Sato, Takumi; Otobe, Haruyoshi; Morishita, Kazuki; Marufuji, Takato; Ishikawa, Takashi; Fujishima, Tadatsune; Nakano, Tomoyuki
JAEA-Technology 2023-016, 41 Pages, 2023/09
This report summarizes the results of the stabilization treatments of post-experiment nuclear materials in Plutonium Fuel Research Facility (PFRF) from August 2018 to March 2021. Based on the management standards for nuclear materials enacted after the contamination accident that occurred at PFRF on June 6, 2017, the post-experiment nuclear materials containing plutonium (Pu): samples mixed with organic substances that cause an increase in internal pressure due to radiolysis (including X-ray diffraction samples mixed with epoxy resin and plutonium powder which caused contamination accidents), carbides and nitrides samples which is reactive in air, and chloride samples which may cause corrosion of storage containers, were selected as targets of the stabilization. The samples containing organic materials, carbides and nitrides were heated in an air flow at 650 C and 950 C for 2 hours respectively to remove organic materials and convert uranium (U) and Pu into oxides. U and Pu chlorides in LiCl-KCl eutectic melt were reduced and extracted into liquid Cd metal by a reaction with lithium (Li) -cadmium (Cd) alloy and converted to U-Pu-Cd alloy at 500 C or higher. All of the samples were stabilized and stored at PFRF. We hope that the contents of this report will be utilized to consider methods for stabilizing post experiment nuclear materials at other nuclear fuel material usage facilities.
Department of HTTR
JAEA-Review 2023-016, 82 Pages, 2023/09
The High Temperature Engineering Test Reactor (HTTR) is the first Japanese High Temperature Gas-cooled Reactor (HTGR) with 30MW in thermal power and 950C of maximum outlet coolant temperature that is constructed by the Japan Atomic Energy Agency located at Oarai-machi, Higashiibaraki-gun, Ibaraki-ken, Japan. The purpose of the HTTR is establishment of basic HTGR technologies, demonstration of HTGR safety characteristics and so on. The HTTR has had a lot of experience of HTGRs' operation and maintenance throughout rated power operations, safety demonstration tests, long-term high temperature operations and demonstration tests relevant to HTGRs' R&Ds. In the fiscal year 2021, as the HTTR completed activities to conform to the New Regulatory Requirements of Nuclear Regulation Authority, The HTTR restarted since the 2011 off the Pacific coast of Tohoku Earthquake and carried out the Loss-of-forced cooling test without Vessel Cooling System (VCS) operational at 9MW (Three gas circulators trip and VCS is stopped.) as the safety demonstration test. This report summarizes the activities carried out in the fiscal year 2021, which were the situation of the New Regulatory Requirements screening of the HTTR, the operation and maintenance of the HTTR, R&Ds relevant to commercial-scale HTGRs, the international cooperation on HTGRs and so on.
Akiyama, Yoichi; Shibanuma, So; Yanagisawa, Kenichi*; Yamada, Taichi; Suzuki, Kenta; Yoshida, Moeka; Ono, Takahiro; Kawabata, Kuniaki; Watanabe, Kaho; Morimoto, Kyoichi; et al.
JAEA-Review 2023-015, 60 Pages, 2023/09
Naraha Center for Remote Control Technology Development (NARREC) was established in Japan Atomic Energy Agency to promote a decommissioning work of Fukushima Daiichi Nuclear Power Station (Fukushima Daiichi NPS). NARREC consists of a Full-scale Mock-up Test Building and Research Management Building. Various test facilities are installed in these buildings for the decommissioning work of Fukushima Daiichi NPS. These test facilities are intended to be used for various users, such as companies engaged in the decommissioning work, research and development institutions, educational institutions and so on. The number of NARREC facility uses was 84 in FY2021. We participated booth exhibitions and presentations on the decommissioning related events. Moreover, we also contributed to the development of human resources by supporting the 6th Creative Robot Contest for Decommissioning. As a new project, "Narahakko Children's Classroom" was implemented for elementary school students in Naraha Town. This report summarizes the activities of NARREC in FY2021, such as the utilization of facilities and equipment of NARREC, the development of remote-control technologies for supporting the decommissioning work, arrangement of the remote-control machines for emergency response, and training for operators by using the machines.
Aomori Research and Development Center
JAEA-Review 2023-014, 31 Pages, 2023/09
With regard to "Offshore Floating Nuclear Power", which is currently under-consideration for design and development, the findings from the Nuclear Ship "MUTSU" are attracting attention from the perspective of operating at sea. The Nuclear Ship "MUTSU" is the only nuclear-powered ship designed, built and operated in Japan. Utilizing this knowledge will be extremely useful for the realization of future "Offshore Floating Nuclear Power". For this purpose, we examined the materials related to the Nuclear Ship "MUTSU" and confirmed the materials that proposed the points to be improved in equipment, based on the power increase test and the experimental voyage, etc. by the persons concerned at that time. We believe that these materials are useful for the design and construction of next-generation nuclear-powered vessels and will be helpful in considering the design and development of "Offshore Floating Nuclear Power". Since these materials have not yet been released, they will be re-edited the contents of 1994 so that they can be made available to the public, and their findings will be able to be made widely available.
Nagai, Takayuki; Okamoto, Yoshihiro; Yamagishi, Hirona*; Shibata, Daisuke*; Kojima, Kazuo*; Hasegawa, Takehiko*; Sato, Seiichi*; Fukaya, Akane*; Hatakeyama, Kiyoshi*
JAEA-Research 2023-004, 45 Pages, 2023/09
The local structure of glass-forming elements and waste elements in borosilicate glasses varies with its chemical composition. In this study, simulated waste glass samples were prepared and the chemical state regarding boron (B), silicon (Si) and waste elements of iron (Fe), cesium (Cs) were estimated by using XAFS measurement in soft X-ray region. To understand the chemical stability of simulated waste glasses, XANES spectra of B K-edge, Fe L, L-edge, and Cs M, M-edge were measured on the glass surface exposed to the leachate. As a result, it was found that the glass surface exposed to the leachate was changed and it was difficult to obtain a clear XANES spectrum. From the B K-edge XANES spectra on glass surfaces exposed to the leachate, an increase in three-coordination of B-O (BO) and a decrease in four-coordination of B-O (BO) were observed compared to the glass surfaces before immersion. The XANES spectra of Fe L, L-edge, and Cs M, M-edge show that as the exposure time in the leachate increases, the Cs present on the glass surface dissolves into the leachate. The XANES spectra of Si K-edge were measured on simulated waste glass surfaces before immersion, and it was confirmed that the change in XANES spectra given by NaO concentration had a larger effect than the waste component concentration.
Sato, Hisashi*; Takayama, Yusuke; Suzuki, Hideaki*; Sato, Daisuke*
JAEA-Data/Code 2023-010, 47 Pages, 2023/09
When a high-level radioactive waste repository is constructed in a coastal area, it is necessary to fully evaluate the impact of seawater-based groundwater on engineered barriers, including buffer materials. In this report, one-dimensional saltwater infiltration tests were conducted to obtain data to understand the impact of seawater-based groundwater on the migration phenomena of water and solutes in the buffer material during the transient period. As a result, it was confirmed that the infiltration rate increased as the NaCl concentration in the infiltration solution increased. And it was confirmed that the water content ratio distribution changed as the NaCl concentration in the infiltration solution increased. As a result of analysis of the chloride ion concentration of the post-test specimens confirmed that chloride ion enrichment was occurred with infiltration. As a result of verifying the mechanism by which chloride ion enrichment occurs, it was confirmed that the phenomenon of chloride ion enrichment due to infiltration depends on the initial water content ratio.
Miyakawa, Kazuya; Hayano, Akira; Sato, Naomi; Nakata, Kotaro*; Hasegawa, Takuma*
JAEA-Data/Code 2023-009, 103 Pages, 2023/09
This borehole investigation was carried out to confirm the validity of the distribution of low flow areas deep underground estimated based on the geophysical survey in FY 2020, as a part of an R&D supporting program titled "Research and development on Groundwater Flow Evaluation Technology in Bedrock" under contract to the Ministry of Economy, Trade and Industry (2021, 2022 FY, Grant Number: JPJ007597). The borehole name is Horonobe Fossil seawater Boring-1 and is referred to as HFB-1 borehole. HFB-1 is a vertical borehole drilled adjacent to the Horonobe Underground Research Laboratory (URL), which was drilled from the surface to a depth of 200 m in FY2021 and from a depth of 200 m to 500 m in FY2022. This report summarizes information related to the drilling of HFB-1 and various data (rock core description, geophysical logging, chemical analysis, etc.) obtained from the borehole investigation.
Local Exhaust Device Development Team in Analysis Section
JAEA-Technology 2023-015, 19 Pages, 2023/08
In the analytical laboratory of Tokai Reprocessing Plant, samples for operation and facility maintenance are analyzed in glove-box. Analytical reagents and equipment are carried inside the glove-box, and radioactive wastes generated through the analytical work are carried out using plastic bag (vinyl-bag) attached to the glove-box. The work carrying in and out from the glove-box is called as bag-in and bag-out. During these works, if the vinyl-bag is damaged, radioactive materials inside the glove-box may be leaked out and radioactive materials contaminate the vinyl-bag surface and the work area. In addition to that, if the radioactive contamination floats into the air, air in the work area may be contaminated. In this study, actual situation of the vinyl-bag work, specifications, and features of a local exhaust device for glove exchange work, which is an existing local exhaust device for gloves with a similar installation structure to vinyl-bags, have been investigated. Then, local exhaust device for vinyl-bag work have been developed. The developed local exhaust device has the same dimensions and shape as worktable that are conventionally used for vinyl-bag work. Also, a hood, HEPA filter, and exhaust blower, which are main components of the exhaust device for glove exchange work, are installed inside of this worktable. As a result, it has been confirmed that the developed local exhaust device is effective to prevent air contamination in vinyl-bag work without increasing the work procedures, manpower, and work time.
Kawano, Takahiro*; Mizuta, Naoki; Ueta, Shohei; Tachibana, Yukio; Yoshida, Katsumi*
JAEA-Technology 2023-014, 37 Pages, 2023/08
Fuel compact for High Temperature Gas-cooled Reactor (HTGR) is fabricated by calcinating a matrix consisting of graphite and binder with the coated fuel particle. The SiC-matrixed fuel compact uses a new matrix made of silicon carbide (SiC) replacing the conventional graphite. Applying the SiC-matrixed fuel compact for HTGRs is expected to improve their performance such as power densities. In this study, the sintering conditions for applying SiC as the matrix of fuel compacts for HTGR are selected, and the density and thermal conductivity of the prototype SiC are measured.
Togawa, Orihiko; Hokama, Tomonori; Hiraoka, Hirokazu
JAEA-Review 2023-013, 48 Pages, 2023/08
When radionuclides are released into the atmospheric environment at a nuclear emergency, protective measures such as evacuation and temporal relocation are carried out using motor vehicles such as private cars and buses to reduce radiation exposure to residents. To confirm conditions of contamination for the evacuated or relocated residents, contamination inspection is conducted, in which it is important not to spoil its rapidity. In the present inspection, wipers and tires are designated to first measuring parts, and they are basically inspected by persons using GM survey meters. Utilization of portable radiation portal monitors is also being considered for rapid and efficient inspection of motor vehicles. In order to contribute to rapid and efficient operation of contamination inspection, this report investigated conditions of contamination and measures of decontaminations for motor vehicles at a nuclear emergency. Although available documents and information were quite few, results of the investigations described in the related documents were extracted and rearranged according to the objectives of this report. Furthermore, these results were considered from a viewpoint of rapid and efficient operation of contamination inspection.
Nakazawa, Osamu; Takiya, Hiroaki; Murakami, Masashi; Donomae, Yasushi; Meguro, Yoshihiro
JAEA-Review 2023-012, 6 Pages, 2023/08
The selection of back-end technology development issues to be prioritized and their schedule of the Japan Atomic Energy Agency (JAEA) have been put together as the "Strategic Roadmap for Back-end Technology Development." The results of questionnaires on development technologies (seeds) and technical issues (needs) within JAEA conducted in FY2022 were reflected in the selection. The issues were extracted from among those that match the seeds and needs, from the perspective of early implementation in the work front and the perspective of common issues, and nine themes were selected. We will build a cross-organizational implementation framework within JAEA and aim to implement the development results in the work front as well as social implementation.
Ogawa, Rina; Amazawa, Hiroya; Nakata, Hisakazu; Sugaya, Toshikatsu; Sakai, Akihiro
JAEA-Review 2023-011, 116 Pages, 2023/08
Japan Atomic Energy Agency (JAEA) is the implementing agency for the disposal business of radioactive waste generated from research, industrial and medical facilities (Institutional radioactive waste). In 2010, JAEA implemented a conceptual design of the disposal facility that conformed to the laws and regulations at the time. However, since 2013, the laws and regulations for nuclear facilities including the Category-2 Waste Disposal were amended. Since then, design of various nuclear facilities including disposal facilities has been reviewed. Therefore, JAEA decided to do additional studies toward the basic design for the disposal facility. When JAEA gets a license of the disposal business of Institutional radioactive waste, it is necessary to show that the disposal facility complies with the rule of design for disposal facility under the law. Therefore, JAEA is examining technical studies of the disposal facility to conform to the new standard. In this report, we organized the requirements of the rule for design of trench disposal facility and extracted the issues to design the disposal facility that conform to the requirements.
JAEA-Review 2023-010, 108 Pages, 2023/08
Tc (technetium-99m) is the most widely used radioisotope in radiopharmaceutical and is decayed from the parent nuclide Mo (molybdenum-99). Most of Mo is generated as one of the fission products of uranium, but recently, from the viewpoint of nuclear security and nuclear nonproliferation, a uranium-free Mo production method is desired. One such method is the (n,) method, in which Mo is irradiated by neutrons. However, since the specific activity of Mo produced by this method is extremely low, it is necessary to improve the Mo adsorption and Tc elution property of alumina (AlO), which is used as a Mo adsorbent, to apply this method to the Mo/Tc generator, a device for separation and concentration of Tc from Mo. Therefore, the objective of this thesis is to elucidate the parameters effective for improving the performance of alumina for the practical use of the Mo/Tc generator using the (n,) method, and to contribute to the development of alumina columns that may be applicable to low specific activity Mo. In this study, alumina with different starting materials was prepared and its applicability as Mo adsorbent for Mo/Tc generator was evaluated. The effects of crystal structure and specific surface area of alumina on Mo adsorption properties were clarified, and the Mo adsorption mechanism was elucidated based on the results of surface analysis of alumina. In addition, Tc elution properties and Tc solution quality were evaluated using MoO irradiated in the Kyoto University Research Reactor (KUR), and a new column shape with potential application to generators was proposed based on the experiment results of alumina columns designed for current generators.
Aomori Research and Development Center
JAEA-Review 2023-005, 87 Pages, 2023/08
Aomori Research and Development Center consists of Nuclear Facilities Management Section, General Affairs and Purchase Section, Facility Maintenance and Engineering Section, AMS Management Section and Nuclear Fuel Cycle Cooperation Office. Each sections are each sections carrying out management of facility operation, decommissioning of reactor facility, etc. to achieve the Medium to long-term plan. In this report, the activities of Aomori Research and Development Center are described to contribute to future facility management and business promotion.
Sato, Yuji; Miyamoto, Yuta; Awatani, Yuto; Yamamoto, Kosuke; Hatakeyama, Takumi
JAEA-Review 2023-002, 59 Pages, 2023/08
"Fugen Decommissioning Engineering Center", in planning and carrying out our decommissioning technical development, organizes "Technical special committee on Fugen decommissioning" which consists of the members well-informed, aiming to make good use of Fugen as a place for technological development which is opened domestic and international, as the central place in research and development base of Fukui prefecture, and to utilize the outcome in our decommissioning to the technical development effectively. This report consists of presentation paper are "Achievements and Considerations for Sampling and Analysis of Reactor Core Components", "Treatment of liquid scintillator waste liquid" and "Results and issues of rationalization of decontamination related to the clearance and considerations related to surface contamination monitoring" which is presented in the 39th Technical Special Committee on Fugen Decommissioning.
Ogawa, Rina; Totsuka, Masayoshi*; Sakai, Akihiro
JAEA-Technology 2023-012, 57 Pages, 2023/07
Concrete vault disposal facility is assumed to be installed below the groundwater table because it is necessary to install them on the ground that has enough bearing capacity. Therefore, the flow rates of groundwater into and out of concrete vault were evaluated by taking into account the permeability coefficients of the geological environment surrounding the facility and of the engineered structure of the facility. Groundwater flow analysis was performed by using the groundwater flow analysis code MIG2DF based on finite element method. In the evaluation of considering the geological environment, since the flow rate of groundwater into and out of the bottom of concrete vault was larger than the flow rates into and out of other sides of the vault in previous technical studies, the evaluation of the flow rate was performed by varying the permeability coefficient of the bedrock adjacent to the bottom of concrete vault. In addition, the other evaluation of the flow rate was conducted assuming the deterioration of concrete vault and of bentonite-mixed soil. As a result, it was found that the permeability coefficient of bedrock adjacent to concrete vault greatly contributed to flow rates of groundwater into and out of concrete vault. In addition, as the permeability coefficient of the bentonite-mixed soil increased due to chemical deterioration, the flow rate of leachate into the surrounding cover soil increased. From the above results, it was found that these permeability coefficients were important influencing factors in the engineering design and safety evaluation of concrete vault disposal facilities.
Nuclear Human Resource Development Center
JAEA-Review 2023-008, 58 Pages, 2023/07
This annual report summarizes the activities of Nuclear Human Resource Development Center (NuHRDeC) of Japan Atomic Energy Agency (JAEA) in the fiscal year (FY) 2021. In FY 2021, in addition to the regular training programs at NuHRDeC, we actively organized special training courses responding to the external training needs, cooperated with universities, offered international training courses for Asian countries and promoted activities of the Japan Nuclear Human Resource Development Network (JN-HRD.net). In FY2021, due to the spread of the new coronavirus infection over the world, some training courses were conducted online using web conference systems. Regular national training programs; training courses for radioisotopes and radiation engineers, nuclear energy engineers and national qualification examinations, were conducted as scheduled in the annual plan. We also delivered training for the Japan Atomic Power Company. We continued cooperative activities with universities, such as acceptance of postdoctoral researchers, and activities in line with the cooperative graduate school system, including the acceptance of students from Nuclear Professional School, the University of Tokyo. Furthermore, joint course among seven universities was successfully held by utilizing remote education system. The joint course and the intensive summer course were conducted as part of the collaboration network with universities. The Instructor Training Program (ITP) under contract with Ministry of Education, Culture, Sports, Science and Technology, was continually offered to the ITP participating countries. As part of the ITP, the Instructor Training Courses such as "Reactor Engineering Course" and the Nuclear Technology Seminar "Basic Radiation Knowledge for School Education Seminar" were conducted online at NuHRDeC. As secretariat of JN-HRD.net, we steadily facilitated the network and conducted webinar and online training despite circulation of the new coronavirus infection.
Takeuchi, Ryuji; Mikake, Shinichiro; Ikeda, Koki; Nishio, Kazuhisa*; Kokubu, Yoko; Hanamuro, Takahiro
JAEA-Review 2023-007, 114 Pages, 2023/07
Japan Atomic Energy Agency (JAEA) at Tono Geoscience Center has been conducting the Mizunami Underground Research Laboratory (MIU) Project to enhance the reliability of geological disposal technologies through investigations of the deep geological environment in the crystalline rock (granite) at Mizunami City, Gifu Prefecture, central Japan since fiscal year 1996. Backfilling and restoration works in the MIU site have been being conducted based on "the MIU Project from FY2020 onwards" which is defined the way forward of backfilling and restoration works and environmental monitoring investigations in the MIU site, since fiscal year 2020. This report summarizes the outline, process, and achievements of the construction and the safety patrol of the backfilling and restoration works in the MIU site performed from May 16, 2020 to January 16, 2022.
Center for Computational Science & e-Systems
JAEA-Evaluation 2023-001, 38 Pages, 2023/07
Research on advanced computational science for nuclear applications, based on "the plan to achieve the medium- and long-term goal of the Japan Atomic Energy Agency", has been performed by Center for Computational Science & e-Systems (CCSE), Japan Atomic Energy Agency. CCSE established a committee consisting of external experts and authorities which evaluates and advises toward the future research and development. This report summarizes the results of the R&D performed by CCSE in FY2022 (April 1st, 2022 - March 31st, 2023) and their evaluation by the committee.
JAEA-Data/Code 2023-008, 49 Pages, 2023/07
Japan Atomic Energy Agency had been conducting "geoscientific study" and "research and development on geological disposal" in the Horonobe Underground Research Laboratory (URL) for safe geological disposal of high-level radioactive waste. In the Horonobe underground research project for FY 2020 and subsequent years, the pressure and water quality of groundwater have been continuously monitored using monitoring systems in order to obtain the data necessary for conducting the remaining important issues. This report presents groundwater pressure which have been obtained from April 2019 to March 2022 by the monitoring systems installed at the 140 m and 350 m gallery.