Development of a phoswich detector for low-energy gamma rays emitted from alpha emitters

Morishita, Yuki; Yamada, Tsutomu*; Nakasone, Takamasa*; Kanno, Marina*; Sasaki, Miyuki; Sanada, Yukihisa; Torii, Tatsuo*

Radiation Measurements, 188, p.107502_1 - 107502_7, 2025/11

https://doi.org/10.1016/j.radmeas.2025.107502

The decommissioning of the Fukushima Daiichi Nuclear Power Station requires thorough inspection of piping for contamination, including alpha nuclides. Since external alpha particle measurements are impractical, detection relies on gamma-rays emitted by the alpha nuclides. Therefore, a phoswich detector for detecting low-energy gamma-rays was developed and experimentally validated. The detector was designed with consideration of energy deposition characteristics and consists of YAP:Ce or HR-GAGG scintillators in combination with BGO scintillators, employing a photomultiplier tube for signal amplification. Validation procedures included Monte Carlo simulations and measurements using actual radiation sources. Both measurement and simulation results demonstrate a correlation in scintillator energy depositions across different gamma-ray energies. Pulse Shape Discrimination (PSD) plots effectively differentiate between low-energy and high-energy gamma-rays, thereby confirming the predictions from simulations. These results suggest promising potential for developing a sensitive low-energy gamma-ray detector utilizing various scintillator combinations. The phoswich detector shows promise for effectively detecting low-energy gamma-rays emitted by alpha nuclides in piping.

Research on radioactive aerosol control and decontamination at Fukushima Daiichi Nuclear Power Station Decommissioning (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2025-015, 73 Pages, 2025/09

JAEA-Review-2025-015.pdf:5.9MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Research on radioactive aerosol control and decontamination at Fukushima Daiichi Nuclear Power Station decommissioning" conducted from FY2021 to FY2023. The present study aims to develop a safe laser decontamination system that integrates advanced particle detection and characterization systems with aerosol dispersion control, in collaboration with UK researchers. For aerosol dispersion control, new containment methods ranging from simple mechanical containment hoods to optical laser shields are jointly investigated. The Japanese team will develop a radioactive dispersion control method based on the use of water mist and water spray to reduce radiation risks during laser cutting and decontamination applications. Based on data on aerosol particles provided by the UK team, the potential to enhance aerosol scrubbing efficiency will be explored. Additionally, the effect of charge enhancement will be evaluated. The UK team will develop laser-based aerosol containment methods and conducting experiments to improve the condensation of aerosol particles and mist in spray scrubbing. The development of aerosol removal technologies and strategies will be carried out through comprehensive experimental and computational studies. Experiments will be conducted at UTARTS facility to verify simultaneous operations such as laser decontamination, cutting, and spray operations. Aerosol measurements will also be performed to obtain high spatial resolution data that can better validate CFD models. In the final year, mock-up tests will be conducted to verify the system's operation and decontamination performance at full scale, evaluating the decontamination system developed through this research.

Assessment report on research and development activities in FY2024 Activity; Research and development related to the accident at TEPCO's Fukushima Daiichi Nuclear Power Station (Achievements in environmental behavior research) (Ex-post evaluations)

Fukushima Research and Engineering Institute*

JAEA-Evaluation 2025-001, 23 Pages, 2025/09

JAEA-Evaluation-2025-001.pdf:0.72MB
JAEA-Evaluation-2025-001-appendix(CD-ROM).zip:185.38MB

Japan Atomic Energy Agency (hereinafter referred to as "JAEA") consulted an assessment committee, "Evaluation Committee of Research and Development related to the Accident at TEPCO's Fukushima Daiichi Nuclear Power Station" (hereinafter referred to as "Committee") for ex-ante evaluations of "Research and Development Related to the Accident at TEPCO's Fukushima Daiichi Nuclear Power Station" in accordance with "General Guideline for the Evaluation of Government Research and Development (R&D) Activities" by Cabinet Office, Government of Japan, "Guideline for Evaluation of R&D in Ministry of Education, Culture, Sports, Science and Technology" and "Regulation on Conduct for Evaluation of R&D Activities" by JAEA. Based on a request from JAEA, the committee conducted a post-evaluation of research and development activities in the fourth phase (April 2022 to March 2029) of the medium-term research plan. This report summarizes the results of the assessment by the Committee.

Detection of beta-emitting radioactive hotspots inside the Fukushima Daiichi Nuclear Power Station Unit 3 reactor building using an optical fiber radiation sensor based on wavelength-resolving analysis

Terasaka, Yuta; Sato, Yuki; Ichiba, Yuta*

Radiation Measurements, 187, p.107486_1 - 107486_8, 2025/09

https://doi.org/10.1016/j.radmeas.2025.107486

Fuel debris criticality analysis technology using non-contact measurement method (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Institute of Science Tokyo*

JAEA-Review 2025-010, 62 Pages, 2025/08

JAEA-Review-2025-010.pdf:3.63MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Fuel debris criticality analysis technology using non-contact measurement method" conducted from FY2021 to FY2023. The purpose of research was to improve the fuel debris criticality analysis technology using non-contact measurement method by the development of the fuel debris criticality characteristics measurement system and the multi-region integral kinetic analysis code. It was performed by Institute of Science Tokyo, Tokyo City University, National Institute of Advanced Industrial Science and Technology, and Nagaoka University of Technology. We developed the fuel debris criticality characteristics measurement system which has a two layer structure surrounding a canister containing fuel debris fragments with He proportional counters. The operational validation and performance evaluation were performed on the developed detector system. We have demonstrated the feasibility and accuracy of measuring the amount of fissile material and water content. MIK2.0-MVP code, which can calculate fission reaction rate attributed to both prompt and delayed neutrons and also can take the movement of fuel debris into calculation, was developed. After parallelizing the tally process of C() function, MIK2.0-MVP code will be applicable to weakly coupled reactors which include moving fuel debris particles if a supercomputer will be used for the tally process of C() function and if the coupling of MIK2.0-MVP code with MPS will be weak.

Characteristics of droplet evaporation on high-temperature porous surfaces for estimating cooling time of fuel debris

Yuki, Kohei*; Horiguchi, Naoki; Yoshida, Hiroyuki; Yuki, Kazuhisa*

Mechanical Engineering Journal (Internet), 12(4), p.24-00451_1 - 24-00451_8, 2025/08

https://doi.org/10.1299/mej.24-00451

Fuel debris at the Fukushima Daiichi nuclear power station is typically cooled under immersion. However, an unexpected significant drop in water level results in coolant contact with high-temperature fuel debris having porous structure. In such scenarios, rapid cooling is essential, yet the thermal behavior at the liquid-solid interface, including capillary phenomena, is not well understood. This paper presents basic research evaluating the evaporation characteristics of droplets upon contact with metallic porous media featuring small pores under 1 mm. We conducted experiments using bronze or stainless steel porous media with pore diameters of 1, 40, or 100 m to derive lifetime curves for droplets. Our findings indicate that Leidenfrost effect is mitigated on porous surfaces as the vapor can escape through the pores. Moreover, in bronze porous media, as the temperature increases, oxide film with a fine structure facilitates capillary action. In contrast, the low wettability of stainless steel porous media prevents capillary action, inhibiting droplet absorption and dispersion into the pores. Consequently, rapid cooling via the capillary action is unlikely if the fuel debris shares similar characteristics with steel porous media. Therefore, for risk management, the cooling system should be established assuming that capillary force does not act in the fuel debris.

Development of the continuous monitoring of tritium water by mid-infrared laser spectroscopy (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; National Institutes of Natural Sciences*

JAEA-Review 2025-009, 48 Pages, 2025/07

JAEA-Review-2025-009.pdf:2.19MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Development of the continuous monitoring of tritium water by mid-infrared laser spectroscopy" conducted from FY2021 to FY2023. The present study aims to demonstrate the principle for rapid measurement of tritiated water at a concentration level of 60 Bq/cc using a cavity ring-down spectroscopy system with a mid-infrared laser. In fiscal year 2023, research focused on (1) developing the cavity ring-down apparatus and (2) evaluating hydrogen isotope composition and preparing standard samples under environmental conditions (subcontracted to Hirosaki University). For (1), an optical bench was set up at the NIFS to perform laser absorption spectroscopy of various hydrogen isotope concentrations, enabling the evaluation of measurement sensitivity and establishment of guidelines. The light amplification of a quantum cascade laser, was further developed, achieving light amplification of a 4.3 m quantum cascade laser with an iron ion-doped medium, yielding a maximum output of 390 mW with a linewidth of less than 30 MHz. For (2), standard samples were prepared by diluting commercially available heavy water with BG water (tritium-free water) to create samples with approximately 100 Bq/L. Isotope ratio measurements were conducted indoors and outdoors using a high-time-resolution atmospheric water vapor collection system for tritium measurement, and daily measurements of the hydrogen isotope ratio (D) were conducted. The relationship between D and tritium concentration in atmospheric water vapor in Hirosaki City was evaluated. Thus, the principle for the rapid measurement of tritiated water using a mid-infrared laser was successfully demonstrated.

Development of methodology combining chemical analysis technology with informatics technology to understand perspectives property of debris and tie-up style human resource development (Contract research); FY2023 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Fukushima University*

JAEA-Review 2025-002, 108 Pages, 2025/07

JAEA-Review-2025-002.pdf:5.25MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2023. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Development of methodology combining chemical analysis technology with informatics technology to understand perspectives property of debris and tie-up style human resource development" conducted from FY2019 to FY2023. The present study aims to Goal of this study is to implement a research plan relate to a development of combinational technology of new chemical analysis with informatics, and the aim is to develop new system for whole image estimation system using small quantities of information. Conducting the collaboration study with JAEA researchers (tie-up style) make connect to the development of human resource from master's course student to post-doctoral researchers who are progress in the local-based and/or many academics fields research. We are in progress to grow international-minded human resources.

Evaluation of Co inventory in the core of the Fukushima Daiichi Nuclear Power Plant; Contribution of fuel deposits to the reactor core inventory

Uchida, Shunsuke*; Kino, Chiaki*; Karasawa, Hidetoshi; Takahatake, Yoko; Koma, Yoshikazu

Journal of Nuclear Science and Technology, 17 Pages, 2025/07

https://doi.org/10.1080/00223131.2025.2499187

Evaluation of radioactive nuclide behavior on and after the accident is important for the estimating radioactive nuclide composition in the wastes. The reactor core inventories have been obtained from the ORIGEN2 analysis, but the inventory of activation products is determined by the amount of their parent nuclides which are impurities contained in the structural materials. The ORIGEN2 does not treat fuel deposits including the impurities. Estimation of the initial Co-60 inventory in accurate is needed on the evaluation of some kinds of radioactive nuclide amount, since it is possible Co-60 is standard in the scaling factor. In this study, contribution of fuel deposits to the reactor core inventory was estimated by comparing the amount of Co-60 and Ni-63 calculated by the amounts of deposition by the microlayer-evaporation and drying-out model (MEDO model) and the result of the ORIGEN2 analysis, and then the method of estimating the reactor core inventory was proposed.

Solidification treatment of simulated decontamination equipment sludge using alkali-activated materials

Matsuzawa, Kazuki*; Yamamoto, Takeshi*; Taniguchi, Takumi; Osugi, Takeshi

Konkurito Kogaku Rombunshu, 36, p.37 - 47, 2025/07

https://doi.org/10.3151/crt.36.37

To dispose the decontamination sludge made from contaminated water in Fukushima Daiichi Nuclear Power Station using alkali-activated materials (AAM), we solidified barium sulfate powder (BS) and potassium hexacyanocobalt(II)-ferrate(II) powder (FCN) with AAM and searched proper compositions corresponding to the standards. At first, we made solidified bodies controlling HO/base ratio, Si/Al molar ratio, and Na/Si molar ratio. When base materials consisted of metakaolin and blast-furnace slag, we found out some proper compositions and two applicable concentrations of solutions to make solidified bodies corresponding to the standards. Secondly, using solutions with the applicable concentrations, we made solidified bodies controlling the amounts of BS, BS+FCN, and HO. The maximum amount of BS+FCN at the proper compositions was larger than that of BS.