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ソースターム評価手法の高度化に向けたFPの化学に関する研究,2; FP移行挙動におよぼす制御材ホウ素の影響

Evaluation of fission product release and transport behavior during severe accident focusing on the chemical forms, 2; Effects of a control material of boron for FP transport behavior

佐藤 勇; 大西 貴士  ; 廣沢 孝志  ; 田中 康介  ; 逢坂 正彦  ; 小山 真一  ; 所 大志郎*; 石ヶ森 俊夫*; 関 崇行*; 品田 雅則*; 関岡 健*

Sato, Isamu; Onishi, Takashi; Hirosawa, Takashi; Tanaka, Kosuke; Osaka, Masahiko; Koyama, Shinichi; Tokoro, Daishiro*; Ishigamori, Toshio*; Seki, Takayuki*; Shinada, Masanori*; Sekioka, Ken*

FPの模擬物質としてCsIを加熱・蒸発させ、移行経路にある温度分布を有する配管に沈着させた。このCsI沈着表面に、より高温で加熱・蒸発したB$$_{2}$$O$$_{3}$$を接触させることで、Cs及びIの沈着・移行挙動に及ぼすホウ素の影響を調べた。その結果、沈着したCsIがホウ素蒸気により再び気相化学形となり、低温部へ移行している可能性を明らかにした。

As a material simulating FP, CsI was heated and evaporated to be decomposited on the surface of a tube having a temperature gradient. Gaseous B$$_{2}$$O$$_{3}$$ made by heating it at higher temperature was react with CsI decomposited on the surface, and then the boron effects for decomposition and migration behavior of Cs and I were observed. Consequently, it was indicated that boron vapor could strip decomposited CsI to make it gaseous species again and then the guseous CsI could move to the colder position.

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