Fuel debris criticality analysis technology using non-contact measurement method (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*

JAEA-Review 2024-013, 48 Pages, 2024/07

JAEA-Review-2024-013.pdf:1.99MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Fuel debris criticality analysis technology using non-contact measurement method" conducted in FY2022. The purpose of research was to improve the fuel debris criticality analysis technology using non-contact measurement method by the development of the fuel debris criticality characteristics measurement system and the multi-region integral kinetic analysis code. It was performed by Tokyo Institute of Technology, National Institute of Advanced Industrial Science and Technology, and Nagaoka University of Technology as the second year of three years research project.

Human resource development related to remote control technology for monitoring inside RPV pedestal during retrieval of fuel debris (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2023-023, 99 Pages, 2024/03

JAEA-Review-2023-023.pdf:6.0MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Human Resource Development Related to Remote Control Technology for Monitoring Inside RPV Pedestal during Retrieval of Fuel Debris" conducted in FY2022. The present study aims to construct a monitoring platform for understanding the status inside a reactor during fuel debris removal, and measurement and visualization by sensors moving on the platform. In addition, to develop research personnel through research education by participating in such research projects, classroom lectures, and facility tours is also a goal of this project. In FY2022, each system was improved and expanded toward the final year, and verification experiments were conducted in simulated environments.

Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of , , and X-rays (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*

JAEA-Review 2023-022, 93 Pages, 2023/12

JAEA-Review-2023-022.pdf:4.7MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of , , and X-rays" conducted from FY2020 to FY2022. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, we have established the latest measurement system, such as the multiple -ray detection methods, and the Spectral Determination Method (hereinafter referred to as "SDM") was developed. In the research in 2022, we developed a code that handles measurement data of LSC, singles Ge, and 2D spectra (multiple ). In addition, to develop an integrated database, spectral data of 40 nuclides were obtained by actual measurements and simulation calculations.

Development of correction method for sample density effect on PGA

Maeda, Makoto; Segawa, Mariko; Toh, Yosuke; Endo, Shunsuke; Nakamura, Shoji; Kimura, Atsushi

Journal of Radioanalytical and Nuclear Chemistry, 332(8), p.2995 - 2999, 2023/08

https://doi.org/10.1007/s10967-023-08961-x

New measurement system based on small-angle neutron scattering for structural analysis of light-responsive materials

Iwase, Hiroki*; Akamatsu, Masaaki*; Inamura, Yasuhiro; Sakaguchi, Yoshifumi*; Morikawa, Toshiaki*; Kasai, Satoshi*; Ouchi, Keiichi*; Kobayashi, Kazuki*; Sakai, Hideki*

Journal of Applied Crystallography, 56(1), p.110 - 115, 2023/02

https://doi.org/10.1107/S1600576722011104

With the increasing importance of light-responsive materials, it is vital to analyze the relationship between function and structural changes induced by light irradiation. Small-angle scattering (SAS) is effective for such structural analysis. However, quantitatively capturing local molecular structure formation and molecular reactions at a scale of less than 1 nm via SAS is difficult. In this study, to analyze the structure of non-equilibrium phenomena in light-responsive materials, a new sample environment has been developed for a time-of-flight small- and wide-angle neutron scattering instrument (TAIKAN), comprising a UV-Vis irradiation system, UV-Vis absorption measurement equipment and photodetector. Simultaneous measurement of small-angle neutron scattering and UV-Vis absorption was achieved. This system was used to demonstrate the in situ observation of UV-Vis irradiation-induced structural change of micelles formed by a light-responsive surfactant sample in an aqueous solution.

Consideration on roles and relationship between observations/measurements and model predictions for environmental consequence assessments for nuclear facilities

Togawa, Orihiko; Okura, Takehisa; Kimura, Masanori

JAEA-Review 2022-049, 76 Pages, 2023/01

JAEA-Review-2022-049.pdf:3.74MB

Before construction and after operation of nuclear facilities, environmental consequence assessments are conducted for normal operation and an emergency. These assessments mainly aim at confirming safety for the public around the facilities and producing relief for them. Environmental consequence assessments are carried out using observations/ measurements by environmental monitoring and/or model predictions by calculation models, sometimes using either of which and at other times using both them, according to the situations and necessities. First, this report investigates methods, roles, merits/demerits and relationship between observations/measurements and model predictions which are used for environmental consequence assessments of nuclear facilities, especially holding up a spent nuclear fuel reprocessing plant at Rokkasho, Aomori as an example. Next, it explains representative examples of utilization of data on observations/measurements and results on model predictions, and considers points of attention at using them. Finally, the report describes future direction, for example, improvements of observations/measurements and model predictions, and fusion of both them.

Challenge to advancement of debris composition and direct isotope measurement by microwave-enhanced LIBS (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; i-Lab*

JAEA-Review 2022-042, 67 Pages, 2023/01

JAEA-Review-2022-042.pdf:7.42MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Challenge to advancement of debris composition and direct isotope measurement by microwave-enhanced LIBS" conducted in FY2021. The present study aims to increase the emission intensity of LIBS (laser-induced breakdown spectroscopy) by superimposing MW (microwave) and apply it to uranium isotope measurement. In FY2021, after confirming that there was no problem in terms of specifications including noise leakage by downsizing the semiconductor MW oscillator and evaluating it as a single unit, the possibility of uranium isotope measurement was examined by applying it to the LIBS experiment. In addition, the optimized design of the MW antenna was carried out. By applying them, we confirmed the actual performance, …

Human resource development related to remote control technology for monitoring inside RPV pedestal during retrieval of fuel debris (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2022-032, 102 Pages, 2022/12

JAEA-Review-2022-032.pdf:9.83MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Human resource development related to remote control technology for monitoring inside RPV pedestal during retrieval of fuel debris" conducted in FY2021. The present study aims to construct a monitoring platform for understanding the status inside a reactor during fuel debris removal, and measurement and visualization by sensors moving on the platform. In addition, to develop research personnel through research education by participating in such research projects, classroom lectures, and facility tours is also a goal of this project. In FY2021, we mainly worked on improving the base design and technology development that we had worked on in the previous year, and we also prepared for integration experiments.

Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of , , and X-rays (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*

JAEA-Review 2021-060, 105 Pages, 2022/03

JAEA-Review-2021-060.pdf:4.59MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of , , and X-rays" conducted in FY2020. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, and develops the measurement system such as multiple -ray detection method. We develop a spectral determination method (SDM method) for integrated analysis by constructing a spectral database for nuclides including -rays and X-rays by measurement using this system and radiation simulation calculation. This method enables simultaneous quantification of multiple nuclides and reduces the chemical separation process.

Human resource development related to remote control technology for monitoring inside RPV pedestal during retrieval of fuel debris (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2021-030, 79 Pages, 2021/12

JAEA-Review-2021-030.pdf:3.82MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Human resource development related to remote control technology for monitoring inside RPV pedestal during retrieval of fuel debris" conducted in FY2020. This study deals with construction of a monitoring platform for understanding the status inside a reactor during fuel debris removal, and measurement and visualization by sensors moving on the platform. In addition, to develop research personnel through research education by participating in such research projects, classroom lectures, and facility tours is also a goal of this project. In FY2020, the main activities were base design and underlying technology development.