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Noseck, U.*; Sch
fer, T.*; Alonso, U.*; Hamamoto, Takafumi*; Havlova, V.*; Hibberd, R.*; Ishidera, Takamitsu; Kitamura, Akira; Klajmon, M.*; Missana, T.*; et al.
Applied Geochemistry, 201, p.106762_1 - 106762_23, 2026/04
Times Cited Count:0 Percentile:0.00Thermodynamic benchmark calculations have been performed to better understand the behavior of
Se(VI),
Tc(VII),
U(VI),
Np(V),
Am(III), Th(IV) and
Pu(IV)) in the evolving geochemical conditions of the Long-term In-situ Test (LIT) at the Grimsel Test Site (GTS) and corresponding mock-up experiment. It also aims to identify the status of the geochemical speciation models and databases for these elements. The experiments are simulating the near-field conditions in some radioactive waste repository concept including a bentonite engineered barrier emplaced in crystalline rock and the findings are contributing to the long-term safety assessment of these facilities.
Kondo, Masatoshi*; Kitamura, Yoshiki*; Kawarai, Atsushi*; Saito, Shigeru; Obayashi, Hironari
Corrosion Science, 262, p.113646_1 - 113646_14, 2026/04
Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)The corrosion resistance of FeCrAl alloy APMT (Fe-21Cr-5Al-3Mo) in flowing lead-bismuth eutectic (LBE) was investigated by corrosion tests performed at 723 K using a non-isothermal forced convection loop. The oxygen concentration in flowing LBE was controlled at 1
10
wt%. No severe corrosion or erosion was detected on the specimens exposed to flowing LBE for 2000 h and 4000 h. Multiple oxide layers consisting of Fe-rich, Cr-rich and Al-rich sub-layers were formed in situ on the surface of APMT during the corrosion tests, which effectively suppressed corrosion and erosion. The oxide layers were intentionally removed by gentle abrasion prior to re-immersion and the specimens were then re-immersed in flowing LBE for an additional 2000 h. The oxide layers were spontaneously re-formed in situ on the abraded surface. This behavior indicates a self-healing capability. The results of micro-scratch tests indicated that the in-situ formed multiple oxide layers exhibited high adhesion strength in the shear direction after the 2000 h corrosion test.
Batsaikhan, M.; Oba, Hironori*; Karino, Takahiro; Akaoka, Katsuaki; Wakaida, Ikuo*; Iwata, Yoshihiro; Sakamoto, Kan*
Journal of Analytical Atomic Spectrometry, 41(4), p.1324 - 1335, 2026/04
Times Cited Count:0 Percentile:0.00Materials Sciences Research Center
JAEA-Review 2025-058, 175 Pages, 2026/03
Fifteen neutron beam experimental instruments managed by JAEA are installed in JRR-3 (Japan Research Reactor No.3) and are available for internal use including upgrading of instruments and for external users to produce various research results. This report summarizes the progress of internal application research and technical development such as upgrading of neutron beam instruments in the fiscal years 2023 and 2024 after the restart of operation.
Hoshino, Masato; Sasaki, Yoshifumi; Horikoshi, Hidehiko*; Tani, Kosuke*
JAEA-Review 2025-047, 122 Pages, 2026/03
Horonobe Underground Research Center managed by Japan Atomic Energy Agency (JAEA) is the Japan's best environment to understand the project of geological disposal of high-level radioactive waste, because there is an Underground Research Laboratory (URL) in the center besides an exhibition facility which explains the content of research conducted in the URL. In the area of the center, there is also an exhibition facility for the full-scale model of engineered barrier system of geological disposal. JAEA takes advantage of this opportunity to conduct public hearing including questionnaire research regarding the questions, anxieties and comments by the visitors for geological disposal project. This report summarizes the result of statistical analysis of 2,830 visitors from April 2024 to January 2025.
Nagaoka, Mika; Maehara, Yushi; Ono, Masako*; Nihei, Hidekazu*; Hirao, Moe; Fujita, Hiroki
JAEA-Research 2026-001, 115 Pages, 2026/03
In fiscal year 2021, Japan Atomic Energy Agency conducted a joint research with Tokyo Electric Power Company Holdings, Inc. to develop a bioassay method. This report presents the results of studies on a systematic analysis method for
-ray and pure
-ray nuclides in urine samples. Specifically, experiments with tracer-containing samples were conducted to verify the nuclide separation performance of the systematic analysis method utilizing multiple solid-phase extraction resins and the sample preparation method for radioactivity measurement. Furthermore, calculation methods for uncertainty and detection limit of radioactivity in
-ray nuclide analysis were summarized.
Nakayama, Masashi; Ishii, Eiichi; Aoyagi, Kazuhei; Hayano, Akira; Ono, Hirokazu; Ozaki, Yusuke; Mochizuki, Akihito; Takeda, Masaki; Kimura, Shun
JAEA-Research 2025-016, 141 Pages, 2026/03
The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA). The main aim of the project is to enhance the reliability of relevant technologies for the geological disposal of high-level radioactive waste by investigating the deep geological environment within the host sedimentary rocks at Horonobe in Hokkaido, northern Japan. These investigations have been conducted in three phases: "Phase 1: Surface-based investigation", "Phase 2: Construction" (investigation during tunnel excavation) and "Phase 3: Operation" (investigation in subsurface facilities). Since the fiscal year 2020, we have been conducting R&D based on the Horonobe Underground Research Plan for the Fiscal Year 2020 Onwards, which was approved by Hokkaido Prefecture and Horonobe Town. In particular, we are working on the following key tasks with the aim of completing JAEA's 3rd and 4th Mid- and Long-Term Plans: "Study on near-field system performance in geological environments", "Demonstration of repository design options" and "Understanding of buffering behaviour of sedimentary rocks to natural perturbations". This report summarizes the R&D activities on the three above-mentioned key tasks, the goals of which were achieved between fiscal years 2020 and 2024. The results obtained from these tasks will be systematically organized as part of the "Systematic integration of technologies towards EBS emplacement" which has been in progress since fiscal year 2024. This task includes concepts related to the layout of galleries and pits, installation methods for engineered barrier materials, and methods for evaluating their containment performance.
Nishihara, Kenji; Fukushima, Masahiro; Abe, Takumi; Katano, Ryota; Yee-Rendon, B.; Iwamoto, Hiroki; Sugawara, Takanori; Obayashi, Hironari; Saito, Shigeru
JAEA-Research 2025-013, 125 Pages, 2026/03
A conceptual design for a pilot Accelerator Driven subcritical System (ADS) was developed as a precursor to a commercial ADS aimed at partitioning and transmutation of minor actinides. The output of the pilot ADS was set at 200 MW. Based on safety assessment results, the design incorporates deep subcriticality and safety rods. Core design, accelerator design, target design, and in-vessel equipment design were performed, clarifying the specific concept.
Okamoto, Naritoshi; Komeno, Akira; Seya, Atsumasa; Inaba, Hideki*; Terakado, Shinichi*; Higuchi, Masashi*
JAEA-Data/Code 2025-022, 497 Pages, 2026/03
The Plutonium Fuel Third Development Laboratory of the Nuclear Fuel Cycle Engineering Laboratories has applied for a change of use permit (hereinafter referred to as "license") for plutonium fuel facilities. For the criticality safety design of gloveboxes and equipment/instruments handling mixed oxide (MOX), various criticality calculation codes are used. The most recent employs the 3D Monte Carlo calculation code KENO-V.a embedded in the SCALE 4.4 code system, along with the 27-group ENDF/B-IV neutron cross-section library. SCALE 4.4 was released by the Oak Ridge National Laboratory (ORNL) in the US in 1998, and has now been in use for 27 years. ORNL has continuously improved its functionality, with SCALE 6.3.2 released in 2024. When designing and constructing new MOX fuel facilities, it is desirable to obtain a license using criticality calculation codes based on the latest knowledge. However, it is necessary to verify that these codes have sufficient reliability. Therefore, in 2018, benchmark calculations were performed using the 252-group ENDF/B-VII.1 neutron cross-section library (v7-252n) for two versions of the criticality calculation sequences KENO-V.a and KENO-VI from SCALE 6.2.3, based on past criticality experimental setups. The estimated critical-limiting multiplication factor was calculated. The results indicate that these codes can be used with sufficient confidence for criticality safety design of MOX fuel facilities.
-ray beam measurementsOmer, M.; Shizuma, Toshiyuki*; Koizumi, Mitsuo; Taira, Yoshitaka*; Zen, H.*; Ogaki, Hideaki*; Hajima, Ryoichi*
Radiation Physics and Chemistry, 240, p.113467_1 - 113467_8, 2026/03
Times Cited Count:0 Percentile:0.00(Chemistry, Physical)Yoshida, Ryu*; Kurikami, Hiroshi; Nagao, Fumiya; Takahashi, Shigeo*; Sanada, Yukihisa
Journal of Environmental Radioactivity, 293, p.107900_1 - 10790_13, 2026/02
Times Cited Count:0 Percentile:0.00(Environmental Sciences)Miyahara, Shinya*; Koie, Ryusuke*; Uno, Masayoshi*; Kawaguchi, Munemichi*; Sato, Rika; Seino, Hiroshi
Nuclear Engineering and Design, 446(Part A), p.114523_1 - 114523_14, 2026/01
Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)Yoneyama, Kai; Nitta, Ayako; Tanaka, Yasuyuki; Kodaka, Noriyasu; Kikuchi, Riku; Sakano, Takuma; Furuse, Takahiro; Sato, Soichi; Sambongi, Mitsuru; Tanaka, Kosuke
JAEA-Technology 2025-008, 44 Pages, 2025/12
At the TEPCO's Fukushima Daiichi Nuclear Power Station (1F), an investigation inside the reactors has been carried out. In order to safely carry out the decommissioning work such as fuel debris retrieval and building demolition, it is important to estimate the contamination in primary containment vessel for control the decommissioning planning and the worker radiation exposure levels. Therefore, the analysis of the deposit inside the penetration for the 1F Unit 2 primary containment vessel ("X-6 penetration") was performed to clarify the components and activity. The smears from the deposit were used for the analysis. Non-destructive analysis such as gamma-ray spectrometry, X-ray Fluorescence (XRF) and Scanning Electron Microscope-Energy dispersive X-ray spectroscopy (SEM-EDX) for the smear-samples were performed to determine the gamma-nuclides and the morphology of elements in the deposit. Furthermore, in order to evaluate the nuclides and nuclide composition of the deposit in detail, the smear-samples were dissolved and the quantitative analysis of gamma-nuclides, Sr-90, alpha-nuclides in the dissolved solution were conducted. The results (non-destructive analysis and quantitative analysis) were compared with the results of samples collected at different locations in the X-6 penetration in 2020. In the gamma-ray spectrometry as non-destructive analysis where the smears were analyzed directly, Co-60, Sb-125, Cs-134, Cs-137, Eu-154, Eu-155 and Am-241 were detected. In XRF results, Fe originating from construction material was detected as a major element and small amount of U and Zr originating from the fuel and fuel cladding were also detected. In SEM-EDX results, O and Fe were found as a major element of the deposit and U particles coexisting with Fe, Si, Cr, Ni and Zr were also found. These results were consistent with the SEM-EDX results of the samples collected in 2020. In radioactivity analysis, quantitative values for gamma-nuclides (Co-60, Sb-125, Cs-134, Cs-137, Eu-154, Eu-155), Sr-90, Pu-238, Pu-239+240, Am-241, Cm-244, U-235 and U-238 were obtained. Using the results, the ratios of radioactivity based on Cs-137 and U-238 were calculated. Both sets of the ratios were compared to the calculated value of the Unit 2 fuel composition from ORIGEN.
Nakayama, Masashi; Ishii, Eiichi; Aoyagi, Kazuhei; Hayano, Akira; Murakami, Hiroaki; Ono, Hirokazu; Takeda, Masaki; Fukatsu, Yuta; Mochizuki, Akihito; Ozaki, Yusuke; et al.
JAEA-Review 2025-042, 136 Pages, 2025/12
The Horonobe Underground Research Laboratory (URL) Project is being pursued by the Japan Atomic Energy Agency (JAEA) to enhance the reliability of relevant technologies for geological disposal of high-level radioactive waste through investigating the deep geological environment within the host sedimentary rocks at Horonobe-cho in Hokkaido, north Japan. In the fiscal year 2024, we continued R&D on "Study on near-field system performance in geological environment", "Demonstration of repository design options", and "Understanding of buffering behaviour of sedimentary rock to natural perturbations". These are identified as key R&D on challenges to be tackled in the Horonobe underground research plan for the fiscal year 2020 onwards. Specifically, "full-scale engineered barrier system (EBS) performance experiment" and "solute transport experiment with model testing" were carried out as part of "Study on near-field system performance in geological environment". "Demonstration of engineering feasibility of repository technology" and "evaluation of EBS behaviour over 100
C" were addressed for "Demonstration of repository design options". The validation of a method for assessing permeability using the Ductility Index and a method for estimating the state of in-situ ground pressure from hydraulic perturbation tests were investigated as part of the study "Understanding of buffering behaviour of sedimentary rock to natural perturbations". In FY2024, we continued construction of the East Access Shaft and the Ventilation Shaft, and construction of these shafts were completed to a depth of 500 m. After the completion of the East Access Shaft, excavation of the West Access Shaft and 500 m gallery has began. As of the end of FY2024, excavation progress is as follows, the East Access Shaft and the Ventilation Shaft were 500 m depth, the West Access Shaft was 472 m depth, 500 m gallery was 112.9 m, respectively. In the Horonobe International Project (HIP), Management Board and Joint Task Meeting was held at the Horonobe URL in June 2024 to review the progress of construction of galleries and preparations of experiments. Task Meetings to review the implementation plan for in-situ testing and analysis were also held. HIP will be implemented in two phases: Phase 1 (from FY2022 to FY2024) and Phase 2 (from FY2025 to FY2028), the research results of Phase 1 were compiled in FY2024.
Teshigawara, Makoto; Ikeda, Yujiro*; Muramatsu, Kazuo*; Sutani, Koichi*; Kimijima, Koichi*; Fukuzumi, Masafumi*; Noda, Yohei*; Koizumi, Satoshi*; Kawamura, Yuji*; Saruta, Koichi; et al.
Canadian Journal of Physics, 103(12), p.1225 - 1231, 2025/12
Times Cited Count:0 Percentile:0.00(Physics, Multidisciplinary)Science using neutrons in the nanometer (nm) wavelength region as probes is expanding into a wide range of fields, from basic research in materials and life science to industrial applications. Dramatic increase in the intensity of the beam source is required to drive such research. We have focused on coherent scattering caused by nano-sized particle aggregations to increase the intensity of neutron beams. Nanodiamond is being vigorously researched and developed with the aim of practical application. On the other hand, we have focused on graphene, which has higher van der Waals forces by an order of magnitude and stronger bonding, sp2, between carbons than nanodiamond. This is expected to lead to its processability into a lumped for and to adapt to higher radiation fields. By promoting chemical vapor deposition (CVD), we have established a technique to form nano-sized graphene (called graphene flower) with a shape similar to a sunflower flower. In this talk, we report on the neutron scattering properties that contribute to the coherent scattering of the newly developed graphene flower.
Aoyagi, Kazuhei; Tamura, Tomonori; Ozaki, Yusuke; Ishii, Eiichi; Motoshima, Takayuki*; Sugawara, Kentaro*
Dai-51-Kai Gamban Rikigaku Ni Kansuru Shimpojiumu Koen Rombunshu(Internet), p.119 - 124, 2025/12
In a high-level radioactive waste disposal, it is important to understand the extent of the Excavation Damaged Zone (EDZ) because it can be one of the factors to determine whether disposal galleries or pits can be excavated or not in the design or construction phases. In this study, we performed a hydro-mechanical coupling analysis to simulate the three-dimensional excavation of the twin galleries which were excavated at a depth of 500 m in the Horonobe Underground Research Laboratory. The analysis revealed that the EDZ was developed 1.5-2.0 m from the gallery wall. The stress acting on the shotcrete was within the ultimate limit state. Based on these results, we estimated that the stability of the twin galleries will be maintained, despite the relatively large extent of the EDZ.

Shimizu, Yusei*; Kittaka, Shunichiro*; Kono, Yohei*; Nakamura, Shota*; Haga, Yoshinori; Yamamoto, Etsuji; Machida, Kazushige*; Amitsuka, Hiroshi*; Sakakibara, Toshiro*
Physical Review B, 112(24), p.245157_1 - 245157_10, 2025/12
Times Cited Count:0 Percentile:0.00(Materials Science, Multidisciplinary)Collaborative Laboratories for Advanced Decommissioning Science; Tokai National Higher Education and Research System*
JAEA-Review 2025-023, 63 Pages, 2025/11
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Development and evaluation of a real-time 3D positioning embedded system combining wireless UWB and camera image analysis" conducted in FY2023. The present study aims to realize an embedded system that combines two of the latest popular technologies, "wireless UWB (Ultra Width Band)" and "multi-camera object recognition" with the goal of simple real-time 3D positioning with less than 10 cm accuracy by a human or robot for measuring air doses in nuclear reactor buildings. In this research, Gifu Univ. and National Institute of Technology, Fukushima College have developed an embedded system with camera shooting function, camera analysis function, and wireless communication function, in order to realize real-time 3D positioning based on the analysis of camera images by using these multiple devices. The Univ. of Tokyo and LocationMind Inc. will apply UWB real-time positioning technology to the inside of nuclear reactor buildings and attempt to develop technology to improve stability. Nagoya Univ. will be in charge of verifying wireless UWB stability from the hardware side by using electromagnetic wave absorbing materials. The radiation resistance evaluation will be conducted in cooperation with the JAEA and National Institute of Technology, Fukushima College.
vapor-liquid transfer model in the chemical behavior analysis code SCHERN for accident of evaporation to dryness by boiling of reprocessed high level liquid wasteYoshida, Kazuo; Hiyama, Mina*; Tamaki, Hitoshi
JAEA-Research 2025-011, 25 Pages, 2025/11
An accident of evaporation to dryness by boiling of high-level radioactive liquid waste (HLLW) is postulated as one of the severe accidents caused by the loss of cooling function at a fuel reprocessing plant. In this case, volatile radioactive materials, such as ruthenium (RuO
) are released from the tanks with water and nitric-acid mixed vapor into the atmosphere. Accurate quantitative estimation of released Ru is one of the important issues for risk assessment of those facilities. RuO
is expected to be absorbed chemically into water dissolving nitrous acid (HNO
). This behavior has been experimentally confirmed and plays an important role in the migration of Ru in the facility. A new model has been proposed as a chemical and physical absorption model based on the experimental results of the migration of RuO
into nitric acid-water mixtures. In this study, to improve the analytical performance of SCHERN, these new analytical models have been incorporated and attempted to analyze the behavior of RuO
in each phase. As a result, it has been observed a tendency that HNO
in the liquid phase increases rapidly during the late boiling phase, when RuO
release increases rapidly, and confirmed that this HNO
concentration change significantly affects the subsequent migration behavior of RuO
. These results indicate that it is essential to improve the analytical accuracy of the chemical behavior of HNO
in each phase.
Yanagisawa, Hiroshi; Motome, Yuiko
JAEA-Research 2025-010, 197 Pages, 2025/11
For understandings of nuclear criticality risks of TRIGA fuel rods and review of safety measures for handling them, nuclear criticality characteristics for infinite and finite heterogeneous lattice systems composed of the NSRR fuel rods were re-evaluated with the use of a detailed computational model for the fuel rod. The MVP version 3 code was used with the JENDL libraries including the latest version, JENDL-5, for the re-evaluation. As the criticality characteristics, variations of neutron multiplication factors of the infinite and water-reflected finite systems were examined in detail with parameters of the lattice pitch and density of moderator water. From the results of the re-evaluated criticality characteristics, the minimum critical number of fuel rods for the water-reflected hexagonal shaped lattice system was obtained to be 46.8
0.2 using the JENDL-5 library. Moreover, the attainability of criticality without the water as moderator and reflector was examined because the zirconium hydride moderator and graphite reflector are equipped with the TRIGA fuel rod. It was found that the criticality is possible to be attained by 115.7
0.6 of the number of fuel rods, which is the smaller number of fuel rods than loaded in the NSRR standard core, even though no water exists.