Validation of underwater radiation monitoring detector

Ji, W.*; Lee, E.*; Ji, Y.-Y.*; Ochi, Kotaro; Yoshimura, Kazuya; Funaki, Hironori; Sanada, Yukihisa

Nuclear Engineering and Technology, 58(2), p.103933_1 - 103933_6, 2026/02

https://doi.org/10.1016/j.net.2025.103933

We aimed to validate the performance of an in situ underwater radiation detector, MARK-U1 (Monitoring of Ambient Radiation of KAERI - Underwater), was used to estimate Cs activity concentration in river and reservoir sediment at predicted sites of contamination. Additionally, underwater core samples were collected to measure the radioactivity using a high-purity germanium (HPGe) detector. To estimate radioactivity, a conversion factor was derived by comparing the measured spectrum and Cs activity in the sample. A Monte Carlo N-Particle (MCNP) simulation was conducted to determine the effective source geometry for in situ measurement. The simulation results correlated well with the on-site MARK-U1 monitoring results, with a deviation of 31.62%. These findings validate the performance of the in situ detector. This device can therefore be used to estimate Cs activity concentration in the underwater sediment via on-site monitoring, without requiring sample collection.

Analysis of deposits inside "X-6 penetration" for the Unit 2 primary containment vessel at Fukushima Daiichi Nuclear Power Station

Yoneyama, Kai; Nitta, Ayako; Tanaka, Yasuyuki; Kodaka, Noriyasu; Kikuchi, Riku; Sakano, Takuma; Furuse, Takahiro; Sato, Soichi; Sambongi, Mitsuru; Tanaka, Kosuke

JAEA-Technology 2025-008, 44 Pages, 2025/12

JAEA-Technology-2025-008.pdf:4.3MB

At the TEPCO's Fukushima Daiichi Nuclear Power Station (1F), an investigation inside the reactors has been carried out. In order to safely carry out the decommissioning work such as fuel debris retrieval and building demolition, it is important to estimate the contamination in primary containment vessel for control the decommissioning planning and the worker radiation exposure levels. Therefore, the analysis of the deposit inside the penetration for the 1F Unit 2 primary containment vessel ("X-6 penetration") was performed to clarify the components and activity. The smears from the deposit were used for the analysis. Non-destructive analysis such as gamma-ray spectrometry, X-ray Fluorescence (XRF) and Scanning Electron Microscope-Energy dispersive X-ray spectroscopy (SEM-EDX) for the smear-samples were performed to determine the gamma-nuclides and the morphology of elements in the deposit. Furthermore, in order to evaluate the nuclides and nuclide composition of the deposit in detail, the smear-samples were dissolved and the quantitative analysis of gamma-nuclides, Sr-90, alpha-nuclides in the dissolved solution were conducted. The results (nondestructive analysis and quantitative analysis) were compared with the results of samples collected at different locations in the X-6 penetration in 2020. In the gamma-ray spectrometry as non-destructive analysis where the smears were analyzed directly, Co- 60, Sb-125, Cs-134, Cs-137, Eu-154, Eu-155 and Am-241 were detected. In XRF results, Fe originating from construction material was detected as a major element and small amount of U and Zr originating from the fuel and fuel cladding were also detected. In SEM-EDX results, O and Fe were found as a major element of the deposit and U particles coexisting with Fe, Si, Cr, Ni and Zr were also found. These results were consistent with the SEM-EDX results of the samples collected in 2020. In radioactivity analysis, quantitative values for gamma-nuclides (Co-60, Sb-125, Cs-134, Cs-137, Eu-154, Eu-155), Sr-90, Pu-238, Pu-239+240, Am-241, Cm-244, U-235 and U-238 were obtained. Using the results, the ratios of radioactivity based on Cs-137 and U-238 were calculated. Both sets of the ratios were compared to the calculated value of the Unit 2 fuel composition from ORIGEN.

A Study on the methodology for rational treatment/disposal of contaminated concrete waste considering volume reduction of waste (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*

JAEA-Review 2025-037, 103 Pages, 2025/12

JAEA-Review-2025-037.pdf:7.28MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "A study on the methodology for rational treatment/disposal of contaminated concrete waste considering volume reduction of waste" conducted in FY2023. The present study aims to evaluate rational waste management strategies incorporating reuse and recycling focusing on radioactive concrete waste, which will be massively generated from dismantling. Feasibility and challenges of aggregate recycling are considered assuming a typical recycled aggregate production technique, based on the characteristics of the concrete. In 2023, the migration behaviors of radionuclides and ions in cementitious materials having interfacial transition zones (ITZ) were investigated through diffusion and leaching experiments using radioactive and non-radioactive tracers and modeled by random walk particle tracking method with a sampling technique using a probabilistic distribution model for two media with an interface. Properties of surrogate contaminated concrete samples prepared by immersing in Cs solution were examined. Migration of ions was studied for surrogate contaminated aggregates and recycled concrete using the surrogate. In addition, surrogate waste package was prepared using by-product powder to study mechanical and chemical properties as well as leaching behavior of radionuclides. Information on properties of the contaminated concrete and tools to estimate the amount of concrete were organized in order to evaluate different waste management scenarios incorporating reuse/recycling.

Plastics as vectors of radiocesium in river environments of Fukushima, Japan

Battulga, B.*; Nakanishi, Takahiro; Ikenoue, Tsubasa; Atarashi-Andoh, Mariko; Koarashi, Jun

Journal of Hazardous Materials, 500, p.140593_1 - 140593_11, 2025/12

https://doi.org/10.1016/j.jhazmat.2025.140593

Development of a Ce:GPS scintillator-based spectrometer and its demonstration in radioactive cesium contamination sites

Morishita, Yuki; Nakama, Shigeo; Ochi, Kotaro; Urabe, Yoshimi*; Kanno, Marina*

Radiation Measurements, 189, p.107513_1 - 107513_6, 2025/12

https://doi.org/10.1016/j.radmeas.2025.107513

Following the Fukushima Daiichi Nuclear Power Plant accident, radioactive cesium contamination posed a significant environmental concern. This study developed a compact gamma-ray spectrometer utilizing a Ce:GPS scintillator and a compact photomultiplier tube (PMT) for environmental monitoring. The spectrometer was designed to overcome limitations of traditional NaI(Tl) detectors, leveraging the non-hygroscopic nature and high energy resolution of Ce:GPS scintillators. Performance was evaluated through measurements of a Cs source and comparison with a commercial NaI(Tl) survey meter. The spectrometer's potential for effective and portable monitoring of radioactive cesium in contaminated environments was demonstrated. The system was tested using sealed sources, confirming its ability to detect the 662 keV photopeak of Cs with high accuracy. Field measurements in radiocesium-contaminated areas showed the spectrometer's effectiveness in detecting dose rate variations and high-dose hotspots. This portable, durable spectrometer shows promise for applications in environmental radiation monitoring and remote sensing technologies.

High-speed 3D modeling for nuclear reactor environment based on feature extraction results from video images (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Sapporo University*

JAEA-Review 2025-033, 71 Pages, 2025/11

JAEA-Review-2025-033.pdf:4.48MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2023, this report summarizes the research results of the "High-speed 3D modeling for nuclear reactor environment based on feature extraction results from video images" conducted in FY2023. The present study aims to develop a 3D model for a workspace that maximizes the amount of information based on the features extracted from video, which is taken when surveying the primary containment vessel and inside the reactor building as part of the decommissioning of 1F, considering within a specified time. In FY2023, we verified extracting effective shooting conditions for obtaining 3D reconstruction based on photogrammetry and the method extracting feature values that can generate 3D restoration results from a small amount of data within a specified time based on deep learning. In addition, we applied point cloud data extracted from video to segmentation and classified it into parts with instance labels.

Investigation of effects of nano interfacial phenomena on dissolution aggregation of alpha nanoparticles by using micro nano technologies (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Institute of Science Tokyo*

JAEA-Review 2025-026, 72 Pages, 2025/11

JAEA-Review-2025-026.pdf:7.97MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Investigation of effects of nano interfacial phenomena on dissolution aggregation of alpha nanoparticles by using micro nano technologies" conducted in FY2023. To ensure the safety of retrieval and storage management of nuclear fuel debris generated by the Fukushima-Daiichi Nuclear Power Station accident, understanding of dissolution-denaturation behavior of the fuel debris alpha particles is one of the most crucial issues. This research aims to create novel microfluidic real-time measurement device for elucidating dissolution, aggregation, and denaturation processes of metal oxide nanoparticles under various solution environments, and clarify their nano-size and interfacial effects. In this year, we conducted bulk and micro dissolution tests of simulated fuel debris particles (UO mechanical-treated nanoparticles, UO chemical-treated nanoparticles, and (U,Zr)O nanoparticles), and successfully clarified that the effects of particle sizes, reaction times, and HO concentrations on the dissolution behavior of each nanoparticle. In particular, it was found that (U,Zr)O nanoparticles have different degrees of Zr catalytic reactions depending on HO concentrations, resulting in the generation of different amounts of gas and U. Moreover, we developed a new microfluidic device which enables to instantly react the nanoparticles with HO solutions, and determined dynamic aggregation and dissolution rates of the nanoparticles. The research was carried out in close collaboration with UK researchers, and achieved the expected goal of this year.

Differential microbial roles in the organic layer and mineral soil determine radioactive cesium fate in forest ecosystems

Koarashi, Jun; Nagano, Hirohiko*; Nakayama, Masataka*; Atarashi-Andoh, Mariko; Nagaoka, Mika

Chemosphere, 389, p.144715_1 - 144715_11, 2025/11

https://doi.org/10.1016/j.chemosphere.2025.144715

Radiocesium (Cs) contamination poses a long-term ecological challenge, particularly in forest ecosystems. The role of soil microorganisms in determining its fate remains insufficiently understood. This study presents a dynamic assessment of microbial Cs retention, focusing on the complex interplay among microorganisms, organic matter, and clay minerals within the organic layer-mineral soil system. Our results show that rapid microbial cycling sustains a potentially bioavailable Cs pool in the organic layer. This microbial involvement diminishes as Cs activity concentrations in the organic layer decline. In the mineral soil, minimal microbial Cs retention was observed, suggesting an indirect role in facilitating Cs immobilization by clay minerals. Notably, microbial Cs retention in the organic layer is regulated by Cs availability, independent of region, forest type, and time since deposition. These findings provide a unified explanation for observed differences in Cs persistence in organic layers between European and Japanese forests.

Improving the analysis method of the Compton camera system mounted on the unmanned helicopter by correcting scintillator coordinates data at each event timing

Shikaze, Yoshiaki

Radioisotopes, 74(3), p.273 - 287, 2025/11

https://doi.org/10.3769/radioisotopes.740302

The previous method used the data during the stable period for the position and attitude angles of the unmanned helicopter as a countermeasure to improve the measurement data analysis of the Compton camera system mounted on the unmanned helicopter. However, this reduced the number of events used for analysis, allowing statistical accuracy to be improved in future. Therefore, all event data were corrected and used this time. The scintillator coordinates of two layers fixed in the previous analysis were replaced with those corrected for the ever-changing positions and tilts for each event. I reconstructed gamma-ray images using the corrected events to improve their statistical accuracy and spatial resolution. I compared the ground measurement results to evaluate the improvement in the accuracy of the reconstructed images of gamma-ray intensity. As for the effect of the improved statistics, a decrease in the residual sum of squares (RSS) was noted after improvement, indicating the effectiveness of this method through good correlations with the ground-measured values. Moreover, from the RSS value comparison, compared to changing from the previous method to the improved method, expanding the range of averaging the measured values was confirmed to be more effective, showing better correlations with the ground-measured values.

Embedded system using a radiation-hardened processor (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Okayama University*

JAEA-Review 2025-022, 51 Pages, 2025/10

JAEA-Review-2025-022.pdf:3.05MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Embedded system using a radiation-hardened processor" conducted in FY2023. The present study aims to develop a radiation-hardened optoelectronic processor with 10 MGy total-ionizing-dose (TID) tolerance, a radiation-hardened processor with 4 MGy TID tolerance, a radiation-hardened memory with 4 MGy TID tolerance, and a radiation-hardened power supply unit with 1 MGy TID tolerance. Up to now, we have successfully developed a radiation-hardened optoelectronic processor with 10 MGy TID tolerance, a radiation-hardened memory with 4 MGy TID tolerance. Moreover, Japanese research group will support radiation-hardened field programmable gate arrays, power supply units, and radiation-hardened optical systems for radiation-hardened robot systems and radiation sensor systems developed by UK team. Finally, we will provide our radiation-hardened robot system which can identify the intensity and type of radiation.