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論文

Hyperfine splitting and nuclear spin polarization in NdPd$$_5$$Al$$_2$$ and Nd$$_3$$Pd$$_{20}$$Ge$$_6$$

目時 直人; 柴田 薫; 松浦 直人*; 北澤 英明*; 鈴木 博之*; 山内 宏樹; 萩原 雅人; Frontzek, M. D.*; 松田 雅昌*

Journal of the Physical Society of Japan, 91(5), p.054710_1 - 054710_6, 2022/05

NdPd$$_5$$Al$$_2$$におけるNdの超微細相互作用分裂を高分解能の中性子非弾性散乱によって研究した。Nd核の核スピン($$I$$=7/2)と、$$|pm9/2rangle$$の軌道が主成分の$$Gamma_6$$基底状態を示す4$$f$$電子との間の超微細相互作用によって、磁気秩序相において生じた超微細相互作用分裂に起因する中性子非弾性散乱ピークを、$$hbaromega$$ = $$pm$$3$$mu$$eVのエネルギーに観察した。低温では、Nd核スピンの低エネルギー状態の占拠確率が増加することによりNd核スピンが偏極し、反強磁性散乱ピーク強度に寄与するが、その際、中性子の非スピン反転過程の寄与が最も大きい。この現象の応用として反強磁性散乱ピーク強度の温度変化から、Nd$$_3$$Pd$$_{20}$$Ge$$_6$$のNd磁気モーメント及び超微細相互作用分裂の大きさを見積もることに成功した。

論文

KeV-region analysis of the neutron capture cross-section of $$^{237}$$Np

Rovira Leveroni, G.; 片渕 竜也*; 登坂 健一*; 松浦 翔太*; 児玉 有*; 中野 秀仁*; 岩本 修; 木村 敦; 中村 詔司; 岩本 信之

Journal of Nuclear Science and Technology, 59(1), p.110 - 122, 2022/01

Neutron capture cross-section measurements for $$^{237}$$Np have been conducted with the Accurate Neutron Nucleus Reaction Measurement Instrument (ANNRI) at the Materials and Life Science Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC) using neutrons with energy ranging from thermal energy to 1 MeV. A Time of Flight (TOF) method using a NaI(Tl) detector was employed for these measurements and the data were analyzed based on the pulse-height weighting technique in order to derive the neutron capture cross-section. The absolute capture cross-section was determined using the whole shape of the first resonance from JENDL-4.0 together with the total neutron flux derived from a $$^{197}$$Au sample measurement in which the first resonance was completely saturated. Both normalization techniques present agreement within 2%. The present results are also compared evaluated data libraries. There is a discrepancy of 10-25% discrepancy from 0.5 to 20 keV with JENDL-4.0. Nonetheless, above this energy, the JENDL-4.0 seems to reproduce the present data better as the results agree within uncertainties up to 500 keV. The cross-section results contain errors below 4% from 0.5 to 30 keV. However, the total uncertainty increases to over 8% over that energy. Along with the cross section measurement, theoretical calculations were performed to reproduce the present results.

論文

Microscopic dynamics of lithium diffusion in single crystal of the solid-state electrolyte La$$_{2/3-x}$$Li$$_{3x}$$TiO$$_{3}$$ (x = 0.13) studied by quasielastic neutron scattering

松浦 直人*; 藤原 靖幸*; 森分 博紀*; 尾原 幸治*; 川北 至信

Physical Review B, 104(9), p.094305_1 - 094305_7, 2021/09

 被引用回数:0

Quasielastic neutron scattering (QENS) measurements combined with first principles based molecular dynamics calculations were conducted to study the dynamics of Li$$^{+}$$ ions in a solid-state electrolyte La$$_{2/3-x}$$Li$$_{3x}$$TiO$$_{3}$$ (LLTO) with $$x = 0.13$$. By using a large $$^{7}$$Li-enriched single crystal sample, a QENS signal was clearly observed along the three principal axes [110], [111], and [001] at a temperature ($$T$$) of 600 K. Wave vector dependence of the linewidth of the QENS signal along each direction was explained well using the Chudley-Elliot model for jumps between the A sites of the perovskite lattice through the bottleneck square, which was also supported by molecular dynamics calculations. The estimated self-diffusion coefficient of Li$$^{+}$$ ($$D_{rm Li}$$) in the ab plane was slightly larger than that along the c axis, suggesting quasi-isotropic diffusion, that is, the three-dimensional diffusion of Li$$^{+}$$ ions. The decrease in $$D_{rm Li}$$ with decreasing $$T$$ was reasonably explained by a thermal activation process with the activation energy determined from ionic-conductivity measurements. Furthermore, the estimated values of the self-diffusion coefficient are comparable to those in the sulfide-based Li$$^{+}$$ ion conductor, Li$$_{7}$$P$$_{3}$$S$$_{11}$$, with 10 times larger ionic conductivity, which clarifies how to understand the Li conduction mechanism in LLTO and Li$$_{7}$$P$$_{3}$$S$$_{11}$$ in a unified manner.

論文

Position dependency of the scattered intensity in the time-of-flight backscattering spectrometer DNA

松浦 直人*; 山田 武*; 富永 大輝*; 小林 誠*; 中川 洋; 川北 至信

JPS Conference Proceedings (Internet), 33, p.011068_1 - 011068_6, 2021/03

飛行時間分析型後方散乱分光器DNAにおける散乱強度の位置依存性を調査した。垂直方向(位置敏感一次元検出器(PSD)のピクセル方向)と水平方向(PSD毎)の両方で周期的な構造が見られた。DNAに設置されたソラースリットとアナライザー結晶の設計値を超えた過度な湾曲が、強度分布の起源であると考えられる。我々は、強度の位置依存性と弾性散乱のエネルギーオフセットを系統的に補正できるソフトウェアを開発した。このソフトウェアにより、本来の散乱強度からのずれが補正でき、エネルギー分解能などのデータの質も向上させることができる。

論文

Position-encoded automatic cell elevator for BL02, J-PARC MLF

富永 大輝*; 小林 誠*; 山田 武*; 松浦 直人*; 川北 至信; 笠井 聡*

JPS Conference Proceedings (Internet), 33, p.011095_1 - 011095_5, 2021/03

トップローディング型冷凍機用の垂直移動型試料交換機が、J-PARC MLFのBL02に設置された中性子分光器の利用支援のために開発された。PEACEと名付けられたこの試料交換機は、中性子照射位置での試料位置の再現性を、PEEKと呼ぶ物質でできたガイドを利用して制御している。3つの試料位置でのバックグラウンド散乱のプロファイルの変化は$$pm$$1.6%以内であることが分かった。この結果は、垂直軸からの試料位置の偏差が$$pm$$0.3mmであることを考えると妥当である。

論文

Magnetism induced by interlayer electrons in the quasi-two-dimensional electride Y$$_{2}$$C; Inelastic neutron scattering study

玉造 博夢; 村上 洋一*; 倉本 義夫*; 佐賀山 基*; 松浦 直人*; 川北 至信; 松石 聡*; 鷲尾 康仁*; 井下 猛*; 浜田 典昭*; et al.

Physical Review B, 102(22), p.224406_1 - 224406_5, 2020/12

 被引用回数:3 パーセンタイル:58.93(Materials Science, Multidisciplinary)

Magnetic excitations in layered electride Y$$_{2}$$C have been found by inelastic neutron scattering. We have observed weak but clear magnetic scattering around the wave number $$Q = 0$$, but no magnetic order down to the lowest temperature measured (7 K). The imaginary part of the dynamical susceptibility deduced is well described by the Lorentz function of energy $$E$$ for each momentum $$Q$$. The width $$mathit{Gamma}(Q)$$ of the Lorentzian is proportional to $$Q(Q^2+kappa^{2})$$ with $$kappa^{-1} sim 4{rm AA}$$ at $$T=7$$ K. We have also found that with increasing $$Q$$ the magnetic form factor decays faster than that of a $$4d$$ electron in a single Y atom, which indicates a more extended magnetic moment in Y$$_{2}$$C. These results provide experimental evidence that the itinerant magnetism in Y$$_{2}$$C originates from the anionic electrons that reside in the interlayers. The Curie-Weiss-like behavior of the magnetic susceptibility reported in Y$$_{2}$$C is ascribed to the mode coupling effects of spin fluctuations.

論文

Fast neutron capture reaction data measurement of minor actinides for development of nuclear transmutation systems

片渕 竜也*; 岩本 修; 堀 順一*; 木村 敦; 岩本 信之; 中村 詔司; 芝原 雄司*; 寺田 和司*; Rovira, G.*; 松浦 翔太*

EPJ Web of Conferences, 239, p.01044_1 - 01044_4, 2020/09

 被引用回数:1 パーセンタイル:89.98

In 2017, a research project entitled "Study on accuracy improvement of fast-neutron capture reaction data of long-lived MAs for development of nuclear transmutation systems" started as a joint collaboration, including Tokyo Tech, Japan Atomic Energy Agency and Kyoto University. This project focuses on neutron capture reaction of MAs, especially $$^{237}$$Np, $$^{241}$$Am and $$^{243}$$Am, in the fast neutron energy region. The final goal of this project is to improve the neutron capture cross sections of $$^{237}$$Np, $$^{241}$$Am and $$^{243}$$Am employing a high-intensity neutron beam from a spallation source of the Japan Proton Accelerator Research Complex (J-PARC) that reduces uncertainties of measurement. In this contribution, the overview of the project and the current progress will be presented.

論文

Ultralow-energy magnon anomaly in yttrium iron garnet

社本 真一; 安井 幸夫*; 松浦 直人*; 赤津 光洋*; 小林 義明*; 根本 祐一*; 家田 淳一

Physical Review Research (Internet), 2(3), p.033235_1 - 033235_6, 2020/08

イットリウム鉄ガーネット結晶の超低エネルギーマグノンを、非弾性中性子散乱によって45$$mu$$eV以下のエネルギー範囲で調べたところ、[111]方向に約0.1Tの磁場が印加した場合に、10Kで超低エネルギーのマグノン異常を発見した。

論文

Magnetically induced electric polarization in Ba$$_{3}$$Fe$$_{2}$$O$$_{5}$$Cl$$_{2}$$ with tunable direction in three dimensions

阿部 伸行*; 塩澤 俊介*; 松浦 慧介*; 佐賀山 基*; 中尾 朗子*; 大原 高志; 徳永 祐介*; 有馬 孝尚*

Physical Review B, 101(18), p.180407_1 - 180407_5, 2020/05

 被引用回数:0 パーセンタイル:0(Materials Science, Multidisciplinary)

The correlation between magnetism and electric polarization in a chiral insulating magnet Ba$$_{3}$$Fe$$_{2}$$O$$_{5}$$Cl$$_{2}$$ has been investigated. The temperature dependence of magnetic susceptibility shows an anomaly at 564 K, suggesting the onset of antiferromagnetic order of Fe$$^{3+}$$ moments. Electric polarization appears in a magnetic field below TN due to the spin-direction-dependent metal-ligand hybridization. The direction of the electric polarization can be controlled in three-dimensional space by changing the direction of an external magnetic field. This compound also shows an antiferromagnetic-to-weak-ferromagnetic transition accompanied by a structural phase transition at 140 K.

論文

Neutron capture cross-section measurement and resolved resonance analysis of $$^{237}$$Np

Rovira, G.*; 片渕 竜也*; 登坂 健一*; 松浦 翔太*; 寺田 和司*; 岩本 修; 木村 敦; 中村 詔司; 岩本 信之; 瀬川 麻里子; et al.

Journal of Nuclear Science and Technology, 57(1), p.24 - 39, 2020/01

 被引用回数:4 パーセンタイル:84.6(Nuclear Science & Technology)

The neutron capture cross-section of $$^{237}$$Np has been measured in the neutron energy region of 10 meV to 500 eV. A neutron time-of-flight method was employed using the NaI(Tl) spectrometer in the ANNRI beam-line at the Japanese Proton Accelerator Re-search Complex (J-PARC). The experimental capture yield was derived using the pulse-height weighting technique and an energy dependent cross-section was obtained relative to the incident neutron spectrum derived from a $$^{10}$$B(n, $$alpha$$)$$^{7}$$Li reaction yield. The absolute cross-section was determined by normalizing the results to JENDL-4.0 cross-section data at the first resonance of $$^{237}$$Np. The thermal cross-section was measured to be 177.6 $$pm$$ 3.8 b. The resolved resonance region was analyzed with the REFIT code.

論文

Improvement in flow-sheet of extraction chromatography for trivalent minor actinides recovery

渡部 創; 先崎 達也; 柴田 淳広; 野村 和則; 竹内 正行; 中谷 清治*; 松浦 治明*; 堀内 勇輔*; 新井 剛*

Journal of Radioanalytical and Nuclear Chemistry, 322(3), p.1273 - 1277, 2019/12

 被引用回数:0 パーセンタイル:0.01(Chemistry, Analytical)

Extraction chromatography flow-sheet employing octyl(phenyl)-$$N,N$$-diisobutylcarbonoylmethylphosphine oxide (CMPO) and $$bis$$(2-ethylhexyl) hydrogen phosphate (HDEHP) extractants for trivalent minor actinide recovery was modified to improve column separation performance. Excellent trivalent minor actinides recovery performance was obtained by column separation experiments on nitric acid solution containing the trivalent minor actinides and representative fission product elements, i.e. recovery yields $$>$$ 93% with sufficient decontamination factors against the fission products. Those are the best performance which we have ever obtained by experiments inside hot cell.

論文

Estimation of planes of a rock mass in a gallery wall from point cloud data based on MD PSO

松浦 勇斗*; 早野 明; 板倉 賢一*; 鈴木 幸司*

Applied Soft Computing, 84, p.105737_1 - 105737_9, 2019/11

 被引用回数:1 パーセンタイル:16.64(Computer Science, Artificial Intelligence)

三次元レーザスキャナの計測では、計測対象物表面に対して高解像度の距離計測が行われ、その計測結果として、計測対象物表面の三次元形状を表す点群データが取得される。取得される点群データは、トンネル壁面の岩盤に分布する割れ目といった不連続面の抽出に活用することができ、その際、点群データから小平面を推定する必要がある。本研究では、点群データから小平面を推定するアルゴリズムとして多次元粒子群最適化(MD PSO)に基づく手法を開発した。MD PSOでは、点群データをバウンディングボックスにより区分し、それぞれの点の法線ベクトルを求め、それに基づき点群データを複数のクラスターに分類する。そして、それぞれのクラスターの点群データに対する最小二乗法により面が推定される。新しく開発されたMD PSOに基づくアルゴリズムを実際の坑道壁面の点群データを用いて適用性を評価した。MD PSOアルゴリズムを適用した場合、従来手法の可変格子分割法(VBS)に基づくアルゴリズムと比較して、7%高い正確性を示した。

論文

Status of neutron spectrometers at J-PARC

梶本 亮一; 横尾 哲也*; 中村 充孝; 川北 至信; 松浦 直人*; 遠藤 仁*; 瀬戸 秀紀*; 伊藤 晋一*; 中島 健次; 河村 聖子

Physica B; Condensed Matter, 562, p.148 - 154, 2019/06

BB2018-0526.pdf:2.45MB

 被引用回数:5 パーセンタイル:48.71(Physics, Condensed Matter)

Seven time-of-flight quasielastic/inelastic neutron scattering instruments are installed on six beamlines in the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (JPARC). Four of these instruments are chopper-type direct-geometry spectrometers, one is a near-backscattering indirect-geometry spectrometer, and the other two are spin-echo-type spectrometers. This paper reviews the characteristic features, recent scientific outcomes, and progress in development of MLF spectrometers.

論文

The Surface composition of asteroid 162173 Ryugu from Hayabusa2 near-infrared spectroscopy

北里 宏平*; Milliken, R. E.*; 岩田 隆浩*; 安部 正真*; 大竹 真紀子*; 松浦 周二*; 荒井 武彦*; 仲内 悠祐*; 中村 智樹*; 松岡 萌*; et al.

Science, 364(6437), p.272 - 275, 2019/04

 被引用回数:140 パーセンタイル:99.81(Multidisciplinary Sciences)

小惑星探査機はやぶさ2のターゲット天体であるリュウグウは、始原的な炭素質物質で構成されていると考えられている。はやぶさ2に搭載された近赤外分光計(NIRS3)によって、天体の表面組成を得た。天体全体の観測で、弱く細い吸収が2.72ミクロンに確認され、OHを含む鉱物の存在を示している。弱いOH吸収と低いアルベドは熱やショックによって変質を受けた炭素質コンドライトに似ている。OHバンドの位置はほとんど一定であり、衝撃片の集合によって形成されたリュウグウは組成的に均質であることを示している。

論文

Development of an alpha dust monitor using a GPS scintillator plate

森下 祐樹; 金子 純一*; 樋口 幹雄*; 井崎 賢二; 矢島 辰雄*; 松浦 貢*; 田村 健; 鳥居 建男

Radiation Measurements, 122, p.115 - 120, 2019/03

 被引用回数:5 パーセンタイル:75.46(Nuclear Science & Technology)

A dust monitor with a silicon surface barrier detector (SSBD) is introduced at a nuclear fuel facility to detect airborne contamination of $$^{238}$$Pu and $$^{239}$$Pu released by past accidents. However, an SSBD frequently produces false alarms, especially in a room with high humidity. We developed an alpha-particle spectrometer based on a cerium-doped Gd$$_{2}$$Si$$_{2}$$O$$_{7}$$ (GPS) scintillator plate and a photomultiplier tube (PMT). The energy resolution for 5.5-MeV alpha particles was $$sim$$11.9% $$pm$$ 0.2% of the FWHM. The efficiency was 92%, and it had a uniform sensitivity. By applying an energy window, the count-rate of the Rn progeny decreased by 77%. The GPS scintillator plate was able to measure the alpha spectrum even though the GPS scintillator got wet.

論文

Nuclear and thermal feasibility of lithium-loaded high temperature gas-cooled reactor for tritium production for fusion reactors

後藤 実; 奥村 啓介; 中川 繁昭; 稲葉 良知; 松浦 秀明*; 中屋 裕行*; 片山 一成*

Fusion Engineering and Design, 136(Part A), p.357 - 361, 2018/11

 被引用回数:1 パーセンタイル:17.98(Nuclear Science & Technology)

高温ガス炉にリチウム化合物を装荷し、$$^{6}$$Li(n,$$alpha$$)反応を用いて核融合炉用燃料であるトリチウムを製造する方法が提案されている。一般的な高温ガス炉の設計においては、過剰反応度を抑制するために、可燃性毒物としてホウ素が炉心に装荷される。本研究では、熱エネルギーとトリチウムの生産を両立するために、リチウムをホウ素の代わりに炉心に装荷することとした。リチウムを装荷した高温ガス炉の成立性を確認するために、核特性値及び燃料温度を計算した。これらの計算結果は設計要求を満たし、熱エネルギーとトリチウムの生産を両立するリチウム装荷高温ガス炉の成立性を確認した。

論文

Magnetic excitations in the orbital disordered phase of MnV$$_2$$O$$_4$$

松浦 慧介*; 佐賀山 基*; 上原 周*; 新居 陽一*; 梶本 亮一; 蒲沢 和也*; 池内 和彦*; Ji, S.*; 阿部 伸行*; 有馬 孝尚*

Physica B; Condensed Matter, 536, p.372 - 376, 2018/05

 被引用回数:2 パーセンタイル:16.65(Physics, Condensed Matter)

We have investigated the temperature dependence of magnetic dynamics in a spinel-type vanadium oxide MnV$$_2$$O$$_4$$ by inelastic neutron scattering. The scattering intensity of excitation around 20 meV disappears in the collinear intermediate-temperature cubic-ferrimagnetic phase, which reveals that this excitation should be peculiar to the orbital ordered phase. We have found a weakly dispersive mode emergent from a non-integer wavevector $$(1.4,1.4,0)$$ at 56 K, which lies in the cubic-ferrimagnetic phase between non-coplanar ferrimagnetic and paramagnetic phases. This indicates that the probable presence of an incommensurate instability in the simple collinear structure.

論文

Maximizing $$T_c$$ by tuning nematicity and magnetism in FeSe$$_{1-x}$$S$$_x$$ superconductors

松浦 康平*; 水上 雄太*; 新井 佑基*; 杉村 優一*; 前島 尚行*; 町田 晃彦*; 綿貫 徹*; 福田 竜生; 矢島 健*; 広井 善二*; et al.

Nature Communications (Internet), 8, p.1143_1 - 1143_6, 2017/10

 被引用回数:59 パーセンタイル:92.87(Multidisciplinary Sciences)

A fundamental issue concerning iron-based superconductivity is the roles of electronic nematicity and magnetism in realising high transition temperature ($$T_c$$). To address this issue, FeSe is a key material, as it exhibits a unique pressure phase diagram involving nonmagnetic nematic and pressure-induced antiferromagnetic ordered phases. However, as these two phases in FeSe have considerable overlap, how each order affects superconductivity remains perplexing. Here we construct the three-dimensional electronic phase diagram, temperature ($$T$$) against pressure ($$P$$) and iso-valent S-substitution ($$x$$), for FeSe$$_{1-x}$$S$$_x$$. By simultaneously tuning chemical and physical pressures, against which the chalcogen height shows a contrasting variation, we achieve a complete separation of nematic and antiferromagnetic phases. In between, an extended nonmagnetic tetragonal phase emerges, where $$T_c$$ shows a striking enhancement. The completed phase diagram uncovers that high-$$T_c$$ superconductivity lies near both ends of the dome-shaped antiferromagnetic phase, whereas $$T_c$$ remainslow near the nematic critical point.

論文

Spin-orbital correlated dynamics in the spinel-type vanadium oxide MnV$$_{2}$$O$$_{4}$$

松浦 慧介*; 佐賀山 基*; 上原 周*; 新居 陽一*; 梶本 亮一; 蒲沢 和也*; 池内 和彦*; Ji, S.*; 阿部 伸行*; 有馬 孝尚*

Physical Review Letters, 119(1), p.017201_1 - 017201_6, 2017/07

 被引用回数:8 パーセンタイル:63.32(Physics, Multidisciplinary)

We investigate the magnetic dynamics in the spinel-type vanadium oxide MnV$$_2$$O$$_4$$. Inelastic neutron scattering around 10 meV and a Heisenberg model analysis have revealed that V$$^{3+}$$ spin-wave modes exist at a lower-energy region than previously reported. The scattering around 20 meV cannot be reproduced with the spin-wave analysis. We propose that this scattering could originate from the spin-orbital coupled excitation. This scattering is most likely attributable to V$$^{3+}$$ spin-wave modes, entangled with the orbital hybridization between $$t_{2g}$$ orbitals.

論文

Polar rotor scattering as atomic-level origin of low mobility and thermal conductivity of perovskite CH$$_{3}$$NH$$_{3}$$PbI$$_{3}$$

Li, B.; 川北 至信; Liu, Y.*; Wang, M.*; 松浦 直人*; 柴田 薫; 河村 聖子; 山田 武*; Lin, S.*; 中島 健次; et al.

Nature Communications (Internet), 8, p.16086_1 - 16086_9, 2017/06

 被引用回数:52 パーセンタイル:91.93(Multidisciplinary Sciences)

Perovskite CH$$_{3}$$NH$$_{3}$$PbI$$_{3}$$ exhibits outstanding photovoltaic performances, but the understanding of the atomic motions remains inadequate even though they take a fundamental role in transport properties. Here, we present a complete atomic dynamic picture consisting of molecular jumping rotational modes and phonons, which is established by carrying out high-resolution time-of-flight quasi-elastic and inelastic neutron scattering measurements in a wide energy window ranging from 0.0036 to 54 meV on a large single crystal sample, respectively. The ultrafast orientational disorder of molecular dipoles, activated at approximately 165 K, acts as an additional scattering source for optical phonons as well as for charge carriers. It is revealed that acoustic phonons dominate the thermal transport, rather than optical phonons due to sub-picosecond lifetimes. These microscopic insights provide a solid standing point, on which perovskite solar cells can be understood more accurately and their performances are perhaps further optimized.

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