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Terada, Hiroaki; Nagai, Haruyasu; Kadowaki, Masanao; Tsuzuki, Katsunori
Journal of Nuclear Science and Technology, 60(8), p.980 - 1001, 2023/08
Times Cited Count:1 Percentile:82.84(Nuclear Science & Technology)It is essential to establish a method for reconstructing the source term and spatiotemporal distribution of radionuclides released into the atmosphere due to a nuclear accident for emergency countermeasures. We examined the dependency of a source term estimation method based on Bayesian inference using atmospheric dispersion simulation and environmental monitoring data on the availability of various monitoring data. Additionally, we examined the applicability of this method to a real-time estimation conducted immediately after an accident. A sensitivity analysis of the estimated source term during the Fukushima Daiichi Nuclear Power Station (FDNPS) accident for combinations of various monitoring data indicated that using monitoring data with a high temporal and spatial resolution and the concurrent use of air concentration and surface deposition data is effective for accurate estimation. A real-time source term estimation experiment assuming the situation of monitoring data acquisition during the FDNPS accident revealed that this method could provide the necessary source term for grasping the overview of surface contamination in the early phase and evaluating the approximate accident scale. If the immediate online acquisition of monitoring data and regular operation of an atmospheric dispersion simulation are established, this method can provide the source term in near-real time.
Dong, F.*; Chen, S.*; Demachi, Kazuyuki*; Yoshikawa, Masanori; Seki, Akiyuki; Takaya, Shigeru
Nuclear Engineering and Design, 404, p.112161_1 - 112161_15, 2023/04
Times Cited Count:0 Percentile:95.45(Nuclear Science & Technology)Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*
JAEA-Review 2022-071, 123 Pages, 2023/03
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Development of a hybrid method for evaluating the long-term structural soundness of nuclear reactor buildings using response monitoring and damage imaging technologies" conducted in FY2021. The present study aims to develop an evaluation method necessary to obtain a perspective on the long-term structural soundness of accident-damaged reactor buildings, where accessibility to work sites is extremely limited due to high radiation dose rate and high contamination. In FY2021, the first year of the three-year plan, the following research items were undertaken by clarifying specific research methods, setting research directions, making necessary preparations, and conducting some tests and other activities.
Futemma, Akira; Sanada, Yukihisa; Sasaki, Miyuki; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Hokama, Tomonori; et al.
JAEA-Technology 2022-028, 127 Pages, 2023/02
A large amount of radioactive material was released by the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company, caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011. After the nuclear disaster, airborne radiation monitoring via manned helicopter has been utilized to grasp rapidly and widely the distribution of the radioactive materials surrounding FDNPS. We prepare the data of background radiation dose, geomorphic characteristics and the controlled airspace surrounding nuclear facilities of the whole country in order to make effective use of the monitoring technique as a way of emergency radiation monitoring and supply the results during an accident of a facility. This report has summarized the knowledge noted above achieved by the aerial radiation monitoring around Ohi and Takahama nuclear power stations. In addition, the examination's progress aimed at introducing airborne radiation monitoring via an unmanned plane during a nuclear disaster and the technical issues are summarized in this report.
Futemma, Akira; Sanada, Yukihisa; Nagakubo, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Urabe, Yoshimi*; et al.
JAEA-Technology 2022-027, 148 Pages, 2023/02
By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company (TEPCO), caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011, a large amount of radioactive material was released from the FDNPS. After the nuclear disaster, airborne radiation monitoring via manned helicopter has been conducted around FDNPS. The results of the airborne radiation monitoring and the evaluation for temporal change of dose rate in the fiscal 2021 were summarized in this report. Analysis considering topographical effects was applied to the result of the airborne monitoring to improve the accuracy of the conventional method. In addition, technique for discriminating gamma rays from the ground and those from the airborne Rn-progenies was also utilized to evaluate their effect on airborne radiation monitoring.
Group for Fukushima Mapping Project
JAEA-Technology 2022-026, 152 Pages, 2023/01
This report presents results of the investigations on the distribution-mapping project of radioactive substances owing to TEPCO Fukushima Daiichi Nuclear Power Station (FDNPS) conducted in FY2021. Car-borne surveys, a flat ground measurement using survey meters, a walk survey and an unmanned helicopter survey were carried out to obtain air dose rate data to create air dose rate distribution maps, and temporal changes of the air dose rates were analyzed. Surveys on depth profile of radiocesium and in-situ measurements as for radiocesium deposition were performed. Based on these measurement results, effective half-lives of the temporal changes in the air dose rates and the deposition were evaluated. Score maps to classify the importance of the measurement points were created for Fukushima Prefecture and the 80 km zone from the FDNPS, and the factors causing changes in the score when monitoring data from multiple years were used were discussed. Monitoring data in coastal area performed owing to the comprehensive radiation monitoring plan until 2020 was summarized, and temporal changes in cesium-137 were analyzed. Using the Bayesian hierarchical modeling approach, we obtained maps that integrated the air dose rate distribution data obtained in this project with respect to the region within 80 km from the FDNPS and Fukushima Prefecture. The measurement results for FY2021 were published on the "Expansion Site of Distribution Map of Radiation Dose", and measurement data were stored as CSV format. Radiation monitoring and analysis of environmental samples owing to the comprehensive radiation monitoring plan were carried out.
Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*
JAEA-Review 2022-032, 102 Pages, 2022/12
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Human resource development related to remote control technology for monitoring inside RPV pedestal during retrieval of fuel debris" conducted in FY2021. The present study aims to construct a monitoring platform for understanding the status inside a reactor during fuel debris removal, and measurement and visualization by sensors moving on the platform. In addition, to develop research personnel through research education by participating in such research projects, classroom lectures, and facility tours is also a goal of this project. In FY2021, we mainly worked on improving the base design and technology development that we had worked on in the previous year, and we also prepared for integration experiments.
Collaborative Laboratories for Advanced Decommissioning Science; High Energy Accelerator Research Organization*
JAEA-Review 2022-031, 89 Pages, 2022/12
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Technology development of diamond-base neutron sensors and radiation-resistive integrated-circuits for shielding-free criticality approach monitoring system" conducted in FY2021. The present study aims to develop key components of neutron detection system without a radiation shield for a criticality approach monitoring system. It is required high neutron detection efficiency for a few cps/nv under 1 kGy/h and compact-light-weight to fit constraints of the penetration size and the payload. The project aims to design and evaluate neutron detection devices based on diamond sensors and a high radiation resistive signal-processing data-transfer system based on radiation resistive integrated circuit technologies …
Tsubota, Yoichi; Honda, Fumiya; Tokonami, Shinji*; Tamakuma, Yuki*; Nakagawa, Takahiro; Ikeda, Atsushi
Nuclear Instruments and Methods in Physics Research A, 1030, p.166475_1 - 166475_7, 2022/05
Times Cited Count:1 Percentile:40.11(Instruments & Instrumentation)In the long-lasting decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), the dismantling of nuclear fuel debris (NFD) remaining in the damaged reactors is an unavoidable but significant issue with many technical difficulties. The dismantling is presumed to involve mechanical cutting, generating significant concentrations of particulates containing -radionuclides (
-aerosols) that pose significant health risk upon inhalation. In order to minimize the radiation exposure of workers with
-aerosols during the dismantling/decommissioning process at 1F, it is essential to monitor the concentration of
-aerosols at the point of initial generation, i.e. inside the primary containment vessels (PCV) of the damaged reactors. Toward this end, an
monitoring system for
-aerosols (
alpha air monitor: IAAM) was developed and its technical performance was investigated under the conditions expected for the actual environments at 1F. IAAM was confirmed to fulfill four technical requirements: (1) steady operation under high humidity, (2) operation without using filters, (3) capability of measuring a high counting rate of
-radiation, and (4) selective measurement of
-radiation even under high radiation background with
/
-rays. IAAM is capable of selectively measuring
-aerosols with a concentration of 3.3
10
Bq/cm
or higher without saturation under a high humid environment (100%-relative humidity) and under high background with
/
-radiation (up to 100 mSv/h of
-radiation). These results demonstrate promising potential of IAAM to be utilized as a reliable monitoring system for
-aerosols during the dismantling of NFD, as well as the whole long-lasting decommissioning of 1F.
Collaborative Laboratories for Advanced Decommissioning Science; Osaka University*
JAEA-Review 2021-074, 104 Pages, 2022/03
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Basic study for on-line monitoring of tiny particles including alpha emitters by aerosol time-of-flight mass spectroscopy" conducted in FY2019 and FY2020. Since the final year of this proposal was FY2020, the results for two fiscal years were summarized. The present study aims to conduct a feasibility study of Aerosol time-of-flight mass spectroscopy (ATOFMS) to on-line measurement of tiny particles containing alpha emitters which might be dispersed in cutting the debris in reactors of the Fukushima Daiichi Nuclear Power Station for realizing their real-time monitoring.
Futemma, Akira; Sanada, Yukihisa; Ishizaki, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Sato, Kazuhiko*; Haginoya, Masashi*; Matsunaga, Yuki*; Kikuchi, Hikaru*; et al.
JAEA-Technology 2021-029, 132 Pages, 2022/02
By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company (TEPCO), caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011, a large amount of radioactive material was released from the FDNPS. After the nuclear disaster, airborne radiation monitoring using manned helicopter has been conducted around FDNPS. The results of the airborne radiation monitoring and the evaluation for temporal change of dose rate in the fiscal 2020 were summarized in this report. Analysis considering topographical effects was applied to the result of the airborne monitoring to improve the accuracy of conventional method. In addition, technique for discriminating gamma rays from the ground and those from the airborne Rn-progenies was also utilized to evaluate their effect on airborne radiation monitoring.
Collaborative Laboratories for Advanced Decommissioning Science; High Energy Accelerator Research Organization*
JAEA-Review 2021-038, 65 Pages, 2022/01
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Technology development of diamond-base neutron sensors and radiation-resistive integrated-circuits for shielding-free criticality approach monitoring system" conducted in FY2020. The present study aims to develop key components of neutron detection system without a radiation shield for a criticality approach monitoring system. It is required high neutron detection efficiency for a few cps/nv under high gamma ray radiation environment (i.e. 1 kGy/h maximum) and compact-light-weight to fit constraints of the penetration size and the payload.
Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*
JAEA-Review 2021-030, 79 Pages, 2021/12
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Human resource development related to remote control technology for monitoring inside RPV pedestal during retrieval of fuel debris" conducted in FY2020. This study deals with construction of a monitoring platform for understanding the status inside a reactor during fuel debris removal, and measurement and visualization by sensors moving on the platform. In addition, to develop research personnel through research education by participating in such research projects, classroom lectures, and facility tours is also a goal of this project. In FY2020, the main activities were base design and underlying technology development.
Futemma, Akira; Sanada, Yukihisa; Sasaki, Miyuki; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Sato, Kazuhiko*; Haginoya, Masashi*; Matsunaga, Yuki*; Kikuchi, Hikaru*; et al.
JAEA-Technology 2021-020, 138 Pages, 2021/11
A large amount of radioactive material was released by the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company, caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011. After the nuclear disaster, airborne radiation monitoring via manned helicopter has been utilized to grasp rapidly and widely the distribution of the radioactive materials surrounding FDNPS. We prepare the data of background radiation dose, geomorphic characteristics and the controlled airspace surrounding nuclear facilities of the whole country in order to make effective use of the monitoring technique as a way of emergency radiation monitoring and supply the results during an accident of a facility. This report is summarized that the knowledge as noted above achieved by the aerial radiation monitoring around Tsuruga and Mihama nuclear power station, research reactors in Kindai University Atomic Energy Research Institute and Institute for Integrated Radiation and Nuclear Science, Kyoto University. In addition, examination's progress aimed at introduction of airborne radiation monitoring via unmanned plane during nuclear disaster and the technical issues are summarized in this report.
Nakano, Masanao
Hoken Butsuri (Internet), 56(1), p.17 - 25, 2021/03
The Tokai Reprocessing Plant is the first reprocessing plant in Japan which started hot test in 1977, and had reprocessed 1140 tons of spent nuclear fuel by May 2007. The gaseous and liquid radioactive wastes has been discharged to the environment. Since iodine-129 (I) is one of the most important nuclides for environmental impact assessment. Therefore,
I in the exhaust and effluent has been controlled, and a precise analysis method of
I in the environmental samples was developed, and the concentration of 129I in the environment was investigated. This report presents an overview of these activities. Not limited to
I on reprocessing facilities, it is essential for nuclear operators to reduce the amount released to the environment in the spirit of ALARA, and to continuously develop the further upgrading environmental monitoring methods and evaluation methods in order to foster a sense of safety and security among residents living in the vicinity of the facilities.
Futemma, Akira; Sanada, Yukihisa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Sato, Kazuhiko*; Haginoya, Masashi*; Matsunaga, Yuki*; Kikuchi, Hikaru*; Ishizaki, Azusa; et al.
JAEA-Technology 2020-019, 128 Pages, 2021/02
A large amount of radioactive material was released by the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company, caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011. After the nuclear disaster, airborne radiation monitoring using manned helicopter has been utilized to grasp rapidly and widely the distribution of the radioactive materials around FDNPS. We prepare the data of background radiation dose, geomorphic characteristics and the controlled airspace around nuclear facilities of the whole country in order to make effective use of the monitoring technique as a way of emergency radiation monitoring and supply the results during accidents of the facilities. Furthermore, the airborne radiation monitoring has been conducted in Integrated Nuclear Emergency Response Drill to increase effectiveness of the monitoring. This report is summarized that the knowledge as noted above achieved by the aerial radiation monitoring around Higashidori nuclear power station, the nuclear fuel reprocessing plant in Rokkasho village and Shika nuclear power station, the full details of the aerial radiation monitoring in Integrated Nuclear Emergency Response Drill in the fiscal 2019. In addition, examination's progress aimed at introduction of airborne radiation monitoring using unmanned helicopter during nuclear disaster and the technical issues are summarized in this report.
Futemma, Akira; Sanada, Yukihisa; Ishizaki, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Sato, Kazuhiko*; Haginoya, Masashi*; Matsunaga, Yuki*; Kikuchi, Hikaru*; et al.
JAEA-Technology 2020-018, 121 Pages, 2021/02
By the nuclear disaster of Fukushima Daiichi Nuclear Power Station (FDNPS), Tokyo Electric Power Company (TEPCO), caused by the Great East Japan Earthquake and the following tsunami on March 11, 2011, a large amount of radioactive material was released from the FDNPS. After the nuclear disaster, airborne radiation monitoring using manned helicopter has been conducted around FDNPS. The results in the fiscal 2019 were summarized in this report. Analysis taken topographical effects into consideration was applied to the result of airborne monitoring to improve the precision of conventional method. In addition, discrimination method of gamma rays from Rn-progenies was also utilized to evaluate their effect on aerial radiation monitoring.
Aoki, Katsunori; Yamanaka, Hiroki*; Watanabe, Kazuhiko*; Sugihara, Kozo
JAEA-Data/Code 2020-018, 45 Pages, 2021/02
Mizunami Underground Research Laboratory (MIU) Project is pursued by Japan Atomic Energy Agency (JAEA) in the crystalline host rock (granite) as a part of geoscientific study of JAEA, and underground facilities of MIU are constructed down to 500m blow the ground surface. As small amount of Uranium is normally contained in granite, high concentration of radon is sometimes detected in the air of the underground facilities constructed in granitic rocks depending on their ventilation conditions. Radon concentrations in underground facilities of MIU have been measured according to the excavation progress of underground facilities or the change of ventilation system. It is recognized that the data obtained by the actual measurement of radon concentration in such underground facilities are rare and valuable. This repot summarizes the measured data from fiscal 2010 to fiscal 2020, together with the information of ventilation conditions and air temperature which affect radon concentrations in underground facilities. The variation of the equilibrium factors of radon is also examined with the actually measured data. As a result, it has been found that radon concentration in the drift is high in summer and low in winter according to the natural ventilation caused by the seasonal temperature difference between in and out of the underground facilities. Furthermore, the temporary increase in the equilibrium factor of radon in the drift at the start of ventilation is supposed to be due to the aerosol increase by the ventilation flow, such as the dust blown up.
Nagaoka, Mika; Fujita, Hiroki; Aida, Taku*; Guo, H.*; Smith, R. L. Jr.*
Applied Radiation and Isotopes, 168, p.109465_1 - 109465_6, 2021/02
Times Cited Count:0 Percentile:0.01(Chemistry, Inorganic & Nuclear)The radioactivities in the environmental samples are analyzed to monitor the nuclear power facilities. The pretreatment of radioactive nuclides of alpha and beta emitters in the environmental samples is performed with acid to decompose organic matter and extract object nuclide such as Sr, U and Pu. However, the pretreatment methods are time-consuming and used many concentrated acid solutions that are unsafe and hazardous. Therefore, we develop to the new pretreatment method using supercritical water instead of acid. Hydrothermal pretreatment of soils (Andosols) from Ibaraki prefecture (Japan) was used to improve methods for monitoring radioactive Sr and U. Calcined samples were pretreated with subcritical or supercritical water (SCW) followed by extraction with 0.5 M HNO
solutions. With SCW pretreatment, recoveries of Sr and U were 70% and 40%, respectively. Experimental recoveries obtained can be described by a linear relationship in water density. The proposed method is robust and can lower environmental burden of routine analytical protocols.
Collaborative Laboratories for Advanced Decommissioning Science; Osaka University*
JAEA-Review 2020-050, 69 Pages, 2021/01
The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2019. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Basic study for On-Line Monitoring of Tiny Particles including Alpha Emitters by Aerosol Time-Of-Flight Mass Spectroscopy" conducted in FY2019. The present study aims to conduct a feasibility study of Aerosol Time-Of-Flight Mass Spectroscopy (ATOFMS) technique to on-line measurement of tiny particles including alpha emitters which might be dispersed in cutting debris in reactors of the Fukushima Daiichi Nuclear Power Station for realizing real-time monitoring of the tiny particles. In FY2019, we prepared the solid (U, Zr)O samples and the acidic and basic U solutions as model materials.