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Rajeev, H. S.*; Hu, X.*; Chen, W.-L.*; Zhang, D.*; Chen, T.*; 古府 麻衣子*; 梶本 亮一; 中村 充孝; Chen, A. Z.*; Johnson, G. C.*; et al.
Journal of the Physical Society of Japan, 94(3), p.034602_1 - 034602_14, 2025/03
被引用回数：0 パーセンタイル：0.00(Physics, Multidisciplinary)Two-dimensional hybrid organic-inorganic perovskites (HOIPs) have emerged as promising materials for light-emitting diode applications. In this study, by using time-of-flight neutron spectroscopy we identified and quantitatively separated the lattice vibrational and molecular rotational dynamics of two perovskites, butylammonium lead iodide (BA)
PbI
and phenethyl-ammonium lead iodide (PEA)PbI. By examining the corresponding temperature dependence, we found that the lattice vibrations, as evidenced by neutron spectra, are consistent with the lattice dynamics obtained from Raman scattering. We revealed that the rotational dynamics of organic molecules in these materials tend to suppress their photoluminescence quantum yield (PLQY) while the vibrational dynamics did not show predominant correlations with the same. Additionally, we observed photoluminescence emission peak splitting for both systems, which becomes prominent above certain critical temperatures where the suppression of PLQY begins. This study suggests that the rotational motions of polarized molecules may lead to a reduction in exciton binding energy or the breaking of degeneracy in exciton binding energy levels, enhancing non-radiative recombination rates, and consequently reducing photoluminescence yield. These findings offer a deeper understanding of fundamental interactions in 2D HOIPs and could guide the design of more efficient light-emitting materials for advanced technological applications.
SR study on the noncentrosymmetric superconductor NbGe
Jiao, J. C.*; Chen, K. W.*; Hillier, A. D.*; 伊藤 孝; 髭本 亘; Li, Z.*; Lv, B.*; Xu, Z.-A.*; Shu, L.*
Physical Review B, 110(21), p.214516_1 - 214516_9, 2024/12
被引用回数：0 パーセンタイル：0.00(Materials Science, Multidisciplinary)We report on a muon spin relaxation (SR) study on the polycrystalline noncentrosymmetric superconductor NbGe with superconducting transition temperature 
= 2.0-2.1 K. The zero-field SR experiment indicates the absence of a spontaneous magnetic field in the superconducting state, showing the preservation of time-reversal symmetry in the superconducting state. The transverse-field SR experiment is performed to map the phase diagram of NbGe, from which clear evidence of both type-I and type-II superconductivities is obtained. More importantly, we clearly delineate the region in the phase diagram where type-I and type-II superconductivities coexist.
Zheng, X.-G.*; 山内 一宏*; 萩原 雅人; 西堀 英治*; 河江 達也*; 渡邊 功雄*; 内山 智貴*; Chen, Y.*; Xu, C.-N.*
Nature Communications (Internet), 15, p.9989_1 - 9989_12, 2024/11
被引用回数：0 パーセンタイル：0.00(Multidisciplinary Sciences)Like the crystallization of water to ice, magnetic transition occurs at a critical temperature after the slowing down of dynamically fluctuating short-range correlated spins. Here, we report a unique type of magnetic transition characterized by a linear increase in the volume fraction of unconventional static short-range-ordered spin clusters, which triggered a transition into a long-range order at a threshold fraction perfectly matching the bond percolation theory in a new quantum antiferromagnet of pseudo-trigonal Cu(OH)
Cl. Static short-range order appeared in its Kagome lattice plane below Ca. 20 K from a pool of coexisting spin liquid, linearly increasing its fraction to 0.492(8), then all Kagome spins transitioned into a stable two-dimensional spin order at 
_
_
_
_
$. The unconventional static nature of the short-range order was inferred to be due to a pinning effect by the strongly correlated coexisting spin liquids. This work presents a unique magnetic system to demonstrate a complete bond percolation process toward the critical transition. Meanwhile, the unconventionally developed magnetic order in this chemically clean system should shed new light on spin-liquid physics.
Chen, H. F.*; Liu, B. X.*; 徐 平光; Fang, W.*; Tong, H. C.*; Yin, F. X.*
Journal of Materials Research and Technology, 32, p.3060 - 3069, 2024/09
被引用回数：1 パーセンタイル：0.00(Materials Science, Multidisciplinary)The hot-rolled microstructure of medium Mn steel has coarse grains and severe elemental segregation, resulting in low strength and plasticity. Constructing a multiphase structure, refining the microstructure, and regulating elemental segregation enhance the mechanical properties. In this study, liquid nitrogen treatment created a layered distribution of austenite and martensite. Warm rolling was then used to reduce layer thickness and refine grain structure. After liquid nitrogen and warm rolling treatments, the strength and plasticity of medium Mn steel increased to 1270 MPa and 23.3%, respectively, far exceeding the hot-rolled state (724 MPa, 12.8%). Warm rolling also triggers austenite reverted transformation (ART) and introduces high-density dislocations, further improving austenite stability. This strengthening effect is higher than that from intercritical annealing alone. Improved austenite stability delays the transformation induced plasticity (TRIP) effect, preventing brittle fracture and enhancing deformation coordination between layers, significantly increasing the plastic deformation capacity of medium Mn steel.
archaea host diverse and interacting extrachromosomal elementsShi, L.-D.*; West-Roberts, J.*; Schoelmerich, M. C.*; Penev, P. I.*; Chen, L.-X.*; 天野 由記; Lei, S.*; Sachdeva, R.*; Banfield, J. F.*
Nature Microbiology (Internet), 9(9), p.2422 - 2433, 2024/09
被引用回数：1 パーセンタイル：39.49(Microbiology)Methane emissions that contribute to climate change can be mitigated by anaerobic methane-oxidizing archaea such as . Some have huge extrachromosomal genetic elements (ECEs) called Borgs that may modulate their activity, yet the broader diversity of ECEs is little studied. Here, we report small enigmatic linear ECEs, circular viruses and unclassified ECEs, that we predict replicate within . The linear ECEs have features such as inverted terminal repeats, pervasive tandem repeats, and coding patterns that are strongly reminiscent of Borgs, but they are only 52 kb to 145 kb in length. They share proteins with Borgs and . Thus, we refer to them as mini-Borgs. Mini-Borgs are genetically diverse and we assign them to at least five family-level groups. We also identify eight novel families of viruses, some of which encode multiheme cytochromes, and unclassified circular ECEs that encode TnpB genes. A population-heterogeneous CRISPR array is encoded in close proximity to TnpB and has spacers that target other ECEs including previously reported plasmids. The diverse groups of ECEs exchange genetic information with each other and with , likely impacting the activity and evolution of these environmentally important archaea.
Hu, F. F.*; Qin, T. Y.*; Ao, N.*; Su, Y. H.; Zhou, L.*; 徐 平光; Parker, J. D.*; 篠原 武尚; Chen, J.*; Wu, S. C.*
Engineering Fracture Mechanics, 306, p.110267_1 - 110267_18, 2024/08
被引用回数：2 パーセンタイル：55.14(Mechanics)Non-destructive and quantitative mapping of gradient residual strain distribution in surface-hardened railway S38C axles could provide a positive reference for determining service lifetime and maintenance strategy. To tackle this concern, time-of-flight neutron Bragg-edge transmission imaging was employed by real axle samples with and without impacted crater. A novel and simple procedure to formulate the residual strain field was also developed in this work, with the transmission batch code in Appendix A. By mapping the global two- dimensional residual strains, it can be verified that the residual strains into the axle are uniformly distributed in the hoop direction. Subsequently, it was revealed that the axial and hoop residual strains, respectively in the cylinder and the long strip samples prepared from a real S38C hollow axle, indicated a gradient evolution distribution with a depth of 
8 mm, covering a range of -5500 1000 
for axial strains and -6500 1000 for hoop strains. More importantly, the maximum compressive lattice strain of the cylinder sample was increased by 15.61%, and 22.35% at the impacting speeds of 100, and 125 m/s, respectively; and that of the long strip sample increased by 29.17%, and 43.70%, respectively. It can thus be concluded that lattice strains have redistributed around the impact crater, demonstrating the local alteration of the residual strain field. These new findings suggest the localized variation in residual strains should be taken into account while evaluating the service damage evolution of railway axles, especially those affected by high-speed impacts during operation.
Wang, S.*; Wang, J.*; Zhang, S.*; Wei, D.*; Chen, Y.*; Rong, X.*; Gong, W.; Harjo, S.; Liu, X.*; Jiao, Z.*; et al.
Journal of Materials Science & Technology, 185, p.245 - 258, 2024/06
被引用回数：17 パーセンタイル：98.00(Materials Science, Multidisciplinary)Nanoprecipitates and nanoscale retained austenite (RA) with suitable stability play crucial roles in determining the yield strength (YS) and ductility of ultrahigh strength steels (UHSSs). However, owing to the kinetics incompatibility between nanoprecipitation and austenite reversion, it is highly challenging to simultaneously introduce high-density nanoprecipitates and optimized RA in UHSSs. In this work, through the combination of austenite reversion treatment (ART) and subsequent flash austenitizing (FA), nanoscale chemical heterogeneity was successfully introduced into a low-cost UHSS prior to the aging process. This chemical heterogeneity involved the enrichment of Mn and Ni in the austenite phase. The resulting UHSS exhibited dual-nanoprecipitation of Ni(Al,Mn) and (Mo,Cr) C and nanoscale austenite stabilized via Mn and Ni enrichment. The hard martensitic matrix strengthened by high-density dual-nanoprecipitates constrains the plastic deformation of soft RA with a relatively low fraction, and the presence of relatively stable nanoscale RA with adequate Mn and Ni enrichment leads to a marginal loss in YS but keeps a persistent transformation-induced plasticity (TRIP) effect. As a result, the newly-developed UHSS exhibits an ultrahigh YS of 1.7 GPa, an ultimate tensile strength (UTS) of 1.8 GPa, a large uniform elongation (UE) of 8.5 percent, and a total elongation (TE) of 13 percent. The strategy of presetting chemical heterogeneity to introduce proper metastable phases before aging can be extended to other UHSSs and precipitation-hardened alloys.
CNguyen, B. V. C.*; 村上 健太*; Chena, L.*; Phongsakorn, P. T.*; Chen, X.*; 橋本 貴司; Hwang, T.*; 古澤 彰憲; 鈴木 達也*
Nuclear Materials and Energy (Internet), 39, p.101639_1 - 101639_9, 2024/06
被引用回数：1 パーセンタイル：0.00(Nuclear Science & Technology)In reactor pressure vessel materials, the formation of Mn- and Ni-rich nanoclusters is a major cause of neutron irradiation embrittlement. The segregation of these solute atoms into dislocation loops has attracted attention as a mechanism to accelerate solute clustering. In this study, the behaviors of solute Mn and Ni atoms in Fe-0.6wt.%Ni, Fe-1.4wt.%Mn, and Fe-1.4wt.%Mn-0.6wt.%Ni alloys irradiated at 400 C up to 3 dpa were analyzed using three-dimensional atom probe tomography. Solute atom clusters were observed in all materials, and their shapes were spherical, flat, and torus in FeNi, FeMn, and FeMnNi, respectively. In ternary alloy FeMnNi, Mn and Ni atoms were concentrated in the sample in the form of arcs, and the orientation of the plane containing the arcs was estimated by comparing field desorption images. The size, number density, and orientation of this structure were found to be in good agreement with those of both types of dislocation loops, namely, b = 1/2 
111
and b = 100, identified in a previous study using the same material. The positions of Ni and Mn enrichment did not fully overlap. Ni atoms tended to be concentrated more in the inner part of the loop than the Mn atoms. Mn atoms were enriched only in the vicinity of the dislocation loops, whereas Ni atoms showed a higher concentration inside the dislocation loops than in the bulk.
Linh, B. D.*; Corsi, A.*; Gillibert, A.*; Obertelli, A.*; Doornenbal, P.*; Barbieri, C.*; Duguet, T.*; G
mez-Ramos, M.*; Holt, J. D.*; Hu, B. S.*; et al.
Physical Review C, 109(3), p.034312_1 - 034312_15, 2024/03
被引用回数：2 パーセンタイル：74.11(Physics, Nuclear)理化学研究所RIビームファクトリーにて中性子過剰核
Arビームからの1中性子ノックアウト反応実験を行い、
Arのエネルギー準位および分光学的因子を導出した。特に、第一励起状態の
への分光学的因子が大きいことから、始状態のArの基底状態において中性子が
軌道を多く占めていることがわかった。これは、中性子数32がよい魔法数として知られる
Caとは異なった性質であり、カルシウムからアルゴンへと陽子が2個減ることで閉殻構造が大きく崩れることが明らかになった。
R
hm, W.*; 伴 信彦*; Chen, J.*; Li, C.*; Dobynde, M.*; Durante, M.*; El-Jaby, S.*; 込山 立人*; 小笹 晃太郎*; 佐藤 達彦; et al.
Journal of Medical Physics - Zeitschrift fr medizinische Physik -, 34(1), p.4 - 13, 2024/02
国際放射線防護委員会(ICRP)は、過去90年間に渡って世界各国や国際的な放射線防護の枠組み作りに貢献してきた。2019年、ICRPは宇宙飛行士の放射線防護に関わる様々な問題に対応したタスクグループ(TG115)を立ち上げ、地上の放射線防護体系と宇宙の放射線防護体系との共通の枠組み作りに取り組んでいる。本論文では、現時点でICRPが定めている宇宙放射線防護体系についてとりまとめて報告する。
Shavers, M. R.*; Semones, E. J.*; Shurshakov, V.*; Dobynde, M.*; 佐藤 達彦; 込山 立人*; Tomi, L.*; Chen, J.*; El-Jaby, S.*; Straube, U.*; et al.
Journal of Medical Physics - Zeitschrift fr medizinische Physik -, 34(1), p.31 - 43, 2024/02
本論文では、国際宇宙ステーションに協力している宇宙機関が、それぞれの評価方法で推定した宇宙線被ばく線量及びそのリスクを相互比較した結果を報告する。比較するミッションには、30日間の磁気圏外ミッションを選択し、宇宙線源として銀河宇宙線と太陽高エネルギー粒子の両方を考慮した。本比較結果より、各機関の線量・リスク評価方法に関する一貫性を確認することができた。本成果は、国際放射線防護委員会(ICRP)のタスクグループ115のレポートとして将来、まとめられる予定である。
都留 智仁; Han, S.*; 松浦 周太郎*; Chen, Z.*; 岸田 恭輔*; Lobzenko, I.; Rao, S.*; Woodward, C.*; George, E.*; 乾 晴行*
Nature Communications (Internet), 15, p.1706_1 - 1706_10, 2024/02
被引用回数：31 パーセンタイル：98.70(Multidisciplinary Sciences)耐火ハイエントロピー合金(RHEA)は、超高温用途への応用の可能性から注目されている。しかし、体心立方結晶をもつため面心立方HEAよりも脆く、さらに、主要なNi基超合金やFCC合金系の材料よりも著しく低いクリープ強度を示す。これらの欠点を克服し、RHEAを実用的な構造材料に発展させるためには、強度と延性を制御する要因の基礎的な理解を深める必要がある。本研究では、TiZrHfNbTaとVNbMoTaWという2つのモデルRHEAを調査し、前者は77Kまで塑性圧縮可能であるのに対し、後者は298K以下では圧縮不可能であることを示した。TiZrHfNbTaの六方最密充填(HCP)元素は、すべての構成元素がBCCであるVNbMoTaWと比較して、転位芯エネルギーを下げ、格子歪みを大きくし、せん断弾性率を下げることで、高い延性と相対的に高い降伏強度につながることがわかった。転位芯構造はVNbTaMoWではコンパクトで、TiZrHfNbTaでは拡張しており、2つのRHEAで異なる滑り面が活性化していることがわかった。これらは、いずれもHCP元素の濃度に起因していることが第一原理計算により明らかになった。この結果は、HCP元素とBCC元素の比率に関連した電子構造の変化を利用して、強度、延性、すべり挙動を制御し、より効率的な発電所や輸送のための次世代高温材料を開発できることを実証している。
Hwang, Y.*; Puebla, J.*; 近藤 浩太*; Gonzalez-Ballestero, C.*; 一色 弘成*; S
nchez Mu
oz, C.*; Liao, L.*; Chen, F.*; Luo, W.*; 前川 禎通*; et al.
Physical Review Letters, 132(5), p.056704_1 - 056704_7, 2024/01
被引用回数：17 パーセンタイル：97.80(Physics, Multidisciplinary)Here, we report the observation of strong coupling between magnons and surface acoustic wave (SAW) phonons in a thin CoFeB film constructed in an on-chip SAW resonator by analyzing SAW phonon dispersion anticrossings. We employ a nanostructured SAW resonator design that, in contrast to conventional SAW resonators, allows us to enhance shear-horizontal strain. Crucially, this type of strain couples strongly to magnons. Our device design provides the tunability of the film thickness with a fixed phonon wavelength, which is a departure from the conventional approach in strong magnon-phonon coupling research. We detect a monotonic increase in the coupling strength by expanding the film thickness, which agrees with our theoretical model. Our work offers a significant way to advance fundamental research and the development of devices based on magnon-phonon hybrid quasiparticles.
Zhang, A.*; Deng, K.*; Sheng, J.*; Liu, P.*; Kumar, S.*; 島田 賢也*; Jiang, Z.*; Liu, Z.*; Shen, D.*; Li, J.*; et al.
Chinese Physics Letters, 40(12), p.126101_1 - 126101_8, 2023/12
被引用回数：11 パーセンタイル：85.96(Physics, Multidisciplinary)In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect. Recently, itis predicted that in the nonrelativistic limit of certain collinear antiferromagnets, there exists a type of chiral "Dirac-like" fermion, whose dispersion manifests four-fold degenerate crossing points formed by spin-degenerate linear bands, with topologically protected Fermi arcs. Here, by combining with neutron diffraction and first-principles calculations, we suggest a multidomain collinear antiferromagnetic configuration, rendering the existence of the Fermi-arc surface states induced by chiral Dirac-like fermions.
Ca cast doubt on a doubly magic 
CaChen, S.*; Browne, F.*; Doornenbal, P.*; Lee, J.*; Obertelli, A.*; 角田 佑介*; 大塚 孝治*; 茶園 亮樹*; Hagen, G.*; Holt, J. D.*; et al.
Physics Letters B, 843, p.138025_1 - 138025_7, 2023/08
被引用回数：9 パーセンタイル：89.00(Astronomy & Astrophysics)
Scからの1陽子ノックアウト反応を用いて、
Caと
Caのガンマ崩壊を観測した。Caでは1456(12)keVの
線遷移が、Caでは1115(34)keVの遷移が観測された。どちらの遷移も暫定的に
と割り当てられた。有効核子間相互作用をわずかに修正した広い模型空間での殻模型計算では、
準位エネルギー、2中性子分離エネルギー、反応断面積が実験とよく一致し、N=34閉殻の上に新しい殻が形成されていることを裏付けた。その構成要素である
と
軌道はほぼ縮退しており、これはCaが二重魔法核である可能性を排除し、Ca同位体のドリップラインを
Caあるいはそれ以上にまで広げる可能性がある。
Jiang, X.*; 服部 高典; Xu, X.*; Li, M.*; Yu, C.*; Yu, D.*; Mole, R.*; 矢野 真一郎*; Chen, J.*; He, L.*; et al.
Materials Horizons, 10(3), p.977 - 982, 2023/03
被引用回数：26 パーセンタイル：93.14(Chemistry, Multidisciplinary)現在の蒸気圧縮式冷凍機に代わる環境に優しい冷凍機として、バロカロリック効果に基づく固体冷凍機が世界的に注目されている。一般に、バロカロリック効果が発現する相はいずれも常圧でも存在する。ここでは、それらの物質と違って、KPFが高圧の菱面体晶相を生成することにより、巨大なバロカロリック効果を示すことを実証した。相図は、圧力依存の熱量測定、ラマン散乱測定、中性子回折測定に基づいて構築されたものである。本研究は、巨大バロカロリー効果に、高圧相の生成という新たな手法をもたらすと期待される。
Chen, J.*; 山本 慧; Zhang, J.*; Ma, J.*; Wang, H.*; Sun, Y.*; Chen, M.*; Liu, S.*; Gao, P.*; Yu, D.*; et al.
Physical Review Applied (Internet), 19(2), p.024046_1 - 024046_9, 2023/02
被引用回数：6 パーセンタイル：62.75(Physics, Applied)Coherent coupling in magnon based hybrid system has many potential applications in quantum information processing. Magnons can propagate in magnetically ordered materials without any motion of electrons, offering a unique method to build low-power-consumption devices and information channels free of heat dissipation. In this article, we demonstrate the coherent propagation of hybridized modes between spin waves and Love surface acoustic waves in a multiferroic BiFeO
and ferromagnetic La
Sr
MnO based heterostructure. The magneto-elastic coupling enables a giant enhancement of strength of the hybridized mode by a factor of 26 compared to that of the pure spin waves. A short wavelength down to 250 nm is demonstrated for the hybridized mode, which is desirable for nanoscale acousto-magnonic applications. Our combined experimental and theoretical analyses represent an important step towards the coherent control in hybrid magnonics, which may inspire the study of magnon-phonon hybrid systems for coherent information processing and manipulation.
island of inversion; First study of low-lying bound excited states in 
V and 
VElekes, Z.*; Juhsz, M. M.*; Sohler, D.*; Sieja, K.*; 吉田 数貴; 緒方 一介*; Doornenbal, P.*; Obertelli, A.*; Achouri, N. L.*; 馬場 秀忠*; et al.
Physical Review C, 106(6), p.064321_1 - 064321_10, 2022/12
被引用回数：3 パーセンタイル：43.00(Physics, Nuclear)VとVの低励起準位構造を初めて探索した。Vについては中性子ノックアウト反応と陽子非弾性散乱が、Vについては中性子ノックアウト反応データが得られた。Vについては4つ、Vについては5つの新たな遷移が確認された。Lenzi-Nowacki-Poves-Sieja (LNPS)相互作用に基づく殻模型計算との比較によって、それぞれの同位体について確認されたガンマ線のうち3つが、first 11/2
状態とfirst 9/2状態からの崩壊と決定された。Vについては、(
,
)非弾性散乱断面積は四重極変形と十六重極変形を想定したチャネル結合法により解析されたが、十六重極変形の影響により、明確に反転の島に属するとは決定できなかった。
neutron orbital and the 
shell closure in CaEnciu, M.*; Liu, H. N.*; Obertelli, A.*; Doornenbal, P.*; Nowacki, F.*; 緒方 一介*; Poves, A.*; 吉田 数貴; Achouri, N. L.*; 馬場 秀忠*; et al.
Physical Review Letters, 129(26), p.262501_1 - 262501_7, 2022/12
被引用回数：18 パーセンタイル：86.28(Physics, Multidisciplinary)230MeV/nucleonでのCaからの中性子ノックアウト反応が線分光と行われ、
と
軌道からの中性子ノックアウト反応の運動量分布が測定された。断面積はの閉殻と整合し、Ca同位体での
と
閉殻と同程度に強い閉殻であることが確認された。運動量分布の分析から
と軌道の平均二乗根半径の差は0.61(23)fmと決定され、これはmodified-shell-modelによる予言の0.7fmと整合した。これは、中性子過剰なCa同位体での軌道半径が大きいことが、中性子数にしたがって線形的に荷電半径が増える意外な現象の原因であることを示唆している。
Chen, L.*; Mao, C.*; Chung, J.-H.*; Stone, M. B.*; Kolesnikov, A. I.*; Wang, X.*; 村井 直樹; Gao, B.*; Delaire, O.*; Dai, P.*
Nature Communications (Internet), 13, p.4037_1 - 4037_7, 2022/07
被引用回数：22 パーセンタイル：81.53(Multidisciplinary Sciences)Spin and lattice are two fundamental degrees of freedom in a solid, and their fluctuations about the equilibrium values in a magnetic ordered crystalline lattice form quasiparticles termed magnons (spin waves) and phonons (lattice waves), respectively. In most materials with strong spin-lattice coupling (SLC), the interaction of spin and lattice induces energy gaps in the spin wave dispersion at the nominal intersections of magnon and phonon modes. Here we use neutron scattering to show that in the two-dimensional (2D) van der Waals honeycomb lattice ferromagnetic CrGeTe, spin waves propagating within the 2D plane exhibit an anomalous dispersion, damping, and breakdown of quasiparticle conservation, while magnons along the c axis behave as expected for a local moment ferromagnet. These results indicate the presence of dynamical SLC arising from the zero-temperature quantum fluctuations in CrGeTe, suggesting that the observed in-plane spin waves are mixed spin and lattice quasiparticles fundamentally different from pure magnons and phonons.
