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JAEA Reports

Radiation monitoring via manned helicopter around the nuclear power station in the fiscal year 2022 (Contract research)

Futemma, Akira; Sanada, Yukihisa; Nagakubo, Azusa; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Arai, Yoshinori*; et al.

JAEA-Technology 2023-027, 146 Pages, 2024/03

JAEA-Technology-2023-027.pdf:18.12MB

By the accident at Tokyo Electric Power Company's (TEPCO's) Fukushima Daiichi Nuclear Power Station (FDNPS), caused by tsunami triggered by the 2011 off the Pacific coast of Tohoku Earthquake, a large amount of radioactive material was released into the surrounding environment. After the accident, Airborne Radiation Monitoring (ARM) via manned helicopter has been applied as a method to quickly and extensively measure the distribution of radiation. Japan Atomic Energy Agency (JAEA) has continuously conducted ARM via manned helicopter around FDNPS. In this report, we summarize the results of the ARM around FDNPS in the fiscal year 2022, evaluate the changes of ambient dose rates and other parameters based on the comparison to the past ARM results, and discuss the causes of such changes. In order to contribute to improve the accuracy of ambient dose rate conversion, we analyzed the ARM data taking into account undulating topography, and evaluated the effect of this method. Furthermore, the effect of radon progenies in the air on the ARM was evaluated by applying the discrimination method to the measurement results.

JAEA Reports

Background radiation monitoring via manned helicopter and development of technology for radiation monitoring via unmanned airplane for application of nuclear emergency response technique in the fiscal year 2022 (Contract research)

Futemma, Akira; Sanada, Yukihisa; Sasaki, Miyuki; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Akutsu, Yuichiro*; Arai, Yoshinori*; et al.

JAEA-Technology 2023-026, 161 Pages, 2024/03

JAEA-Technology-2023-026.pdf:14.66MB

By the accident at Tokyo Electric Power Company's (TEPCO's) Fukushima Daiichi Nuclear Power Station (FDNPS), caused by tsunami triggered by the 2011 off the Pacific coast of Tohoku Earthquake, a large amount of radioactive material was released into the surrounding environment. After the accident, Airborne Radiation Monitoring (ARM) via manned helicopter has been utilized as a method to quickly and extensively measure radiation distribution surrounding FDNPS. In order to utilize ARM and to promptly provide the results during a nuclear emergency, information on background radiation levels, topographical features, and controlled airspace surrounding nationwide nuclear facilities have been prepared in advance. In the fiscal year 2022, we conducted ARM around the Mihama Nuclear Power Station of Kansai Electric Power Company (KEPCO), the Tsuruga Power Station of Japan Atomic Power Company (JAPC), and the Ikata Power Station of Shikoku Electric Power Company (YONDEN), and prepared information on background radiation doses and controlled airspace. In addition, we have developed an aerial radiation detection system via unmanned airplane, which is expected to be an alternative to ARM, during a nuclear emergency. This report summarizes the results and technical issues identified.

JAEA Reports

Investigations on distribution of radioactive substances owing to the Fukushima Daiichi Nuclear Power Station Accident in the fiscal year 2022 (Contract research)

Group for Fukushima Mapping Project

JAEA-Technology 2023-024, 176 Pages, 2024/03

JAEA-Technology-2023-024.pdf:22.16MB

This report presents results of the investigations on the distribution-mapping project of radioactive substances owing to TEPCO Fukushima Daiichi Nuclear Power Station (FDNPS) conducted in FY2022. Car-borne surveys, a measurement using survey meters, a walk survey and an unmanned helicopter survey were carried out to obtain air dose rate data to create their distribution maps, and temporal changes of the air dose rates were analyzed. Surveys on depth profile of radiocesium and in-situ measurements as for radiocesium deposition were performed. Based on these measurement results, effective half-lives of the temporal changes in the air dose rates and the deposition were evaluated. Score maps to classify the importance of the measurement points were created, and the factors causing changes in the score when monitoring data from multiple years were used were discussed. The range of fluctuation of past tritium concentration data in seawater was determined, and the causes of the fluctuation were discussed. Monitoring data in coastal area performed in 2022 owing to the comprehensive radiation monitoring plan was summarized, and temporal changes in cesium-137 were analyzed. Using the Bayesian hierarchical modeling approach, we obtained maps that integrated air dose rate distribution data acquired through surveys such as car-borne and walk surveys with respect to the region within 80 km from the FDNPS and Fukushima Prefecture. The measurement results for FY2022 were published on the "Database for Radioactive Substance Monitoring Data", and measurement data were stored as CSV format. Radiation monitoring and analysis of environmental samples owing to the comprehensive radiation monitoring plan were carried out.

JAEA Reports

Improvement of aerosol time-of-flight mass spectrometer for on-line measurement of tiny particles containing alpha emitters (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Osaka University*

JAEA-Review 2023-039, 71 Pages, 2024/03

JAEA-Review-2023-039.pdf:4.43MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY20 21, this report summarizes the research results of the "Improvement of aerosol time-of-flight mass spectrometer for on-line measurement of tiny particles containing alpha emitters" conducted in FY2021. The present study aims to improve Aerosol Time-Of-Flight Mass Spectrometer in order to monitor tiny particles containing alpha emitters such as U and Pu generated in removing debris from the reactors of 1F. In FY2021, for improving mass-resolution, we designed the optimized structure of mass spectrometer with much better mass resolution and ion transmittance than commercial ATOFMS by a PC simulation. Further, design of a detection part of ATOFMS fitted to the mass spectrometer was completed.

JAEA Reports

Embedded system using a radiation-hardened processor (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Okayama University*

JAEA-Review 2023-038, 48 Pages, 2024/03

JAEA-Review-2023-038.pdf:2.58MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems inthe nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Embedded system using a radiation-hardened processor" conducted in FY2022. The present study aims to be developing a radiation-hardened optoelectronic processor with a 10 MGy total-ionizing-dose (TID) tolerance, a radiation-hardened processor without any optical component with a 4 MGy TID tolerance, a radiation-hardened memory with a 4 MGy TID tolerance, and a radiation-hardened power supply unit with a 1 MGy TID tolerance. Moreover, Japanese research group will support radiation- hardened field programmable gate arrays, power supply units, and radiation-hardened optical systems for radiation-hardened robot systems and radiation sensor systems developed by UK team.

JAEA Reports

Development of a cooperative operation robot system for radiation source exploration (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*

JAEA-Review 2023-030, 80 Pages, 2024/03

JAEA-Review-2023-030.pdf:4.96MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems inthe nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2021, this report summarizes the research results of the "Development of a cooperative operation robot system for radiation source exploration" conducted in FY2022. The present study aims to develop a Cooperative Operation Robot system for RAdiation Source Exploration (CORRASE). The multiple robot system provides radiation source exploration with wide field of view, rapidity, and low cost. The radiation source exploration is realized with multiple robots carrying directional gamma-ray detectors determining the incident direction of the incoming gamma-rays. We will develop the system by the final year of this proposal aiming for application in the Fukushima Daiichi Nuclear Power Station.

JAEA Reports

Establishment of 3-D dose dispersion forecasting method and development of in-structure survey using the transparency difference of each line gamma-ray (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Kyoto University*

JAEA-Review 2023-028, 54 Pages, 2024/03

JAEA-Review-2023-028.pdf:3.81MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2022, this report summarizes the research results of the "Establishment of 3-D dose dispersion forecasting method and development of in-structure survey using the transparency difference of each line gamma-ray" conducted in FY2022. We realized an electron track detecting Compton camera (ETCC) that can measure $$gamma$$-ray images (linear images) with the bijective projection. In the "Quantitative analysis of radioactivity distribution by imaging of high radiation field environment using gamma-ray imaging spectroscopy" (hereinafter referred to as the previous project) adopted in FY2018, the 1 km square area including the reactor buildings was imaged at once.

JAEA Reports

Study on rational treatment/disposal of contaminated concrete waste considering leaching alteration (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Hokkaido University*

JAEA-Review 2023-027, 126 Pages, 2024/03

JAEA-Review-2023-027.pdf:5.51MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Study on rational treatment/disposal of contaminated concrete waste considering leaching alteration" conducted from FY2020 to FY2022. The present study aims to understand migration behaviors of radionuclides in relation to the properties of concrete altered by leaching, to develop migration model of radionuclides, and to evaluate waste management scenarios, focusing on underground concrete structures in contact with contaminated water.

JAEA Reports

Development of extremely small amount analysis technology for fuel debris analysis (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tohoku University*

JAEA-Review 2023-025, 117 Pages, 2024/03

JAEA-Review-2023-025.pdf:7.29MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Development of extremely small amount analysis technology for fuel debris analysis" conducted in FY2022. Understanding the properties of fuel debris is necessary for handling, criticality control, storage control, etc. A key technique is the chemical analysis of actinide nuclides. We develop sample pretreatment technology and separation / analysis process required for chemical analysis. The purpose of this study is to streamline future planned fuel debris analysis. To promote 1F decommissioning, we will train human resources through on-the-job training.

JAEA Reports

Development of methodology combining chemical analysis technology with informatics technology to understand perspectives property of debris and tie-up style human resource development (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Fukushima University*

JAEA-Review 2023-024, 109 Pages, 2024/03

JAEA-Review-2023-024.pdf:5.42MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Development of methodology combining chemical analysis technology with informatics technology to understand perspectives property of debris and tie-up style human resource development" conducted in FY2022. The present study aims to goal of this study is to implement a research plan relate to a development of combinational technology of new chemical analysis with informatics, and the aim is to develop new system for whole image estimation system using small quantities of information.

JAEA Reports

Human resource development related to remote control technology for monitoring inside rpv pedestal during retrieval of fuel debris (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2023-023, 99 Pages, 2024/03

JAEA-Review-2023-023.pdf:6.0MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems inthe nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Human Resource Development Related to Remote Control Technology for Monitoring Inside RPV Pedestal during Retrieval of Fuel Debris" conducted in FY2022. The present study aims to construct a monitoring platform for understanding the status inside a reactor during fuel debris removal, and measurement and visualization by sensors moving on the platform. In addition, to develop research personnel through research education by participating in such research projects, classroom lectures, and facility tours is also a goal of this project. In FY2022, each system was improved and expanded toward the final year, and verification experiments were conducted in simulated environments.

JAEA Reports

Contribution to risk reduction in decommissioning works by the elucidation of basic property of radioactive microparticles (Contract Research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Ibaraki University*

JAEA-Review 2023-021, 112 Pages, 2024/02

JAEA-Review-2023-021.pdf:7.1MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Contribution to Risk Reduction in Decommissioning Works by the Elucidation of Basic Property of Radioactive Microparticles" conducted from FY2018 to FY2021 (this contract was extended to FY2021). The present study aims to understand the basic properties (size, chemical composition, isotopic composition - including concentration of $$alpha$$-emitters, electrostatic properties, and optical properties, etc.) of fine particles composed of silicate with insoluble properties which contain regions of highly concentrated radioactive cesium (Cs) released to the environment by the accident at the Fukushima Daiichi Nuclear Power Station of TEPCO in 2011 March.

JAEA Reports

Development of genetic and electrochemical diagnosis and inhibition technologies for invisible corrosion caused by microorganisms (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; National Institute for Materials Science*

JAEA-Review 2023-031, 101 Pages, 2024/01

JAEA-Review-2023-031.pdf:24.47MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of genetic and electrochemical diagnosis and inhibition technologies for invisible corrosion caused by microorganisms" conducted from FY2020 to FY2022. The present study aims to develop innovative diagnostic techniques such as accelerated test specimens and on-site genetic testing for microbially induced and accelerated corrosion of metallic materials (microbially influenced corrosion, MIC), and to identify the conditions that promote MIC at 1F for proposing methods to prevent MIC through water quality and environmental control.

JAEA Reports

Annual report of Nuclear Emergency Assistance and Training Center (April 1, 2022 - March 31, 2023)

Nuclear Emergency Assistance and Training Center

JAEA-Review 2023-026, 54 Pages, 2023/12

JAEA-Review-2023-026.pdf:3.26MB

The Japan Atomic Energy Agency (JAEA) is one of the designated public corporations, which is the agency dealing with emergency situations in cooperation with the Japanese and local governments under the Disaster Countermeasures Basic Act and under the Armed Attack Situation Response Law. JAEA has, therefore, responsibilities of providing technical assistances to the Japanese and local governments in case of nuclear or radiological emergencies based on these acts. To fulfill the assistances, the JAEA has prepared the Nuclear Emergency Support Measures Regulation, Disaster Prevention Work Plan and Civil Protection Work Plan. The Nuclear Emergency Assistance and Training Center (NEAT) is the main center of the technical assistance in case of emergency, and dispatches experts of JAEA, supplies equipment and materials and gives technical advice and information, to the Japanese and local governments for emergency based on the regulation and plans. In normal time, the NEAT provides the technical assistances such as the exercises and training courses concerning the nuclear preparedness and response to the JAEA experts and to emergency responders including the Japanese and local government officers. This report introduces the results of activities in Japanese Fiscal Year 2022, conducted by the NEAT.

JAEA Reports

Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of $$beta$$, $$gamma$$, and X-rays (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*

JAEA-Review 2023-022, 93 Pages, 2023/12

JAEA-Review-2023-022.pdf:4.7MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of $$beta$$, $$gamma$$, and X-rays" conducted from FY2020 to FY2022. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, we have established the latest measurement system, such as the multiple $$gamma$$-ray detection methods, and the Spectral Determination Method (hereinafter referred to as "SDM") was developed. In the research in 2022, we developed a code that handles measurement data of LSC, singles Ge, and 2D spectra (multiple $$gamma$$). In addition, to develop an integrated database, spectral data of 40 nuclides were obtained by actual measurements and simulation calculations.

JAEA Reports

Technology development of diamond-base neutron sensors and radiation-resistive integrated-circuits for shielding-free criticality approach monitoring system (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; High Energy Accelerator Research Organization*

JAEA-Review 2023-020, 90 Pages, 2023/12

JAEA-Review-2023-020.pdf:6.59MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Technology development of diamond-base neutron sensors and radiation-resistive integrated-circuits for shielding-free criticality approach monitoring system" conducted from FY2020 to FY2022. The present study aims to develop key components of neutron detection system without a radiation shield for a criticality approach monitoring system with high neutron detection efficiency (a few count/nv) under high gamma ray background (1kGy/h). Developed components are neutron detection devices based on diamond sensors and a high radiation resistive signal-processing data-transfer system based on radiation resistive integrated circuit technologies.

JAEA Reports

Analysis of deposits inside the reactor at Fukushima Daiichi Nuclear Power Station in JFY2021; The Subsidy program of "Project of Decommissioning and Contaminated Water Management (Development of Analysis and Estimation Technology for Characterization of Fuel Debris)" starting FY2021

Ikeuchi, Hirotomo; Sasaki, Shinji; Onishi, Takashi; Nakayoshi, Akira; Arai, Yoichi; Sato, Takumi; Ohgi, Hiroshi; Sekio, Yoshihiro; Yamaguchi, Yukako; Morishita, Kazuki; et al.

JAEA-Data/Code 2023-005, 418 Pages, 2023/12

JAEA-Data-Code-2023-005-01.pdf:24.59MB
JAEA-Data-Code-2023-005-02.pdf:32.18MB

For safe and steady decommissioning of Tokyo Electric Power Company Holdings' Fukushima Daiichi Nuclear Power Station (1F), information concerning composition and physical/chemical properties of fuel debris generated in the reactors should be estimated and provided to other projects conducting the decommissioning work including the retrieval of fuel debris and the subsequent storage. For this purpose, in FY2021, samples of contaminants (the wiped smear samples and the deposits) obtained through the internal investigation of the 1F Unit 2 were analyzed to clarify the components and to characterize the micro-particles containing uranium originated from fuel (U-bearing particles) in detail. This report summarized the results of analyses performed in FY2021, including the microscopic analysis by SEM and TEM, radiation analysis, and elemental analysis by ICP-MS, as a database for evaluating the main features of each sample and the probable formation mechanism of the U-bearing particles.

JAEA Reports

Effect of preparation conditions and storage time on characteristic and rheological properties of carbonate slurries

Kato, Tomoaki; Yamagishi, Isao

JAEA-Technology 2023-018, 53 Pages, 2023/11

JAEA-Technology-2023-018.pdf:2.6MB

In the decommissioning of Fukushima Daiichi Nuclear Power Station, radioactive carbonate slurry waste was generated using the Advanced Liquid Processing System (ALPS) pretreatment and temporarily stored in a high integrity container (HIC). In 2015, overflow of supernatant from HIC estimate as bubble retention in the carbonate slurry was discovered, increasing the need for a safety assessment of the carbonate slurry stored the HIC (HIC slurry). In this study, a carbonate slurry (simulated slurry) was prepared according to the Mg/Ca mass ratio in the ALPS inlet water of the HIC slurry which overflew the HIC. The effects of reaction time during the pretreatment process, suspended solids concentration (SS concentration), and settling time on the particle composition, morphology and rheological properties of the slurry were investigated. Evaluating the effect of reaction time and concentration process on chemical properties in slurry production, the effect of the reaction time was not confirmed in the simulated slurry that had undergone the concentration process, and slurry prepared at SS concentration of 150 g/L was composed of formless particles have a particle diameter of 0.4 $$mu$$m or less. We also investigate the effect of SS concentration on sedimentability, decrease in SS concentration by dilution with processing solution contributed to an increase in the initial slurry settling velocity. Furthermore, two different flow characteristics were observed depending on the settling time, suggesting that the slurry at the initial settling time has non-Bingham flow properties, whereas it changes to Bingham flow properties as the settling time becomes longer. In addition, yield stress was increased with settling time, and this yield stress was found to be exponentially proportional to the density of the slurry. These results provide knowledge to estimate the current state of HIC slurry and are expected to contribute to the safety assessment.

JAEA Reports

Segregation of components of molten core oxidic materials using cold crucible induction heating technique (Joint research)

Sudo, Ayako; M$'e$sz$'a$ros, B.*; Sato, Takumi; Nagae, Yuji

JAEA-Research 2023-007, 31 Pages, 2023/11

JAEA-Research-2023-007.pdf:3.61MB

For the criticality assessment of fuel debris generated by the accident in Fukushima Daiichi Nuclear Power Station, understanding of the elemental localization in fuel debris is important. Especially, the distribution of Fe and Gd, which may behave as potential neutron absorber materials in the fuel debris, is of particular important from the viewpoint of nuclear criticality safety. To investigate the localization tendency of Gd and Fe in molten core materials during solidification progress, liquefaction/solidification tests on core materials containing UO$$_{2}$$, ZrO$$_{2}$$, FeO, Gd$$_{2}$$O$$_{3}$$, and simulated fission products (MoO$$_{3}$$, Nd$$_{2}$$O$$_{3}$$, SrO, and RuO$$_{2}$$) and concrete (SiO$$_{2}$$, Al$$_{2}$$O$$_{3}$$, and CaO) were performed using cold crucible induction heating technique. During the test, the molten core materials gradually subsided and solidified from the bottom to the top of the melt. Elemental analysis showed that Fe content in the inner region increased approximately up to 3.4 times that in the bottom region. The concentration of Fe into the inner region was observed in all the samples regardless of the initial FeO composition, cooling rates, and phase separation. This suggests that FeO may be concentrated into the low temperature region, where the melt solidified later. In contrast, Gd content in the bottom region increased approximately up to 2.6 times that in the inner region. The concentration of Gd into the bottom region was observed when the initial Gd$$_{2}$$O$$_{3}$$ content was higher than 1 at.%. This suggests that Gd$$_{2}$$O$$_{3}$$ may be concentrated into the earlier solidified region. On the other hand, no significant localization was observed on the simulated fission products.

JAEA Reports

Annual report for FY2021 on the activities of Naraha Center for Remote Control Technology Development (April 1, 2021 - March 31, 2022)

Akiyama, Yoichi; Shibanuma, So; Yanagisawa, Kenichi*; Yamada, Taichi; Suzuki, Kenta; Yoshida, Moeka; Ono, Takahiro; Kawabata, Kuniaki; Watanabe, Kaho; Morimoto, Kyoichi; et al.

JAEA-Review 2023-015, 60 Pages, 2023/09

JAEA-Review-2023-015.pdf:4.78MB

Naraha Center for Remote Control Technology Development (NARREC) was established in Japan Atomic Energy Agency to promote a decommissioning work of Fukushima Daiichi Nuclear Power Station (Fukushima Daiichi NPS). NARREC consists of a Full-scale Mock-up Test Building and Research Management Building. Various test facilities are installed in these buildings for the decommissioning work of Fukushima Daiichi NPS. These test facilities are intended to be used for various users, such as companies engaged in the decommissioning work, research and development institutions, educational institutions and so on. The number of NARREC facility uses was 84 in FY2021. We participated booth exhibitions and presentations on the decommissioning related events. Moreover, we also contributed to the development of human resources by supporting the 6th Creative Robot Contest for Decommissioning. As a new project, "Narahakko Children's Classroom" was implemented for elementary school students in Naraha Town. This report summarizes the activities of NARREC in FY2021, such as the utilization of facilities and equipment of NARREC, the development of remote-control technologies for supporting the decommissioning work, arrangement of the remote-control machines for emergency response, and training for operators by using the machines.

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