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論文

Tolerance of spin-Seebeck thermoelectricity against irradiation by swift heavy ions

岡安 悟; 針井 一哉*; 小畠 雅明; 吉井 賢資; 福田 竜生; 石田 真彦*; 家田 淳一; 齊藤 英治

Journal of Applied Physics, 128(8), p.083902_1 - 083902_7, 2020/08

The ion-irradiation tolerance of thermoelectric devices based on the spin Seebeck effect (SSE) was investigated by using 320 MeV gold ion (Au$$^{24+}$$) beams modeling cumulative damages due to fission products emitted from the surface of spent nuclear fuels. For this purpose, prototypical Pt/Y$$_3$$Fe$$_5$$O$$_{12}$$/Gd$$_3$$Ga$$_5$$O$$_{12}$$ SSE elements were irradiated with varying the dose level at room temperature and measured the SSE voltage of them. We confirmed that the thermoelectric and magnetic properties of the SSE elements are not affected by the ion-irradiation up to $$10^{10}$$ ions/cm$$^2$$ fluence and that the SSE signal is extinguished around $$10^{12}$$ ions/cm$$^2$$, in which the ion tracks almost fully cover the sample surface. We also performed the hard X-ray photoemission spectroscopy (HAXPES) measurements to understand the effects at the interface of Pt/Y$$_3$$Fe$$_5$$O$$_{12}$$. The HAXPES measurements suggest that the chemical reaction that diminishes the SSE signals is enhanced with the increase of the irradiation dose. The present study demonstrates that SSE-based devices are applicable to thermoelectric generation even in harsh environments for a long time period.

論文

Hard X-ray photoelectron spectroscopy study of Pt/Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$

小畠 雅明; 吉井 賢資; 福田 竜生; 川崎 郁斗; 岡根 哲夫; 山上 浩志; 矢板 毅; 針井 一哉; 家田 淳一; 岡安 悟; et al.

JPS Conference Proceedings (Internet), 30, p.011192_1 - 011192_6, 2020/03

スピンゼーベック効果を示す系として注目されているPt/Y$$_{3}$$Fe$$_{5}$$O$$_{12}$$(YIG)系に対し、放射光を用いた硬X線光電子分光(HAXPES)により表面及び界面の電子状態測定を行った。本系ではスピンゼーベック効果のほかに特異な性質を示すことが報告されている。例えば、外部磁場が存在しない状況でもホール効果を発現する。この起源として、YIG中のFe$$^{3+}$$イオンがPt膜に染み出し、磁性を持つ金属間化合物を生成している可能性が提案されている。そこでHAXPESの分析深さを利用し、界面近傍の鉄イオン等の電子状態を測定した。Ptの厚みが2nm, 5nm, 8nm, 10nmの試料を測定したところ、2nmと5nmの試料において鉄イオンの分析を行うことができた。Fe 1s光電子スペクトルからは、鉄イオンが3+のものと金属的な0価に近い2つの状態が存在することが判明し、上記の可能性を支持する結果が得られた。Pt 4fやO 1sスペクトルなども測定しており、詳しい結果は当日報告する。

論文

Negative muonium ion production with a C12A7 electride film

大谷 将士*; 深尾 祥紀*; 二ツ川 健太*; 河村 成肇*; 的場 史郎*; 三部 勉*; 三宅 康宏*; 下村 浩一郎*; 山崎 高幸*; 長谷川 和男; et al.

Journal of Physics; Conference Series, 1350, p.012067_1 - 012067_6, 2019/12

 被引用回数:0 パーセンタイル:100

負ミューオニウムはそのユニークな性質から様々な科学の分野で応用される可能性がある。1980年代に真空中で初めて生成されて以来、仕事関数の低い物質を用いて負ミューオニウム生成効率を高めることが議論されてきた。アルミナセメントの構成物質であるC12A7は良く知られた絶縁体であるが、電子をドープすることで導体として振舞うことが近年発見された。このC12A7エレクトライドは2.9eVという比較的低い仕事関数を持ち、負イオン生成効率を示すと期待されている。本論文では、従来用いていたアルミニウム、C12A7エレクトライド、さらにステンレスターゲット用いた負ミューオニウムイオン生成効率の比較について述べる。測定された生成率は10$$^{-3}$$/sであり、現状セットアップではエレクトライドにおいても大きな生成率向上は確認されず、表面状態をより注意深く整える必要であることが推定される。また、生成された負ミューオニウムの平均エネルギーに材質依存はなく、0.2$$pm$$0.1keVであった。

論文

Genetic survey of indigenous microbial eukaryotic communities, mainly fungi, in sedimentary rock matrices of deep terrestrial subsurface

齋藤 禎一*; 平野 伸一*; 長岡 亨*; 天野 由記

Ecological Genetics and Genomics, 12, p.100042_1 - 100042_9, 2019/10

培養に依存しない分子生物学的手法によって、さまざまな環境中の微生物群集組成について分析が可能となった。これらの手法により、嫌気的で太陽光の存在しない、高温・高圧の極限環境からも多くの未培養原核生物が検出されている。近年、深海環境においても真核生物が検出されており、その結果真核生物が従来考えられてきたよりも広範囲にわたって生息可能であることが示された。本研究では、幌延深地層研究センターの地下施設深度250mの環境において、分子生物学的手法を用いた真核生物に関する研究を行った。その結果、幌延の深部堆積岩環境において、菌類が真核生物群集の優占種であることが示された。また、岩石試料中からZygomycete, Basidiomycete, Ascomyceteのような様々な種の菌類が検出された。本研究は、深部堆積岩地下環境における真核生物の多様性に関する研究として世界初の成果である。

論文

Beam commissioning of muon beamline using negative hydrogen ions generated by ultraviolet light

中沢 雄河*; Bae, S.*; Choi, H.*; Choi, S.*; 飯嶋 徹*; 飯沼 裕美*; 河村 成肇*; 北村 遼; Kim, B.*; Ko, H. S.*; et al.

Nuclear Instruments and Methods in Physics Research A, 937, p.164 - 167, 2019/09

 被引用回数:1 パーセンタイル:53.3(Instruments & Instrumentation)

再加速された熱ミューオンビームを用いたミューオンの異常磁気モーメント及び電気双極子モーメント精密測定実験用のミューオンリニアックを開発中である。このリニアックのためのUV光駆動の負水素イオン源を開発した。ミューオン加速実験の前にこのイオン源を用いたビームラインの調整を行った。加速ミューオンの分別に必要な偏向電磁石の磁場強度を負水素ビームを用いて確認することができた。このイオン源はミューオンビームラインのコミッショニングに広く用いることができる。

論文

Study on optical properties of metallic sodium by vacuum ultra violet in UVSOR

河口 宗道; 斉藤 淳一; 大道 博行*; 末元 徹*

UVSOR-46, P. 89, 2019/08

本研究は、真空紫外光が金属ナトリウムを透過する現象を理論的に解明するために、UVSORを利用して正確なスペクトルを取得するのが目的である。特別な容器を設計製作することにより、ナトリウム試料は測定時においても金属光沢を維持していることを確認した。UVSORの測定の結果から、MgF$$_2$$窓に真空紫外光を透過しにくい層が出来てしまった可能性が示されたので、今後解決して再測定を行う計画である。

論文

Revising the 4${it f}$ symmetry in CeCu$$_{2}$$Ge$$_{2}$$; Soft X-ray absorption and hard X-ray photoemission spectroscopy

荒谷 秀和*; 中谷 泰博*; 藤原 秀紀*; 川田 萌樹*; 金井 惟奈*; 山神 光平*; 藤岡 修平*; 濱本 諭*; 久我 健太郎*; 木須 孝幸*; et al.

Physical Review B, 98(12), p.121113_1 - 121113_6, 2018/09

AA2018-0352.pdf:1.16MB

 被引用回数:3 パーセンタイル:61.62(Materials Science, Multidisciplinary)

We present a detailed study on the $$4f$$ ground state symmetry of the pressure-induced superconductor CeCu$$_2$$Ge$$_2$$ probed by soft X-ray absorption and hard X-ray photoemission spectroscopy. The revised Ce $$4f$$ ground states are determined as $$|{Gamma_7}rangle=sqrt{0.45}|{J_{z}=pm frac{5}{2}}rangle - sqrt{0.55}|{mp frac{3}{2}}rangle$$ with $$Sigmamathchar`-{rm type}$$ in-plane rotational symmetry. This gives an in-plane magnetic moment consistent with the antiferromagnetic moment as reported in neutron measurements. Since the in-plane symmetry is the same as that for the superconductor CeCu$$_2$$Si$$_2$$, we propose that the charge distribution along the $$c$$-axis plays an essential role in driving the system into a superconducting phase.

論文

First muon acceleration using a radio-frequency accelerator

Bae, S.*; Choi, H.*; Choi, S.*; 深尾 祥紀*; 二ツ川 健太*; 長谷川 和男; 飯嶋 徹*; 飯沼 裕美*; 石田 勝彦*; 河村 成肇*; et al.

Physical Review Accelerators and Beams (Internet), 21(5), p.050101_1 - 050101_6, 2018/05

 被引用回数:9 パーセンタイル:13.16(Physics, Nuclear)

ミューオンがRF加速器によって初めて加速された。正ミューオンと電子の束縛状態である負ミューオニウムをアルミ標的中での電子獲得反応によって生成し、静電加速器により初期加速する。それを高周波四重極加速空洞(RFQ)によって89keVまで加速した。加速された負ミューオニウムは、偏向電磁石による運動量の測定と飛行時間により同定された。このコンパクトなミューオン加速器は、素粒子物理や物性物理などのミューオン加速器の様々な応用への第一歩である。

論文

Evaluation of thermal strain induced in components of Nb$$_{3}$$Sn strand during cooling

諏訪 友音*; 辺見 努*; 齊藤 徹*; 高橋 良和*; 小泉 徳潔*; Luzin, V.*; 鈴木 裕士; Harjo, S.

IEEE Transactions on Applied Superconductivity, 28(3), p.6001104_1 - 6001104_4, 2018/04

 被引用回数:0 パーセンタイル:100(Engineering, Electrical & Electronic)

Nb$$_{3}$$Sn strands, whose properties are very sensitive to stress/strain, are utilized for ITER cable-in-conduit conductor (CICC) of the central solenoids. The Nb$$_{3}$$Sn strands experience temperature range of $$sim$$1000 K from the temperature of the heat treatment with the initiation of the Nb$$_{3}$$Sn reaction to the operation temperature of $$sim$$4 K. Due to this large temperature range, large thermal strain is induced in the Nb$$_{3}$$Sn filaments due to the differences between the coefficients of thermal expansion and Young's moduli of the components of the strand. Therefore, it is considered that initial performance of the CICC is influenced by the thermal strain on the Nb$$_{3}$$Sn, and it is important to evaluate the strain state of the Nb$$_{3}$$Sn strand at low temperature. In this study, the thermal strain of the components of free Nb$$_{3}$$Sn strand was measured by neutron diffraction and stress/strain state was assessed from room temperature to low temperature. As the results of diffraction measurements, it was found that 0.111 % and 0.209 % compressive strain were generated in Nb$$_{3}$$Sn filaments at 300 and 10 K, respectively.

論文

New precise measurement of muonium hyperfine structure interval at J-PARC

上野 恭裕*; 青木 正治*; 深尾 祥紀*; 東 芳隆*; 樋口 嵩*; 飯沼 裕美*; 池戸 豊*; 石田 啓一*; 伊藤 孝; 岩崎 雅彦*; et al.

Hyperfine Interactions, 238(1), p.14_1 - 14_6, 2017/11

 被引用回数:3 パーセンタイル:12.84

MuSEUM is an international collaboration aiming at a new precise measurement of the muonium hyperfine structure at J-PARC (Japan Proton Accelerator Research Complex). Utilizing its intense pulsed muon beam, we expect a ten-fold improvement for both measurements at high magnetic field and zero magnetic field. We have developed a sophisticated monitoring system, including a beam profile monitor to measure the 3D distribution of muonium atoms to suppress the systematic uncertainty.

論文

Shell evolution beyond $$Z$$=28 and $$N$$=50; Spectroscopy of $$^{81,82,83,84}$$Zn

Shand, C. M.*; Podoly$'a$k, Zs.*; G$'o$rska, M.*; Doornenbal, P.*; Obertelli, A.*; Nowacki, F.*; Otsuka, T.*; Sieja, K.*; Tostevin, J. A.*; Tsunoda, T.*; et al.

Physics Letters B, 773, p.492 - 497, 2017/10

 被引用回数:13 パーセンタイル:12.29(Astronomy & Astrophysics)

Low-lying states in neutron-rich $$^{81,82.83.84}$$Zn nuclei were measured for the first time via in-beam $$gamma$$-ray spectroscopy at RIKEN. These include the 4$$_1^+$$ to 2$$_1^+$$ in $$^{82}$$Zn and the 2$$_1^+$$ to 0$$_1^+$$ and 4$$_1^+$$ to 2$$_1^+$$ in $$^{84}$$Zn. The reduced E($$2^+$$) energies and increased E(4$$^+$$)/E(2$$^+$$) ratios at $$N$$=52,54 compared to $$^{80}$$Zn attest that the magicity is confined just on the neutron number $$N$$=50 only. The levels observed in $$^{84}$$Zn suggest the onset of deformation towards heavier Zn isotopes. The data were compared to state-of-the-art shell model calculations.

論文

Two-phase flow measurements in a simulated debris bed

伊藤 大介*; Rivera, M. N.*; 齊藤 泰司*; 青柳 光裕; 神山 健司; 鈴木 徹*

Proceedings of 17th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-17) (USB Flash Drive), 10 Pages, 2017/09

Two-phase flow through porous media must be well understood to develop a severe accident analysis code not only for light water reactor (LWR) but also sodium-cooled fast reactor (SFR). When a core disruptive accident occurs in SFR, the fuel inside the core become melted and interacts with the coolant. As a result, gas-liquid two-phase flow will be formed in the debris bed, which may have porous nature depending on the cooling process. Thus, as first step, the present work focuses on the characteristics of pressure drop in two-phase flows in different porous media conditions (porous size, liquid and gas flow velocity). To construct an experimental database, the measured pressure drop under different conditions was compared with existing correlations. In addition, X-ray radiography, which is very helpful to understand the two-phase structure inside the porous media, was applied to measure porosity and void fraction distribution in the packed bed of spheres.

論文

Measurements of two-phase pressure drop in a simulated debris bed

Nava, M.*; 伊藤 大介*; 齊藤 泰司*; 青柳 光裕; 神山 健司; 鈴木 徹*

Proceedings of 25th International Conference on Nuclear Engineering (ICONE-25) (CD-ROM), 5 Pages, 2017/07

Two-phase flow through porous media should be well understood to develop a severe accident analysis code not only for light water reactor but also sodium cooled fast reactor (SFR). When a core disruptive accident occurs in SFR, the fuel inside the core become melted and interacts with the coolant. As a result, gas-liquid two-phase flow will be formed in the debris bed, which may have porous nature depending on the cooling process. Thus, as first step, the present work focuses on the characteristics of pressure drop in single and two-phase flows in different porous media conditions (porous size, liquid and gas flow velocity). In addition, in order to construct an experimental database, the measured pressure drop under different conditions was compared with existing correlations.

論文

Evaluation of bending strain in Nb$$_{3}$$Sn strands of CIC conductor using neutron diffraction

辺見 努*; Harjo, S.; 梶谷 秀樹*; 諏訪 友音*; 齊藤 徹*; 相澤 一也; 長村 光造*; 小泉 徳潔*

IEEE Transactions on Applied Superconductivity, 27(4), p.4200905_1 - 4200905_5, 2017/06

 被引用回数:0 パーセンタイル:100(Engineering, Electrical & Electronic)

The superconducting property of Nb$$_{3}$$Sn strands is very sensitive to strain. The transverse electromagnetic loading has been considered as a major origin of the degradation of Nb$$_{3}$$Sn cable-in-conduit conductors (CICCs) due to the local bending. Since the bending pitch is around 5 mm due to contacting of strands compacted by the electromagnetic transverse loading, there is a possibility of a large bending strain with small deflection of strands. The bending strain of the strands cannot be evaluated from only the small deflection obtained visually. Measuring bending strain of Nb$$_{3}$$Sn strand in CICCs is important for evaluating the conductor performance. Neutrons, which have a large penetration depth, are a powerful tool to evaluate the internal strain of Nb$$_{3}$$Sn in the CICC. This paper shows that the bending strain in Nb$$_{3}$$Sn strands of CICCs can be determined by the neutron diffraction profile nondestructively and quantitatively.

論文

Shape evolution in neutron-rich krypton isotopes beyond N=60; First spectroscopy of $$^{98,100}$$Kr

Flavigny, F.*; Doornenbal, P.*; Obertelli, A.*; Delaroche, J.-P.*; Girod, M.*; Libert, J.*; Rodriguez, T. R.*; Authelet, G.*; 馬場 秀忠*; Calvet, D.*; et al.

Physical Review Letters, 118(24), p.242501_1 - 242501_6, 2017/06

 被引用回数:21 パーセンタイル:10.34(Physics, Multidisciplinary)

The first $$gamma$$-ray spectroscopy of very neutron rich $$^{98,100}$$Kr isotopes was carried out at the RIBF at RIKEN Nishina center. Excited states in these isotopes were populated via (p,2p) reactions using radioactive $$^{99,101}$$Rb beams accelerated to 220 MeV/nucleon. The new data show a significant increase in deformation beyond N=60, as well as competing configurations (shape-coexistence) at low energy. The data were compared with beyond-mean-field calculations which predict level energies in good agreement with observation, and suggest oblate-prolate shape coexistence.

論文

Characteristics of pressure drop and void fraction in a simulated debris bed

伊藤 大介*; Nava, M.*; 齊藤 泰司*; 青柳 光裕; 神山 健司; 鈴木 徹*

Proceedings of 2017 Japan-US Seminar on Two-Phase Flow Dynamics (JUS 2017), 4 Pages, 2017/06

Two-phase flow through porous media should be well understood to develop a severe accident analysis code not only for light water reactor but also sodium-cooled fast reactor (SFR). When a core disruptive accident occurs in SFR, the fuel inside the core become melted and interacts with the coolant. As a result, gas-liquid two-phase flow will be formed in the debris bed, which may have porous nature depending on the cooling process. Thus, as first step, the present work focuses on the characteristics of pressure drop in two-phase flows in different porous media conditions (porous size, liquid and gas flow velocity). In addition, to construct an experimental database, the measured pressure drop under different conditions was compared with existing correlations.

論文

$$gamma$$ decay of unbound neutron-hole states in $$^{133}$$Sn

Vaquero, V.*; Jungclaus, A.*; Doornenbal, P.*; Wimmer, K.*; Gargano, A.*; Tostevin, J. A.*; Chen, S.*; N$'a$cher, E.*; Sahin, E.*; 志賀 慶明*; et al.

Physical Review Letters, 118(20), p.202502_1 - 202502_5, 2017/05

 被引用回数:13 パーセンタイル:17.71(Physics, Multidisciplinary)

Excited states in $$^{133}$$Sn were populated following one-neutron knockout reaction from an unstable $$^{134}$$Sn beam at the RIBF laboratory in RIKEN. In addition to the already known $$gamma$$ rays, additional $$gamma$$ strength was observed for the first time in the excitation-energy range 3.5-5.5 MeV. Since the neutron separation energy of $$^{133}$$Sn is low, this observation provides direct evidence for the radioactive decay of neutron-unbound states in this nucleus. The ability of $$gamma$$ decay to compete with neutron emission was attributed to a mismatch between the wave functions of the initial and final states in the neutron emission case. These findings suggest that in the region south-east of $$^{132}$$Sn, nuclear structure effects play a significant role in the decay of unbound states, which are instead usually ignored in the evaluation of neutron-emission probabilities in astrophysical simulations.

論文

Low-lying structure and shape evolution in neutron-rich Se isotopes

Chen, S.*; Doornenbal, P.*; Obertelli, A.*; Rodriguez, T. R.*; Authelet, G.*; 馬場 秀忠*; Calvet, D.*; Ch$^a$teau, F.*; Corsi, A.*; Delbart, A.*; et al.

Physical Review C, 95(4), p.041302_1 - 041302_6, 2017/04

 被引用回数:15 パーセンタイル:9.29(Physics, Nuclear)

Neutron-rich isotopes of selenium, $$^{88,90,92,94}$$Se, where studied via in beam $$gamma$$-ray spectroscopy after nucleon removal reactions at RIBF in RIKEN. The low-energy excitations of these nuclei were investigated using $$gamma$$-$$gamma$$ coincidences, and the first and second excited 2$$^+$$ states were found at remarkably low energies. The analysis and comparison with self-consistent beyond-mean field calculations suggest that both shape coexistence and triaxiality are needed to describe these isotopes.

論文

Are there signatures of harmonic oscillator shells far from stability?; First spectroscopy of $$^{110}$$Zr

Paul, N.*; Corsi, A.*; Obertelli, A.*; Doornenbal, P.*; Authelet, G.*; 馬場 秀忠*; Bally, B.*; Bender, M.*; Calvet, D.*; Ch$^a$teau, F.*; et al.

Physical Review Letters, 118(3), p.032501_1 - 032501_7, 2017/01

 被引用回数:23 パーセンタイル:9.11(Physics, Multidisciplinary)

The first measurement of $$gamma$$ rays emitted by the very neutron rich nuclei $$^{112}$$Mo (Z=42) and $$^{110}$$Zr (Z=40) was carried out at the RIBF facility at RIKEN. These data shine light on the postulated N=70 harmonic oscillator shell. If the spin-orbit splitting which gives rise to the N=82 shell gap is reduced in very neutron-rich nuclei, the harmonic oscillator gap at N=70 should open instead. However, both the measured energy of the first excited state $$^{112}$$Mo and $$^{110}$$Zr, respectively 235(7) keV and 185(11) keV, and their E(4$$^+$$)/E(2$$^+$$) ratio, indicate that these nuclei are good rotors, and exclude the shell stabilization scenario at Z=40 and N=70. These results were compared to state-of-the-art density functional theoretical calculations using Gogny and Skyrme effective interactions.

論文

New muonium HFS measurements at J-PARC/MUSE

Strasser, P.*; 青木 正治*; 深尾 祥紀*; 東 芳隆*; 樋口 嵩*; 飯沼 裕美*; 池戸 豊*; 石田 啓一*; 伊藤 孝; 岩崎 雅彦*; et al.

Hyperfine Interactions, 237(1), p.124_1 - 124_9, 2016/12

 被引用回数:5 パーセンタイル:6.58

At the Muon Science Facility (MUSE) of J-PARC (Japan Proton Accelerator Research Complex), the MuSEUM collaboration is planning new measurements of the ground state hyperfine structure (HFS) of muonium both at zero field and at high magnetic field. The previous measurements were performed both at LAMPF (Los Alamos Meson Physics Facility) with experimental uncertainties mostly dominated by statistical errors. The new high intensity muon beam that will soon be available at MUSE H-Line will provide an opportunity to improve the precision of these measurements by one order of magnitude. An overview of the different aspects of these new muonium HFS measurements, the current status of the preparation, and the results of a first commissioning test experiment at zero field are presented.

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