Uranium-plutonium-oxygen phase diagram; Investigating the solvus of fluorite's exsolution

Vauchy, R.; Hirooka, Shun; Horii, Yuta; Ogasawara, Masahiro*; Sunaoshi, Takeo*; Yamada, Tadahisa*; Tamura, Tetsuya*; Murakami, Tatsutoshi

Journal of Nuclear Materials, 599, p.155233_1 - 155233_11, 2024/10

https://doi.org/10.1016/j.jnucmat.2024.155233

The fluorite exsolution/recombination in UPuO (y = 0.30 and 0.45) and PuO was investigated using differential scanning calorimetry. The results are in relatively good agreement with the literature data, except for plutonia. Our values indicate that the critical temperature of the miscibility gap in Pu-O is 3050 K lower than previously reported. Finally, the systematic experimental procedure allowed us refining the locus of the solvus existing in hypostoichiometric U0PuO, UPuO, and PuO dioxides.

Trivalent lanthanide sorption onto illite in the presence of carbonate; A Study combining thermodynamic sorption modeling, time-resolved laser fluorescence spectroscopy, and parallel factor analysis

Sugiura, Yuki; Ishidera, Takamitsu; Aoyagi, Noboru; Mei, H.; Saito, Takumi*; Tachi, Yukio

Applied Clay Science, 258, p.107476_1 - 107476_10, 2024/09

https://doi.org/10.1016/j.clay.2024.107476

Trial analysis of chemical behavior in high-level radioactive liquid waste tank at accident of evaporation to dryness by boiling of reprocessing plant

Yoshida, Kazuo; Hiyama, Mina*; Tamaki, Hitoshi

JAEA-Research 2024-007, 24 Pages, 2024/08

JAEA-Research-2024-007.pdf:2.1MB

An accident of evaporation to dryness by boiling of high-level radioactive liquid waste (HLLW) is postulated as one of the severe accidents caused by the loss of cooling function at a fuel reprocessing plant. In this case, volatile radioactive materials, such as ruthenium (Ru) are released from the tanks with water and nitric-acid mixed vapor into the atmosphere. Accurate quantitative estimation of released Ru is one of the important issues for risk assessment of those facilities. It has been observed experimentally that volatility of RuO is suppressed by HNO generated by HNO radiolysis. The analysis of chemical reactions of NO including HNO and HNO in the waste tank is essential to simulate of these phenomena. To resolve this issue, an analytical approach has been attempted to couple dynamically two computer codes SHAWED and SCHERN. The simulation of boiling behavior in the tank is conducted with SHAWED. SCHERN simulates chemical behaviors of HNO, HNO and NO in the tank. A programmatic coupling algorithm and a trial simulation of the accident are presented in this report.

GPV2OSC, meteorological data format conversion program for OSCAAR

Risk Analysis Research Group, Reactor Safety Research Division, Nuclear Safety Research Center

JAEA-Data/Code 2024-006, 40 Pages, 2024/07

JAEA-Data-Code-2024-006.pdf:1.92MB

The Risk Analysis Research Group, Reactor Safety Research Division, Nuclear Safety Research Center, Sector of Nuclear Safety Research and Emergency Preparedness, Japan Atomic Energy Agency has been developing OSCAAR, a probabilistic risk assessment program for nuclear facility accidents. OSCAAR has the feature to calculate atmospheric concentrations of radioactive materials using an atmospheric dispersion model. This feature requires the input of meteorological data about wind speed, precipitation rate, atmospheric stability and so on. However, to use numerical weather prediction data created from the Japan Meteorological Agency (JMA) on OSCAAR, it is necessary to convert the data format to match OSCAAR input format in advance. Therefore, we developed GPV2OSC, a pre-processing program for OSCAAR, to create meteorological data converted from JMA weather prediction data format to OSCAAR input format when the target region and period are specified. This report describes the outline and usage of GPV2OSC.

The Development of Petri Net-based continuous Markov Chain Monte Carlo methodology applying to dynamic probability risk assessment for multi-state resilience systems with repairable multi-component interdependency under longtermly thereat

Li, C.-Y.; Watanabe, Akira*; Uchibori, Akihiro; Okano, Yasushi

Journal of Nuclear Science and Technology, 61(7), p.935 - 957, 2024/07

https://doi.org/10.1080/00223131.2023.2290067

High temperature nanoindentation of (U,Ce)O compounds

Frazer, D.*; Saleh, T. A.*; Matsumoto, Taku; Hirooka, Shun; Kato, Masato; McClellan, K.*; White, J. T.*

Nuclear Engineering and Design, 423, p.113136_1 - 113136_7, 2024/07

https://doi.org/10.1016/j.nucengdes.2024.113136

Nanoindentation based techniques can be employed on minute volumes of material to measure mechanical properties, including Young's modulus, hardness, and creep stress exponents. In this study, (U,Ce)O solid solutions samples are used to develop elevated temperature nanoindentation and nanoindentation creep testing methods for use on mixed oxide fuels. Nanoindentation testing was performed on 3 separate (Ux-1,Cex)O compounds ranging from x equals 0.1 to 0.3 at up to 800 C: their Young's modulus, hardness, and creep stress exponents were evaluated. The Young's modulus decreases in the expected linear manner while the hardness decreases in the expected exponential manner. The nanoindentation creep experiments at 800 C give stress exponent values, n=4.7-6.9, that suggests dislocation motion as the deformation mechanism.

A Proposed regulatory framework for small modular reactors

Nuclear System Technology Review Committee

JAEA-Review 2024-018, 38 Pages, 2024/06

JAEA-Review-2024-018.pdf:1.46MB

In the R&D activities related to the Ministry of Education, Culture, Sports, Science and Technology's Innovative Nuclear R&D Program, "Development of Integrated Energy System Simulation Method Utilizing Small Modular Reactors for Enhanced System Decarbonization and Resilience," Japan Atomic Energy Agency (JAEA) established the "Nuclear System Technology Review Committee," consisting of experts in the subject areas, to obtain advice on the feasibility of deploying Design-standardized, Factory-built, Site-independent Small Modular Reactors (DFS-SMRs) in Japan and other countries. The Committee met three times during the 2021-2024 project period to discuss proposals for a regulatory framework for the potential commercial deployment of DFS-SMRs in Japan. The starting point for the Committee's discussions was the view that Japan's nuclear regulatory framework, like most other countries with existing commercial nuclear power plants in operation, focuses on large Light Water Reactors. Another consideration was the Committee's view on the basic structure of the regulatory framework, consistent with other regulatory initiatives around the world. Specifically, that the most effective regulatory frameworks need to be less prescriptive, less technology-dependent, and more performance-based. This report focuses on the United States, which has played a leading role in the deployment of SMRs and other advanced reactors, and summarizes the discussions regarding the proposal for a licensing framework for SMRs in Japan, an analysis of the gaps between Japan's current licensing framework and the proposed framework, and specific recommendations for closing the gaps. The Committee is hopeful that the changes to the regulatory framework proposed in this report will become a reality.

Numerical simulation of accidents involving core damage with integrative severe accident analysis code, SPECTRA

Ishida, Shinya; Uchibori, Akihiro; Okano, Yasushi

Dai-28-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (Internet), 4 Pages, 2024/06

no abstracts in English

Quantitative analysis of microstructure evolution, stress partitioning and thermodynamics in the dynamic transformation of Fe-14Ni alloy

Li, L.*; Miyamoto, Goro*; Zhang, Y.*; Li, M.*; Morooka, Satoshi; Oikawa, Katsunari*; Tomota, Yo*; Furuhara, Tadashi*

Journal of Materials Science & Technology, 184, p.221 - 234, 2024/06

https://doi.org/10.1016/j.jmst.2023.10.037

Development of a hybrid method for evaluating the long-term structural soundness of nuclear reactor buildings using response monitoring and damage imaging technologies (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*

JAEA-Review 2023-048, 151 Pages, 2024/05

JAEA-Review-2023-048.pdf:8.48MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Development of a hybrid method for evaluating the long-term structural soundness of nuclear reactor buildings using response monitoring and damage imaging technologies" conducted in FY2022. The present study aims to develop an evaluation method necessary to obtain a perspective on the long term structural soundness of accident-damaged reactor buildings, where accessibility to work sites is extremely limited due to high radiation dose rate and high contamination. In FY2022, the second year of the three-year plan, some tests and other activities on the following research items were conducted following FY2021, based on the specific research methods and research directions clarified in FY2021.