are identified as key R&D challenges to be tackled in the Horonobe underground research plan for the fiscal year 2020 onwards. In the "Study on near-field system performance in geological environment", we continue to obtain data from the full-scale engineered barrier system performance experiment, and work on the specifics of the full-scale engineered barrier system dismantling experiment. As for "Demonstration of repository design options", the investigation, design, and evaluation techniques are to be systemized at various scales, from the tunnel to the pit, by means of an organized set of evaluation methodologies for confinement performance at these respective scales. Preliminary borehole investigations will be conducted within a 500 m gallery, with the objectives of obtaining rock strength and rock permeability data, as well as surveying the extent of the excavation damaged zone surrounding the test tunnel via tomographic analysis. A planning study for the in-situ construction test will be conducted to investigate the construction of backfill material and watertight plugs. The volume of water inflow associated with the excavation of the 500 m gallery will be observed, and its magnitude will be compared with the range of water inflow predicted in the analysis. The test plan to determine the extent of the excavation damaged zone around the pit, which is planned to be constructed in the 500 m gallery, will be studied to determine the in-situ excavation damaged zone. In addition, the investigation and evaluation methods for the amount of water inflow from fractures and the extent of the excavation damaged zone around the pit will be organized. Concerning the construction and maintenance of the subsurface facilities, excavation of the West Access Shaft and the 500 m gallery will continue. It is anticipated that the construction of the facilities will be completed by the end of the fiscal year 2025. In addition, we continue R&D on the following three tasks in the Horonobe International Project; Task A: Solute transport experiment with model testing, Task B: Systematic integration of repository technology options, and Task C: Full-scale engineered barrier system dismantling experiment.
Yamaguchi, Yuji; Kondo, Yasuhiro; Meigo, Shinichiro; Shinozaki, Shinichi; Takayanagi, Tomohiro; Fujimori, Hiroshi*; Kawamura, Naritoshi*
Journal of Physics; Conference Series, 3094(1), p.012023_1 - 012023_5, 2025/09
The 3-GeV proton beam from the rapid cycling synchrotron (RCS) of J-PARC is transported to the spallation neutron source at Materials and Life Science Experimental Facility (MLF) by a 3-GeV RCS to Neutron facility Beam Transport (3NBT) line. Recently, the first design idea of a new proton beam transport line has been proposed for a future target station of the MLF (TS2). In the present study, proton beam transport is simulated near the TS2 target where a bending magnet and a solenoid are located for muon beam transport. The purposes are to clarify the magnetic field effects on the proton beam by the magnets and to present a method to correct each effect. Orbit deviation by the bending magnet and vertical size expansion due to profile rotation by the solenoid can be corrected by installing additional bending magnets and a solenoid with reversal magnetic field, respectively. The correction method is expected to be effective and also needs to be studied further for detail design.
Che, G.*; Tang, X.*; Liu, J.*; Lang, P.*; Fei, Y.*; Yang, X.*; Wang, Y.*; Gao, D.*; Wang, X.*; Ju, J.*; et al.
Nano Letters, 25(39), p.14467 - 14472, 2025/09
Mechanochemical radical polymerization has unique advantages in the synthesis of polymer due to its reduced solvent consumption and adaptability of insoluble monomers. However, it suffers from the uncontrollable degradation of the formed polymers during reaction and new synthetic strategy with precise controllability needs to be developed. Here, by employing high static pressure up to 30 GPa, we found 1,3,5-trifluorobenzene undergoes radical polymerization by breaking the conjugated
-bonds, and forms a carbon nanothread with high selectivity (Polymer-I polymorph). Based on the crystal structure at the threshold pressure and the calculated energy barriers for the bonding pathway, we concluded that the benzene-rings react via a 1-2 radical polymerization pathway. Our work highlights high pressure is a robust method to initiate the solid-state radical polymerization, even for very stable aromatics, and offers fresh insights for the synthesis of polymeric carbon-based materials with high selectivity.
Sato, Rika; Kondo, Toshiki; Umeda, Ryota; Kikuchi, Shin; Yamano, Hidemasa
Progress in Nuclear Science and Technology (Internet), 8, p.137 - 142, 2025/09
In a sodium-cooled fast reactor (SFR) coupled to thermal energy storage (TES) system, the reaction between nitrate molten salt as thermal energy storage medium and sodium (Na) as reactor coolant might occur under postulated accidental conditions. Thus, the reaction behavior of Na-nitrate molten salt is one of the important phenomena in terms of safety assessment of the SFR with TES system. In this study, reaction experiments on Na-solar salt were performed. It was found that Na-solar salt reaction occurred after the NaNO
-KNO
eutectic melting. Based on the measured reaction temperature, the kinetic parameters and rate constant were obtained and compared with the sodium-water reaction. From the results of kinetic analysis, it could be assumed that Na-solar salt reaction occurs in the time frame of the accident such as the failure of heat transfer tube of sodium-molten salt heat exchanger.
Terasaka, Yuta; Sato, Yuki; Ichiba, Yuta*
Radiation Measurements, 187, p.107486_1 - 107486_8, 2025/09
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)Chauvin, N.*; Martin, P.*; Ogata, Takanari*; Calabrese, R.*; Janney, D.*; Hirooka, Shun; Kato, Masato; Staicu, D.*; McClellan, K.*; White, J.*; et al.
NEA/NSC/R(2024)1 (Internet), 289 Pages, 2025/07
no abstracts in English
Yoshida, Kazuo; Hiyama, Mina*; Tamaki, Hitoshi
JAEA-Research 2025-003, 24 Pages, 2025/06
An accident of evaporation to dryness by boiling of high-level radioactive liquid waste (HLLW) is postulated as one of the severe accidents caused by the loss of cooling function at a fuel reprocessing plant. In this case, volatile radioactive materials, such as ruthenium (RuO
) are released from the tanks with water and nitric-acid mixed vapor into the atmosphere. Accurate quantitative estimation of released Ru is one of the important issues for risk assessment of those facilities. RuO
is expected to be absorbed chemically into water dissolving nitrous acid. Condensation of mixed vapor plays an important role for Ru transporting behavior in the facility building. The thermal-hydraulic behavior in the facility building is simulated with MELCOR code. The latent heat, which is a governing factor for vapor condensing behavior, has almost same value for nitric acid and water at the temperature range under 120 centigrade. Considering this thermal characteristic, it is assumed that the amount of nitric acid is substituted with mole-equivalent water in MELCOR simulation. Compensating modeling induced deviation by this assumption have been assembled with control function features of MELCOR. The comparison results have been described conducted between original simulation and modified simulation with compensating model in this report. It has been revealed that the total amount of pool water in the facility was as same as both simulations.
Yanagisawa, Hiroshi; Motome, Yuiko
JAEA-Research 2025-001, 99 Pages, 2025/06
The detailed computational models for nuclear criticality analyses on the first startup cores of NSRR (Nuclear Safety Research Reactor), which is categorized as a TRIGA-ACPR (Annular Core Pulse Reactor), were created for the purposes of deeper understandings of safety inspection data on the neutron absorber rod worths of reactivity and improvement of determination technique of the reactivity worths. The uncertainties in effective neutron multiplication factor (k
) propagated from errors in the geometry, material, and operation data for the present models were evaluated in detail by using the MVP version 3 code with the latest Japanese nuclear data library, JENDL-5, and the previous versions of JENDL libraries. As a result, the overall uncertainties in k
for the present models were evaluated to be in the range of 0.0027 to 0.0029
k
. It is expected that the present models will be utilized as the benchmark on k
for TRIGA-ACPR. Moreover, it is confirmed that the overall uncertainties were sufficiently smaller than the values of absorber rod worths determined in NSRR. Thus, it is also considered that the present models are applicable to further analyses on the absorber rod worths in NSRR.
Shimada, Asako; Hemmi, Ko; Ohira, Saki; Iida, Yoshihisa
Analytical Sciences, 9 Pages, 2025/06
Times Cited Count:0 Percentile:0.00(Chemistry, Analytical)Sugita, Yutaka; Ono, Hirokazu; Beese, S.*; Pan, P.*; Kim, M.*; Lee, C.*; Jove-Colon, C.*; Lopez, C. M.*; Liang, S.-Y.*
Geomechanics for Energy and the Environment, 42, p.100668_1 - 100668_21, 2025/06
Times Cited Count:1 Percentile:65.19(Energy & Fuels)The international cooperative project DECOVALEX 2023 focused on the Horonobe EBS experiment in the Task D, which was undertaken to study, using numerical analyses, the thermo-hydro-mechanical (or thermo-hydro) interactions in bentonite based engineered barriers. One full-scale in-situ experiment and four laboratory experiments, largely complementary, were selected for modelling. The Horonobe EBS experiment is a temperature-controlled non-isothermal experiment combined with artificial groundwater injection. The Horonobe EBS experiment consists of the heating and cooling phases. Six research teams performed the THM or TH (depended on research team approach) numerical analyses using a variety of computer codes, formulations and constitutive laws.
sp. nov., a novel hydrogen-producing bacterium isolated from a deep diatomaceous shale formationUeno, Akio*; Sato, Kiyoshi*; Tamamura, Shuji*; Murakami, Takuma*; Inomata, Hidenori*; Tamazawa, Satoshi*; Amano, Yuki; Miyakawa, Kazuya; Naganuma, Takeshi*; Igarashi, Toshifumi*
International Journal of Systematic and Evolutionary Microbiology, 75(6), p.006802_1 - 006802_11, 2025/06
Times Cited Count:0 Percentile:0.00(Microbiology)no abstracts in English