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Mechanical and thermal properties of Zr-B and Fe-B alloys

Sun, Y.*; 阿部 雄太; 牟田 浩明*; 大石 佑治*

Journal of Nuclear Science and Technology, 57(8), p.917 - 925, 2020/08

 被引用回数:0 パーセンタイル:100(Nuclear Science & Technology)

After the core meltdown in the Fukushima Daiichi (1F) nuclear power plant, various compounds in metal boride systems could potentially form as a result of the reactions between B$$_{4}$$C (control material) and Fe, Zr alloys (control-blade sheaths, zircaloy claddings, channel box, etc.). Some previous studies have focused on the properties of intermetallic compounds of the Zr-B and Fe-B systems, such as ZrB$$_{2}$$, FeB, and Fe$$_{2}$$B. However, during the solidification of fuel debris, composites of these intermetallics rather than large chunks of single-phase intermetallics will form. This situation makes the understanding of the composition dependence of the mechanical and thermal properties of these metal borides a major task before debris retrieval takes place. In this study, we first investigated the temperature-dependent thermal conductivity of Fe-B and Zr-B eutectics from room temperature up to 900 $$^{circ}$$C. We were then able to evaluate the composition-dependent indentation hardness of these metal borides at room temperature. Based on our experimental data, we concluded that the hardness and thermal conductivity of the Fe-B, Zr-B composites can be well estimated using the properties of the composites' corresponding components, with Rule of Mixtures and Effective Medium Theory (EMT) calculations, respectively.


Chemical forms of uranium evaluated by thermodynamic calculation associated with distribution of core materials in the damaged reactor pressure vessel

池内 宏知; 矢野 公彦; 鷲谷 忠博

Journal of Nuclear Science and Technology, 57(6), p.704 - 718, 2020/06

 被引用回数:0 パーセンタイル:100(Nuclear Science & Technology)

福島第一原子力発電所から取り出された燃料デブリへの効果的な処置方策を提案する上では、燃料デブリ中でUがとりうる化学形についての詳細な調査が不可欠である。特に、アクセス性に乏しい圧力容器内に残留する燃料デブリに関する情報が重要である。本研究では、圧力容器内燃料デブリ中、特にマイナー相におけるUの化学形を評価することを目的とし、1F-2号機の事故進展での材料のリロケーション及び環境変化を考慮した熱力学計算を実施した。組成,温度,酸素量といった計算条件は、既存の事故進展解析の結果から設定した。計算の結果、Uの化学形はFeとOの量によって変化し、Feの少ない領域で$$alpha$$-(Zr,U)(O)、Feの多い領域でFe$$_{2}$$(Zr,U) (Laves相)の生成が顕著であった。還元性条件で生成するこれらの金属相中には数パーセントのUが移行しており、燃料デブリの処置において核物質の化学分離を考慮する場合はこれらの相の生成に留意すべきと考えられる。


Gamma detector response simulation inside the pedestal of Fukushima Daiichi Nuclear Power Station

Riyana, E. S.; 奥村 啓介; 寺島 顕一; 松村 太伊知; 坂本 雅洋

Mechanical Engineering Journal (Internet), 7(3), p.19-00543_1 - 19-00543_8, 2020/06

Prediction of the fuel debris location and distribution inside the primary containment vessel (PCV) of the Fukushima Daiichi Nuclear Power Plant is important to decide further decommissioning step and strategy. The radiation measurements in the past internal investigations have not yet provided enough information to predict fuel debris location and its distribution inside PCV. To support further measurement efforts, we simulate the detector response inside the PCV. The calculation result could provide a base on deciding suitable detector systems to assist the efforts on searching, localizing and defining distributions of the fuel debris.




JAEA-Review 2020-004, 140 Pages, 2020/05




Experimental and analytical investigation of formation and cooling phenomena in high temperature debris bed

堀田 亮年*; 秋葉 美幸*; 森田 彰伸*; Konovalenko, A.*; Vilanueva, W.*; Bechta, S.*; Komlev, A.*; Thakre, S.*; Hoseyni, S. M.*; Sk$"o$ld, P.*; et al.

Journal of Nuclear Science and Technology, 57(4), p.353 - 369, 2020/04

 被引用回数:0 パーセンタイル:100(Nuclear Science & Technology)

Key phenomena in the cooling states of debris beds under wet cavity conditions were classified into several groups based on the complicated geometry, nonhomogeneous porosity and volumetric heat of debris beds. These configurations may change due to the molten jet breakup, droplet agglomeration, anisotropic melt spreading, two-phase flow in a debris bed, particle self-leveling and penetration of molten metals into a particle bed. The modular code system THERMOS was designed for evaluating the cooling states of underwater debris beds. Three additional tests, DEFOR-A, PULiMS and REMCOD were employed to validate implemented models. This paper summarizes the entire test plan and representative data trends prior to starting individual data analyses and validations of specific models that are planned to be performed in the later phases. It also tries to report research questions to be answered in future works, such as various scales of melt-coolant interactions observed in the PULiMS tests.


放射線耐性の高い薄型SiC中性子検出器の開発(委託研究); 平成30年度英知を結集した原子力科学技術・人材育成推進事業

廃炉国際共同研究センター; 京都大学*

JAEA-Review 2019-042, 43 Pages, 2020/03




先端計測技術の融合で実現する高耐放射線燃料デブリセンサーの研究開発(委託研究); 平成30年度英知を結集した原子力科学技術・人材育成推進事業

廃炉国際共同研究センター; 高エネルギー加速器研究機構*

JAEA-Review 2019-040, 77 Pages, 2020/03




燃料デブリ取出し時における放射性核種飛散防止技術の開発(委託研究); 平成30年度英知を結集した原子力科学技術・人材育成推進事業

廃炉国際共同研究センター; 東京大学*

JAEA-Review 2019-037, 90 Pages, 2020/03




合金相を含む燃料デブリの安定性評価のための基盤研究(委託研究); 平成30年度英知を結集した原子力科学技術・人材育成推進事業

廃炉国際共同研究センター; 東北大学*

JAEA-Review 2019-035, 61 Pages, 2020/03




レーザー蛍光法を用いた燃料デブリ変質相の同定(委託研究); 平成30年度英知を結集した原子力科学技術・人材育成推進事業

廃炉国際共同研究センター; 東京大学*

JAEA-Review 2019-030, 66 Pages, 2020/03


日本原子力研究開発機構(JAEA)廃炉国際共同研究センター(CLADS)では、平成30年度英知を結集した原子力科学技術・人材育成推進事業(以下、「本事業」という)を実施している。本事業は、東京電力ホールディングス福島第一原子力発電所の廃炉等をはじめとした原子力分野の課題解決に貢献するため、国内外の英知を結集し、様々な分野の知見や経験を、従前の機関や分野の壁を越えて緊密に融合・連携させた基礎的・基盤的研究及び人材育成を推進することを目的としている。平成30年度の新規採択課題から実施主体を文部科学省からJAEAに移行することで、JAEAとアカデミアとの連携を強化し、廃炉に資する中長期的な研究開発・人材育成をより安定的かつ継続的に実施する体制を構築した。本研究は、研究課題のうち、平成30年度「レーザー蛍光法を用いた燃料デブリ変質相の同定」について取りまとめたものである。本研究は、デブリの主要構成元素であるウランに着目し、酸化的環境で安定な6価ウラン(U(VI))に選択的な時間分解型レーザー蛍光分光(TRLFS)法を用い、様々な条件下でデブリ表面に生成する変質相の同定を行う。特に、極低温での測定を行い、蛍光収率を向上させ、ピーク広がりを抑えることで、さらなる高感度・高分解能測定を実現するとともに、量子化学計算や多変量解析, 機械学習を援用することで、多成分、不均質なデブリ変質相の同定に繋げる。


Current situation of OECD/NEA, Preparatory Study on Analysis of Fuel debris (PreADES) project

仲吉 彬; Journeau, C.*; Rempe, J.*; Barrachin, M.*; Bottomley, D.; Nauchi, Y.*; Song, J. H.*

Proceedings of 2019 International Workshop on Post-Fukushima Challenges on Severe Accident Mitigation and Research Collaboration (SAMRC 2019) (USB Flash Drive),  ( ), 6 Pages, 2019/11

In recognition of the broad international interest in learning from post-accident examinations and other activities related to the Fukushima Daiichi Nuclear Power Station (1F), Japan recommended, to the Organization for Economic Co-operation and Development/Nuclear energy Agency/Committee on Safety of Nuclear Installations (OECD/NEA/CSNI) in 2013, that they identified and followed up on opportunities to address safety research gaps. The CSNI set up the Senior Expert Group (SEG) on Safety Research Opportunities Post-Fukushima (SAREF). In 2016-2017, Preparatory Study on Analysis of Fuel Debris (PreADES) project was recommended by the SEG on SAREF as a near-term project. The PreADES project will summarize the collected knowledge and expertise of debris characterization and identify the needs for debris analyses that will most contribute to the decommissioning of 1F. The project also aims to improve the understanding of severe accidents and reactor safety assessments as well as creating appropriate and optimal methodologies for future debris sampling, retrieval, and storage. Consequently, the project provides important input for a future international project of sample examination based on long-term considerations. The PreADES project launched discussions among interested organizations at the preliminary meeting in July 2017 about the objectives, scope, output, and direction of the project. The contents of the PreADES project were agreed as the three following tasks: Task 1: Joint study on fuel debris' expected properties and characterization, Task 2: Identifying needs and major issues for future fuel debris sampling, retrieval, and analyses, Task 3: Planning of future international R&D framework. Currently, 4th meeting took place on July in Tokyo Japan. Task 1 is almost completed and Task 2 will be summarized soon.


Effect of quenching on molten core-concrete interaction product

北垣 徹; 池内 宏知; 矢野 公彦; Brissonneau, L.*; Tormos, B.*; Domenger, R.*; Roger, J.*; 鷲谷 忠博

Journal of Nuclear Science and Technology, 56(9-10), p.902 - 914, 2019/09

 被引用回数:1 パーセンタイル:53.3(Nuclear Science & Technology)

Characterization of fuel debris is required to develop fuel debris removal tools. Especially, knowledge pertaining to the characteristics of molten core-concrete interaction (MCCI) product is needed because of the limited information available at present. The samples of a large-scale MCCI test performed under quenching conditions, VULCANO VW-U1, by CEA were analyzed to evaluate the characteristics of the surface of MCCI product generated just below the cooling water. As a result, the microstructure of the samples were found to be similar despite the different locations of the test sections. The Vickers hardness of each of the phases in these samples was higher than that of previously analyzed samples in another VULCANO test campaign, VBS-U4. From the comparison between analytical results of VULCANO MCCI test product, MCCI product generated under quenching condition is homogeneous and its hardness could be higher than that of the bulk MCCI product.


Calculation of gamma and neutron emission characteristics emitted from fuel debris of Fukushima Daiichi Nuclear Power Station

Riyana, E. S.; 奥村 啓介; 寺島 顕一

Journal of Nuclear Science and Technology, 56(9-10), p.922 - 931, 2019/09

 被引用回数:1 パーセンタイル:53.3(Nuclear Science & Technology)

Determination of fuel debris location and distribution inside primary containment vessel of Fukushima Daiichi Nuclear Power Station is important to decide further decommissioning step and strategy. We calculate neutron flux produced from fuel debris and secondary particles photon resulted from neutron reaction with nuclides inside fuel debris, including direct photon emission from FPs in fuel debris. Neutron and gamma characteristics resulted from calculation could be use as basis for determination suitable spectrometer system or detector for searching, localizing and treatment of fuel debris.


Exploratory investigation for estimation of fuel debris criticality risk

山根 祐一; 沼田 良明*; 外池 幸太郎

Proceedings of 11th International Conference on Nuclear Criticality Safety (ICNC 2019) (Internet), 10 Pages, 2019/09



Simulation study on the design of nondestructive measurement system using fast neutron direct interrogation method to nuclear materials in fuel debris

前田 亮; 古高 和禎; 呉田 昌俊; 大図 章; 米田 政夫; 藤 暢輔

Journal of Nuclear Science and Technology, 56(7), p.617 - 628, 2019/07

 被引用回数:1 パーセンタイル:53.3(Nuclear Science & Technology)

In order to measure the amount of nuclear materials in the fuel debris produced in the Fukushima Daiichi Nuclear Power Plant accident, we have designed a measurement system based on a Fast Neutron Direct Interrogation (FNDI) method. In particular, we have developed a fast response detector bank for fast neutron measurements by Monte Carlo simulations. The new bank has more than an order of magnitude faster response compared to the standard ones. We have also simulated the nondestructive measurements of the nuclear materials in homogeneously mixed fuel debris with various matrices which contain Stainless Steel (JIS SUS304), concrete, and various control-rod (CR) contents in the designed system. The results show that at least some types of the fissile materials in the debris can be measured by using the designed system.


An Interpretation of Fukushima-Daiichi Unit 3 plant data covering the two-week accident-progression phase based on correction for pressure data

佐藤 一憲

Journal of Nuclear Science and Technology, 56(5), p.394 - 411, 2019/05

 被引用回数:1 パーセンタイル:53.3(Nuclear Science & Technology)

福島第一3号機の圧力測定システムでは、運転中の蒸発/凝縮を補正するためにその一部に水柱が採用されている。これらの水柱の一部は事故条件下において蒸発し、正しい圧力データが示されていなかった。RPV(原子炉圧力容器), S/C(圧力抑制室)及びD/W(ドライウェル)の各圧力の比較を通し、水柱変化の効果を評価した。これによりRPV, S/C圧力データに対して水柱変化の効果の補正を行った。補正された圧力を用いて、事故進展中のRPV, S/C, D/W間のわずかな圧力差を評価した。この情報を、3号機の水位、CAMS(格納系雰囲気モニタリングシステム)および環境線量率などのデータとともに活用し、RPVおよびPCVの圧力上昇・下降および放射性物質の環境への放出に着目して事故進展挙動の解釈を行った。RPV内およびRPV外の燃料デブリのドライアウトはこれらの圧力低下を引き起こしている可能性がある一方、S/Cからペデスタルに流入したS/C水がペデスタルに移行した燃料デブリによって加熱されたことがPCV加圧の原因となっている。ペデスタル移行燃料デブリの周期的な再冠水とそのドライアウトは、最終的なデブリの再冠水まで数回の周期的な圧力変化をもたらしている。


Calculation of gamma and neutron emission characteristics emitted from fuel debris as a basis for determination of suitable detector system

Riyana, E. S.; 奥村 啓介; 寺島 顕一

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 4 Pages, 2019/05

Determination of fuel debris location and distribution inside primary containment vessel (PCV) of Fukushima Daiichi Nuclear Power Station is important to decide further decommissioning step and strategy. Past measurements not yet provide enough information to determine fuel debris location and its distribution inside PCV. To support further measurements effort, we simulate detector response inside PCV based on calculated photon and neutron emission spectrum produced from fuel debris. The Calculation result could be use as basis for determination of suitable spectrometer system or detector for search, localized, define fuel debris distributions and treatment of fuel debris.


Knowledge obtained from dismantling of large-scale MCCI experiment products for decommissioning of Fukushima Daiichi Nuclear Power Station

仲吉 彬; 池内 宏知; 北垣 徹; 鷲谷 忠博; Bouyer, V.*; Journeau, C.*; Piluso, P.*; Excoffier, E.*; David, C.*; Testud, V.*

Proceedings of International Topical Workshop on Fukushima Decommissioning Research (FDR 2019) (Internet),  ( ), 4 Pages, 2019/05

A large-scale Molten Core-Concrete Interaction (MCCI) test (VF-U1) under the Fukushima Daiichi Nuclear Power Station (1F) conditions (core material composition, concrete, and decay heat) was conducted at the large MCCI test facility (VULCANO) owned by French Alternative Energies and Atomic Energy Commission (CEA) in France. About 50 kg of simulated debris was melted and brought into contact with concrete to erode concrete under 1F conditions. After cooling, the concrete test section (concrete and MCCI product) was dismantled. Main observations of the structure of solidified pool (crust, porosity, oxide/metal layer, etc.) and of the ablation are given. The technical results obtained herein are summarized, and they provide interesting knowledge that will help with the decommissioning of 1F.


A Laboratory investigation of microbial degradation of simulant fuel debris by oxidizing microorganisms

Liu, J.; 土津田 雄馬; 北垣 徹; 香西 直文; 山路 恵子*; 大貫 敏彦

Proceedings of International Topical Workshop on Fukushima Decommissioning Research (FDR 2019) (Internet), 2 Pages, 2019/05



Observation of simulated fuel debris using synchrotron radiation

米田 安宏; 原田 誠; 高野 公秀

Transactions of the Materials Research Society of Japan, 44(2), p.61 - 64, 2019/04

Computed Tomography(CT)を用いて、模擬燃料デブリの3次元観察を行った。CTを使用して得られた模擬燃料デブリの内部は、ジルコニアリッチ部分およびコンクリートリッチ部分における明確なコントラストを示した。溶融状態からまず融点の高いジルコニアが析出する。コンクリートより重いジルコニアは結晶が析出すると下部へ移動し底面付近に凝集するため相分離が生じる。相分離はジルコニアの組成比の違いによって生じているが、組成比による結晶モードの違いも観察することができた。

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